Analytic solutions to the time-dependent Schrödinger equation for cutoff wave initial conditions are used to investigate the time evolution of the transmitted probability density for tunneling. For a broad range of values of the potential barrier opacity $α$, we find that the probability density exhibits two evolving structures. One refers to the propagation of a {\it forerunner} related to a {\it time domain resonance} [Phys. Rev. A {\bf 64}, 0121907 (2001)], while the other consists of a semiclassical propagating wavefront. We find a regime where the {\it forerunners} are absent, corresponding to positive {\it time delays}, and show that this regime is characterized by opacities $α< α_c$. The critical opacity $α_c$ is derived from the analytical expression for the {\it delay time}, that reflects a link between transient effects in tunneling and the {\it delay time}
Transient {\it time-domain resonances} found recently in time-dependent solutions to Schrödinger's equation are used to investigate the issue of the tunneling time in rectangular potential barriers. In general, a time frequency analysis shows that these transients have frequencies above the cutoff frequency associated with the barrier height, and hence correspond to non-tunneling processes. We find, however, a regime characterized by the barrier opacity, where the peak maximum $t_{max}$ of the {\it time-domain resonance} corresponds to under-the-barrier tunneling. We argue that $t_{max}$ repre…
Transient tunneling effects in triple barrier systems are investigated by considering a time-dependent solution to the Schrödinger equation with a cutoff wave initial condition. We derive a two-level formula for incidence energies $E$ near the first resonance doublet of the system. Based on that expression we find that the probability density along the internal region of the potential, is governed by three oscillation frequencies: one of them refers to the well known Bohr frequency, given in terms of the first and second resonance energies of the doublet, and the two others, represent a coupli…
We investigate the transient evolution of finite-frequency current noise after abrupt switching on of the tunneling coupling in two paradigmatic, exactly solvable models of mesoscopic physics: the resonant level model and the Majorana resonant level model, which emerges as an effective model for a Kondo quantum dot at the Toulouse point. We find a parameter window in which the transient noise can become negative, a property it shares with the transient current. However, in contrast to the transient current, which approaches the steady state exponentially fast, we observe an algebraic decay in …
We calculate the response of a molecular magnet subject to a time-varying magnetic field and coupled to a heat bath. We propose that observations of calculated oscillations transverse to the field direction may be an effective way of demonstrating quantum tunneling and thus probing the details of level repulsion. The effective model of a triangle of Heisenberg spins and weak anisotropies, as has been used to model the molecular magnets V15 and Cu3, is used to illustrate this.
In this work we study the behaviour of Wigner phase delay time for tunneling in the reflection mode. Our system consists of a circular loop connected to a single wire of semi-infinite length in the presence of Aharonov-Bohm flux. We calculate the analytical expression for the saturated delay time. This saturated delay time is independent of Aharonov- Bohm flux and the width of the opaque barrier thereby generalizing the Hartman effect. This effect implies superluminal group velocities as a consequence. We also briefly discuss the concept called "space collapse or space destroyer".
We show that the group delay in tunneling is not a traversal time but a lifetime of stored energy or stored probability escaping through both ends of the barrier. Because it is a lifetime associated with both forward (transmitted) and backward (reflected) fluxes, it cannot be used to define a group velocity for forward transit in cases where a wavepacket is mostly reflected. For photonic tunneling barriers the group delay is identical to the dwell time which is also a property of an entire wave function with reflected and transmitted components. Theoretical predictions and experimental reports…
Tunneling Dynamics and Time Delay in Electron Transport through Time-Dependent Barriers with Finite-Bandwidth Reservoirs
Weizmann Institute（魏茨曼科学研究所）；BCAM - Basque Center for Applied Mathematics（巴斯克应用数学中心）；Departmento de Química-Física, Universidad del País Vasco, UPV/EHU（巴斯克大学物理化学系）；IKERBASQUE, Basque Foundation for Science（伊克尔巴斯基克科学基金会）
The transit times are obtained for a symmetrized (two identical bosons) and an antisymmetrized (two identical fermions) quantum colliding configuration. Considering two identical particles symmetrically impinging on a one-dimensional barrier, we demonstrate that the phase time and the dwell time give connected results where, however, the exact position of the scattered particles is explicitly determined by the phase time (group delay). For the antisymmetrized wave function configuration, an unusual effect of {\em accelerated} transmission is clearly identified in a simultaneous tunneling of tw…
We study the tunneling zone solutions of a one-dimensional electrostatic potential for the relativistic (Dirac to Klein-Gordon) wave equation when the incoming wave packet exhibits the possibility of being almost totally transmitted through the barrier. The transmission probabilities, the phase times and the dwell times for the proposed relativistic dynamics are obtained and the conditions for the occurrence of accelerated tunneling transmission are all quantified. We show that, in some limiting cases, the analytical difficulties that arise when the stationary phase method is employed for obta…
Transient phenomena of phase modulated cut-off wavepackets are explored by deriving an exact general solution to Schrödinger's equation for finite range potentials involving arbitrary initial quantum states. We show that the dynamical features of the probability density are governed by a virtual \textit{self-induced two-level system} with energies $E_{+}$, and $E_{-}$, due to the phase modulation of the initial state. The asymptotic probability density exhibits Rabi-oscillations characterized by a frequency $Ω=(E_{+}-E_{-})/\hbar$, which are independent of the potential profile. It is also fou…
The electron dynamics in the classically forbidden region during relativistic tunnel-ionization is investigated. The classical forbidden region in the relativistic regime is identified by defining a gauge invariant total energy operator. Introducing position dependent energy levels inside the tunneling barrier, we demonstrate that the relativistic tunnel-ionization can be well described by a one-dimensional intuitive picture. This picture predicts that, in contrast to the well-known nonrelativistic regime, the ionized electron wave packet arises with a momentum shift along the laser's propagat…
Several recent attoclock experiments have investigated the fundamental question of a quantum mechanically induced time delay in tunneling ionization via extremely precise photoelectron momentum spectroscopy. The interpretations of those attoclock experimental results were controversially discussed, because the entanglement of the laser and Coulomb field did not allow for theoretical treatments without undisputed approximations. The method of semiclassical propagation matched with the tunneled wavefunction, the quasistatic Wigner theory, the analytical R-matrix theory, the backpropagation metho…
Motivated by recent time domain experiments on ultrafast atom ionization, we analyze the transients and timescales that characterize, besides the relatively long lifetime, the decay by tunneling of a localized state. While the tunneling starts immediately, some time is required for the outgoing flux to develop. This short-term behavior depends strongly on the initial state. For the initial state tightly localized so that the initial transients are dominated by over-the-barrier motion, the timescale for the flux propagation through the barrier is close to the Büttiker-Landauer traversal time. T…
This report deals with the basic concepts on deducing transit times for quantum scattering: the stationary phase method and its relation with delay times for relativistic and non-relativistic tunneling particles. We notice that the applicability of this method is constrained by several subtleties in deriving the phase time that describes the localization of scattered wave packets. We investigate the general relation between phase times and dwell times for quantum tunneling/scattering. Considering a symmetrical collision of two identical wave packets with an one-dimensional barrier, we demonstr…
The measurement of the tunneling time in attosecond experiments, termed attoclock, triggered a hot debate about the tunneling time, the role of time in quantum mechanics, where the interaction with the laser pulse involves two regimes of a different character, the multiphoton and the tunneling (field-) ionization. In the adiabatic field calibration, one of us (O. K.) developed in earlier works a real tunneling time model and showed that the model fits well to the experimental data of Landsmann et al. (Optica {\bf 1}, 343 2014). In the present work, it is shown that the model explains the exper…
The general and explicit relation between the phase time and the dwell time for quantum tunneling of a relativistically propagating particle is investigated and quantified. In analogy with previously obtained non-relativistic results, it is shown that the group delay can be described in terms of the dwell time and a self-interference delay. Lessons concerning the phenomenology of the relativistic tunneling are drawn.
Tunneling delay times of wavepackets in quantum mechanical penetration of rectangular barriers have long been known to show a perplexing independence with respect to the width of the barrier. This also has relevence to the transmission of evanescent waves in optics. Some authors have claimed that in the presence of absorption or inelastic channels (which they model by taking a complex barrier potential) this effect no longer exists, in that the time delay becomes proportional to the barrier width. Taking the point of view that complex potentials imply non-Hermitian Hamiltonians and are as such…
We explore the dynamics of relativistic quantum waves in a potential step by using an exact solution to the Klein-Gordon equation with a point source initial condition. We show that in both the propagation, and Klein-tunneling regimes, the Zitterbewegung effect manifests itself as a series of quantum beats of the particle density in the long-time limit. We demonstrate that the beating phenomenon is characterized by the Zitterbewegung frequency, and that the amplitude of these oscillations decays as $t^{-3/2}$. We show that beating effect also manifests itself in the free Klein-Gordon and Dirac…
We report on the measurement of the time required for a wave packet to tunnel through the potential barriers of an optical lattice. The experiment is carried out by loading adiabatically a Bose-Einstein condensate into a 1D optical lattice. A sudden displacement of the lattice by a few tens of nm excites the micromotion of the dipole mode. We then directly observe in momentum space the splitting of the wave packet at the turning points and measure the delay between the reflected and the tunneled packets for various initial displacements. Using this atomic beam splitter twice, we realize a chai…
We solve the Dirac equation in three regions of graphene to get the solutions of the energy spectrum in connection to the strain, energy gap, and magnetic field. The Goos-Hänchen shifts and group delay time will be obtained by applying the stationary phase approximation after the wave functions at the interfaces have been matched. Our results suggest that the group delay time is influenced by the presence of strain along the armchair and zigzag directions. We show that the gate voltage and strain have the ability to change the group delay from subluminality to superluminality. This may have si…
We study the temporal aspects of quantum tunneling as manifested in time-of-arrival experiments in which the detected particle tunnels through a potential barrier. In particular, we present a general method for constructing temporal probabilities in tunneling systems that (i) defines `classical' time observables for quantum systems and (ii) applies to relativistic particles interacting through quantum fields. We show that the relevant probabilities are defined in terms of specific correlations functions of the quantum field associated with tunneling particles. We construct a probability distri…
Exact analytical solutions of the time-dependent Schrödinger equation with the initial condition of an incident cutoff wave are used to investigate the traversal time for tunneling. The probability density starts from a vanishing value along the tunneling and transmitted regions of the potential. At the barrier width it exhibits, at early times, a distribution of traversal times that typically has a peak $τ_p$ and a width $Δτ$. Numerical results for other tunneling times, as the phase-delay time, fall within $Δτ$. The Büttiker traversal time is the closest to $τ_p$. Our results resemble calcul…
The transient processes of electron transport in nano-scale devices exhibit special phenomena that exist only in the transient regime. Besides how fast the steady states are approached, one interesting aspect of transient transport arises from its strong dependence on the initial state of the system. Here we address the issue of how the symmetries embedded in the initial state interplay with those of the system structure in the course of transient transports. We explicitly explore the transient currents arising from various initial occupations in a double-quantum-dot Aharonov-Bohm interferomet…
We study the tunneling time of Dirac fermions in graphene magnetic barrier through an electrostatic potential and a mass term. This latter generates an energy gap in the spectrum and therefore affects the proprieties of tunneling of the system. For clarification, we first start by deriving the eigenspinors solutions of Dirac equation and second connect them to the incident, reflected and transmitted beam waves. This connection allows us to obtain the corresponding phases shifts and consequently compute the group delay time in transmission and reflection. Our numerical results show that the gro…
Recent attoclock experiments using the attsecond angular streaking technique enabled the measurement of the tunneling time delay during laser induced strong field ionization. Theoretically the tunneling time delay is commonly modelled by the Wigner time delay concept which is derived from the derivative of the electron wave function phase with respect to energy. Here, we present an alternative method for the calculation of the Wigner time delay by using the fixed energy propagator. The developed formalism is applied to the nonrelativistic as well as to the relativistic regime of the tunnel-ion…
I show that the MacColl-Hartman effect, namely, the saturation of the group delay time of sub-barrier quantum tunneling as a function of the barrier width, comes from the saturating behavior of a more fundamental concept - the phase of the stationary wave function. The explanation of saturation is given based on the decomposition of the stationary wave function into the spectrum of wave numbers and formulation of the initial condition for the direction of propagation of the incident matter wave. It is also shown that the saturation plateau of MacColl and Hartman actually doesn't continue indef…
The use of adiabatic passage techniques to mediate particle transport through real space, rather than phase space is becoming an interesting possibility. We have investigated the properties of Coherent Tunneling Adiabatic Passage (CTAP) with alternating tunneling matrix elements. This geometry, not previously considered in the donor in silicon paradigm, provides an interesting route to long-range quantum transport. We introduce simplified coupling protocols, and transient eigenspectra as well as a realistic gate design for this transport protocol. Using a pairwise treatment of the tunnel coupl…
For a circularly polarized single-color field at a central frequency of $2ω$ the final electron momentum distribution upon strong field ionization does not carry any information about the phase of the initial momentum distribution. Adding a weak, co-rotating, circularly polarized field at a central frequency of $ω$ gives rise to a sub-cycle interference pattern (holographic angular streaking of electrons (HASE)). This interference pattern allows for the retrieval of the derivative of the phase of the initial momentum distribution after tunneling $ϕ^{\prime}_{\mathrm{off}}(p_i)$. A trajectory-b…
The intermediate domain of strong-field ionization between the tunneling and the multiphoton regimes is investigated using the strong field approximation and the imaginary-time method. An intuitive model for the dynamics is developed which describes the ionization process within a nonadiabatic tunneling picture with a coordinate dependent electron energy during the under-the-barrier motion. The nonadiabatic effects in the elliptically polarized laser field induce a transversal momentum shift of the tunneled electron wave packet at the tunnel exit, a delayed appearance in the continuum as well …
We study the quantum Goos-Hänchen (GH) shift and the tunneling transmission at a curved step potential by investigating the time evolution of a wave packet. An initial wave packet is expanded in terms of the eigenmodes of a circular step potential. Its time evolution is then given by the interference of their simple eigenmode oscillations. We show that the GH shift along the step boundary can be explained by the energy-dependent phase loss upon reflection, which is defined by modifying the one-dimensional (1D) effective potential derived from the 2D circular system. We also demonstrate that th…
Experiments have shown that individual photons penetrate an optical tunnel barrier with an effective group velocity considerably greater than the vacuum speed of light. The experiments were conducted with a two-photon parametric down-conversion light source, which produced correlated, but random, emissions of photon pairs. The two photons of a given pair were emitted in slightly different directions so that one photon passed through the tunnel barrier, while the other photon passed through the vacuum. The time delay for the tunneling photon relative to its twin was measured by adjusting the pa…
The conundrum parameter-operator of time in quantum mechanics (QM), as well as the time-energy uncertainty relation and the tunneling delay time, have recently been addressed in attosecond optical ioniza- tion experiments. The parameter status of time in the time dependent Schrödinger equation (TDSE) is supported by the well-known Pauli's ob- jection as well as by its interpretation as an emerging property of entangle- ment with a classical environment. On the other hand, the introduction of a self-adjoint dynamical time operator in Dirac's formulation of elec- tron's relativistic quantum mech…
The buildup process of the probability density inside the quantum well of a double-barrier resonant structure is studied by considering the analytic solution of the time dependent Schrödinger equation with the initial condition of a cutoff plane wave. For one level systems at resonance condition we show that the buildup of the probability density obeys a simple charging up law, $| Ψ(τ) / ϕ| =1-e^{-τ/τ_0},$ where $ϕ$ is the stationary wave function and the transient time constant $τ_0$ is exactly two lifetimes. We illustrate that the above formula holds both for symmetrical and asymmetrical pot…
The general and explicit relation between the phase time and the dwell time for quantum tunneling or scattering is investigated. Considering a symmetrical collision of two identical wave packets with an one-dimensional barrier, here we demonstrate that these two distinct transit time definitions give connected results where, however, the phase time (group delay) accurately describes the exact position of the scattered particles. The analytical difficulties that arise when the stationary phase method is employed for obtaining phase (traversal) times are all overcome. Multiple wave packet decomp…
We present a spin-adapted time-dependent coupled cluster singles and doubles model for the molecular response to a sequence of ultrashort laser pulses. The implementation is used to calculate the electronic response to a valence-exciting pump pulse, and a subsequent core-exciting probe pulse. We assess the accuracy of the integration procedures used in solving the dynamic coupled cluster equations, in order to find a compromise between computational cost and accuracy. The transient absorption spectrum of lithium fluoride is calculated for various delays of the probe pulse with respect to the p…
Using a time operator, we define a tunneling time for a particle going through a barrier. This tunneling time is the average of the phase time introduced by other authors. In addition to the delay time caused by the resonances over the barrier, the present tunneling time is also affected by the branch point at the edge of the energy continuum. We find that when the particle energy is near the branch point, the tunneling time becomes strongly dependent on the width of the incoming wave packet, which implies that there is no intrinsic tunneling time. This effect is related to the quantum uncerta…
Tunneling of spinless electrons from a single-channel emitter into an empty collector through an interacting resonant level of the quantum dot (QD) is studied, when all Coulomb screening of charge variations on the dot is realized by the emitter channel and the system is mapped onto an exactly solvable model of a dissipative qubit. In this model we describe the qubit density matrix evolution with a generalized Lindblad equation, which permit us to count the tunneling electrons and therefore relate the qubit dynamics to the charge transfer statistics. In particular, the coefficients of its gene…
The Hartman effect for the tunneling particle implies the independence of group delay time on the opaque barrier width, with superluminal velocities as a consequence. This effect is further examined on a quantum ring geometry in the presence of Aharonov-Bohm flux. We show that while tunneling through an opaque barrier the group delay time for given incident energy becomes independent of the barrier thickness as well as the magnitude of the flux. The Hartman effect is thereby extended beyond one dimension and in the presence of Aharonov-Bohm flux.
Visualizing and controlling electron dynamics over femtosecond timescale play a key role in the design of next-generation electronic devices. Using simulations, we demonstrate the electronic oscillation inside the naphthalene molecule can be tracked by means of the tuning of delay time between two identical femtosecond laser pulses. Both the frequency and decay time of the oscillation are detected by the tunneling charge through the junction of scanning tunneling microscopy. And the tunneling charge is sensitive to the carrier-envelope phase (CEP) for few-cycle long optical pulses. While this …
We compare the main competing theories of tunneling time against experimental measurements using the attoclock in strong laser field ionization of helium atoms. Refined attoclock measurements reveal a real and not instantaneous tunneling delay time over a large intensity regime, using two different experimental apparatus. Only two of the theoretical predictions are compatible within our experimental error: the Larmor time, and the probability distribution of tunneling times constructed using a Feynman Path Integral (FPI) formulation. The latter better matches the observed qualitative change in…
The tunneling dynamics in relativistic strong-field ionization is investigated with the aim to develop an intuitive picture for the relativistic tunneling regime. We demonstrate that the tunneling picture applies also in the relativistic regime by introducing position dependent energy levels. The quantum dynamics in the classically forbidden region features two time scales, the typical time that characterizes the probability density's decay of the ionizing electron under the barrier (Keldysh time) and the time interval which the electron spends inside the barrier (Eisenbud-Wigner-Smith tunneli…
We investigate ultrafast dynamics of the lowest singlet excited electronic state in liquid nitrobenzene using Ultrafast Transient Polarization Spectroscopy (UTPS), extending the well-known technique of Optical-Kerr Effect (OKE) spectroscopy to excited electronic states. The third-order non-linear response of the excited molecular ensemble is highly sensitive to details of excited state character and geometries and is measured using two femtosecond pulses following a third femtosecond pulse that populates the S1 excited state. By measuring this response as a function of time delays between the …
