In this paper we extend current perspectives in engineering reservoirs by producing a time-dependent master equation leading to a nonstationary superposition equilibrium state that can be nonadiabatically controlled by the system-reservoir parameters. Working with an ion trapped inside a nonindeal cavity we first engineer effective Hamiltonians that couple the electronic states of the ion with the cavity mode. Subsequently, two classes of decoherence-free evolution of the superposition of the ground and decaying excited levels are achieved: those with time-dependent azimuthal or polar angle. As an application, we generalise the purpose of an earlier study [Phys. Rev. Lett. 96, 150403 (2006)], showing how to observe the geometric phases acquired by the protected nonstationary states even under a nonadiabatic evolution.
In this paper, we propose a scheme for implementing the nonadiabatic holonomic quantum computation (NHQC+) of two Rydberg atoms by using invariant-based reverse engineering (IBRE). The scheme is based on Förster resonance induced by strong dipole-dipole interaction between two Rydberg atoms, which provides a selective coupling mechanism to simply the dynamics of system. Moreover, for improving the fidelity of the scheme, the optimal control method is introduced to enhance the gate robustness against systematic errors. Numerical simulations show the scheme is robust against the random noise in …
Coherent control experiments in molecules are often done with shaped laser fields. The electric field is described classically and control over the time evolution of the system is achieved by shaping the laser pulses in the time or frequency domain. Moving on from a classical to a quantum description of the light field allows to engineer the quantum state of light to steer chemical processes. The quantum field description of the photon mode allows to manipulate the light-matter interaction directly in phase-space. In this paper we will demonstrate the basic principle of coherent control with q…
Based only on the parallel transport condition, we present a general method to compute Abelian or non-Abelian geometric phases acquired by the basis states of pure or mixed density operators, which also holds for nonadiabatic and noncyclic evolution. Two interesting features of the non-Abelian geometric phase obtained by our method stand out: i) it is a generalization of Wilczek and Zee's non-Abelian holonomy, in that it describes nonadiabatic evolution where the basis states are parallelly transported between distinct degenerate subspaces, and ii) the non-Abelian character of our geometric ph…
Experimental and theoretical evidence point out to the crucial role of specific resonant intramolecular vibrational modes in the interpretation of long-lived coherences observed in two-dimensional spectra of some natural and synthetic light harvesting complexes. For the natural situation of illumination by incoherent (sun)light, the relevance of these vibrations is analyzed here for light-harvesting vibronic prototype dimers. The detailed analysis of the density matrix dynamics reveals that the inclusion of the intramolecular vibrational modes reinforce up to one order of magnitude the exciton…
We investigate the spontaneous emission from an inverted Y-type atomic system coupled by three coherent fields. We use the Schrödinger equation to calculate the probability amplitudes of the wave function of the system and derive an analytical expression of the spontaneous emission spectrum to trace the origin of the spectral features. Quantum interference effects, such as the spectral line narrowing, spectrum splitting and dark resonance are observed. The number of spectral components, the spectral linewidth, and relative heights can be very different depending on the physical parameters. A v…
We present a proposal for realizing local decoherence-free evolution of given entangled states of two two-level (TL) ions. For two TL ions coupled to a single heavily damped cavity, we can use engineering reservoir scheme to obtain a decoherence-free subspace which can be nonadiabatically controlled by the system and reservoir parameters. Then the local decoherence-free evolution of the entangled states are achieved. And we also discuss the relation between the geometric phases and the entanglement of the two ions under the nonadiabatic coherent evolution.
Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an additional phase information, which can be retrieved by the streaking technique. In this contribution we extend the streaking formalism to include coupled electron and nuclear dynamics in molecules as well as initial coherences and demonstrate how it offers a novel tool to monitor non-adiabatic dynamics as it occurs in the vicinity of conical intersections and …
Coherent control of collective spontaneous emission in an extended atomic ensemble resonantly interacting with single-photon wave packets is analyzed. A scheme for coherent manipulation of collective atomic states is developed such that superradiant states of the atomic system can be converted into subradiant ones and vice versa. Possible applications of such a scheme for optical quantum state storage and single-photon wave packet shaping are discussed. It is shown that also in the absence of inhomogeneous broadening of the resonant line, single-photon wave packets with arbitrary pulse shape m…
In spontaneous emission an atom in an excited state undergoes a transition to the ground state and emits a single photon. Associated with the emission is a change of the atomic momentum due to photon recoil. Photon emission can be modified close to surfaces and in cavities. For an ion, localized in front of a mirror, coherence of the emitted resonance fluorescence has been reported. In free space experiments demonstrated that spontaneous emission destroys motional coherence. Here we report on motional coherence created by a single spontaneous emission event close to a mirror surface. The coher…
We investigate the entanglement dynamics of two two-level emitters (qubits) mediated by a semiinfinite, one-dimensional (1D) photonic waveguide. The coupling of each qubit to the waveguide is chiral, which depends on the propagation direction of light. The finite end of the waveguide is terminated by a perfect mirror, such that coherent quantum feedback is introduced to the system. We show that the chirally generated entanglement between the qubits can be preserved by controlling the time delay of the feedback. Moreover, when the time delay is negligible, the qubit-qubit reduced system evolves…
An optical resonator with intracavity Kerr nonlinearity can exhibit dispersive bistability suitable for all-optical switching. With nanophotonic elements it may be possible to achieve attojoule switching energies, which would be very attractive for ultra-low power operation but potentially problematic because of quantum fluctuation-induced spontaneous switching. In this manuscript I derive a quantum-optical model of two Kerr-nonlinear ring resonators connected in a coherent feedback loop, and show via numerical simulation that a properly designed `controller' cavity can significantly reduce th…
We study the spontaneous emission, the absorption and dispersion properties of a ${\bf Λ}$-type atom where one transition interacts near resonantly with a double-band photonic crystal. Assuming an isotropic dispersion relation near the band edges, we show that two distinct coherent phenomena can occur. First, the spontaneous emission spectrum of the adjacent free space transition obtains `dark lines' (zeroes in the spectrum). Second, the atom can become transparent to a probe laser field coupling to the adjacent free space transition.
A three-level atom in a $Λ$ configuration trapped in an optical cavity forms a basic unit in a number of proposed protocols for quantum information processing. Through control with an appropriate laser, this system allows for efficient storage of cavity photons into long-lived atomic excitations, and their retrieval with high fidelity. This process presumes an adiabatic transfer through the `dark state', a coherent superposition of the two lower levels of the $Λ$ system, by a slow variation of the intensity of the control laser. We study the full quantum mechanics of this transfer process with…
Laser cooling of molecules employing broadband optical pumping involves a timescale separation between laser excitation and spontaneous emission. Here, we optimize the optical pumping step using shaped laser pulses. We derive two optimization functionals to drive population into those excited state levels that have the largest spontaneous emission rates to the target state. We show that, when using optimal control, laser cooling of molecules works even if the Franck-Condon map governing the transitions is preferential to heating rather than cooling. Our optimization functional is also applicab…
We report an interference experiment of spontaneous emission of light from two distant solid-state ensembles of atoms that are coherently excited by a short laser pulse. The ensembles are Erbium ions doped into two LiNbO3 crystals with channel waveguides, which are placed in the two arms of a Mach-Zehnder interferometer. The light that is spontaneously emitted after the excitation pulse shows first-order interference. By a strong collective enhancement of the emission, the atoms behave as ideal two-level quantum systems and no which-path information is left in the atomic ensembles after emissi…
We investigate the occurrence of a phase transition, characterized by the spontaneous breaking of a discrete symmetry, in a driven-dissipative Bose-Hubbard lattice in presence of two-photon coherent driving. The driving term does not lift the original $U(1)$ symmetry completely and a discrete $\mathbb{Z}_2$ symmetry is left. When driving the bottom of the Bose-Hubbard band, a mean-field analysis of the steady state reveals a second-order transition from a symmetric phase to a quasi-coherent state with a finite expectation value of the Bose field. For larger driving frequency, the phase diagram…
We present the formulation of the problem of the coherent dynamics of quantum mechanical two-level systems in the adiabatic region in terms of the differential geometry of plane curves. We show that there is a natural plane curve corresponding to the Hamiltonian of the system for which the geometrical quantities have a simple physical interpretation. In particular, the curvature of the curve has the role of the nonadiabatic coupling.
We show lasing without population inversion in a closed four-level atomic system which is no longer incoherently pumped on the transition at which lasing occurs. The four-level system can overcome some limits in the typical lambda-type and V-type three-level systems, furthermore it is possible to achieve lasing even in the absence of the inversion condition for the thermal radiation fields or of the inversion of spontaneous decay rate. We find that when the detuning of probe field is equal to that of coherent coupling field, there is a peak value along with the increase of the detuning. To exp…
The interaction of a moving charged particle with its coherent electromagnetic field is analysed in the framework of non-relativistic quantum mechanics. It is shown that, when this interaction is taken into account, a spatially localized state may have a mean energy lower than the one corresponding to a delocalized state.
The spontaneous emission of an excited two-level emitter driven by a strong classical coherent low-frequency electromagnetic field is investigated. We find that for relatively strong laser driving, multi-photon processes are induced, thereby opening additional decay channels for the atom. We analyze the interplay between the strong low-frequency driving and the interfering multiphoton decay channels, and discuss its implications for the spontaneous emission dynamics.
As one of the central topics in quantum optics, collective spontaneous emission such as superradiance has been realized in a variety of systems. This work proposes an innovative scheme to coherently control collective emission rates via a self-interference mechanism in a nonlinear waveguide setting. The self-interference is made possible by photon backward scattering incurred by quantum scatterers in a waveguide working as quantum switches. Whether the interference is constructive or destructive is found to depend strongly on the distance between the scatterers and the emitters. The interferen…
Amplified spontaneous emission is a common noise source in active optical systems, it is generally seen as being an incoherent process. Here we excite an ensemble of rare earth ion dopants in a solid with a π-pulse, resulting in amplified spontaneous emission. The application of a second π-pulse leads to a coherent echo of the amplified spontaneous emission that is correlated in both amplitude and phase. For small optical thicknesses, we see evidence that the amplified spontaneous emission and its echo are entangled.
We propose two quantum error correction schemes which increase the maximum storage time for qubits in a system of cold trapped ions, using a minimal number of ancillary qubits. Both schemes consider only the errors introduced by the decoherence due to spontaneous emission from the upper levels of the ions. Continuous monitoring of the ion fluorescence is used in conjunction with selective coherent feedback to eliminate these errors immediately following spontaneous emission events, and the conditional time evolution between quantum jumps is removed by symmetrizing the quantum codewords.
We propose a scheme to engineer Schrödinger-cat states of propagating optical pulses. Multi-dimensional and multi-partite cat states can be generated simply by reflecting coherent optical pulses successively from a single-atom cavity. The influences of various sources of noise, including the atomic spontaneous emission and the pulse shape distortion, are characterized through detailed numerical simulation, which demonstrates practicality of this scheme within the reach of current experimental technology.
In quantum information processing, quantum cavities play an important role by providing the mechanisms to transfer information between atom qubits and photon qubits, or to couple single atoms with the optical modes of the cavity field. We explore numerically the population transfer in an atom + cavity system by using the $π$-pulse and adiabatic passage methods. While the first method is very efficient transferring the atomic population for no radiative decay of the intermediate level, the second method shows very interesting nonadiabatic, resonance-like properties that can be used to achieve v…
We discuss the spontaneous emission from a coherently prepared and microwave driven doublet of potentially closely spaced excited states to a common ground level. Multiple interference mechanisms are identified which may lead to fluorescence inhibition in well-separated regions of the spectrum or act jointly in cancelling the spontaneous emission. In addition to phase independent quantum interferences due to combined absorptions and emissions of driving field photons, we distinguish two competing phase dependent interference mechanisms as means of controlling the fluorescence. The indistinguis…
We study the light generated by spontaneous emission into a mode of a cavity QED system under weak excitation of the orthogonally polarized mode. Operating in the intermediate regime of cavity QED with comparable coherent and decoherent coupling constants, we find an enhancement of the emission into the undriven cavity mode by more than a factor of 18.5 over that expected by the solid angle subtended by the mode. A model that incorporates three atomic levels and two polarization modes quantitatively explains the observations.
We study the resonance fluorescence from a coherently driven four-level atom in the Y-type configuration. The effects of quantum interference induced by spontaneous emission on the fluorescence properties of the atom are investigated. It is found that the quantum interference resulting from cascade emission decays of the atom leads to a splitting of resonances in the excited level populations calculated as a function of light detuning. For some parameters, interference assisted enhancement of inner sidebands and narrowing of central peaks may also occur in the fluorescence spectrum. We present…
We propose the use of stimulated Raman adiabatic passage (STIRAP) to offer a fast high fidelity method of performing SU(2) rotations on spinor Bose Einstein condensates (BEC). Past demonstrations of BEC optical control suffer from difficulties arising from collective enhancement of spontaneous emission and inefficient two-photon transitions originating from selection rules. We present here a novel scheme which allows for arbitrary coherent rotations of two-component BECs while overcoming these issues. Numerical tests of the method show that for BECs of \ce{^{87}Rb} with up to $ 10^4 $ atoms an…
We propose and demonstrate a robust control scheme by ultrafast nonadiabatic chirped laser pulse, designed for targeting coherent superpositions of two-level systems. Robustness against power fluctuation is proved by our numerical study and a proof-of-principle experiment performed with femtosecond laser interaction on cold atoms. They exhibit for the final driven dynamics a cusp on the Bloch sphere, corresponding to a zero curvature of fidelity. This solution is particularly simple and thus applicable to a wide range of potential applications.
We theoretically examine photoassociation of a two-component Fermi degenerate gas, focusing on light-induced atom-atom interactions as a means to raise the critical temperature of the BCS transition to a superfluid state. As it stands, photoassociation-induced superfluidity is limited by spontaneous decay to experimentally inconvenient light intensities [Mackie et al., Opt. Express 8, 118 (2000)]. We therefore propose to use coherent control in photoassociation to a pair of molecular levels to cancel spontaneous emission, whereby the BCS transition should occur within reach of current experime…
A completely quantum description of Raman process is used to investigate the nonclassical properties of the modes in the stimulated, spontaneous and partially spontaneous Raman process. Both coherent scattering (where all the initial modes are coherent) and chaotic scattering (where initial phonon mode is chaotic and all the other modes are coherent) are studied. Nonclassical character of Raman process is observed by means of intermodal entanglement, single mode and intermodal squeezing of vacuum fluctuations, sub-shot noise and wave variances. Joint photon-phonon number and integrated-intensi…
This is the third of a series of papers devoted to develop a microscopical approach to the dipole emission process and its relation to coherent transport in random media. In this paper, we compute the power emitted by an induced dipole and the spontaneous decay rate of a Lorentzian-type dipole. In both cases, the emitter is placed at the center of a real cavity drilled in a continuous medium.
Warm rubidium vapours are known to be a versatile medium for a variety of experiments in atomic physics and quantum optics. Here we present experimental results on producing the frequency converted light for quantum applications based on spontaneous and stimulated processes in rubidium vapours. In particular, we study the efficiency of spontaneously initiated stimulated Raman scattering in the Λ-level configuration and conditions of generating the coherent blue light assisted by multi-photon transitions in the diamond-level configuration. Our results will be helpful in search for new types of …
We study coherent photoassociation, phenomena analogous to coherent optical transients in few-level systems, which may take place in photoassociation of an atomic Bose-Einstein condensate but not in a nondegenerate gas. We develop a second-quantized Hamiltonian to describe photoassociation, and apply the Hamiltonian both in the momentum representation and in the position representation (field theory). Solution of the two-mode problem including only one mode each for the atomic and molecular condensates displays analogs of Rabi oscillations and rapid adiabatic passage. A classical version of th…
