We study the effect of quantum interference on the structure and properties of spontaneous and stimulated transitions in a degenerate V-type three-level atom with an arbitrary total momentum of each state. Explicit expressions for the factors in the terms of the relaxation operator and stimulated transition operator with account of quantum interference effects are obtained. It has been demonstrated that the condition for the dipole transition moments to be parallel is insufficient and for conventional atoms the interference cross terms are zeros for both operators. The conditions when quantum interference influences the properties of the relaxation operators have been analysed. For the stimulated transitions this condition is shown to be anisotropy of the photon field interacting with the atoms. This case is minutely studied for the D-line of alkali metals.
We theoretically discuss one-photon and two-photon double-slit interferences for spontaneous and stimulated parametric down-conversions. We show that the two-photon sub-wavelength interference can exist in a general spontaneous parametric down-conversion (SPDC) for both type I and type II crystals. We propose an alternative way to observe sub-wavelength interference by a joint-intensity measurement which occurs for only type I crystal in a higher gain of SPDC. When a signal beam injects into the crystal, it may create two interference patterns by two stimulated down-converted beams, showing no…
In a recent paper [I.I. Arkhipov, Phys. Rev. A 98, 021803 (2018)], it was shown that one can completely identify the nonclassicality of single- and two-mode Gaussian states by means of certain nonclassicality witnesses which are based on intensity moments up to the third order of optical fields, provided that an appropriate coherent displacement is applied to a given Gaussian state. Here, we utilize a mathematical equivalence between the description of the coherent displaced Gaussian states generated in the spontaneous parametric processes and the Gaussian states generated in the corresponding…
We examine the conditions needed to accomplish stimulated Raman adiabatic passage (STIRAP) when the three levels (g, e and f) are degenerate, with arbitrary couplings contributing to the pump-pulse interaction (g - e) and to the Stokes-pulse interaction (e-f). We show that in general a sufficient condition for complete population removal from the g set of degenerate states for arbitrary, pure or mixed, initial state is that the degeneracies should not decrease along the sequence g, e and f. We show that when this condition holds it is possible to achieve the degenerate counterpart of conventio…
Spontaneous parametric down conversion has been largely exploited as a tool for absolute calibration of photon counting detectors, photomultiplier tubes or avalanche photodiodes working in Geiger regime. In this work we investigate the extension of this technique from very low photon flux of photon counting regime to the absolute calibration of analog photodetectors at higher photon flux. Moving toward higher photon rate, i.e. at high gain regime, with the spontaneous parametric down conversion shows intrinsic limitations of the method, while the stimulated parametric down conversion process, …
We report on four-wave mixing in coupled photonic crystal nano-cavities on a silicon-on-insulator platform. Three photonic wire cavities are side-coupled to obtain three modes equally separated in energy. The structure is designed to be self-filtering, and we show that the pump is rejected by almost two orders of magnitudes. We study both the stimulated and the spontaneous four-wave mixing processes: owing to the small modal volume, we find that signal and idler photons are generated with a hundred-fold increase in efficiency as compared to silicon micro-ring resonators.
Frequency non-degenerate entangled photon pairs have been employed in quantum communication, imaging, and sensing. To characterize quantum entangled state with long-wavelength (infrared, IR or even terahertz, THz) photon, one needs to either develop the single-photon detectors at the corresponding wavelengths or use novel tomography technique, which does not rely on single-photon detections, such as stimulated emission tomography (SET). We use standard quantum state tomography and SET to measure the density matrix of entangled photon pairs, with one photon at 1550 nm and the other one at 810 n…
We show how stimulated parametric processes can be employed in experiments on beyond the diffraction limit to overcome the problem of low visibility obtained by using spontaneous down conversion operating in the high gain regime. We further show enhancement of the count rate by several orders when stimulated parametric processes are used. Both the two photon counts and the visibility can be controlled by the phase of the stimulating coherent beam.
Stimulated emission of two photons is observed experimentally in the parametric amplification process and is compared to a three-photon interference scheme. We find that the underlying physics of stimulated emission is simply the constructive interference due to photon indistinguishability. So the observed signal enhancement upon the input of photons is a result of multi-photon interference of the input photons and the otherwise spontaneously emitted photon from the amplifier.
Nanoscale semiconductor lasers have been developed recently using either metal, metallo-dielectric or photonic crystal nanocavities. While the technology of nanolasers is steadily being deployed, their expected performance for on-chip optical interconnects is still largely unknown due to a limited understanding of some of their key features. Specifically, as the cavity size is reduced with respect to the emission wavelength, the stimulated and the spontaneous emission rates are modified, which is known as the Purcell effect in the context of cavity quantum electrodynamics. This effect is expec…
Do the wavepacket-size of free-electron wavefunction and its history have physical effect in its interaction with light? Here we answer this problem by analyzing a QED model, considering both spontaneous and stimulated emission of quantized radiation field. For coherent radiation (Glauber state), we confirm that stimulated emission/absorption of photons has a dependence on wavepacket size that decays when it exceeds the interacting radiation wavelength, consistently and complementarily with Schrodinger equation analysis of wavepacket acceleration in classical electromagnetic field. Furthermore…
The general expressions for the time development of the ensemble averages of E^- and E^-E^+ are found for N two level molecules (TLMs) interacting with a single mode electromagnetic field. The TLMs are assumed to be at equivalent mode positions in the field. In the main body of the paper, the general results are then simplified by assuming that all TLMs are in the up state at time 0. Examples of spontaneous emission behavior including both Super Radiant behavior and emission suppression are shown in Appendix E while stimulated emission with all TLMs initially in the lower state is examined in …
We propose the use of stimulated Raman adiabatic passage (STIRAP) to offer a fast high fidelity method of performing SU(2) rotations on spinor Bose Einstein condensates (BEC). Past demonstrations of BEC optical control suffer from difficulties arising from collective enhancement of spontaneous emission and inefficient two-photon transitions originating from selection rules. We present here a novel scheme which allows for arbitrary coherent rotations of two-component BECs while overcoming these issues. Numerical tests of the method show that for BECs of \ce{^{87}Rb} with up to $ 10^4 $ atoms an…
Scattering of a short (much shorter then the spontaneous lifetime) laser pulse has been considered in a dense resonant medium subject to local field effects. The system was studied in the limit of Hartree-Fock approximation for Bogolubov-Born-Green-Kirkwood-Yvon (BBGKY) hierarchy of equations for reduced density operators. A closed set of equations for atomic and field density operators was derived to describe stimulated scattering of radiation. Numerically as well as theoretically the capability of multicomponent spectrum with maximums multiple to Rabi frequency has been demonstrated. Relativ…
Here we present a semiclassical analysis of spontaneous and stimulated radiative emission from unmodulated and optically-modulated electron quantum wavepackets. We show that the radiative emission/absorption and corresponding deceleration/acceleration of the wavepackets depend on the controllable 'history-dependent' wavepacket size. The characteristics of the radiative interaction when a wavepacket of size (duration) is short relative to the radiation wavelength, are close to the predictions of the classical point-particle modeling. On the other hand, in the long-sized wavepacket limit, the in…
We present a general formalism for describing stimulated Raman adiabatic passage in a multi-level atom. The atom is assumed to have two ground state manifolds a and b and an excited state manifold e, and the adiabatic passage is carried out by resonantly driving the a-e and b-e transitions with time-dependent fields. Our formalism gives a complete description of the adiabatic passage process, and can be applied to systems with arbitrary numbers of degenerate states in each manifold and arbitrary couplings of the a-e and b-e transitions. We illustrate the formalism by applying it to both a simp…
Vacuum-stimulated Raman scattering in strongly coupled atom-cavity systems allows one to generate free-running single photon pulses on demand. Most properties of the emitted photons are well defined, provided spontaneous emission processes do not contribute. Therefore, electronic excitation of the atom must not occur, which is assured for a system adiabatically following a dark state during the photon-generation process. We experimentally investigate the conditions that must be met for adiabatic following in a time-of-flight driven system, with atoms passing through a cavity and a pump beam or…
Photoassociation and the Feshbach resonance are, in principle, feasible means for creating a molecular Bose-Einstein condensate from an already-quantum-degenerate gas of atoms; however, mean-field shifts and irreversible decay place practical constraints on the efficient delivery of stable molecules using either mechanism alone. We therefore propose Feshbach-stimulated Raman photoproduction, i.e., a combination of magnetic and optical methods, as a viable means to collectively convert degenerate atoms into a stable molecular condensate with near-unit efficiency.
Stimulated Raman interaction of a classically pumped single three-level $Λ$-type atom in a resonator cavity featuring both radiative and unwanted losses is studied. It is shown that in the regime of stimulated adiabatic Raman passage the excited outgoing wave packet of the cavity-assisted electromagnetic field can be prepared in a one-photon Fock state with high efficiency. In this regime, the spatio-temporal shape of the wave packet does not depend on the interaction shape of the pump field, provided that the interaction of the atom with the pump is time-delayed with respect to the interactio…
The existence of higher order entanglement in the stimulated and spontaneous Raman processes is established using the perturbative solutions of the Heisenberg equations of motion for various field modes that are obtained using the Sen-Mandal technique and a fully quantum mechanical Hamiltonian that describes the stimulated and spontaneous Raman processes. Specifically, the perturbative Sen-Mandal solutions are exploited here to show the signature of the higher order two-mode and multi-mode entanglement. In some special cases, we have also observed higher order entanglement in the partially spo…
We consider ultracold atoms in a far detuned optical lattice orientated across a high-Q optical resonator. Applying an external driving laser to the atoms, which is red detuned from the cavity mode by one vibrational quantum, induces cavity-enhanced sideband cooling. For a dense and cold enough atomic ensemble we predict an oscillation threshold for optical Raman sideband lasing concurrent with coherent matter-wave amplification. Above this oscillation threshold photons and atoms in the lowest band are dominantly created pairwise via stimulated emission with a strong suppression of competing s…
Warm rubidium vapours are known to be a versatile medium for a variety of experiments in atomic physics and quantum optics. Here we present experimental results on producing the frequency converted light for quantum applications based on spontaneous and stimulated processes in rubidium vapours. In particular, we study the efficiency of spontaneously initiated stimulated Raman scattering in the Λ-level configuration and conditions of generating the coherent blue light assisted by multi-photon transitions in the diamond-level configuration. Our results will be helpful in search for new types of …
A five-level four-pulse phase-sensitive extended stimulated Raman adiabatic passage scheme is proposed to realize complete control of the population transfer branching ratio between two degenerate target states. The control is achieved via a three-node null eigenstate that can be correlated with an arbitrary superposition of the target states. Our results suggest that complete suppression of the yield of one of two degenerate product states, and therefore absolute selectivity in photochemistry, is achievable and predictable, even without studying the properties of the unwanted product state be…
We present a quantum optics approach for describing stimulated parametric down conversion in the two type-I crystal "sandwich" configuration, which allows for parametric interaction of vector vortex beams. We analyze the conditions for which phase conjugation of the seed vector beam occurs. We then use two strategies for defining generalized Stokes parameters to describe phase conjugation of vector vortex beams. These allow for geometrical representations, such as higher-order Poincaré spheres. Our results are useful for description and design of stimulated and spontaneous parametric down conv…
We investigate the performance of a certain nonclassicality identifier, expressed via integrated second-order intensity moments of optical fields, in revealing bipartite entanglement of quantum-optical frequency combs (QOFCs), which are generated in both spontaneous and stimulated parametric down-conversion processes. We show that, by utilizing that nonclassicality identifier, one can well identify the entanglement of the QOFC directly from the experimentally measured intensity moments without invoking any state reconstruction techniques or homodyne detection. Moreover, we demonstrate that the…
We analyze the error in trapped-ion, hyperfine qubit, quantum gates due to spontaneous scattering of photons from the gate laser beams. We investigate single-qubit rotations that are based on stimulated Raman transitions and two-qubit entangling phase-gates that are based on spin-dependent optical dipole forces. This error is compared between different ion species currently being investigated as possible quantum information carriers. For both gate types we show that with realistic laser powers the scattering error can be reduced to below current estimates of the fault-tolerance error threshold…
The phenomenon of spontaneous symmetry breaking is investigated in the dynamic thermalization of a degenerate quantum system. A three-level system interacting with a heat bath is carefully studied to this end. It is shown that the three-level system with degenerate ground states might have different behaviors depending on the details of the interaction with the heat bath when the temperature approaches zero. If we introduce an external field to break the degeneracy of the ground states and let it approach zero after letting the temperature approach zero, then two possibilities will arise: the …
We characterise the spontaneous emission time and direction from small numbers of dipole-coupled two-level atoms (2LAs) in the presence of incident fields. We show how to use adiabatic passage to admit population transfer between states in the one-quantum subspace for two and three 2LAs. Our method is a multi-atom generalisation of stimulated-Raman-adiabatic-passage (STIRAP) for a single multi-level atom. We use numerical results to justify an ansatz that enables us to give analytical expressions for the directional emission which depends on the incident fields. Our results admit a characteris…
We show that the two-photon transition rates of quantum dots coupled to nanocavities are enhanced by up to 8 orders of magnitude relative to quantum dots in bulk host. We then propose how to take advantage of this enhancement to implement coherent quantum dot excitation by two-photon absorption, entangled photon pair generation by two-photon spontaneous emission, and single-photon generation at telecommunication wavelengths by two-photon stimulated and spontaneous emission.
We study two-photon excitation of Rydberg states of atoms under stimulated adiabatic passage with delayed laser pulses. We find that the combination of strong interaction between the atoms in Rydberg state and the spontaneous decay of the intermediate exited atomic state leads to the Rydberg excitation of precisely one atom within the atomic ensemble. The quantum Zeno effect offers a lucid interpretation of this result: the Rydberg blocked atoms repetitively scattering photons effectively monitor a randomly excited atom which therefore remains in the Rydberg state. This system can be used for …
We investigate the effect of the cumulative phase on the photon statistics of the three-mode state whose evolution is described by the trilinear Hamiltonian $\hat{H}_{I}=i\hbarκ\big(\hat{a}\hat{b}\hat{c}^{\dagger}-\hat{a}^{\dagger}\hat{b}^{\dagger}c\big)$, wherein the pump is taken to be quantized (and prepared in a coherent state) and the signal and idler modes are initially seeded with coherent states. We provide a brief review of the two-mode squeezed coherent states generated by non-degenerate coherently-stimulated parametric down-conversion, whereby the nonlinear crystal is driven by a st…
Bridging quantum mechanics and nonlinear optics in Raman scattering
Nikon Corporation（尼康公司）；Institute of Pure and Applied Science, University of Tsukuba（筑波大学纯应用科学研究所）；Department of Biosciences and Informatics, Faculty of Science and Technology, Keio University（庆应义塾大学理工学部生物信息学科）
The interaction between light and an atom proceeds via three paradigmatic mechanisms: spontaneous emission, stimulated emission, and absorption. All three are resonant processes in the sense that they require that the radiation field be resonant with the atomic transition. The non-resonant counterparts of these effects, while necessary to maintain locality of the interaction in principle, are usually negligible because their effects tend to average out over multiple cycles of the radiation field. This state of affairs does not hold if the atom is accelerated. We show that, when accelerated, th…
The coherent interaction of electromagnetic fields with solid-state two-level systems can yield deterministic quantum light sources for photonic quantum technologies. To date, the performance of semiconductor single-photon sources based on three-level systems is limited mainly due to a lack of high photon indistinguishability. Here, we tailor the cavity-enhanced spontaneous emission from a ladder-type three-level system in a single epitaxial quantum dot (QD) through stimulated emission. After populating the biexciton (XX) of the QD through two-photon resonant excitation (TPE), we use another l…
The adiabatic manipulation of quantum states is a powerful technique that has opened up new directions in quantum engineering, enabling tests of fundamental concepts such as the Berry phase and its nonabelian generalization, the observation of topological transitions, and holds the promise of alternative models of quantum computation. Here we benchmark the stimulated Raman adiabatic passage process for circuit quantum electrodynamics, by using the first three levels of a transmon qubit. We demonstrate a population transfer efficiency above 80% between the ground state and the second excited st…
A model for quantum Zeno effect based upon an effective Schrödinger equation originated by the path-integral approach is developed and applied to a two-level system simultaneously stimulated by a resonant perturbation. It is shown that inhibition of stimulated transitions between the two levels appears as a consequence of the influence of the meter whenever measurements of energy, either continuous or pulsed, are performed at quantum level of sensitivity. The generality of this approach allows to qualitatively understand the inhibition of spontaneous transitions as the decay of unstable partic…
We have measured the 2-particle correlation function of atoms from a Bose--Einstein condensate participating in a superradiance process, which directly reflects the 2nd order coherence of the emitted light. We compare this correlation function with that of atoms undergoing stimulated emission. Whereas the stimulated process produces correlations resembling those of a coherent state, we find that superradiance, even in the presence of strong gain, shows a correlation function close to that of a thermal state, just as for ordinary spontaneous emission.
We study the process of co-polarized spontaneous four-wave mixing in single-mode optical fibers, with an emphasis on an analysis of the conversion efficiency. We consider both the monochromatic-pumps and pulsed-pumps regimes, as well as both the degenerate-pumps and non-degenerate-pumps configurations. We present analytical expressions for the conversion efficiency, which are given in terms of double integrals. In the case of pulsed pumps we take these expressions to closed analytical form with the help of certain approximations. We present results of numerical simulations, and compare them to…
Quantum adiabatic evolution, an important fundamental concept inphysics, describes the dynamical evolution arbitrarily close to the instantaneous eigenstate of a slowly driven Hamiltonian. In most systems undergoing spontaneous symmetry-breaking transitions, their two lowest eigenstates change from non-degenerate to degenerate. Therefore, due to the corresponding energy-gap vanishes, the conventional adiabatic condition becomes invalid. Here we explore the existence of quantum adiabatic evolutions in spontaneous symmetry-breaking transitions and derive a symmetry-dependent adiabatic condition.…
We consider pulsed-pump spontaneous parametric downconversion (SPDC) as well as pulsed single- and dual-pump spontaneous four-wave mixing processes in waveguides within a unified Hamiltonian theoretical framework. Working with linear operator equations in $k$-space, our approach allows inclusion of linear losses, self- and cross-phase modulation, and dispersion to any order. We describe state evolution in terms of second-order moments, for which we develop explicit expressions. We use our approach to calculate the joint spectral amplitude of degenerate squeezing using SPDC analytically in the …
