A bosonic state is commonly considered nonclassical (or quantum) if its Glauber-Sudarshan $P$ function is not a classical probability density, which implies that only coherent states and their statistical mixtures are classical. We quantify the nonclassicality of a single qubit, defined by the vacuum and single-photon states, by applying the following four well-known measures of nonclassicality: (1) the nonclassical depth, $τ$, related to the minimal amount of Gaussian noise which changes a nonpositive $P$ function into a positive one; (2) the nonclassical distance $D$, defined as the Bures distance of a given state to the closest classical state, which is the vacuum for the single-qubit Hilbert space; together with (3) the negativity potential (NP) and (4) concurrence potential, which are the nonclassicality measures corresponding to the entanglement measures (i.e., the negativity and concurrence, respectively) for the state generated by mixing a single-qubit state with the vacuum on a balanced beam splitter. We show that complete statistical mixtures of the vacuum and single-photon states are the most nonclassical single-qubit states regarding the distance $D$ for a fixed value of both the depth $τ$ and NP in the whole range $[0,1]$ of their values, as well as the NP for a given value of $τ$ such that $τ>0.3154$. Conversely, pure states are the most nonclassical single-qubit states with respect to $τ$ for a given $D$, NP versus $D$, and $τ$ versus NP. We also show the "relativity" of these nonclassicality measures by comparing pairs of single-qubit states: if a state is less nonclassical than another state according to some measure then it might be more nonclassical according to another measure. Moreover, we find that the concurrence potential is equal to the nonclassical distance for single-qubit states.
In this paper, we use the characteristic function, i.e., the Fourier transform of the Glauber-Sudarshan phase-space distribution, to find the degree of nonclassicality of a given state. This degree of nonclassicality quantifies the nonclassicality in terms of quantum superpositions. We demonstrate two ways to determine or to estimate the degree of nonclassicality by studying the properties of the characteristic functions. The developed criteria are applied to two examples of squeezed states undergoing a classical mixing or a nonclassical superposition with vacuum.
The degree of nonclassicality of states of a field mode is analysed considering both phase-space and distance-type measures of nonclassicality. By working out some general examples, it is shown explicitly that the phase-space measure is rather sensitive to superposition of states, with finite superpositions possessing maximum nonclassical depth (the highest degree of nonclassicality) irrespective to the nature of the component states. Mixed states are also discussed and examples with nonclassical depth varying between the minimum and the maximum allowed values are exhibited. For pure Gaussian …
A measure of nonclassicality of quantum states based on the volume of the negative part of the Wigner function is proposed. We analyze this quantity for Fock states, squeezed displaced Fock states and cat-like states defined as coherent superposition of two Gaussian wave packets.
We introduce a new non-Gaussian state, generated by m times coherent superposition operation $a\cos θ+a^{\dagger }e^{iφ}\sin θ$ (MCSO) on odd-Schrodinger-cat state (OSCS). Its normalized constant is turned out to be related with the Hermite polynomial. We further investigate the nonclassical properties of the MCSO-OSCS through Mandel's Q-parameter, quadrature squeezing, the photocount distribution and Wigner function (WF). It is shown that the nonclassicality of the MCSO-OSCS is influenced by the number of times (m) of coherent superpositon operation, the angle $θ$ and the amplitude of the coh…
There are quantum states of light that can be expressed as finite superpositions of Fock states (FSFS). We demonstrate the nonclassicality of an arbitrary FSFS by means of its phase space distributions such as the Wigner function and the $Q$-function. The decoherence of the FSFS is studied by considering the time evolution of its Wigner function in amplitude decay and phase damping channels. As examples, we determine the nonclassicality and decoherence of generalized and reciprocal binomial states.
The nonclassicality of single-mode quantum states is studied in relation to the entanglement created by a beam splitter. It is shown that properly defined quantifications -- based on the quantum superposition principle -- of the amounts of nonclassicality and entanglement are strictly related to each other. This can be generalized to the amount of genuine multipartite entanglement, created from a nonclassical state by an N splitter. As a consequence, a single-mode state of a given amount of nonclassicality is fully equivalent, as a resource, to exactly the same amount of entanglement. This rel…
The algebraic quantification of nonclassicality, which naturally arises from the quantum superposition principle, is related to properties of regular nonclassicality quasiprobabilities. The latter are obtained by non-Gaussian filtering of the Glauber-Sudarshan $P$~function. They yield lower bounds for the degree of nonclassicality. We also derive bounds for convex combinations of Gaussian states for certifying quantum non-Gaussianity directly from the experimentally accessible nonclassicality quasiprobabilities. Other quantum-state representations, such as $s$-parametrized quasiprobabilities, …
We introduce an experimentally accessible method to measure a unique degree of nonclassicality, based on the quantum superposition principle, for arbitrary quantum states. We formulate witnesses and test a given state for any particular value of this measure. The construction of optimal tests is presented as well as the general numerical implementation. We apply this approach on examples such as squeezed states, and we show how to formulate conditions to certify a particular degree of nonclassicality for single- and multimode radiation fields.
We derive and implement a general method to characterize the nonclassicality in compound discrete- and continuous-variable systems. For this purpose, we introduce the operational notion of conditional hybrid nonclassicality which relates to the ability to produce a nonclassical continuous-variable state by projecting onto a general superposition of discrete-variable subsystem. We discuss the importance of this form of quantumness in connection with interfaces for quantum communication. To verify the conditional hybrid nonclassicality, a matrix version of a nonclassicality quasiprobability is d…
Bell nonclassicality of a single photon superposition in two modes, often referred to as `nonlocality of a single photon', is one of the most striking nonclassical phenomena discussed in the context of foundations of quantum physics. Here we show how to robustly violate local realism within the weak-field homodyne measurement scheme for \textit{any} superposition of one photon with vacuum. Our modification of the previously proposed setups involves tunable beamsplitters at the measurement stations, and the local oscillator fields significantly varying between the settings, optimally being {\it…
We discuss the role of nonclassicality of quantum states as a necessary resource in deterministic generation of multipartite entangled states. In particular for three bilinearly coupled modes of the electromagnetic field, tuning of the coupling constants between the parties allows the total system to evolve into both Bell and GHZ states only when one of the parties is initially prepared in a nonclassical state. A superposition resource is then converted into an entanglement resource.
To quantify single mode nonclassicality, we start from an operational approach. A positive semi-definite observable is introduced to describe a measurement setup. The quantification is based on the negativity of the normally ordered version of this observable. Perfect operational quantumness corresponds to the quantum-noise-free measurement of the chosen observable. Surprisingly, even moderately squeezed states may exhibit perfect quantumness for a properly designed measurement. The quantification is also considered from an axiomatic viewpoint, based on the algebraic structure of the quantum s…
Characterizing genuine quantum resources and determining operational rules for their manipulation are crucial steps to appraise possibilities and limitations of quantum technologies. Two such key resources are nonclassicality, manifested as quantum superposition between reference states of a single system, and entanglement, capturing quantum correlations among two or more subsystems. Here we present a general formalism for the conversion of nonclassicality into multipartite entanglement, showing that a faithful reversible transformation between the two resources is always possible within a pre…
Quantum mechanics exhibits a wide range of nonclassical features, of which entanglement in multipartite systems takes a central place. In several specific settings, it is well known that nonclassicality (e.g., squeezing, spin squeezing, coherence) can be converted into entanglement. In this work, we present a general framework, based on superposition, for structurally connecting and converting nonclassicality to entanglement. In addition to capturing the previously known results, this framework also allows us to uncover new entanglement convertibility theorems in two broad scenarios, one which…
A beam's density matrix that is described by the superposition of excitation on coherent states with thermal noise (SECST) is presented, and its matrix elements in Fock space are calculated. The maximum information transmitted by the SECST beam is derived. It is more than that by coherent light beam and increases as the excitation photon number increases. In addition, the nonclassicality of density matrix is demonstrated by calculating its Wigner function.
We reconsider the all-optical homodyne-measurement based experimental schemes that aim to reveal Bell nonclassicality of a single photon, often termed `nonlocality'. We focus on the schemes put forward by Tan, Walls and Collett (TWC, 1991) and Hardy (1994). In the light of our previous work the Tan, Walls and Collett setup can be described by a precise local hidden variable model, hence the claimed nonclassicality of this proposal is apparent, whereas the nonclassicality proof proposed by Hardy is impeccable. In this work we resolve the following problem: which feature of the Hardy's approach …
The constraints arising for a general set of causal relations, both classically and quantumly, are still poorly understood. As a step in exploring this question, we consider a coherently controlled superposition of "direct-cause" and "common-cause" relationships between two events. We propose an implementation involving the spatial superposition of a mass and general relativistic time dilation. Finally, we develop a computationally efficient method to distinguish such genuinely quantum causal structures from classical (incoherent) mixtures of causal structures and show how to design experiment…
We consider an experimentally realizable scheme for manipulating quantum states using a general superposition of products of field annihilation ($\hat{a}$) and creation ($\hat{a}^†$) operators of the type ($s \hat{a}\hat{a}^†+ t \hat{a}^†\hat{a}$), with $s^2 + t^2 = 1$. Such an operation, when applied on states with classical features, is shown to introduce strong nonclassicality. We quantify the generated degree of nonclassicality by the negative volume of Wigner distribution in the phase space and investigate two other observable nonclassical features, sub-Poissonian statistics and squeezing…
Distinguishing quantum states that admit a classical counterpart from those that exhibit nonclassicality has long been a central issue in quantum optics. Finding an implementable criterion certifying optical nonclassicality (i.e, the incompatibility with a statistical mixture of coherent states) is of major importance as it often is a prerequisite to quantum information processes. A hierarchy of conditions for detecting whether a quantum state exhibits optical nonclassicality can be written based on some matrices of moments of the optical field [Phys. Rev. A 72, 043808 (2005)]. Here, we design…
Contrary to previous claims, it is shown that, for an ensemble of either single-particle systems or multi-particle systems, the realistic interpretation of a superposition state that mathematically describes the ensemble does not imply that the ensemble is a mixture. Therefore it cannot be argued that the realistic interpretation is wrong on the basis that some predictions derived from the mixture are different from the corresponding predictions derived from the superposition state.
We present Bell-type tests of nonclassicality and non-Gaussianity for single-mode fields employing a generalized quasiprobability function. Our nonclassicality tests are based on the observation that two orthogonal quadratures in phase space (position and momentum) behave as independent realistic variables for a coherent state. Taking four (three) points at the vertices of a rectangle (right triangle) in phase space, our tests detect every pure nonclassical Gaussian state and a range of mixed Gaussian states. These tests also set an upper bound for all Gaussian states and their mixtures, which…
We theoretically propose and experimentally demonstrate a nonclassicality test of single-mode field in phase space, which has an analogy with the nonlocality test proposed by Banaszek and Wodkiewicz [Phys. Rev. Lett. 82, 2009 (1999)]. Our approach to deriving the classical bound draws on the fact that the Wigner function of a coherent state is a product of two independent distributions as if the orthogonal quadratures (position and momentum) in phase space behave as local realistic variables. Our method detects every pure nonclassical Gaussian state, which can also be extended to mixed states.…
We examine the notion of nonclassicality in terms of quasiprobability distributions. In particular, we do not only ask if a specific quasiprobability can be interpreted as a classical probability density, but require that characteristic features of classical electrodynamics are resembled. We show that the only quasiprobabilities which correctly describe the superposition principle of classical electromagnetic fields are the $s$-parameterized quasiprobabilities. Furthermore, the Glauber-Sudarshan P function is the only quantum-mechanical quasiprobability which is transformed at a classical atte…
We demonstrate, theoretically and experimentally, that statistical mixtures of the vacuum state |0> and the single-photon Fock state |1> are nonclassical according to the Vogel criterion (W. Vogel, Phys. Rev. Lett. 84, 1849 (2000)), regardless of the vacuum fraction. The ensembles are synthesized via conditional measurements on biphotons generated by means of parametric downconversion, and their quadrature statistics are measured using balanced homodyne detection. A comparative review of various quantum state nonclassicality criteria is presented.
In this paper, we detail an orthogonalization procedure that allows for the quantification of the amount of coherence present an arbitrary superposition of coherent states. The present construction is based on the quantum coherence resource theory introduced by Baumgratz et al., and the coherence resource monotone that we identify is found to characterize the nonclassicality traditionally analyzed via the Glauber-Sudarshan $P$ distribution. This suggests that identical quantum resources underlie both quantum coherence in the discrete finite dimensional case and the nonclassicality of quantum l…
It is known that a macroscopic quantum superposition (MQS), when it is exposed to environment, decoheres at a rate scaling with the separation of its component states in phase space. This is more or less consistent with the well known proposition that a more macroscopic quantum state is reduced more quickly to a classical state in general. Effects of initial mixedness, however, on the subsequent decoherence of MQSs have been less known. In this paper, we study the evolution of a highly mixed MQS interacting with an environment, and compare it with that of a pure MQS having the same size of the…
A minimal energy quantum superposition of two maximally distinguishable, isoenergetic single mode Gaussian states is used to construct the system-environment representation of a class of linear bosonic quantum channels acting on a single bosonic mode. The quantum channels are further defined by unitary dynamics of the system and environment corresponding to either a passive linear optical element $U_{\text{BS}}$ or two-mode squeezing $U_{\text{TM}}$. The notion of nonclassicality distance is used to show that the initial environment superposition state becomes maximally nonclassical as the con…
The availability of Bose-Einstein condensates as mesoscopic or macroscopic quantum objects has aroused new interest in the possiblity of making and detecting coherent superpositions involving many atoms. In this article we show that it may be possible to generate such a superposition state in a reasonably short time using Feshbach resonances to tune the inter-atomic interactions in a double-well condensate. We also consider the important problem of distinguishing whether a coherent superposition or a statistical mixture is generated by a given experimental procedure. We find that unambiguously…
The transition from quantum to classical, in the case of a quantum harmonic oscillator, is typically identified with the transition from a quantum superposition of macroscopically distinguishable states, such as the Schrödinger cat state, into the corresponding statistical mixture. This transition is commonly characterized by the asymptotic loss of the interference term in the Wigner representation of the cat state. In this paper we show that the quantum to classical transition has different dynamical features depending on the measure for nonclassicality used. Measures based on an operatorial …
We present a detailed report on the decoherence of quantum states of continuous variable systems under the action of a quantum optical master equation resulting from the interaction with general Gaussian uncorrelated environments. The rate of decoherence is quantified by relating it to the decay rates of various, complementary measures of the quantum nature of a state, such as the purity, some nonclassicality indicators in phase space and, for two-mode states, entanglement measures and total correlations between the modes. Different sets of physically relevant initial configurations are consid…
Conventional Glauber coherent states (CS) can be defined in several equivalent ways, e.g., by displacing the vacuum or, explicitly, by their infinite Poissonian expansion in Fock states. It is well known that these definitions become inequivalent if applied to finite $d$-level systems (qudits). We present a comparative Wigner-function description of the qudit CS defined (i) by the action of the truncated displacement operator on the vacuum and (ii) by the Poissonian expansion in Fock states of the Glauber CS truncated at $(d-1)$-photon Fock state. These states can be generated from a classical…
We present controllable generation of various kinds of highly nonclassical states of light, including the single photon state and superposition states of mesoscopically distinct components. The high nonclassicality of the generated states is measured by the negativity of the Wigner function, which is largest ever observed to our knowledge. Our scheme is based on photon subtraction from a nearly pure squeezed vacuum, generated from an optical parametric oscillator with a periodically-poled KTiOPO$_4$ crystal as a nonlinear medium. This is an important step to realize basic elements of universal…
We consider fundamental limits on the detectable size of macroscopic quantum superpositions. We argue that a full quantum mechanical treatment of system plus measurement device is required, and that a (classical) reference frame for phase or direction needs to be established to certify the quantum state. When taking the size of such a classical reference frame into account, we show that to reliably distinguish a quantum superposition state from an incoherent mixture requires a measurement device that is quadratically bigger than the superposition state. Whereas for moderate system sizes such a…
We study characteristics of superpositions and entanglement of thermal states at high temperatures and discuss their applications to quantum information processing. We introduce thermal-state qubits and thermal-Bell states, which are a generalization of pure-state qubits and Bell states to thermal mixtures. A scheme is then presented to discriminate between the four thermal-Bell states without photon number resolving detection but with Kerr nonlinear interactions and two single-photon detectors. This enables one to perform quantum teleportation and gate operations for quantum computation with …
We study a class of quantum measurement models. A microscopic object is entangled with a macroscopic pointer such that a distinct pointer position is tied to each eigenvalue of the measured object observable. Those different pointer positions mutually decohere under the influence of an environment. Overcoming limitations of previous approaches we (i) cope with initial correlations between pointer and environment by considering them initially in a metastable local thermal equilibrium, (ii) allow for object-pointer entanglement and environment-induced decoherence of distinct pointer readouts to …
The heart of the measurement puzzle, namely the problem of definite outcomes, remains unresolved. This paper shows that Josef Jauch's 1968 reduced density operator approach is the solution, even though many question it: The entangled "Measurement State" implies local mixtures of definite but indeterminate eigenvalues even though the MS continues evolving unitarily. A second, independent, argument based on the quantum's nonlocal entanglement with its measuring apparatus shows that the outcomes must be definite eigenvalues because of relativity's ban on instant signaling. Experiments with entang…
We consider macroscopic, mesoscopic and "S-scopic" quantum superpositions of eigenstates of an observable, and develop some signatures for their existence. We define the extent, or size $S$ of a superposition, with respect to an observable \hat{x}, as being the range of outcomes of \hat{x} predicted by that superposition. Such superpositions are referred to as generalized $S$-scopic superpositions to distinguish them from the extreme superpositions that superpose only the two states that have a difference $S$ in their prediction for the observable. We also consider generalized $S$-scopic super…
We experimentally demonstrate storage and on-demand release of phase-sensitive, photon-number superposition states of the form $α|0\rangle + βe^{iθ} |1\rangle$ for an optical quantized oscillator mode. For this purpose, we introduce a phase-probing mechanism to a storage system composed of two concatenated optical cavities, which was previously employed for storage of phase-insensitive single-photon states [Phys. Rev. X 3, 041028 (2013)]. This is the first demonstration of all-optically storing highly nonclassical and phase-sensitive quantum states of light. The strong nonclassicality of the s…
In finite probability theory, events are subsets of the outcome set. Subsets can be represented by 1-dimensional column vectors. By extending the representation of events to two dimensional matrices, we can introduce "superposition events." Probabilities are introduced for classical events, superposition events, and their mixtures by using density matrices. Then probabilities for experiments or `measurements' of all these events can be determined in a manner exactly like in quantum mechanics (QM) using density matrices. Moreover the transformation of the density matrices induced by the experim…
Construction of an optical quantum computer (OQC) is finished by implementing all necessary ingredients with light (photon). There is, however, one more hurdle to clear. It is scalability, which is easily lost when accommodating many qubits by densely nesting quantum circuits. Any of the reported OQC schemes is not neces-sarily best placed in this regard. Here we demonstrate the power of "frequency" de-gree of freedom of light, which outperforms others with its potentially infinite basis states: as multiple qubits share the same "one-photon" superposition state all along, a realistic OQC desig…
We study a class of quantum measurement models. A microscopic object is entangled with a macroscopic pointer such that each eigenvalue of the measured object observable is tied up with a specific pointer deflection. Different pointer positions mutually decohere under the influence of a bath. Object-pointer entanglement and decoherence of distinct pointer readouts proceed simultaneously. Mixtures of macroscopically distinct object-pointer states may then arise without intervening macroscopic superpositions. Initially, object and apparatus are statistically independent while the latter has point…
The ability to generate light in a pure quantum state is essential for advances in optical quantum technologies. However, obtaining quantum states with control in the photon-number has remained elusive. Optical light fields with zero and one photon can be produced by single atoms, but so far it has been limited to generating incoherent mixtures, or coherent superpositions with a very small one-photon term. Here, we report on the on-demand generation of quantum superpositions of zero, one, and even two photons, via pulsed coherent control of a single artificial atom. Driving the system up to fu…
