We study spontaneous emission from an atom under the action of laser fields. We consider two different energy level diagrams. The first one consists of two levels resonantly driven by laser radiation where either of levels may decay to a separate level. For such a system we show that the presence of the second decay channel may deteriorate the destructive interference occurring in case of one decay channel because of Autler-Townes effect. The second diagram represents two two-level resonantly driven systems with the upper levels decaying to a common level. For this diagram we show that there is no interference between the two decay channels when the laser fields are described in the Fock representation, while in case of definite-phase classical fields such interference takes place and is partially or completely destructive or constructive depending on the initial conditions and on the mutual orientation of the spontaneous emission dipole moments.
We proposed an analytical model to analyze the Landau-Zener interference in a multilevel superconducting flux qubit driven by large amplitude external fields. Our analytical results agree remarkably with those of the experiment [Nature 455, 51 (2008)]. Moreover, we studied the effect of driving-frequency and dephasing rate on the interference. The dephasing generally destroys the interference while increasing frequency rebuilds the interference at large dephasing rate. At certain driving frequency and dephasing rate, the interference shows some anomalous features as observed in recent experime…
We derive a master equation for a superradiant medium which includes multilevel interference betwen the individual scatterers. The derivation relies on the Born-Markov approximation and implements the coarse graining formalism. The master equation fulfils the Lindblad form and contains terms describing single-atom multilevel interference, multi-atom interference between identical transitions, and multi-atom interference between different electronic transitions with parallel dipoles. This formalism is then applied to determine the excitation spectrum of two emitters using the parameters of the …
Recent experiments on Landau-Zener interference in multilevel superconducting flux qubits revealed various interesting characteristics, which have been studied theoretically in our recent work by simply using rate equation method [PRB 79, 094529, (2009)]. In this note we extend this method to the same system but with larger driving amplitude and higher driving frequency. The results show various anomalous characteristics, some of which have been observed in a recent work.
We study the non-Markovian quantum interference phenomenon of a multi-state atomic system coupled to a bosonic dissipative environment by using the exact master equations derived in this paper. Two examples involving four-level systems with or without external control fields are investigated. Our results show that non-Markovian master equations are capable of exhibiting quantum interference phenomena in a temporal domain that has not fully explored before. In particular, we show that the environmental memory is instrumental in the onset of non-Markovian quantum interference pattern in differen…
Vacuum-induced interference in light scattering by multilevel atomic chains
University of Innsbruck（因斯布鲁克大学）；Saarland University（萨尔兰大学）；Center for Quantum Technologies (QuTe), Saarland University（萨尔兰大学量子技术中心）；Università degli Studi di Milano（米兰大学）
Our work is based on the collision-induced coherence of two decay channels along two optical transitions.The quantum interference of pumping processes creates the dark state and the more atoms are pumped in this collision-induced dark state the stronger the suppression of the spontaneous emission. The efficiency of this suppression is quantified by putting it in comparison with the spontaneous emission on the ultraviolet transition which proceeds in a regular fashion. The branching ratio of these two(visible and ultraviolet) transitions is introduced as the effective measure of the degree of t…
We show that radiative coupling between two multilevel atoms having near-degenerate states can produce new interference effects in spontaneous emission. We explicitly demonstrate this possibility by considering two identical V systems each having a pair of transition dipole matrix elements which are orthogonal to each other. We discuss in detail the origin of the new interference terms and their consequences. Such terms lead to the evolution of certain coherences and excitations which would not occur otherwise. The special choice of the orientation of the transition dipole matrix elements enab…
We study the presence of nontrivial bound states of two multilevel quantum emitters and the photons propagating in a linear waveguide. We characterize the conditions for the existence of such states and determine their general properties, focusing in particular on the entanglement between the two emitters, that increases with the number of excitations. We discuss the relevance of the results for entanglement preservation and generation by spontaneous relaxation processes.
We study the spontaneous excitation of a radially polarized static multilevel atom outside a spherically symmetric black hole in multi-polar interaction with quantum electromagnetic fluctuations in the Boulware, Unruh and Hartle-Hawking vacuum states. We find that spontaneous excitation does not occur in the Boulware vacuum, and, in contrast to the scalar field case, spontaneous emission rate is not well-behaved at the event horizon as result of the blow-up of the proper acceleration of the static atom. However, spontaneous excitation can take place both in the Unruh and the Hartle-Hawking vac…
Landau-Zener-Stuckelberg interferometry has been extensively investigated in quantum two-level systems, with particular interests on artificial system such as superconducting flux qubits. With increasing the driving field amplitude, more energy levels will be involved into the quantum evolution, which results in population inversion and many interesting interference patterns. These interference patterns can be used to obtain the parameters characterizing the system and probe dephasing mechanisms of the qubit. Most recently, experiments have been extended to the regime with higher-frequency and…
We study spontaneously generated entanglement (SGE) between two identical multilevel atoms in free space via vacuum-induced radiative coupling. We show that the SGE in two-atom systems may initially increase with time but eventually vanishes in the time scale determined by the excited state lifetime and radiative coupling strength between the two atoms. We demonstrate that a steady-state SGE can be established by incoherently pumping the excited states of the two-atom system. We have shown that an appropriate rate of incoherent pump can help producing optimal SGE. The multilevel systems offer …
We analyze the dynamics of quantum beats in a system of two V-type three-level atoms coupled to a waveguide. We show that quantum beats can be collectively enhanced or suppressed, akin to Dicke super- and sub-radiance, depending on the interatomic separation and the initial correlations between the atoms. In particular, the interference properties of the collective beats are determined by the distance between the atoms modulo the beat wavelength. We study the collective atomic and field dynamics, illustrating a crossover from a Markovian to a non-Markovian regime as the atomic separation becom…
Quantum coherence is one of the clearest departures from classical physics, exhibited when a system is in a superposition of different basis states. Here the coherent superposition of three motional Fock states of a single trapped ion is experimentally certified, with a procedure provably robust against imperfect operation. As the motional state cannot be directly interrogated, our scheme uses an interference pattern generated by projective measurement of the coupled qubit state. The minimum number of coherently superposed states is inferred from a series of threshold values based on analysis …
We theoretically discuss one-photon and two-photon double-slit interferences for spontaneous and stimulated parametric down-conversions. We show that the two-photon sub-wavelength interference can exist in a general spontaneous parametric down-conversion (SPDC) for both type I and type II crystals. We propose an alternative way to observe sub-wavelength interference by a joint-intensity measurement which occurs for only type I crystal in a higher gain of SPDC. When a signal beam injects into the crystal, it may create two interference patterns by two stimulated down-converted beams, showing no…
Recent work using spontaneous parametric down-conversion (SPDC) has made possible investigations of the Einstein-Podolsky-Rosen paradox in its original (position-momentum) form. We propose an experiment that uses SPDC photon pairs to measure through which slit a photon passes while simultaneously observing double-slit interference.
Quantum path interferences or resonances in multilevel dissipative quantum systems play an important and intriguing role in the transport processes of nanoscale systems. Many previous minimalistic models used to describe the quantum path interference driven by incoherent fields are based on the approximations including the second order perturbation for the weak coupling limit, the ad-hoc choices of two-time correlation functions and $\it{etc}$. On the other hand, the similar model to study the non-adiabatic molecular electronic excitation have been extensively developed and many efficient quan…
We implement experimentally a method to generate photon-number$-$path and polarization entangled photon pairs using ``beamlike'' type-II spontaneous parametric down-conversion (SPDC), in which the signal-idler photon pairs are emitted as two separate circular beams with small emission angles rather than as two diverging cones.
We study first-order interference in spontaneous parametric down-conversion generated by two pump pulses that do not overlap in time. The observed modulation in the angular distribution of the signal detector counting rate can only be explained in terms of a quantum mechanical description based on biphoton states. The condition for observing interference in the signal channel is shown to depend on the parameters of the idler radiation.
We discuss an experimental setup where two laser-driven atoms spontaneously emit photons and every photon causes a ``click'' at a point on a screen. By deriving the probability density for an emission into a certain direction from basic quantum mechanical principles we predict a spatial interference pattern. Similarities and differences with the classical double-slit experiment are discussed.
We demonstrate one- and two-photon diffraction and interference experiments utilizing parametric down-converted photon pairs (biphotons) and a transmission grating. With two-photon detection, the biphoton exhibits a diffraction-interference pattern equivalent to that of an effective single particle that is associated with half the wavelength of the constituent photons. With one-photon detection, however no diffraction-interference pattern is observed. We show that these phenomena originate from the spatial quantum correlation between the down-converted photons.
We study the resonance fluorescence from a coherently driven four-level atom in the Y-type configuration. The effects of quantum interference induced by spontaneous emission on the fluorescence properties of the atom are investigated. It is found that the quantum interference resulting from cascade emission decays of the atom leads to a splitting of resonances in the excited level populations calculated as a function of light detuning. For some parameters, interference assisted enhancement of inner sidebands and narrowing of central peaks may also occur in the fluorescence spectrum. We present…
The eigenvalue problem for the dressed bound-state of unstable multilevel systems is examined both outside and inside the continuum, based on the N-level Friedrichs model which describes the couplings between the discrete levels and the continuous spectrum. It is shown that a bound-state eigenenergy always exists below each of the discrete levels that lie outside the continuum. Furthermore, by strengthening the couplings gradually, the eigenenergy corresponding to each of the discrete levels inside the continuum finally emerges. On the other hand, the absence of the eigenenergy inside the cont…
We report an interference experiment of spontaneous emission of light from two distant solid-state ensembles of atoms that are coherently excited by a short laser pulse. The ensembles are Erbium ions doped into two LiNbO3 crystals with channel waveguides, which are placed in the two arms of a Mach-Zehnder interferometer. The light that is spontaneously emitted after the excitation pulse shows first-order interference. By a strong collective enhancement of the emission, the atoms behave as ideal two-level quantum systems and no which-path information is left in the atomic ensembles after emissi…
We study the effect of quantum interference on the structure and properties of spontaneous and stimulated transitions in a degenerate V-type three-level atom with an arbitrary total momentum of each state. Explicit expressions for the factors in the terms of the relaxation operator and stimulated transition operator with account of quantum interference effects are obtained. It has been demonstrated that the condition for the dipole transition moments to be parallel is insufficient and for conventional atoms the interference cross terms are zeros for both operators. The conditions when quantum …
We examine theoretically how dipole-dipole interactions arising from multiple photon scattering lead to a modified distribution of ground state populations in a driven, ordered 1D array of multilevel atoms. Specifically, we devise a level configuration in which a ground-state population accumulated due solely to dipole-dipole interactions can be up to 20\% in regimes accessible to current experiments with neutral atom arrays. For much larger systems, the steady state can consist of an equal distribution of population across the ground state manifold. Our results illustrate how dipole-dipole in…
We show that the quantum interference between downconverted photon pairs and photons from coherent laser light can produce a maximally path entangled N-photon output component with a fidelity greater than 90% for arbitrarily high photon numbers. A simple beam splitter operation can thus transform the 2-photon coherence of down-converted light into an almost optimal N-photon coherence.
Studying the spontaneous emission of a V-type three-level atom embedded in a photonic crystal (PC) by fractional calculus, we found that the atomic excited states in the anisotropic PC can be expressed as a superposition of four dressed states analytically. Through detuning two allowed atomic transition energies with respect to the photonic band edge, the coupling between these two transitions leads to three dynamic regimes, namely non-Markovian decay, damped quantum interference and quantum interference, classified by the numbers of contributed bounded dressed states. From the degree of quant…
The spontaneous emission is investigated for an effective atomic two-level system in an intense coherent field with frequency lower than the vacuum-induced decay width. As this additional low-frequency field is assumed to be intense, multiphoton processes may be induced, which can be seen as alternative transition pathways in addition to the simple spontaneous decay. The interplay of the various interfering transition pathways influences the decay dynamics of the two-level system and may be used to slow down the spontaneous decay considerably. We derive from first principles an expression for …
We theoretically investigate nonresonant spontaneous bremsstrahlung in the scattering of an electron by a nucleus in the field of two linearly polarized light waves propagating in the same direction in the general relativistic case. It is demonstrated that there are two substantially different kinematic ranges: the noninterference range, where the Bunkin-Fedorov quantum parameters serve as multiphoton parameters,and the interference range, where interference effects become significant, and quantum interference parameters play the role of multiphoton parameters. We determine the cross sections …
Resonant spontaneous bremsstrahlung of an electron scattered by a nucleus in the field of two moderately strong pulsed laser waves is studied theoretically. The process is studied in detail within the interference kinematic region. This region is determined by scattering of particles in the same plane at predetermined angles, at that stimulated absorption and emission of photons of external pulsed waves by an electron occurs in correlated manner. The correspondence between the emission angle and the final-electron energy is established in the kinematic region where the resonant parametric inte…
We discuss the spontaneous emission from a coherently prepared and microwave driven doublet of potentially closely spaced excited states to a common ground level. Multiple interference mechanisms are identified which may lead to fluorescence inhibition in well-separated regions of the spectrum or act jointly in cancelling the spontaneous emission. In addition to phase independent quantum interferences due to combined absorptions and emissions of driving field photons, we distinguish two competing phase dependent interference mechanisms as means of controlling the fluorescence. The indistinguis…
Spontaneous emission can create coherences in a multilevel atom having close lying levels, subject to the condition that the atomic dipole matrix elements are non-orthogonal. This condition is rarely met in atomic systems. We report the possibility of bypassing this condition and thereby creating coherences by letting the atom with orthogonal dipoles to interact with the vacuum of a pre-selected polarized cavity mode rather than the free space vacuum. We derive a master equation for the reduced density operator of a model four level atomic system, and obtain its analytical solution to describe…
We consider regimes of Spontaneous Parametric Down-Conversion both noncollinear and nondegenerate in frequencies. Parameters characterizing degrees of noncollinearity and of nondgeneracy are defined, and they are shown to be not independent of each other. At a given degree of nondegeneracy the emitted photons are shown to propagate along two different cones opening angles of which are determined by the degree of nondegeneracy. Based on this, the degree of nondegeneracy can be controlled by means of the angular selection of photons, e.g., with the help of appropriately installed slits. For such…
We investigate theoretically the non-Markovian dynamics of a degenerate V-type quantum emitter in the vicinity of a metallic nanosphere, a system that exhibits quantum interference in spontaneous emission due to the anisotropic Purcell effect. We calculate numerically the electromagnetic Green's tensor and employ the effective modes differential equation method for calculating the quantum dynamics of the emitter population, with respect to the resonance frequency and the initial state of the emitter, as well as its distance from the nanosphere. We find that the emitter population evolution var…
In this work, the effects of quantum interference and spontaneously generated coherence (SGC) are theoretically analyzed in a four level system of a $^{87}\mathrm{Rb}$ atom. For the effects of SGC, we find that a new kind of EIT channel can be induced due to destructive interference, and the nonlinear Kerr absorption can be coherently narrowed or eliminated under different strengths of the coupling and switching fields.
Quantum nonlinear interferometers (QNIs) can measure the infrared physical quantities of a sample by detecting visible photons. A QNI with Michelson geometry based on the spontaneous parametric down-conversion in a second-order nonlinear crystal is studied systematically. A simplified theoretical model of the QNI is presented. The interference visibility, coherence length, equal-inclination interference, and equal-thickness interference for the QNI are demonstrated theoretically and experimentally. As an application example of the QNI, the refractive index and the angle between two surfaces of…
We investigate the collective decay dynamics of atoms with a generic multilevel structure (angular momenta $F\leftrightarrow F'$) coupled to two light modes of different polarization inside a cavity. In contrast to two-level atoms, we find that multilevel atoms can harbour eigenstates that are perfectly dark to cavity decay even within the subspace of permutationally symmetric states (collective Dicke manifold). The dark states arise from destructive interference between different internal transitions and are shown to be entangled. Remarkably, the superradiant decay of multilevel atoms can end…
We investigate the dynamical behavior of the atom-photon entanglement in a V-type three-level quantum system using the atomic reduced entropy. It is shown that an atom and photons are entangled at the steady-state; however disentanglement can also be achieved in an especial condition. It is demonstrated that in the presence of quantum interference induced by spontaneous emission, the reduced entropy and the atom-photon entanglement are phase-dependent. Non-stationary solution is also obtained when the quantum interference due to the spontaneous emission is completely included.
It is a long standing question whether or not one can change the nature of spontaneous emission by a free electron through shaping the electron wavefunction. On one hand, shaping the electron wavefunction changes the respective charge and current densities of the electron. On the other hand, spontaneous emission of an electron is an incoherent process and can often be insensitive to the shape of the electron wavefunction. In this work, we arrive at an affirmative answer examining Bremsstrahlung radiation by free electron superposition states. We find that the radiation can be markedly differen…
We investigate the generation and the evolution of two-mode continuous-variable (CV) entanglement from system of a microwave-driven V-type atom in a quantum beat laser. By taking into account the effects of spontaneously generated quantum interference between two atomic decay channels, we show that the CV entanglement with large mean number of photons can be generated in our scheme, and the property of the filed entanglement can be adjusted by properly modulating the frequency detuning of the fields. More interesting, it is found that the entanglement can be significantly enhanced by the spont…
As one of the central topics in quantum optics, collective spontaneous emission such as superradiance has been realized in a variety of systems. This work proposes an innovative scheme to coherently control collective emission rates via a self-interference mechanism in a nonlinear waveguide setting. The self-interference is made possible by photon backward scattering incurred by quantum scatterers in a waveguide working as quantum switches. Whether the interference is constructive or destructive is found to depend strongly on the distance between the scatterers and the emitters. The interferen…
We discuss the connection between quantum interference effects in optical beams and radiation fields emitted from atomic systems. We illustrate this connection by a study of the first- and second-order correlation functions of optical fields and atomic dipole moments. We explore the role of correlations between the emitting systems and present examples of practical methods to implement two systems with non-orthogonal dipole moments. We also derive general conditions for quantum interference in a two-atom system and for a control of spontaneous emission. The relation between population trapping…
We investigate the question whether Michelson type interferometry is possible if the role of the beam splitter is played by a spontaneous process. This question arises from an inspection of trajectories of atoms bouncing inelastically from an evanescent-wave (EW) mirror. Each final velocity can be reached via two possible paths, with a {\it spontaneous} Raman transition occurring either during the ingoing or the outgoing part of the trajectory. At first sight, one might expect that the spontaneous character of the Raman transfer would destroy the coherence and thus the interference. We investi…
The spontaneous decay of a V-type three-level atom placed in a negative-refractive-index waveguide is analyzed. We find that in thin waveguides, highly efficient surface guided modes are supported, which do not occur in positive index waveguides. In addition, at low absorption, the mode density and thus spontaneous emission into particular regular guided modes is enhanced by several orders of magnitude as compared to regular dielectric waveguides. The asymmetries between emission into the different modes and the enhancement of particular guided modes allow to induce strong spontaneous-emission…
The complex internal atomic structure involved in radiative transitions has an effect on the spectrum of fluctuations (noise) of the transmitted light. A degenerate transition has different properties in this respect than a pure two-level transition. We investigate these variations by studying a certain transition between two degenerate atomic levels for different choices of the polarization state of the driving laser. For circular polarization, corresponding to the textbook two-level atom case, the optical spectrum shows the characteristic Mollow triplet for strong laser drive, while the corr…
We consider a pair of three-level atoms interacting with the vacuum. The process of disentanglement due to spontaneous emission and the role of quantum interference between principal transitions in this process, are analysed. We show that the presence of interference can slow down disentanglement. In the limit of maximal interference, some part of initial entanglement can survive.
With quantum interference of two-path spontaneous emissions, we propose a novel scheme to coherently control the atom--photon momentum entanglement through atomic internal coherence. A novel phenomenon called ``momentum phase entanglement'' is reported, and we found, under certain conditions, that more controllable entangled state can be produced with super--high degree of entanglement.
In a previous paper [B. Deb and G. S. Agarwal, Phys. Rev. A 90, 063417 (2014)], it was theoretically shown that, magneto-optical manipulation of low energy scattering resonances and atom-molecule transitions could lead to the formation of a bound state in continuum (BIC), provided there is no spontaneous emission. We find that even an exceedingly small spontaneous decay from exited molecular states can spoil the BIC. In this paper, we show how to circumvent the detrimental effect of spontaneous emission by making use of vacuum-induced coherence (VIC) which results in the cancellation or suppre…
The quantum mechanical decay of two or more overlapped resonances in a common continuum is largely influenced by Fano interference, leading to important phenomena such as the existence of bound states in the continuum, fractional decay and quiescent dynamics for single particle decay, and signature of particle statistics in the many-body quantum decay. An overlooked yet essential requirement to observe Fano interference is time reversal symmetry of the bath. Here we consider multilevel quantum decay in a bath sustaining unidirectional (chiral) propagating states, such as in quantum Hall or in …
Stimulated emission of two photons is observed experimentally in the parametric amplification process and is compared to a three-photon interference scheme. We find that the underlying physics of stimulated emission is simply the constructive interference due to photon indistinguishability. So the observed signal enhancement upon the input of photons is a result of multi-photon interference of the input photons and the otherwise spontaneously emitted photon from the amplifier.
In spontaneous parametric down conversion (SPDC) based quantum information processing (QIP) experiments, there is a tradeoff between the coincide count rates (i.e. the pumping power of the SPDC), which limits the rate of the protocol, and the visibility of the quantum interference, which limits the quality of the protocol. This tradeoff is mainly caused by the multi-photon pair emissions from the SPDCs. In theory, the problem is how to model the experiments without truncating these multi-photon emissions while including practical imperfections. In this paper, we establish a method to theoretic…
The fluorescence light emitted by a 4-level system in $J=1/2$ to $J=1/2$ configuration driven by a monochromatic laser field and in an external magnetic field is studied. We show that the spectrum of resonance fluorescence emitted on the $π$ transitions shows a signature of spontaneously generated interference effects. The degree of interference in the fluorescence spectrum can be controlled by means of the external magnetic field, provided that the Landé g-factors of the excited and the ground state doublet are different. For a suitably chosen magnetic field strength, the relative weight of t…
We study the spectral properties of Spontaneous Parametric Down Conversion in a periodically poled waveguided structure of KTP crystal pumped by ultra-short pulses. Our theoretical analysis reveals a strongly multimode and asymmetric structure of the two-photon spectral amplitude for type-II SPDC. Experimental evidence, based on Hong-Ou-Mandel polarization interference with narrowband filtering, confirms this result.
