Optical mode characterization of single photons prepared via conditional measurements on a biphoton state
T. Aichele, A. I. Lvovsky, S. Schiller
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submitted to the special issue of the European Physical Journal D "Quantum interference and cryptographic keys: novel physics and advancing technologies"
A detailed theoretical analysis of the spatiotemporal mode of a single photon prepared via conditional measurements on a photon pair generated in the process of parametric down-conversion is presented. The maximum efficiency of coupling the photon into a transform-limited classical optical mode is calculated and ways for its optimization are determined. An experimentally feasible technique of generating the optimally matching classical mode is proposed. The theory is applied to a recent experiment on pulsed homodyne tomography of the single-photon Fock state (A. I. Lvovsky et al., Phys Rev. Lett. 87, 050402 (2001) - preprint at quant-ph/0101051)
We prepare qudits based on angular multimode biphoton states by modulating the pump angular spectrum. The modes are prepared in the Schmidt basis and their intensity distributions do not overlap in space. This allows one to get rid of filtering losses while addressing single modes and to realize a single-shot qudit readout.
We report a scalable linear optical scheme for generating entangled states of multiple ququarts in which the individual single-ququart state is prepared with the biphoton polarization state of frequency-nondegenerate spontaneous parametric down-conversion. The output state is calculated with the full consideration of the higher order effect (double-pair events) of spontaneous parametric down-conversion. Scalability to multiple-ququart entanglement is demonstrated with examples: linear optical entanglement of three and four individual biphoton ququarts.
We report the experimental generation of a class of spin-orbit vector modes of light via an asymmetric Mach-Zehnder interferometer, obtained from an input beam prepared in a product state of its spin and orbital degrees of freedom. These modes contain a spatially varying polarization structure which may be controllably propagated about the beam axis by varying the retardance between the vertical and horizontal polarization components of the light. Additionally, their transverse spatial intensity distributions may be continuously manipulated by tuning the input polarization parameters. In the c…
We measure the transverse entanglement of photon pairs on their propagation from the near to the far field of spontaneous parametric downconversion (SPDC). The Fedorov ratio, depending on the widths of conditional and unconditional intensity measurements, is shown to be only able to characterize entanglement in the near and far field zones of the source. Therefore we also follow a different approach. By evaluating the first-order coherence of a subsystem of the state we can quantify its entanglement. Unlike previous measurements, which determine the Fedorov ratio via intensity correlations, ou…
Spectrally uncorrelated biphoton state generated from the spontaneous nonlinear optical process is an important resource for quantum information. Currently such spectrally uncorrelated biphoton state can only be prepared from limited kinds of nonlinear media, thus limiting their wavelengths. In order to explore wider wavelength range, here we theoretically study the generation of spectrally uncorrelated biphoton state from 14 isomorphs of potassium dihydrogen phosphate (KDP) crystal. We find that 11 crystals from the `KDP family' still maintain similar nonlinear optical properties of KDP, such…
We demonstrate a silicon-chip biphoton source with an unprecedented quantum cross correlation up to ${\rm g_{si}^{(2)}(0) = (2.58 \pm 0.16) \times 10^4}$. The emitted biphotons are intrinsically single-mode, with self correlations of ${\rm g_{ss}^{(2)}(0) = 1.90 \pm 0.05}$ and ${\rm g_{ii}^{(2)}(0) = 1.87 \pm 0.06}$ for signal and idler photons, respectively. We observe the waveform asymmetry of cross correlation between signal and idler photons and reveal the identical and non-exponential nature of self correlations of individual signal and idler photon modes, which is a nature of cavity-enha…
Our last experimental results on the realization of a measurement-conditional unitary operation at single photon level are presented. This gate operates by rotating by $90^o$ the polarization of a photon produced by means of Type-II Parametric Down Conversion conditional to a polarization measurement on the correlated photon. We then propose a new scheme for measuring the quantum efficiency of a single photon detection apparatus by using this set-up. We present experimental results obtained with this scheme compared with {\it traditional} biphoton calibration. Our results show the interesting …
A reliable single photon source is a prerequisite for linear optical quantum computation and for secure quantum key distribution. A criterion yielding a conclusive test of the single photon character of a given source, attainable with realistic detectors, is therefore highly desirable. In the context of heralded single photon sources, such a criterion should be sensitive to the effects of higher photon number contributions, and to vacuum introduced through optical losses, which tend to degrade source performance. In this paper we present, theoretically and experimentally, a criterion meeting t…
Heralded single photons are prepared at a rate of ~100 kHz via conditional measurements on polarization-nondegenerate biphotons produced in a periodically poled KTP crystal. The single-photon Fock state is characterized using high frequency pulsed optical homodyne tomography with a fidelity of (57.6 +- 0.1)%. The state preparation and detection rates allowed us to perform on-the-fly alignment of the apparatus based on real-time analysis of the quadrature measurement statistics.
Photon modes have an important role in characterizing the quantum sources of light. Proper coupling of various photon modes obtained in spontaneous parametric down conversion (SPDC) process in optical fibers is essential to generate an effective source of entangled photons. The two main pre-detection factors affecting the biphoton mode coupling in SPDC are the pump beam focusing parameter and the crystal thickness. We present the numerical and experimental results on the effect of pump focusing on conditional down-converted photon modes for a Type-I BBO crystal. We experimentally verify that b…
We use the Stokes photon of a biphoton pair to set the time origin for electro-optic modulation of the wave function of the anti-Stokes photon thereby allowing arbitrary phase and amplitude modulation. We demonstrate conditional single-photon wave functions composed of several pulses, or instead, having gaussian or exponential shapes.
Preparation of Schrödinger-cat-like states via conditional output measurement on a beam splitter is studied. In the scheme, a mode prepared in a squeezed vacuum is mixed with a mode prepared in a Fock state and photocounting is performed in one of the output channels of the beam splitter. In this way the mode in the other output channel is prepared in a Schrödinger-cat-like state that is either a photon-subtracted or a photon-added Jacobi polynomial squeezed vacuum state, depending upon the difference between the number of photons in the input Fock state and the number of photons in the output…
We propose an experimentally accessible procedure for conditional preparation of highly non-classical states of collective spin of an atomic ensemble. The quantum state engineering is based on a combination of QND interaction between atoms and light previously prepared in a non-Gaussian state using photon subtraction from squeezed vacuum beam, homodyne detection on the output light beam, and a coherent displacement of atomic state. The procedure is capable of non-deterministic preparation of a wide class of superpositions of atomic Dicke states. We present several techniques to optimize the pe…
We show that conditional output measurement on a beam splitter may be used to produce photon-added states for a large class of signal-mode quantum states, such as thermal states, coherent states, squeezed states, displaced photon-number states, and coherent phase states. Combining a mode prepared in such a state and a mode prepared in a photon-number state, the state of the mode in one of the output channels of the beam splitter ``collapses'' to a photon-added state, provided that no photons are detected in the other output channel. We present analytical and numerical results, with special emp…
State preparation via conditional output measurement on a beam splitter is studied, assuming the signal mode is mixed with a mode prepared in a Fock state and photon numbers are measured in one of the output channels. It is shown that the mode in the other output channel is prepared in either a photon-subtracted or a photon-added Jacobi polynomial state, depending upon the difference between the number of photons in the input Fock state and the number of photons in the output Fock state onto which it is projected. The properties of the conditional output states are studied for coherent and squ…
We demonstrate, theoretically and experimentally, that statistical mixtures of the vacuum state |0> and the single-photon Fock state |1> are nonclassical according to the Vogel criterion (W. Vogel, Phys. Rev. Lett. 84, 1849 (2000)), regardless of the vacuum fraction. The ensembles are synthesized via conditional measurements on biphotons generated by means of parametric downconversion, and their quadrature statistics are measured using balanced homodyne detection. A comparative review of various quantum state nonclassicality criteria is presented.
We present a method for computing the action of conditional linear optical transformations, conditioned on photon counting, for arbitrary signal states. The method is based on the Q-function, a quasi probability distribution for anti normally ordered moments. We treat an arbitrary number of signal and ancilla modes. The ancilla modes are prepared in an arbitrary product number state. We construct the conditional, non unitary, signal transformations for an arbitrary photon number count on each of the ancilla modes.
We study the conditional preparation of single photons based on parametric downconversion, where the detection of one photon from a given pair heralds the existence of a single photon in the conjugate mode. We derive conditions on the modal characteristics of the photon pairs, which ensure that the conditionally prepared single photons are quantum-mechanically pure. We propose specific experimental techniques that yield photon pairs ideally suited for single-photon conditional preparation.
The problem of photon adding and subtracting is studied, using conditional output measurement on a beam splitter. It is shown that for various classes of states the corresponding photon-added and -subtracted states can be prepared. Analytical results are presented, with special emphasis on photon-added and -subtracted squeezed vacuum states, which are found to represent two different types of Schroedinger-cat-like states. Effects of realistic photocounting and Fock-state preparation are discussed.
A simple experimental setup consisting of a spontaneous parametric down-conversion source and passive linear optics is proposed for conditional preparation of a maximally entangled polarization state of two photons. Successful preparation is unambiguously heralded by coincident detection of four auxiliary photons. The proposed scheme utilizes the down-conversion term corresponding to the generation of three pairs of photons. We analyze imperfect detection of the auxiliary photons and demonstrate that its deleterious effect on the fidelity of the prepared state can be suppressed at the cost of …
We propose a scheme to prepare optical Schrödinger-cat states in a traveling wave setting. Two states are similarly prepared via the self-Kerr effect and after mixing them, one mode is measured by homodyne detection. In the other mode a superposition of coherent states is conditionally prepared. The advantage of the scheme is that assuming a small Kerr effect one can prepare with high probability one from a set of Schrödinger-cat states. The measured value of the quadrature provides the information, which state from the set is actually prepared.
The polarization analysis of quantized probe light transmitted through an atomic ensemble has been used to prepare entangled collective atomic states. In a "balanced" detection configuration, where the difference signal from two detection ports is analyzed, the continuous monitoring of a component of the Stokes field vector provides a means for conditional projective measurements on the atomic system. Here, we make use of classical driving fields, in the pulsed regime, and of an "unbalanced" detection setup (single detector) where the effective photon number of scattered photons is the detecte…
We present a fiber based source of polarization-entangled photon pairs that is well suited for quantum communication applications in the 1550nm band of standard fiber-optic telecommunications. Polarization entanglement is created by pumping a nonlinear-fiber Sagnac interferometer with two time-delayed orthogonally-polarized pump pulses and subsequently removing the time distinguishability by passing the parametrically scattered signal-idler photon pairs through a piece of birefringent fiber. Coincidence detection of the signal-idler photons yields biphoton interference with visibility greater …
We discuss the conditional preparation of single photons via parametric down-conversion. This technique is commonly used as a single photon source in modern quantum optics experiments. A significant problem facing this technique is the inability of present day photo-detectors to resolve photon number. This results in mixing with higher photon number terms. To overcome this several techniques have been proposed, including multi-port detection and time-division multiplexing. These techniques help approximate number resolving detection even when using non-number resolving detectors. In this paper…
A measurement-induced continuous-variable logical gate is able to prepare Schrödinger cat states if the gate uses a non-Gaussian resource state, such as cubic phase state [I. V. Sokolov, Phys. Lett. A 384, 126762 (2020)]. Our scheme provides an alternative to hybrid circuits which use photon subtraction and (or) Fock resource states and photon number detectors. We reveal the conditions under which the gate conditionally prepares quantum superposition of two undistorted "copies" of an arbitrary input state that occupies a finite area in phase space. A detailed analysis of the fidelity between t…
We study the collective spontaneous emission of three identical two-level atoms initially prepared in the excited states by measuring Glauber's third-order photon correlation function. Assuming two atoms at sub-wavelength distance from each other such that they are subject to the dipole-dipole interaction while the third one is located several wavelengths away, we observe super- and subradiant decay alike, depending on the direction of observation. Unlike the case where no remote atom is introduced or no conditional measurements are performed, the spontaneous emission behavior of the condition…
Non-Gaussian states of an optical field are important as a proposed resource in quantum information applications. While conditional preparation is a highly successful approach to preparing such states, their quality is limited by detector non-idealities such as dead time, narrow dynamic range, limited quantum efficiency and dark noise. Mesoscopic photon counters, with peak performance at higher photon number, offer many practical advantages over single-photon level conditioning detectors. Here we propose a novel approach involving displacement of the ancilla field into the regime where mesosco…
We propose a conditional scheme to generate entangled two-photons generalized binomial states inside two separate single-mode high-Q cavities. This scheme requires that the two cavities are initially prepared in entangled one-photon generalized binomial states and exploits the passage of two appropriately prepared two-level atoms one in each cavity. The measurement of the ground state of both atoms is finally required when they exit the cavities. We also give a brief evaluation of the experimental feasibility of the scheme.
Quantum measurement-induced gate based on entanglement with ideal cubic phase state used as a non-Gaussian resource is able to produce Shrödinger cat state in the form of two high fidelity ``copies'' of the target state on phase plane [N.I. Masalaeva, I.V. Sokolov, Phys. Lett. A 424, 127846 (2022)]. In this work we examine the effect of finite initial squeezing of the resource state on the gate performance. We present exact solution for the gate output state and demonstrate that there exists a degree of squeezing, available in experiment, such that the output cat state quality almost does not …
It was recently pointed out (and demonstrated experimentally) by Lundeen et al. that the wave function of a particle (more precisely, the wave function possessed by each member of an ensemble of identically-prepared particles) can be "directly measured" using weak measurement. Here it is shown that if this same technique is applied, with appropriate post-selection, to one particle from a (perhaps entangled) multi-particle system, the result is precisely the so-called "conditional wave function" of Bohmian mechanics. Thus, a plausibly operationalist method for defining the wave function of a qu…
The dynamics of an ensemble of identically prepared two-qubit systems is investigated which is subjected to the iteratively applied measurements and conditional selection of a typical entanglement purification protocol. It is shown that the resulting measurement-induced non-linear dynamics of the two-qubit state exhibits strong sensitivity to initial conditions and also true chaos. For a special class of initially prepared two-qubit states two types of islands characterize the asymptotic limit. They correspond to a separable and a maximally entangled two-qubit state, respectively, and their bo…
We derived quantum trajectories for a system interacting with the environment prepared in a continuous mode single photon state as the limit of discrete filtering model with an environment defined as series of independent qubits prepared initially in the entangled state being an analogue of a continuous mode state. The environment qubits interact with the quantum system and they are subsequently measured. The initial correlation between the bath qubits is the source of the non-Markovianity. The conditional evolutions of the quantum system for limit of the continuous in time observations togeth…
An approach for generating the entangled photonic states |F1,F2>+|F2,F1> from two arbitrary states |F1> and |F2> is proposed. The protocol is implemented by the conditionally induced beam-splitter coupling which leads to the selective swapping between two photonic modes. Such coupling occurs in a quantum system prepared in the superposition of two ground states with only one of them being involved in the swapping. All the entangled states in the category, such as entangled pairs of coherent states or Fock states (N00N states), can be efficiently produced in the same way by this method.
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We show that a continuous range of nonclassical states of light can be generated using conditional measurements on the idler mode of an optical parametric amplifier. The output state is prepared by introducing a coherent state in the signal mode of the amplifier with a single photon in the idler mode, followed by a conditional measurement of a single photon in the output idler mode. By varying the gain of the amplifier, this approach can produce a coherent state, a photon-added state, a displaced number state, or a continuous range of other nonclassical states with intermediate properties. We …
We show how a qubit can be fault-tolerantly encoded in the infinite-dimensional Hilbert space of an optical mode. The scheme is efficient and realizable with present technologies. In fact, it involves two travelling optical modes coupled by a cross-Kerr interaction, initially prepared in coherent states, one of which is much more intense than the other. At the exit of the Kerr medium, the weak mode is subject to a homodyne measurement and a quantum codeword is conditionally generated in the quantum fluctuations of the intense mode.
We propose and experimentally verify a scheme to engineer arbitrary states of traveling light field up to the two-photon level. The desired state is remotely prepared in the signal channel of spontaneous parametric down-conversion by means of conditional measurements on the idler channel. The measurement consists of bringing the idler field into interference with two ancilla coherent states, followed by two single-photon detectors, which, in coincidence, herald the preparation event. By varying the amplitudes and phases of the ancillae, we can prepare any arbitrary superposition of zero- one- …
We have reconstructed the quantum state of optical pulses containing single photons using the method of phase-randomized pulsed optical homodyne tomography. The single-photon Fock state |1> was prepared using conditional measurements on photon pairs born in the process of parametric down-conversion. A probability distribution of the phase-averaged electric field amplitudes with a strongly non-Gaussian shape is obtained with the total detection efficiency of (55+-1)%. The angle-averaged Wigner function reconstructed from this distribution shows a strong dip reaching classically impossible negat…
The semi-classical gravity sourced by the quantum expectation value of the matter's energy-momentum tensor will change the evolution of the quantum state of matter. This effect can be described by the Schroedinger-Newton (SN) equation, where the semi-classical gravity contributes a gravitational potential term depending on the matter quantum state. This state-dependent potential introduces the complexity of the quantum state evolution and measurement in SN theory, which is different for different quantum measurement prescriptions. Previous theoretical investigations on the SN-theory phenomenol…
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The work is devoted to the theoretical and experimental study of quantum states of light conditionally prepared by subtraction of a random number of photons from the initial multimode thermal state. A fixed number of photons is subtracted from a multimode quantum state, but only a subsystem of a lower number of modes is registered, in which the number of subtracted photons turns out to be a non-fixed random variable. It is shown that the investigation of multiphoton subtracted multimode thermal states provides a direct study of the fundamental quantum-statistical properties of bosons using a s…
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This dissertation studies the statistics and modeling of a quantum system probed by a coherent laser field. We focus on an ensemble of qubits dispersively coupled to a traveling wave light field. The first research topic explores the quantum measurement statistics of a quasi-monochromatic laser probe. We identify the shortest timescale that successive measurements approximately commute. Our model predicts that for a probe in the near infrared, noncommuting measurement effects are apparent for subpicosecond times. The second dissertation topic attempts to find an approximation to a conditional …
We consider an optical probe that interacts with an ensemble of rare earth ions doping a materialin the shape of a cantilever. By optical spectral hole burning, the inhomogeneously broadenedtransition in the ions is prepared to transmit the probe field within a narrow window, but bendingof the cantilever causes strain in the material which shifts the ion resonances. The motion of thecantilever may thus be registered by the phase shift of the probe. By continuously measuringthe optical field we induce a rapid reduction of the position and momentum uncertainty of thecantilever. Doing so, the pro…
Occupation-selective photon-pair interactions in a flux-pumped SQUID resonator
Universidade Estadual de Ponta Grossa（蓬塔格罗萨州立大学）；Universidade Estadual Paulista (UNESP)（圣保罗州立大学）；Hainan Bielefeld University of Applied Sciences（海南比勒费尔德应用科学大学）
