We discuss the connection between quantum interference effects in optical beams and radiation fields emitted from atomic systems. We illustrate this connection by a study of the first- and second-order correlation functions of optical fields and atomic dipole moments. We explore the role of correlations between the emitting systems and present examples of practical methods to implement two systems with non-orthogonal dipole moments. We also derive general conditions for quantum interference in a two-atom system and for a control of spontaneous emission. The relation between population trapping and dark states is also discussed. Moreover, we present quantum dressed-atom models of cancellation of spontaneous emission, amplification on dark transitions, fluorescence quenching and coherent population trapping.
We collect the fluorescence from two trapped atomic ions, and measure quantum interference between photons emitted from the ions. The interference of two photons is a crucial component of schemes to entangle atomic qubits based on a photonic coupling. The ability to preserve the generated entanglement and to repeat the experiment with the same ions is necessary to implement entangling quantum gates between atomic qubits, and allows the implementation of protocols to efficiently scale to larger numbers of atomic qubits.
We demonstrate deterministic generation of two distinct collective excitations in one atomic ensemble, and we realize the Hong-Ou-Mandel interference between them. Using Rydberg blockade we create single collective excitations in two different Zeeman levels, and we use stimulated Raman transitions to perform a beam-splitter operation between the excited atomic modes. By converting the atomic excitations into photons, the two-excitation interference is measured by photon coincidence detection with a visibility of 0.89(6). The Hong-Ou-Mandel interference witnesses an entangled NOON state of the …
We present Hong-Ou-Mandel interference of single photons generated via two different physical processes by two independent atomic systems: scattering by a single atom, and parametric generation via four-wave mixing in a cloud of cold atoms. Without any spectral filtering, we observe a visibility of V=62$\pm$4%. After correcting for accidental coincidences, we obtain V=93$\pm$6%. The observed interference demonstrates the compatibility of the two sources, forming the basis for an efficient quantum interface between different physical systems.
High-visibility interference of photon echoes generated in spatially separated solid-state atomic ensembles is demonstrated. The solid state ensembles were LiNbO$_3$ waveguides doped with Erbium ions absorbing at 1.53 $μ$m. Bright coherent states of light in several temporal modes (up to 3) are stored and retrieved from the optical memories using two-pulse photon echoes. The stored and retrieved optical pulses, when combined at a beam splitter, show almost perfect interference, which demonstrates both phase preserving storage and indistinguishability of photon echoes from separate optical memo…
We observe quantum, Hong-Ou-Mandel, interference of fields produced by two remote atomic memories. High-visibility interference is obtained by utilizing the finite atomic memory time in four-photon delayed coincidence measurements. Interference of fields from remote atomic memories is a crucial element in protocols for scalable generation of multi-node remote qubit entanglement.
In this paper we explore the physical origin of the transparency induced in absorbing three-level cascade atoms by the simultaneous interplay of two coherent beams of light. By utilizing the scattering technique we offer what we believe is a very convincing physical evidence for the existence, or for the absence, of quantum interference effects in the Autler-Townes (AT) and Electromagnetically Induced Transparency (EIT) phenomena.
The exactly analytical solutions for the dynamics of the dissipative three-level V-type and $Λ$-type atomic systems in the vacuum Lorentzian environments are presented. Quantum interference phenomenon between the two transitions in V-type atomic system is studied and the intuitive interference conditions are derived. For the dissipative $Λ$-type atomic system, we demonstrate that the similar quantum interference phenomenon does not exist. Finally, we study the dynamical evolution of quantum Fisher information, quantum entanglement and quantum coherence for the V-type atomic system. We find tha…
The Berry phase acquired by an electromagnetic field undergoing an adiabatic and cyclic evolution in phase space is a purely quantum-mechanical effect of the field. However, this phase is usually accompanied by a dynamical contribution and cannot be manifested in any light-beam interference experiment because it is independent of the field state. We here show that such a phase can be produced using an atom coupled to a quantized field and driven by a slowly changing classical field, and it is manifested in atomic Ramsey interference oscillations. We also show how this effect may be applied to …
We propose a scheme for generation of continuous-wave THz radiation. The scheme requires a medium where three discrete states in a $Λ$ configuration can be selected, with the THz-frequency transition between the two lower metastable states. We consider the propagation of three-frequency continuous-wave electromagnetic (e.m.) radiation through a $Λ$ medium. Under resonant excitation, the medium absorption can be strongly reduced due to quantum interference of transitions, while the nonlinear susceptibility is enhanced. This leads to very efficient energy transfer between the e.m. waves providin…
We report an interference experiment of spontaneous emission of light from two distant solid-state ensembles of atoms that are coherently excited by a short laser pulse. The ensembles are Erbium ions doped into two LiNbO3 crystals with channel waveguides, which are placed in the two arms of a Mach-Zehnder interferometer. The light that is spontaneously emitted after the excitation pulse shows first-order interference. By a strong collective enhancement of the emission, the atoms behave as ideal two-level quantum systems and no which-path information is left in the atomic ensembles after emissi…
The squeezing spectrum of the resonance fluorescence is studied for a coherently driven four-level atom in the Y-type configuration. It is found that the squeezing properties of the fluorescence radiation are modified significantly when quantum interference of the spontaneous decays channels is included. We show a considerable enhancement of steady-state squeezing in spectral components for strong and off-resonant driving fields. The squeezing may be increased in both the inner and outer sidebands of the spectrum depending upon the choice of parameters. We also show that the interference can d…
We study the effect of quantum interference on the structure and properties of spontaneous and stimulated transitions in a degenerate V-type three-level atom with an arbitrary total momentum of each state. Explicit expressions for the factors in the terms of the relaxation operator and stimulated transition operator with account of quantum interference effects are obtained. It has been demonstrated that the condition for the dipole transition moments to be parallel is insufficient and for conventional atoms the interference cross terms are zeros for both operators. The conditions when quantum …
Vacuum-induced interference in light scattering by multilevel atomic chains
University of Innsbruck（因斯布鲁克大学）；Saarland University（萨尔兰大学）；Center for Quantum Technologies (QuTe), Saarland University（萨尔兰大学量子技术中心）；Università degli Studi di Milano（米兰大学）
We theoretically propose a method to enhance Raman scattering by injecting a seeded light field which is correlated with the initially prepared atomic spin wave. Such a light-atom correlation leads to an interference in the Raman scattering. The interference is sensitive to the relative phase between the seeded light field and initially prepared atomic spin wave. For constructive interference, the Raman scattering is greatly enhanced. Such an enhanced Raman scattering may find applications in quantum information, nonlinear optics and optical metrology due to its simplicity.
The beam-splitter (BS) is one of the most common and important components in modern optics, and lossless BS which features unitary transformation induces Hermitian evolution of light. However, the practical BS based on the conversion between different degree of freedoms are naturally non-Hermitian, as a result of essentially open quantum dynamics. In this work, we experimentally demonstrate a non-Hermitian BS for the interference between traveling photonic and localized magnonic modes. The non-Hermitian magnon-photon BS is achieved by the coherent and incoherent interaction mediated by the exc…
The subtle and fundamental issue of indistinguishability and interference between independent pathways to the same target state is examined in the context of coherent control of atomic and molecular processes, with emphasis placed on possible "which-way" information due to quantum entanglement established in the quantum dynamics. Because quantum interference between independent pathways to the same target state occurs only when the independent pathways are indistinguishable, it is first shown that creating useful coherence (as defined in the paper) between nondegenerate states of a molecule fo…
It is a long standing question whether or not one can change the nature of spontaneous emission by a free electron through shaping the electron wavefunction. On one hand, shaping the electron wavefunction changes the respective charge and current densities of the electron. On the other hand, spontaneous emission of an electron is an incoherent process and can often be insensitive to the shape of the electron wavefunction. In this work, we arrive at an affirmative answer examining Bremsstrahlung radiation by free electron superposition states. We find that the radiation can be markedly differen…
Canonical quantum formalism predicts that the interference pattern registered in multi-slit experiments should be a simple combination of patterns observed in two-slit experiments. This has been linked to the validity of Born's rule and verified in precise experiments with photons as well as molecules via nuclear magnetic resonance. Due to the expected universal validity of Born rule, it is instructive to conduct similar tests with yet other physical systems. Here we discuss analogs of triple-slit experiment using atoms allowing tripod energy level configuration, as realisable e.g. with alkali…
To realize a quantum network based on quantum entanglement swapping, bright and completely autonomous sources are essentially required. Here, we experimentally demonstrate Hong-Ou-Mandel (HOM) quantum interference between two independent bright photon pairs generated via the spontaneous four-wave mixing in Doppler-broadened ladder-type 87Rb atoms. Bright autonomous heralded single photons are operated in a continuous-wave (CW) mode with no synchronization or supplemental filters. The four-fold photon coincidence counts per hour correspond to 5000 events for a temporal range of 10 ns, one order…
We present experimental observations of interference between an atomic spin coherence and an optical field in a Λ-type gradient echo memory. The interference is mediated by a strong classical field that couples a weak probe field to the atomic coherence through a resonant Raman transition. Interference can be observed between a prepared spin coherence and another propagating optical field, or between multiple Λ transitions driving a single spin coherence. In principle, the interference in each scheme can yield a near unity visibility.
We demonstrate the existence of new nonclassical correlations in the radiation of two atoms, which are coherently driven by a continuous laser source. The photon-photon-correlations of the fluorescence light show a spatial interferene pattern not present in a classical treatment. A feature of the new phenomenon is, that bunched and antibunched light is emitted in different spatial directions. The calculations are performed analytically. It is pointed out, that the correlations are induced by state reduction due to the measurement process when the detection of the photons does not distinguish b…
Trapped atomic ensembles are convenient systems for quantum information storage in the long-lived sublevels of the electronic ground state and its conversion to propagating optical photons via stimulated Raman processes. Here we investigate a phase-matched emission of photons from a coherently prepared atomic ensemble. We consider an ensemble of cold atoms in an elongated harmonic trap with normal density distribution, and determine the parameters of paraxial optics to match the mode geometry of the emitted radiation and optimally collect it into an optical waveguide.
Spontaneously generated coherence and enhanced dispersion in a V-type, three-level atomic system interacting with a single mode field can considerably reduce the radiative and cavity decay rates. This may eliminate the use of high finesse, miniaturized cavities in optical cavity quantum electrodynamics experiments under strong atom-field coupling conditions.
When N driven atoms emit in phase into a high-Q cavity mode, the intracavity field generated by collective scattering interferes destructively with the pump driving the atoms. Hence atomic fluorescence is suppressed and cavity loss becomes the dominant decay channel for the whole ensemble. Microscopically 3D light-intensity minima are formed in the vicinity of the atoms that prevent atomic excitation and form a regular lattice. The effect gets more pronounced for large atom numbers, when the sum of the atomic decay rates exceeds the rate of cavity losses and one would expect the opposite behav…
Atomic magnetometers are highly sensitive detectors of magnetic fields that monitor the evolution of the macroscopic magnetic moment of atomic vapors, and opening new applications in biological, physical, and chemical science. However, the performance of atomic magnetometers is often limited by hidden systematic effects that may cause misdiagnosis for a variety of applications, e.g., in NMR and in biomagnetism. In this work, we uncover a hitherto unexplained interference effect in atomic magnetometers, which causes an important systematic effect to greatly deteriorate the accuracy of measuring…
We present an experimental and theoretical study of phase-dependent interference effects in multi-photon excitation under bichromatic radio-frequency (rf) field. Using an intense rf pulse, we study the interference between the three-photon and one-photon transition between the Zeeman sub-levels of the ground state of $^{87}$Rb that allows us to determine the carrier-envelope phase of the fields even for long pulses.
Interference effects in quantum transitions, giving rise to amplification without inversion, optical transparency and to enhancements in nonlinear optical frequency conversions are considered. Review of the relevant early theoretical and experimental results is given. The role of relaxation processes, spontaneous cascade of polarizations, local field effects, Doppler-broadening, as well as specific features of the interference in the spectral continuum are discussed.
The Doppler effect of moving atoms can create irreversibility of light. We show that the laser field in electromagnetic induced transparency (EIT) scheme with atomic motion can control the directional propagation of two counter-propagating probe fields in atomic gas cell. The quantum coherence effect serves as an optical transistor. Interference of the two output fields from the cell shows useful feature for determining the mean atomic velocity and can be useful as quantum velocimeter. We also find that the sign of the dispersive phase in EIT has a unique property, which helps to explain certa…
Two approaches used in the description of the channeling radiation emitted from relativistic positrons are compared with each other. In the first (traditional) case, the probability of the process is proportional to a sum of absolute squares of the amplitudes of the transition between two states with definite transverse energy levels of the positrons traversing single crystals. In the second case, we begin with calculation of the sum of amplitudes for transition between states with different transverse energy levels for corresponding radiation frequency, and then the sum is squared. One must k…
It is shown, that radiation spectrum of atoms (or nuclei) in the gravitational field has a red shift since the effective mass of radiating electrons (or nucleons) changes in this field. This red shift is equal to the red shift of radiation spectrum in the gravitational field measured in existence experiments. The same shift must arise when the photon (or $ γ$ quantum) is passing through the gravitational field if it participates in gravitational interactions (photon has no rest mass). The absence of the double effect in the experiments, probably, means that photons (or $ γ$ quanta) are passing…
Studying the spontaneous emission of a V-type three-level atom embedded in a photonic crystal (PC) by fractional calculus, we found that the atomic excited states in the anisotropic PC can be expressed as a superposition of four dressed states analytically. Through detuning two allowed atomic transition energies with respect to the photonic band edge, the coupling between these two transitions leads to three dynamic regimes, namely non-Markovian decay, damped quantum interference and quantum interference, classified by the numbers of contributed bounded dressed states. From the degree of quant…
In this paper we study the evolution of the two two-level atoms interacting with a single-mode quantized radiation field, namely, two-atom multiphoton Jaynes-Cummings model when the radiation field and atoms are initially prepared in the superpostion of displaced number states and excited atomic states, respectively. For this system we investigate the atomic inversion, Wigner function, phase distribution and entanglement.
We investigate an atomic $Λ$-system with one transition coupled to a laser field and a flat continuum of vacuum modes and the other transition coupled to field modes near the edge of a photonic band gap. The system requires simultaneous treatment of Markovian and non-Markovian dissipation processes, but the photonic band gap continuum can not be eliminated within a density matrix treatment. Instead we propose a formalism based on Monte-Carlo wavefunctions, and we present results relevant to an experimental characterization of a structured continuum.
We theoretically investigate the quantum dynamics of the center of mass of trapped atoms, whose internal degrees of freedom are driven in a $Λ$-shaped configuration with the lasers tuned at two-photon resonance. In the Lamb-Dicke regime, when the motional wave packet is well localized over the laser wavelenght, transient coherent population trapping occurs, cancelling transitions at the laser frequency. In this limit the motion can be efficiently cooled to the ground state of the trapping potential. We derive an equation for the center-of-mass motion by adiabatically eliminating the internal d…
Advances in the distribution of quantum information will likely require entanglement shared across a hybrid quantum network. Many entanglement protocols require the generation of indistinguishable photons between the various nodes of the network. This is challenging in a hybrid environment due to typically large differences in the spectral and temporal characteristics of single photons generated in different systems. Here we show, for the first time, quantum interference between photons generated from a single atomic ion and an atomic ensemble, located in different buildings and linked via opt…
A theoretical study of the interference pattern imprinted on the doubly differential momentum distribution of the photoelectron due to atomic ionization induced by a short laser pulse is developed from a semiclassical standpoint. We use the semiclassical two-step model of Shvetsov-Shilovski et al. (Phys. Rev. A 94, 013415) to elucidate the nature of the holographic structure. Three different types of trajectories are characterized during the ionization process by a single cycle pulse with three different types of interferences. We show that the holographic interference arises from the ionizati…
The effect of quantum interference on the optical properties of a pumped-probe three-level V-type atomic system is investigated. The probe absorption, dispersion, group index and optical bistability beyond the two-photon resonance condition are discussed. It is found that the optical properties of a medium in the frequency of the probe field, in general, are phase independent. The phase dependence arises from a scattering of the coupling field into the probe field at a frequency which in general differs from the probe field frequency. It is demonstrated that beyond the two-photon resonance con…
We investigate laser-induced quantum interference phenomena in superradiance processes and in an ensemble of initially excited $Λ-$type closely packed three-level emitters. The lower doublet levels are pumped with a coherent laser field. Due to constructive quantum interference effects, the superradiance occurs on a much weaker atomic transition which is not the case in the absence of the coherent driving. This result may be of visible relevance for enhancing ultraweak transitions in atomic or atomic-like systems, respectively, or for high-frequency lasing effects.
A hybrid quantum system is proposed by coupling the internal hyperfine transitions of a trapped atomic Bose-Einstein condensate (BEC) and a superconducting quantum interference device (SQUID) via the macroscopic quantum field of the flux qubit. The presence of the condensate leads to a bosonic enhancement of the Rabi frequency over the otherwise small single-particle magnetic dipole transition matrix elements. This enhancement allows for the possibility to rapidly transfer and store qubit states in the BEC that were originally prepared in the SQUID. The fidelity of this transfer for different …
We investigate the dynamical behavior of the atom-photon entanglement in a V-type three-level quantum system using the atomic reduced entropy. It is shown that an atom and photons are entangled at the steady-state; however disentanglement can also be achieved in an especial condition. It is demonstrated that in the presence of quantum interference induced by spontaneous emission, the reduced entropy and the atom-photon entanglement are phase-dependent. Non-stationary solution is also obtained when the quantum interference due to the spontaneous emission is completely included.
We report on the observation of quantum interference of a collective single spin excitation with a spin ensemble of $N_{\text{atom}} =10^5$ atoms. Detection of a single photon scattered from the atoms creates the single spin excitation, a Fock state embedded in the collective spin of the ensemble. The state of the atomic ensemble is then detected by tomography via a quantum non-demolition measurement of the collective spin. A macroscopic difference of the order of $\sqrt{N_{\text{atom}}}$ in the marginal distribution of the collective spin state arises from the interference between the single …
We study the effects of many-body interactions on the interference in a Mach-Zehnder interferometer for matter waves of ultracold Bose atoms. After switching off an axial trapping potential, the thermal initial wavepacket expands, and subsequently interference fringes may be observed in a circular 1D trap. These are computed for axial harmonic or $δ$-function traps, and for interaction strengths from the Thomas-Fermi regime to the Tonks-Girardeau limit. It is shown that many-body correlations in a realistic setup destroy interference to a large degree. Analytical expressions allowing to infer …
A measurement scheme of atomic qubits pinned at given positions is studied by analyzing the interference pattern obtained when they emit photons spontaneously. In the case of two qubits, a well-known relation is revisited, in which the interference visibility is equal to the concurrence of the state in the infinite spatial separation limit of the qubits. By taking into account the super-radiant and sub-radiant effects, it is shown that a state tomography is possible when the qubit spatial separation is comparable to the wavelength of the atomic transition. In the case of three qubits, the rela…
Quantum coupling between mechanical oscillators and atomic gases generating entanglement has been recently experimentally demonstrated using their subsequent interaction with light. The next step is to build a hybrid atom-mechanical quantum gate showing bosonic interference effects of single quanta in the atoms and oscillators. We propose an experimental test of Hong-Ou-Mandel interference between single phononic excitation and single collective excitation of atoms using the optical connection between them. A single optical pulse is sufficient to build a hybrid quantum-nondemolition gate to ob…
We investigate the quantum interference induced by a relative phase in the correlated initial state of a system which consists in a two-level atom interacting with a damped mode of the radiation field. We show that the initial relative phase has significant effects on both the evolution of the atomic excited-state population and the information flow between the atom and the reservoir, as quantified by the trace distance. Furthermore, by considering two two-level atoms interacting with a common damped mode of the radiation field, we highlight how initial relative phases can affect the subsequen…
The wave function of an atom passed through a diffraction grating acquires a regular space structure and the interaction of another particle with this atom can be thought of as scattering on a 'quantum grating' composed of a single atom. Probing this 'grating' by collisions with charged projectiles reveals interference effects due to coherent contributions of its 'slits' to the transition amplitude. In particular, the spectra of electrons emitted from the atom in collisions with swift ions exhibit a pronounced interference pattern whose shape can be extremely sensitive to the collision velocit…
We characterize the effect of quantum interference on the line shapes and measured line positions in atomic spectra. These effects, which occur when the excited state splittings are of order the excited state line widths, represent an overlooked but significant systematic effect. We show that excited state interference gives rise to non-Lorenztian line shapes that depend on excitation polarization, and we present expressions for the corrected line shapes. We present spectra of 6,7 Li D lines taken at multiple excitation laser polarizations and show that failure to account for interference chan…
We assess the effect of the heat radiation emitted by mesoscopic particles on their ability to show interference in a double slit arrangement. The analysis is based on a stationary, phase-space based description of matter wave interference in the presence of momentum-exchange mediated decoherence.
We experimentally demonstrate the generation of heralded bi-chromatic single photons from an atomic collective spin excitation (CSE). The photon arrival times display collective quantum beats, a novel interference effect resulting from the relative motion of atoms in the CSE. A combination of velocity-selective excitation with strong laser dressing and the addition of a magnetic field allows for exquisite control of this collective beat phenomenon. The present experiment uses a diamond scheme with near-IR photons that can be extended to include telecommunications-wavelengths or modified to all…
With quantum interference of two-path spontaneous emissions, we propose a novel scheme to coherently control the atom--photon momentum entanglement through atomic internal coherence. A novel phenomenon called ``momentum phase entanglement'' is reported, and we found, under certain conditions, that more controllable entangled state can be produced with super--high degree of entanglement.
The relations between quantum coherence and quantum interference are discussed. A general method for generation of quantum coherence through interference-induced state selection is introduced and then applied to `simple' atomic systems under two-photon transitions, with applications in quantum optics and laser cooling.
The resonance fluorescence from regular atomic systems is shown to represent a continuous source of non-Gaussian entangled radiation propagating in two different directions. For a single atom entanglement occurs under the same conditions as squeezing. For more atoms, the entanglement can be more robust against dephasing than squeezing, hence providing a useful continuous source for various applications of entangled radiation.
Essential for building quantum networks over remote independent nodes, the indistinguishability of photons has been extensively studied by observing the coincidence dip in the Hong-Ou-Mandel interferometer. However, indistinguishability is not limited to the same type of bosons. For the first time, we hereby observe quantum interference between flying photons and a single quantum of stored atomic coherence (magnon) in an atom-light beam splitter interface. We demonstrate that the Hermiticity of this interface determines the type of quantum interference between photons and magnons. Consequently…
We consider the coherent state radiation field inside a micromaser cavity and study the entanglement mediated by it on a pair of two level atoms passing though the cavity one after the other. We then investigate the effects of squeezing of the cavity field on the atomic entanglement. We compute the entanglement of formation for the emerging mixed two-atom state and show that squeezing of the cavity radiation field can increase the atomic entanglement.
We predict the existence of high frequency modes in the interference pattern of two condensates made of fermionic-atom dimers. These modes, which result from fermion exchanges between condensates, constitute a striking signature of the dimer composite nature. From the 2-coboson spatial correlation function, that we derive analytically, and the Shiva diagrams that visualize many-body effects specific to composite bosons, we identify the physical origin of these high frequency modes and determine the conditions to see them experimentally by using bound fermionic-atom pairs trapped on optical lat…
