We demonstrate, theoretically and experimentally, that statistical mixtures of the vacuum state |0> and the single-photon Fock state |1> are nonclassical according to the Vogel criterion (W. Vogel, Phys. Rev. Lett. 84, 1849 (2000)), regardless of the vacuum fraction. The ensembles are synthesized via conditional measurements on biphotons generated by means of parametric downconversion, and their quadrature statistics are measured using balanced homodyne detection. A comparative review of various quantum state nonclassicality criteria is presented.
A bosonic state is commonly considered nonclassical (or quantum) if its Glauber-Sudarshan $P$ function is not a classical probability density, which implies that only coherent states and their statistical mixtures are classical. We quantify the nonclassicality of a single qubit, defined by the vacuum and single-photon states, by applying the following four well-known measures of nonclassicality: (1) the nonclassical depth, $τ$, related to the minimal amount of Gaussian noise which changes a nonpositive $P$ function into a positive one; (2) the nonclassical distance $D$, defined as the Bures di…
Distinguishing quantum states that admit a classical counterpart from those that exhibit nonclassicality has long been a central issue in quantum optics. Finding an implementable criterion certifying optical nonclassicality (i.e, the incompatibility with a statistical mixture of coherent states) is of major importance as it often is a prerequisite to quantum information processes. A hierarchy of conditions for detecting whether a quantum state exhibits optical nonclassicality can be written based on some matrices of moments of the optical field [Phys. Rev. A 72, 043808 (2005)]. Here, we design…
Polya states of single mode radiation field are proposed and their algebraic characterization and nonclassical properties are investigated. They degenerate to the binomial (atomic coherent) and negative binomial (Perelomov's su(1,1) coherent) states in two different limits and further to the number, the ordinary coherent and Susskind-Glogower phase states. The algebra involved turn out to be a two-parameter deformation of both su(2) and su(1,1). Nonclassical properties are investigated in detail.
We experimentally investigate a method of directly characterizing the photon number distribution of nonclassical light beams that is tolerant to losses and makes use only of standard binary detectors. This is achieved in a single measurement by calibrating the detector using some small amount of prior information about the source. We demonstrate the technique on a freely propagating heralded two-photon number state created by conditional detection of a two-mode squeezed state generated by a parametric downconverter.
Numerous inequalities involving moments of integrated intensities and revealing nonclassicality and entanglement in bipartite optical fields are derived using the majorization theory, non-negative polynomials, the matrix approach, as well as the Cauchy-Schwarz inequality. Different approaches for deriving these inequalities are compared. Using the experimental photocount histogram generated by a weak noisy twin beam monitored by a photon-number-resolving iCCD camera the performance of the derived inequalities is compared. A basic set of ten inequalities suitable for monitoring the entanglement…
An analytic operator solution of a generalized quantum mechanical Hamiltonian of two-mode Bose Einstein condensates (BECs) is obtained and the same is used to investigate the nonclassical properties of the modes present in the system. Nonclassical characters are observed by means of single mode and intermodal squeezing, single mode and intermodal sub-Poissonian boson statistics and intermodal entanglement. In addition to the traditionally studied lower order nonclassical properties, signatures of higher order nonclassical characters of two-mode BEC systems are also obtained by investigating th…
We implement the direct sampling of negative phase-space functions via unbalanced homodyne measurement using click-counting detectors. The negativities significantly certify nonclassical light in the high-loss regime using a small number of detectors which cannot resolve individual photons. We apply our method to heralded single-photon states and experimentally demonstrate the most significant certification of nonclassicality for only two detection bins. By contrast, the frequently applied Wigner function fails to indicate such quantum characteristics for the quantum efficiencies present in ou…
Broadband light sources play essential roles in diverse fields, such as high-capacity optical communications, optical coherence tomography, optical spectroscopy, and spectrograph calibration. Though an ultrabroadband nonclassical state from standard spontaneous parametric down-conversion may serve as a quantum counterpart, its detection and quantum characterization have been a challenging task. Here we demonstrate the quantitative characterization of a multimode structure in such an ultrabroadband (150 nm FWHM) squeezed state at telecom wavelength (1.5 μm). The nonclassical photon distribution…
While negativity in phase space is a well-known signature of nonclassicality, a wide variety of nonclassical states require their characterization beyond negativity. We establish a framework of nonclassicality in phase space that addresses nonclassical states comprehensively with a direct experimental evidence. This includes the negativity of phase-space distribution as a special case and further analyzes quantum states with positive distributions effectively. We prove that it detects all nonclassical Gaussian states and all non-Gaussian states of arbitrary dimension remarkably by examining th…
We show that one single experiment can test simultaneously and independently both the nonclassicality of states and measurements by the violation or fulfillment of classical bounds on the statistics. Nonideal measurements affected by imperfections can be characterized by two bounds depending on whether we test the ideal measurement or the real one.
We study the characteristics of the light generated by few emitters in a cavity at strong light-matter coupling. By means of the Glauber $g^{(2)}$-function we can identify clearly distinguished parameter regimes with super-Poissonian and sub-Poissonian photon statistics. We establish a relation between the emission characteristics for one and multiple emitters, and explain its origin in terms of the photon-dressed emitter states. Cooperative effects lead to the generation of nonclassical light already at reduced light-matter coupling if the number of emitters is increased. Our results are obta…
Thermal or chaotic light sources emit radiation characterized by a slightly enhanced probability of emitting photons in bunches, described by a zero-delay second-order correlation function $g^{(2)}(0) = 2$. Here we explore photon-coincidence counting statistics of thermal cavities in the ultrastrong coupling regime, where the atom-cavity coupling rate becomes comparable to the cavity resonance frequency. We find that, depending on the system temperature and coupling rate, thermal photons escaping the cavity can display very different statistical behaviors, characterised by second-order correla…
The measurement of joint signal-idler photon-number distribution of a field obtained from spontaneous parametric downconversion using an intensified CCD camera is presented. It is shown that a classicality criterion is violated directly by the measured data. Characteristic dimensions of the area of correlation are determined in the same experimental setup.
We investigate the nonclassical properties of output fields propagated through a contradirectional asymmetric nonlinear optical coupler consisting of a linear waveguide and a nonlinear (quadratic) waveguide operated by second harmonic generation. In contrast to the earlier results, all the initial fields are considered weak and a completely quantum mechanical model is used here to describe the system. Perturbative solutions of Heisenberg's equations of motion for various field modes are obtained using Sen-Mandal technique. Obtained solutions are subsequently used to show the existence of singl…
A system of two two-level atoms interacting with a squeezed vacuum field can exhibit stationary entanglement associated with nonclassical two-photon correlations characteristic of the squeezed vacuum field. The amount of entanglement present in the system is quantified by the well known measure of entanglement called concurrence. We find analytical formulas describing the concurrence for two identical and nonidentical atoms and show that it is possible to obtain a large degree of steady-state entanglement in the system. Necessary conditions for the entanglement are nonclassical two-photon corr…
We report the experimental realization and tomographic analysis of novel quantum light states obtained by exciting a classical thermal field by a single photon. Such states, although completely incoherent, possess a tunable degree of quantumness which is here exploited to put to a stringent experimental test some of the criteria proposed for the proof and the measurement of state non-classicality. The quantum character of the states is also given in quantum information terms by evaluating the amount of entanglement that they can produce.
We report measurements of two-photon interference using a cw-pumped type-II spontaneous parametric down-conversion source based on a multimode perodically poled potassium titanyl phosphate waveguide. We have used the recently demonstrated technique of controlling the spatial characteristics of the down-conversion process via intermodal dispersion to generate photon pairs in fundamental transverse modes, thus ensuring their spatial indistinguishability. Good spatial overlap of photon modes within pairs has been verified using the Hong-Ou-Mandel interferometer and the preparation of polarization…
A non-Gaussian state being a mixture of the vacuum and single-photon states can be generated by truncating a thermal state in a quantum scissors device of Pegg et al. [Phys. Rev. Lett. 81 (1998) 1604]. In contrast to the thermal state, the generated state shows nonclassical property including the negativity of Wigner function. Besides, signal amplification and signal-to-noise ratio enhancement can be achieved.
Nonclassical states of light are necessary resources for quantum technologies such as cryptography, computation and the definition of metrological standards. Observing signatures of nonclassicality generally requires inferring either the photon number distribution or a quasi-probability distribution indirectly from a set of measurements. Here, we report an experiment in which the nonclassical character of families of quantum states is assessed by direct inspection of the outcomes from a multiplexed photon counter. This scheme does not register the actual photon number distribution; the statist…
We present a robust tool to analyze nonclassical properties of multimode twin-beam states in the mesoscopic photon-number domain. The measurements are performed by direct detection. The analysis exploits three different non-classicality criteria for detected photons exhibiting complementary behavior in the explored intensity regime. Joint signal-idler photon-number distributions and quasi-distributions of integrated intensities are determined and compared with the corresponding distributions of detected photons. Experimental conditions optimal for nonclassical properties of twin-beam states ar…
We theoretically introduce a new kind of non-Gaussian state-----Laguerre polynomial excited coherent states by using the multiphoton catalysis which actually can be considered as a block comprising photon number operator. It is found that the normalized factor is related to the two-variable Hermite polynomials. We then investigate the nonclassical properties in terms of Mandel's Q parameter, quadrature squeezing, second correlation, and the negativity of Wigner function (WF). It is shown that all these properties are related to the amplitude of coherent state, catalysis number and unbalanced b…
Highly nonclassical character of optical quantum detectors, such as single-photon detectors, is essential for preparation of quantum states of light and a vast majority of applications in quantum metrology and quantum information processing. Therefore, it is both fundamentally interesting and practically relevant to investigate the nonclassical features of optical quantum measurements. Here we propose and experimentally demonstrate a procedure for direct certification of quantum non-Gaussianity and Wigner function negativity, two crucial nonclassicality levels, of photonic quantum detectors. R…
Quantum information science attempts to exploit capabilities from the quantum realm to accomplish tasks that are otherwise impossible in the classical domain [1]. Although sufficient conditions have been formulated for the physical resources required to achieve quantum computation and communication [2], there is an evolving understanding of the power of quantum measurement combined with conditional evolution for accomplishing diverse tasks in quantum information science [3-5]. In this regard, a significant advance is the invention of a protocol by Duan, Lukin, Cirac, and Zoller (DLCZ) [6] for …
Taking the decoherence into account, we investigate nonclassical features of the optical Schrödinger cat states in one mode and two coupled-modes systems with two-photon driving. In the one mode system, the relationship between the Schrödinger cat states and the system parameters is derived. We observe that in the presence of single-photon decay the steady states would be a mixture of Schrödinger cats. The dynamics and steady states of such a cat versus single-photon decay are examined. In the two coupled-modes cases with linear and nonlinear couplings, the dynamics of entanglement and mutual …
Characterizing quantum synchronization in the van der Pol oscillator via tomogram and photon correlation
Indian Association for the Cultivation of Science（印度科学文化研究院）；The Institute of Mathematical Sciences（数学科学研究所）；Government Arts and Science College Kozhikode, University of Calicut（卡利卡特大学科泽科德政府文理科学院）；Government College Malappuram, University of Calicut（卡利卡特大学马拉普兰政府学院）
A completely quantum description of Raman process is used to investigate the nonclassical properties of the modes in the stimulated, spontaneous and partially spontaneous Raman process. Both coherent scattering (where all the initial modes are coherent) and chaotic scattering (where initial phonon mode is chaotic and all the other modes are coherent) are studied. Nonclassical character of Raman process is observed by means of intermodal entanglement, single mode and intermodal squeezing of vacuum fluctuations, sub-shot noise and wave variances. Joint photon-phonon number and integrated-intensi…
The vast majority of physical objects we are dealing with are almost exclusively made of atoms. Due to their discrete level structure, single atoms have proved to be emitters of light which is incompatible with the classical description of electromagnetic waves. We demonstrate this incompatibility for atomic fluorescence when scaling up the size of the source ensemble, which consists of trapped atomic ions, by several orders of magnitude. The presented measurements of nonclassical statistics on light unconditionally emitted from ensembles containing up to more than a thousand ions promise furt…
Nonclassical states, having no classical analogue, promise advantage in the performance in several fields of technology, such as computation, communication, sensing. This led to an escalated interest in the recent years for the generation and characterization of nonclassical states in various physical systems of interest. Keeping this in mind, we examined generation of various lower- and higher-order nonclassical states in both codirectional and contradirectional asymmetric nonlinear optical couplers operating under second harmonic generation with the help of moments-based criteria. Using anot…
Quantum mechanics predicts that measurements of incompatible observables carry a minimum uncertainty which is independent of technical deficiencies of the measurement apparatus or incomplete knowledge of the state of the system. Nothing yet seems to prevent a single physical quantity, such as one spin component, from being measured with arbitrary precision. Here we show that an intrinsic quantum uncertainty on a single observable is ineludible in a number of physical situations. When revealed on local observables of a bipartite system, such uncertainty defines an entire class of bona fide meas…
The characterization of mixtures of non-interacting, spectroscopically similar quantum components has important applications in chemistry, biology, and materials science. We introduce an approach based on quantum tracking control that allows for determining the relative concentrations of constituents in a quantum mixture, using a single pulse which enhances the distinguishability of components of the mixture and has a length that scales linearly with the number of mixture constituents. To illustrate the method, we consider two very distinct model systems: mixtures of diatomic molecules in the …
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables, for example in cluster state computation. They can be generated either by mixing different squeezed light sources using linear optical operations, or directly in a multimode optical device. In parallel, frequency combs are perfect tools for high precision metrological applications and for quantum time transfer. Synchronously Pumped Optical Parametric Oscillators (SPOPOs) have been theoretically shown to produce multimode non-classical frequency combs. In this paper, we present the…
We develop a semiclassical method for the determination of the nonlinear dynamics of dissipative quantum optical systems in the limit of large number of photons N, based on the 1/N-expansion and the quantum-classical correspondence. The method has been used to tackle two problems: to study the dynamics of nonclassical state generation in higher-order anharmonic dissipative oscillators and to establish the difference between the quantum and classical dynamics of the second-harmonic generation in a self-pulsing regime. In addressing the first problem, we have obtained an explicit time dependence…
Nonclassical states of a quantized light are described in terms of Glauber-Sudarshan P distribution which is not a genuine classical probability distribution. Despite several attempts, defining a uniform measure of nonclassicality (NC) for the single mode quantum states of light is yet an open task. In our previous work [Phys. Rev. A 95, 012330 (2017)] we have shown that the existing well-known measures fail to quantify the NC of single mode states that are generated under multiple NC-inducing operations. Recently, Ivan et. al. [Quantum. Inf. Process. 11, 853 (2012)] have defined a measure of …
We report demonstrations of both quadrature squeezed vacuum and photon number difference squeezing generated in an integrated nanophotonic device. Squeezed light is generated via strongly driven spontaneous four-wave mixing below threshold in silicon nitride microring resonators. The generated light is characterized with both homodyne detection and direct measurements of photon statistics using photon number-resolving transition edge sensors. We measure $1.0(1)$~dB of broadband quadrature squeezing (${\sim}4$~dB inferred on-chip) and $1.5(3)$~dB of photon number difference squeezing (${\sim}7$…
