A recently developed scheme [S. Scheel, L. Knoll, and D.-G. Welsch, Phys. Rev. A 58, 700 (1998)] for quantizing the macroscopic electromagnetic field in linear dispersive and absorbing dielectrics satisfying the Kramers-Kronig relations is used to derive the quantum local-field correction for the standard virtual-sphere-cavity model. The electric and magnetic local-field operators are shown to be consistent with QED only if the polarization noise is fully taken into account. It is shown that the polarization fluctuations in the local field can dramatically change the spontaneous decay rate, compared with the familiar result obtained from the classical local-field correction. In particular, the spontaneous emission rate strongly depends on the radius of the local-field virtual cavity.
We present a quantum error correcting code that is invariant under the conditional time evolution between spontaneous emissions and which can correct for one general error. The code presented here generalizes previous error correction codes in that not all errors lead to different error syndromes. This idea may lead to shorter codes than previously expected.
We derive dissipative effective Hamiltonian for the unstable Lee model without any ad hoc coarse graining procedure. Generalized radiative corrections, utilizing the in-in formalism of quantum field theory, automatically yield irreversibility as well as the decay of quantum coherence. Especially we do not need to extend the ordinary Hilbert space for describing the intrinsically dissipative system if we use the generalized in-in formalism of quantum field theory.
For a moving atom, the spontaneous emission rate is modified due to the contributions from two factors, the Röntgen interaction term and the recoil effect induced by the emitted photon. Here we investigate the emission rate of a uniformly moving atom near a perfectly conducting plate and obtain the corrections induced by these two factors. We find that the corrections individually induced by the Röntgen term and the recoil effect can be simply added and result in the total correction to the decay rate. Moreover, it is shown that the Röntgen term gives positive correction, while the recoil effe…
The spontaneous emission of an excited two-level emitter driven by a strong classical coherent low-frequency electromagnetic field is investigated. We find that for relatively strong laser driving, multi-photon processes are induced, thereby opening additional decay channels for the atom. We analyze the interplay between the strong low-frequency driving and the interfering multiphoton decay channels, and discuss its implications for the spontaneous emission dynamics.
Using the Born expansion of the Green tensor, we consider the spontaneous decay rate of an excited atom placed in the vicinity of a rectangular plate. We discuss the limitations of the commonly used simplifying assumption that the plate extends to infinity in the lateral directions and examine the effects of the atomic dipole moment orientation, atomic position, and plate boundary and thickness on the atomic decay rate. In particular, it is shown that in the boundary region, the spontaneous decay rate can be strongly modified.
A numerical model of spontaneous decay continuously monitored by a distant detector of emitted particles is constructed. It is shown that there is no quantum Zeno effect in such quantum measurement if the interaction between emitted particle and detector is short-range and the mass of emitted particle is not zero.
It was shown that different mechanisms of perturbation of spontaneous decay constant: inelastic interaction of emitted particles with particle detector, decay onto an unstable level, Rabi transition from the final state of decay (electromagnetic field domination) and some others are really the special kinds of one general effect - perturbation of decay constant by dissipation of the final state of decay. Such phenomena are considered to be Zeno-like effects and general formula for perturbed decay constant is deduced.
Starting from the quantized version of Maxwell's equations for the electromagnetic field in an arbitrary linear Kramers-Kronig dielectric, spontaneous decay of the excited state of a two-level atom embedded in a dispersive and absorbing medium is studied and the decay rate is calculated. The calculations are performed for both the (Clausius-Mosotti) virtual cavity model and the (Glauber-Lewenstein) real cavity model. It is shown that owing to nonradiative decay associated with absorption the rate of spontaneous decay sensitively depends on the cavity radius when the atomic transition frequency…
We study spontaneous radiative decay of translational levels of an atom in the vicinity of a semi-infinite dielectric. We systematically derive the microscopic dynamical equations for the spontaneous decay process. We calculate analytically and numerically the radiative linewidths and the spontaneous transition rates for the translational levels. The roles of the interference between the emitted and reflected fields and of the transmission into the evanescent modes are clearly identified. Our numerical calculations for the silica--cesium interaction show that the radiative linewidths of the bo…
We investigate the nonclassicality of an open quantum system using Leggett-Garg inequality (LGI) which test the correlations of a single system measured at different times. Violation of LGI implies nonclassical behavior of the open system. We investigate the violation of the Leggett-Garg inequality for a two level system (qubit) spontaneously decaying under a general non-Markovian dissipative environment. Our results are exact as we have calculated the two-time correlation functions exactly for a wide range of system-environment parameters beyond Born-Markov regime.
We consider the spontaneous emission of a broadening molecule on the surface of a micro-sphere in this paper. The density of states for the micro-cavity is derived from quasi-normal models(QNM's) expansion of the correlation functions of electromagnetic fields. Through detailed analysis we show that only weak coupling between a broadening atom(molecule) and the electromagnetic fields exists in a dielectric sphere cavity whether the sphere is small or big. From these results we find the explicit expression of the spontaneous emission decay rate for a surfactant broadening molecule on the surfac…
Spontaneous decay of an excited atom in a waveguide is essentially modified by the spatial structure of vacuum reservoir. This is particularly exciting in view of a range of applications for quantum information science. We found out that spontaneous decay can be incomplete, so the time dependence of the excited state population asymptotically approaches to a nonzero value, under the conditions when the atomic transition frequency is larger than the cutoff frequency of a waveguide and far from the vicinities of the cut-offs. Discovered effect is explained by the emergence of the dark state, whi…
A new class of error-correcting quantum codes is introduced capable of stabilizing qubits against spontaneous decay arising from couplings to statistically independent reservoirs. These quantum codes are based on the idea of using an embedded quantum code and exploiting the classical information available about which qubit has been affected by the environment. They are immediately relevant for quantum computation and information processing using arrays of trapped ions or nuclear spins. Interesting relations between these quantum codes and basic notions of design theory are established.
The spontaneous emission is investigated for an effective atomic two-level system in an intense coherent field with frequency lower than the vacuum-induced decay width. As this additional low-frequency field is assumed to be intense, multiphoton processes may be induced, which can be seen as alternative transition pathways in addition to the simple spontaneous decay. The interplay of the various interfering transition pathways influences the decay dynamics of the two-level system and may be used to slow down the spontaneous decay considerably. We derive from first principles an expression for …
We propose a dissipative scheme to prepare a three-dimensional entangled state for two atoms trapped in separate coupled cavities. Our work shows that both atomic spontaneous emission and cavity decay, which are two typical obstacles in unitary-dynamics-based schemes, could be utilized as resources for high-dimensional entangled state preparation without specifying initial state and controlling time precisely. Final numerical simulation with one group of experimental parameters indicates that the performance of our scheme is better than the unitary-dynamics-based scheme.
We present a quantization scheme for the electromagnetic field interacting with atomic systems in the presence of dispersing and absorbing magnetodielectric media, including left-handed material having negative real part of the refractive index. The theory is applied to the spontaneous decay of a two-level atom at the center of a spherical free-space cavity surrounded by magnetodielectric matter of overlapping band-gap zones. Results for both big and small cavities are presented, and the problem of local-field corrections within the real-cavity model is addressed.
The 'disentanglement eraser' or 'entanglement restorer' scheme allows retrieving entanglement by erasing the information about the formation of a classical (or separable) state. It suggests an analogy between the pairs of properties: entangled-separable and wave-particle, the latter as described in the 'quantum eraser'. The scheme illustrates the physical importance of information in quantum systems, and it is also useful as a building block for quantum computation. An optical setup for its simple implementation using three-photon decay in a centro-symmetrical crystal is proposed.
In a previous paper [B. Deb and G. S. Agarwal, Phys. Rev. A 90, 063417 (2014)], it was theoretically shown that, magneto-optical manipulation of low energy scattering resonances and atom-molecule transitions could lead to the formation of a bound state in continuum (BIC), provided there is no spontaneous emission. We find that even an exceedingly small spontaneous decay from exited molecular states can spoil the BIC. In this paper, we show how to circumvent the detrimental effect of spontaneous emission by making use of vacuum-induced coherence (VIC) which results in the cancellation or suppre…
After giving a summary of the basic-theoretical concept of quantization of the electromagnetic field in the presence of dispersing and absorbing (macroscopic) bodies, their effect on spontaneous decay of an excited atom is studied. Various configurations such as bulk material, planar half space media, spherical cavities, and microspheres are considered. In particular, the influence of material absorption on the local-field correction, the decay rate, the line shift, and the emission pattern are examined. Further, the interplay between radiative losses and losses due to material absorption is a…
The influence of the size and shape of a dispersing and absorbing dielectric body on the local-field corrected spontaneous-decay of an excited atom embedded in the body is studied on the basis of the real-cavity model. By means of a Born expansion of the Green tensor of the system it is shown that to linear order in the susceptibility of the body the decay rate exactly follows Tomas's formula found for the special case of an atom at the center of a homogeneous dielectric sphere [Phys. Rev. A 63, 053811 (2001)]. It is further shown that for an atom situated at the interior of an arbitrary diele…
We present a formalism for studying the influence of dispersive and absorbing dielectric bodies on a radiating atom in the framework of quantization of the phenomenological Maxwell equations for given complex permittivities of the bodies. In Markov approximation, the rate of spontaneous decay and the line shift associated with it can then be related to the complex permittivities and geometries of the bodies via the dyadic Green function of the classical boundary value problem of electrodynamics -- a result which is in agreement with second-order calculations for microscopic model systems. The …
We investigate the question whether Michelson type interferometry is possible if the role of the beam splitter is played by a spontaneous process. This question arises from an inspection of trajectories of atoms bouncing inelastically from an evanescent-wave (EW) mirror. Each final velocity can be reached via two possible paths, with a {\it spontaneous} Raman transition occurring either during the ingoing or the outgoing part of the trajectory. At first sight, one might expect that the spontaneous character of the Raman transfer would destroy the coherence and thus the interference. We investi…
We study spontaneous emission from an atom under the action of laser fields. We consider two different energy level diagrams. The first one consists of two levels resonantly driven by laser radiation where either of levels may decay to a separate level. For such a system we show that the presence of the second decay channel may deteriorate the destructive interference occurring in case of one decay channel because of Autler-Townes effect. The second diagram represents two two-level resonantly driven systems with the upper levels decaying to a common level. For this diagram we show that there i…
Within the framework of macroscopic quantum electrodynamics, the resonant van der Waals potential experienced by an excited two-level atom near a planar magneto-electric two-layer system consisting of a slab of left-handed material and a perfect mirror is studied. It is shown that disregarding of material absorption leads to unphysical results, with divergent values for the potential away from the surface. Under appropriate conditions, the setup is found to feature a barrier near the surface which can be employed to levitate particles or used as a trapping or cooling mechanism. Finally, the pr…
In a recent article [Phys. Rev. A 94, 052128 (2016)], the authors compute the predictions of two collapse models on the transition probabilities of neutral mesons. Notably, they claim to find an influence on the decay rates and attempt to prove that a new parameter $θ(0)$ is required to fully characterize the noise of standard collapse models. These two claims are incorrect and motivated by flawed computations. This comment derives the correct transition probabilities exactly from the master equation, explains how they could be computed perturbatively in a safe way and finally shows where the …
Tanabe et al (Phys. Rev. A {\bf 82} 040101(R) 2010) have experimentally demonstrated that the emission properties of unstable atoms in entangled and product states are different. The authors define an apparent decay time as a fitting parameter which falls below the lifetime of the single atom for entangled pairs. We argue that their results about coincidence time spectra are correct, but those concerning lifetimes cannot be considered conclusive because they assume the emission of photons by the two atoms to be independent processes, a doubtful hypothesis for entangled states. We suggest an im…
A formalism for studying spontaneous decay of an excited two-level atom in the presence of dispersing and absorbing dielectric bodies is developed. An integral equation, which is suitable for numerical solution, is derived for the atomic upper-state-probability amplitude. The emission pattern and the power spectrum of the emitted light are expressed in terms of the Green tensor of the dielectric-matter formation including absorption and dispersion. The theory is applied to the spontaneous decay of an excited atom at the center of a three-layered spherical cavity, with the cavity wall being mod…
We consider a complete study of the influence of the cavity size on the spontaneous decay of an atom excited state, roughly approximated by a harmonic oscillator. We confine the oscillator-field system in a spherical cavity of radius $R$, perfectly reflective, and work in the formalism of dressed coordinates and states, which allows to perform non-perturbative calculations for the probability of the atom to decay spontaneously from the first excited state to the ground state. In free space, $R\to\infty$, we obtain known exact results an for sufficiently small $R$ we have developed a power expa…
The electromagnetic field inside an isotropic optically active medium is quantized on the base of Fedorov's model for optical activity. The modified photon propagator is derived. Using this result it is shown that the QED correction to the electron mass contains chiral terms which nevertheless are parity invariant. The spontaneous emission rate of a two-level atom is shown to increase in the medium. The spontaneously emitted radiation is partially polarized.
We present a new method to measure the guided, radiated and total decay rates in one-dimensional waveguides. It is also theoretically shown that large modifications of the total decay rate can be achieved in realistic EDFAs and EDWAs with effective mode area radii smaller than ~ 1 micrometer.
In this paper we extend current perspectives in engineering reservoirs by producing a time-dependent master equation leading to a nonstationary superposition equilibrium state that can be nonadiabatically controlled by the system-reservoir parameters. Working with an ion trapped inside a nonindeal cavity we first engineer effective Hamiltonians that couple the electronic states of the ion with the cavity mode. Subsequently, two classes of decoherence-free evolution of the superposition of the ground and decaying excited levels are achieved: those with time-dependent azimuthal or polar angle. A…
On the basis of general theoretical results developed previously in [I. M. Sokolov et al., J. Exp. Theor. Phys. 112, 246 (2011)], we analyze spontaneous decay of a single atom inside cold atomic clouds under conditions when the averaged interatomic separation is less or comparable with the wavelength of quasi resonant radiation. Beyond the decay dynamics we analyze shifts of resonance as well as distortion of the spectral shape of the atomic transition.
In this paper we discuss the use of the transition operator method for the theoretical description of a multi-qubit system in a one-dimensional waveguide. A general calculation has been performed for the N-qubit system, which was then applied to the case of spontaneous decay for one and two qubits. The probabilities of transitions in such systems, as well as the emission spectra, are investigated in detail.
We propose a linear optics scheme with SPDC process to test the fault tolerance property of quantum error correction code. To transmit an unknown qubit robustly through the noisy channel, one may first encode it into a certain quantum error correction code and then transmit it. The remote party decodes it and stores it. Sending a qubit in such a way can significantly reduces the error rate compared with directly sending the qubit itself. Here we show how to realize such a scheme by linear optics.
We investigate the time evolution of atomic population in a two-level atom driven by a monochromatic radiation field, taking spontaneous emission into account. The Rabi oscillation exhibits amplitude damping in time caused by spontaneous emission. We show that the semiclassical master equation leads in general to an overestimation of the damping rate and that a correct quantitative description of the damped Rabi oscillation can thus be obtained only with a full quantum mechanical theory.
Dynamical reduction models propose a solution to the measurement problem in quantum mechanics: the collapse of the wave function becomes a physical process. We compute the predictions to decaying and Dynamical reduction models propose a solution to the measurement problem in quantum mechanics: the collapse of the wave function becomes a physical process. We compute the predictions to decaying and flavor--oscillating neutral mesons for the two most promising collapse models, the QMUPL (Quantum Mechanics with Universal Position Localization) model and the mass-proportional CSL (Continuous Sponta…
On the basis of the general quantum microscopic theory we study the process of spontaneous decay of an excited atom in a dense and disordered ensemble of point-like impurity atoms embedded into transparent dielectric and located near a charged perfectly conducting surface. We have analyzed the simultaneous influence of the modified spatial structure of field modes near the conductive surface and the electric field on the character of interatomic dipoledipole interaction. This leads to the modification of the transition spectrum of an excited atom inside an ensemble and the spontaneous decay dy…
In this work, we consider atomic spontaneous emission in a system consisting of two identical two-level atoms interacting dispersively with the quantized electromagnetic field in a high-Q cavity. We investigate the destructive effect of the atomic decay on the generation of maximally entangled states, following the proposal by Zheng S B and Guo G C (2000 Phys. Rev. Lett. 85 2392). In particular, we analyze the fidelity of teleportation performed using such a noisy channel and calculatethe maximum spontaneous decay rate we may have in order to realize teleportation.
We have theoretically studied the effect of deterministic temporal control of spontaneous emission in a dynamic optical microcavity. We propose a new paradigm in light emission: we envision an ensemble of two-level emitters in an environment where the local density of optical states is modified on a time scale shorter than the decay time. A rate equation model is developed for the excited state population of two-level emitters in a time-dependent environment in the weak coupling regime in quantum electrodynamics. As a realistic experimental system, we consider emitters in a semiconductor micro…
Spontaneous emission by an excited fermionic atom can be suppressed due to the Pauli exclusion principle if the relevant final states after the decay are already occupied by identical atoms in the ground state. Here we discuss a setup where a single atom is prepared in the first excited state on a single site of an optical lattice under conditions of very tight trapping. We investigate these phenomena in the context of two experimental realizations: (1) with alkali atoms, where the decay rate of the excited state is large and (2) with alkaline earth-like atoms, where the decay rate from metast…
The matrix elements of operators transforming as irreducible representations of an unbroken symmetry group $G$ are governed by the well-known Wigner-Eckart relations. In the case of infinitely-extended systems, with $G$ spontaneously broken, we prove that the corrections to such relations are provided by symmetry breaking Ward identities, and simply reduce to a tadpole term involving Goldstone bosons. The analysis extends to the case in which an explicit symmetry breaking term is present in the Hamiltonian, with the tadpole term now involving pseudo Goldstone bosons. An explicit example is dis…
The local field correction to the spontanous dacay rate of an impurity source atom imbedded in a disordered dielectric is calculated to second order in the dielectric density. The result is found to differ from predictions associated with both "virtual" and "real" cavity models of this decay process. However, if the contributions from two dielectric atoms at the same position are included, the virtual cavity result is reproduced.
Spontaneous emission of a two--level atom in free space is modified by other atoms in its vicinity leading to super- and sub-radiance. In particular, for atomic distances closer than the transition wavelength the maximally entangled antisymmetric superposition state of two individually excited atomic dipole moments possesses no total dipole moment and will not decay spontaneously at all. Such a two-atom dark state does not exist, if the atoms possess alternative decay channels towards other atomic lower energy states. However, we show here that for any atomic state with $N-1$ independent spont…
We propose a very simple scheme to slow down the usual exponential decay of upper state population in an atomic two level system considerably. The scheme makes use of an additional intense field with frequency lower than the total decay width of the atomic transition. This allows for additional decay channels with the exchange of one or more low-frequency photons during an atomic transition. The various channels may then interfere with each other. The intensity and the frequency of the low-frequency field are shown to act as two different control parameters modifying the duration and the amoun…
In contrast to the traditional Spontaneous Generated Coherence (SGC), Field Generated Coherence (FGC)-based atomic scheme is presented for spontaneous emission cancellation. It is easy to achieve externally controllable experimental trapping condition in this 4-field-driven 5-level atomic system. Consequently, due to the FGC the decay from the central dressed \emph{bare-energy-state} of the set of upper three closely spaced hyperfine decaying states of Sodium D2 line is completely cancelled under the trapping condition, exhibiting a novel phenomenon of a \textit{dark bare-energy-state}% . Exte…
We study a two-level model coupled to the electromagnetic vacuum and to an external classic electric field with fixed frequency. The amplitude of the external electric field is supposed to vary very slow in time. Garrison and Wright [{\it Phys. Lett.} {\bf A128} (1988) 177] used the non-hermitian Hamiltonian approach to study the adiabatic limit of this model and obtained that the probability of this two-level system to be in its upper level has an imaginary geometric phase. Using the master equation for describing the time evolution of the two-level system we obtain that the imaginary phase d…
We consider a one-dimensional chain of N equidistantly spaced noninteracting qubits embedded in an open waveguide. In the frame of single-excitation subspace, we systematically study the evolution of qubits amplitudes if the only qubit in the chain was initially excited. We show that the temporal dynamics of qubits amplitudes crucially depend on the value of kd, where k is the wave vector, d is a distance between neighbor qubits. If kd is equal to an integer multiple of $π$, then the qubits are excited to a stationary level which scales as SN^{-1}S. We show that in this case, it is the dark st…
Spontaneous decay of an excited atomic state is a fundamental process that originates from the interaction between matter and vacuum modes of the electromagnetic field. The rate of decay can thus be engineered by modifying the density of final states of the joint atom-photon system. Imposing suitable boundary conditions on the electromagnetic field has been shown to alter the density of vacuum modes near the atomic transition, resulting in modified atomic decay rates. Here we report the first experimental demonstration of suppression of atomic radiative decay by reducing the density of availab…
We introduce a photonic nanostructure made of two dimensional materials that can lead to non-Markovian dynamics in the spontaneous emission of a nearby quantum emitter. Specifically, we investigate the spontaneous emission dynamics of a two-level quantum emitter with picosecond free-space decay time, modelling J-aggregates, close to a MoS$_2$ nanodisk. Reversible population dynamics in the quantum emitter is obtained when the emitter's frequency matches the frequency of an exciton-polariton resonance created by the nanodisk. When such isolated resonances exist, decaying Rabi oscillations may o…
Radiative corrections to an atom are calculated near a half-space that has arbitrarily-shaped small depositions upon its surface. The method is based on calculation of the classical Green's function of the macroscopic Maxwell equations near an arbitrarily perturbed half-space using a Born series expansion about the bare half-space Green's function. The formalism of macroscopic quantum electrodynamics is used to carry this over into the quantum picture. The broad utility of the calculated Green's function is demonstrated by using it to calculate two quantities --- the spontaneous decay rate of …
Spontaneous collapse models aim to resolve the measurement problem in quantum mechanics by considering wave-function collapse as a physical process. We analyze how these models affect a decaying flavor-oscillating system whose evolution is governed by a phenomenological non-Hermitian Hamiltonian. In turn, we apply two popular collapse models, the Quantum Mechanics with Universal Position Localization and the Continuous Spontaneous Localization models, to a neutral meson system. By using the equivalence between the approaches to the time evolution of decaying systems with a non-Hermitian Hamilt…
The dynamics of an electronic two-level system coupled to an electromagnetic field are simulated explicitly for one and three dimensional systems through semiclassical propagation of the Maxwell-Liouville equations. We consider three flavors of mixed quantum-classical dynamics: the classical path approximation (CPA), Ehrenfest dynamics, and symmetrical quantum-classical (SQC) dynamics. The CPA fails to recover a consistent description of spontaneous emission. A consistent "spontaneous" emission can be obtained from Ehrenfest dynamics--provided that one starts in an electronic superposition sta…
In the framework of Bohmian quantum mechanics supplemented with the Chetaev theorem on stable trajectories in dynamics in the presence of dissipative forces we have shown the possibility of the classical (without tunneling) universal description of radioactive decay of heavy nuclei, in which under certain conditions so called noise-induced transition is generated or, in other words, the stochastic channel of alpha decay, cluster radioactivity and spontaneous fission conditioned by the Kramers diffusion mechanism. Based on the ENSDF database we have found the parametrized solutions of the Krame…
