We study spontaneous radiative decay of translational levels of an atom in the vicinity of a semi-infinite dielectric. We systematically derive the microscopic dynamical equations for the spontaneous decay process. We calculate analytically and numerically the radiative linewidths and the spontaneous transition rates for the translational levels. The roles of the interference between the emitted and reflected fields and of the transmission into the evanescent modes are clearly identified. Our numerical calculations for the silica--cesium interaction show that the radiative linewidths of the bound excited levels with large enough but not too large vibrational quantum numbers are moderately enhanced by the emission into the evanescent modes and those for the deep bound levels are substantially reduced by the surface-induced red shift of the transition frequency.
We study the interaction of dielectric rods and disks with the laser field of a high finesse cavity. The quantum master equation for the coupled particle-cavity dynamics, including Rayleigh scattering, is derived for particle sizes comparable to the laser wavelength. We demonstrate that such anisotropic nanoparticles can be captured from free flight at velocities higher than those required to capture dielectric spheres of the same volume, and that efficient ro-translational cavity cooling into the deep quantum regime is achievable.
The local-field renormalization of the spontaneous emission rate in a dielectric is explicitly obtained from a fully microscopic quantum-electrodynamical, many-body derivation of Langevin-Bloch operator equations for two-level atoms embedded in an absorptive and dispersive, linear dielectric host. We find that the dielectric local-field enhancement of the spontaneous emission rate is smaller than indicated by previous studies.
Starting from the quantized version of Maxwell's equations for the electromagnetic field in an arbitrary linear Kramers-Kronig dielectric, spontaneous decay of the excited state of a two-level atom embedded in a dispersive and absorbing medium is studied and the decay rate is calculated. The calculations are performed for both the (Clausius-Mosotti) virtual cavity model and the (Glauber-Lewenstein) real cavity model. It is shown that owing to nonradiative decay associated with absorption the rate of spontaneous decay sensitively depends on the cavity radius when the atomic transition frequency…
We present a formalism for studying the influence of dispersive and absorbing dielectric bodies on a radiating atom in the framework of quantization of the phenomenological Maxwell equations for given complex permittivities of the bodies. In Markov approximation, the rate of spontaneous decay and the line shift associated with it can then be related to the complex permittivities and geometries of the bodies via the dyadic Green function of the classical boundary value problem of electrodynamics -- a result which is in agreement with second-order calculations for microscopic model systems. The …
Spontaneous emission and Lamb shift of atoms in absorbing dielectrics are discussed. A Green's-function approach is used based on the multipolar interaction Hamiltonian of a collection of atomic dipoles with the quantised radiation field. The rate of decay and level shifts are determined by the retarded Green's-function of the interacting electric displacement field, which is calculated from a Dyson equation describing multiple scattering. The positions of the atomic dipoles forming the dielectrics are assumed to be uncorrelated and a continuum approximation is used. The associated unphysical …
We demonstrate how exactly bound cavity modes can be realized in dielectric structures other than 3d photonic crystals. For a microcavity consisting of crossed anisotropic layers, we derive the cavity resonance frequencies, and spontaneous emission rates. For a dielectric structure with dissipative loss and central layer with gain, the beta factor of direct spontaneous emission into a cavity mode and the laser threshold is calculated.
We propose a laser cooling concept for the translational motion of molecules which does not require repeated spontaneous emission by each molecule. The cooling works by repetition of three main steps: velocity selection of a narrow momentum width, deceleration of velocity selected molecules and accumulation of the decelerated molecules by an irreversible process, namely by single spontaneous emission. We develop a cooling model which enables analytical description of the transient populations and entropies for the total molecular system, the center of mass degree of freedom and the internal de…
The local field correction to the spontanous dacay rate of an impurity source atom imbedded in a disordered dielectric is calculated to second order in the dielectric density. The result is found to differ from predictions associated with both "virtual" and "real" cavity models of this decay process. However, if the contributions from two dielectric atoms at the same position are included, the virtual cavity result is reproduced.
We investigate spontaneous emission of a two-level atom with an arbitrarily polarized electric dipole in front of a flat dielectric surface. We treat the general case where the atomic dipole matrix element is a complex vector, that is, the atomic dipole can rotate with time in space. We calculate the rates of spontaneous emission into evanescent and radiation modes and study the angular densities of the rates in the space of wave vectors for the field modes. We show that, when the ellipticity of the atomic dipole is not zero, the angular density of the spontaneous emission rate of the atom may…
Spontaneous down conversion in metal-dielectric interface in case of oblique laser excitation is considered. In this case it is possible to generate pairs of polarization entangled surface plasmon polaritons with high efficiency if to use excitation angle corresponding to the Kretschmann configuration for generated plasmons. The efficiency can be additionally enlarged if to use properly nanostructured metallic film allowing one to directly excite surface plasmon polaritons and to fulfill phase matching condition of them with generated surface plasmon polaritons.
The spontaneous emission rate of a radiating atom reaches its time-independent equilibrium value after an initial transient regime. In this paper we consider the associated relaxation effects of the spontaneous decay rate of atoms in dispersive and absorbing dielectric media for atomic transition frequencies near material resonances. A quantum mechanical description of such media is furnished by a damped-polariton model, in which absorption is taken into account through coupling to a bath. We show how all field and matter operators in this theory can be expressed in terms of the bath operators…
The influence of the size and shape of a dispersing and absorbing dielectric body on the local-field corrected spontaneous-decay of an excited atom embedded in the body is studied on the basis of the real-cavity model. By means of a Born expansion of the Green tensor of the system it is shown that to linear order in the susceptibility of the body the decay rate exactly follows Tomas's formula found for the special case of an atom at the center of a homogeneous dielectric sphere [Phys. Rev. A 63, 053811 (2001)]. It is further shown that for an atom situated at the interior of an arbitrary diele…
We devise new optical antennas that reduce the excited-state radiative lifetimes of emitters to the order of 100 femtoseconds while maintaining quantum efficiencies of about 80% at a broadband operation. Here, we combine metallic nanoparticles with planar dielectric structures and exploit design strategies from plasmonic nanoantennas and concepts from Cavity Quantum Electrodynamics to maximize the local density of states and minimize the nonradiative losses incurred by the metallic constituents. The proposed metallo-dielectric hybrid antennas promise important impact on various fundamental and…
A formalism for studying spontaneous decay of an excited two-level atom in the presence of dispersing and absorbing dielectric bodies is developed. An integral equation, which is suitable for numerical solution, is derived for the atomic upper-state-probability amplitude. The emission pattern and the power spectrum of the emitted light are expressed in terms of the Green tensor of the dielectric-matter formation including absorption and dispersion. The theory is applied to the spontaneous decay of an excited atom at the center of a three-layered spherical cavity, with the cavity wall being mod…
We study from a critical perspective several quantum-electrodynamic phenomena commonly related to vacuum electromagnetic (EM) fluctuations in complex media. We compute the resonance-shift, the spontaneous emission rate, the local density of states and the van-der-Waals-Casimir pressure in a dielectric medium using a microscopic diagrammatic approach. We find, in agreement with some recent works, that these effects cannot be attributed to variations on the energy of the EM vacuum but to variations of the dielectric self-energy. This energy is the result of the interaction of the bare polarizabi…
The emission properties of atoms lie at the foundations of both quantum theory and light-matter interactions. In the context of macroscopic media, exact knowledge thereof is important both in current quantum technologies as well as in fundamental studies. While for isotropic media, this is a very well-studied problem, there are still big gaps in the theory of anisotropic media. In particular, to the best of our knowledge, an explicit expression for the spontaneous emission rate in general anisotropic media has not been presented. In this work, we first derive the quantised electromagnetic fiel…
An atom recoils when it undergoes spontaneous decay. In this paper we present a microscopic calculation of the recoil of a source atom imbedded in a dielectric medium. We find that the source atom recoils with the canonical photon momentum $n\hbar k_{0,}$ where $n$ is the index of refraction and $\hbar k_{0}$ is the photon momentum calculated at the source atom atomic frequency $ω_{0}$. We also show explicitly how the energy is conserved with the photon inside the medium.
A recently developed scheme [S. Scheel, L. Knoll, and D.-G. Welsch, Phys. Rev. A 58, 700 (1998)] for quantizing the macroscopic electromagnetic field in linear dispersive and absorbing dielectrics satisfying the Kramers-Kronig relations is used to derive the quantum local-field correction for the standard virtual-sphere-cavity model. The electric and magnetic local-field operators are shown to be consistent with QED only if the polarization noise is fully taken into account. It is shown that the polarization fluctuations in the local field can dramatically change the spontaneous decay rate, co…
Acoustic spontaneous emission into bulk dielectrics can be a strong source of decoherence in quantum devices, especially when a qubit is in the presence of piezoelectric materials. We study the dynamics of a qubit coupled to an acoustic resonator by a piezoelectric film. By varying the surface topography of the resonator from rough to polished to shaped, we explore the crossover from fast decay of an excited qubit to quantum-coherent coupling between the qubit and an isolated phonon mode. Our experimental approach may be used for precision measurements of crystalline vibrations, the design of …
Quantum mechanical treatment of light inside dielectric media is important to understand the behavior of an optical system. In this paper, a two-level atom embedded in a rectangular waveguide surrounded by a perfect electric conductor is considered. Spontaneous emission, propagation, and detection of a photon are described by the second quantization formalism. The quantized modes for light are divided into two types: photonic propagating modes and localized modes with exponential decay along the direction of waveguide. Though spontaneous emission depends on all possible modes including the loc…
Within the frame of quantum optics we analyze the properties of spontaneous emission of two-level atom in media with indefinite permittivity tensor where the geometry of the dispersion relation is characterized by an ellipsoid or a hyperboloid(hyperbolic medium). The decay rate is explicitly given with the orientation of the dipole transition matrix element taken into account. It indicates that for the ellipsoid case the intensity of the photons coupled into different modes can be tuned by changing the direction of the matrix element and for the hyperboloid case it is found that spontaneous em…
A non-perturbative theory of the spontaneous down conversion (SDC) of surface plasmon polaritons at a metal-dielectric interface is presented. It is shown that the process is resonantly enhanced for the characteristic power of excitation, typically of the order of tens of watts. At a stronger excitation the yield of SDC decreases rapidly. At a stronger excitation the yield of SDC decreases rapidly. The reason for this decrease is the high rate of the change of surface plasmon polaritons by the laser field, exceeding the rate of the zero-point fluctuations responsible for the SDC process. The o…
General physical conditions for the occurrence of photonic Klein tunneling are studied, where (controlled) spontaneous emission from the devices considered plays a key role. The specific example of a simple dielectric slab bounded by two dielectric half spaces with arbitrary refractive indices is worked out quite in detail, the measured reflection and transmission probabilities being calculated analytically. It is found that, in given cases, the measured reflection probability may be arbitrarily large (for large incident wavelengths) irrespective of the fact that the transmission probability i…
We build up a consistent theory of quantum electrodynamics in the presence of macroscopic polarizable media. We use the Huttner-Barnett model of a dispersive and absorbing dielectric medium and formulate the theory in terms of interacting quantum fields. We integrate out the damped polaritons by using diagrammatic techniques and find an exact expression for the displacement field (photon) propagator in the presence of a dispersive and absorbing dielectric half-space. This opens a new route to traceable perturbative calculations of the same kind as in free-space quantum electrodynamics. As a wo…
On the basis of the general quantum microscopic theory we study the process of spontaneous decay of an excited atom in a dense and disordered ensemble of point-like impurity atoms embedded into transparent dielectric and located near a charged perfectly conducting surface. We have analyzed the simultaneous influence of the modified spatial structure of field modes near the conductive surface and the electric field on the character of interatomic dipoledipole interaction. This leads to the modification of the transition spectrum of an excited atom inside an ensemble and the spontaneous decay dy…
We propose that condensed matter phenomena involving the spontaneous emergence and dynamics of crystal lattices can be realized in the setting of ultracold Bose-condensed atoms coupled to multimode cavities. Previously, it was shown that in the case of a transversely pumped single-mode cavity, the atoms self-organize at either the even or the odd antinodes of the cavity mode, given sufficient pump intensity, and hence spontaneously break a discrete translational symmetry. Here, we demonstrate that in multimode cavities the self-organization brings the additional feature of continuous translati…
The Lieb-Schultz-Mattis theorem and its higher dimensional generalizations by Oshikawa and Hastings require that translationally invariant 2D spin systems with a half-integer spin per unit cell must either have a continuum of low energy excitations, spontaneously break some symmetries, or exhibit topological order with anyonic excitations. We establish a connection between these constraints and a remarkably similar set of constraints at the surface of a 3D interacting topological insulator. This, combined with recent work on symmetry-enriched topological phases (SETs) with on-site unitary symm…
In this paper, we propose an effective model including a macroscopic Hamiltonian to describe the interactions between a two-level atom and scattered light in a 1-D dielectric waveguide. The proposed formalism allows us to incorporate the effect of changing optical media inside the continuum while demonstrating a non-classical derivation of Fresnel Law. We obtain the transport characteristics of the two-level system, explore its high-Q bandreject filter property and discuss the implications of radiative and non-radiative dissipation. In addition, we apply our formalism to a modified Fabry-Pérot…
One of the most extraordinary manifestations of the coupling of the optical field and matter is the emission of light by charged particles passing through a dielectric medium: the Vavilov-Cherenkov effect. In this article, it is theoretically predicted that a related phenomenon may be observed when neutral fast polarizable particles travel near a metal surface supporting surface plasmon polaritons. Rather dramatically, it is found that at some critical velocity, even if the initial optical field is vanishingly small, the system may become unstable and may start spontaneously emitting light suc…
