An ideal and reversible transfer technique for the quantum state between light and metastable collective states of matter is presented and analyzed in detail. The method is based on the control of photon propagation in coherently driven 3-level atomic media, in which the group velocity is adiabatically reduced to zero. Form-stable coupled excitations of light and matter (``dark-state polaritons'') associated with the propagation of quantum fields in Electromagnetically Induced Transparency are identified, their basic properties discussed and their application for quantum memories for light analyzed.
Using an extended Tavis-Cummings model, we study the effect of the spin-orbit coupling between the singlet and the triplet molecular excitons in organic microcavities in the strong coupling regime. The model is solved in the single excitation space for polaritons, which contains the bright (permutation symmetric) singlet and triplet excitons, as well as the dark bands consisting of the nonsymmetric excitons of either type. We find that the spin-orbit coupling splits the lower polariton into two branches, and also creates a triplet polariton when the cavity mode is in resonance with the triplet…
Inhomogeneous mass trap for dark-state polaritons in atomic media
National Central University（中央大学）；National Tsing Hua University（清华大学）；National Center for Excellence in Quantum Information Science and Engineering, National Tsing Hua University（国家量子信息科学与工程卓越中心）；Physics Division, National Center for Theoretical Sciences（理论科学国家中心物理部）；Quantum Technology Center, National Central University（量子技术中心）
We consider a two-dimensional extension of the 1D waveguide quantum electrodynamics and investigate the nature of linear excitations in two-dimensional arrays of qubits coupled to networks of chiral waveguides. We show that the combined effects of chirality and long-range photon mediated qubit-qubit interactions lead to the emergence of the two-dimensional flat bands in the polaritonic spectrum, corresponding to slow strongly correlated light.
In resonantly pumped polariton superfluids we recently explored a new regime based on the bistability of the polariton system to enhance the propagation of polariton fluids up to macroscopic distances. This technique together with an all-optical imprinting method allowed the generation and control of various topological excitations such as quantized vortices and dark solitons. The flexibility and scalability of the new experimental scheme opens the way to the systematic study of quantum turbulence in driven dissipative quantum fluids of light. In this article we review the basic working princi…
The quest of utilizing neutral particles to simulate the behaviour of charged particles in a magnetic field makes the generation of artificial magnetic field of great interest. The previous and the only proposal for the production of synthetic magnetic field for the dark state polaritons in electromagnetically induced transparency invokes the mechanical rotation of a sample. Here, we put forward an optical scheme to generate effective gauge potentials for stationary-light polaritons. 5To demonstrate the capabilities of our approach, we present recipes for having dark state polaritons in degene…
Collective strong coupling between a disordered ensemble of $N$ localized molecular vibrations and a resonant optical cavity mode gives rise to 2 polariton and $N-1\gg2$ dark modes. Thus, experimental changes in thermally-activated reaction kinetics due to polariton formation appear entropically unlikely and remain a puzzle. Here we show that the overlooked dark modes, while parked at the same energy as bare molecular vibrations, are robustly delocalized across $\sim$2-3 molecules, yielding enhanced channels of vibrational cooling, concomitantly catalyzing a chemical reaction. As an illustrati…
Information processing and storing by the same physical system is emerging as a promising alternative to traditional computing platforms. In turn, this requires the realization of elementary units whose memory content can be easily tuned and controlled. Here, we introduce a polariton-based quantum memristor where the memristive nature arises from the inter-cavity polariton exchange and is controlled by a time-varying atom-cavity detuning. A dynamical hysteresis is characterized by the fluctuations in the instantaneous polariton number, where the history information is encoded into a dynamical …
Two-photon absorption (TPA) allows accessing dark states of matter otherwise inaccessible to light, which serve as important building blocks for quantum information processing. In a semiconductor microcavity, TPA driven condensation of strongly-coupled light-matter exciton-polaritons can enable new solid-state quantum simulations of dark state-condensate interactions, and was predicted to stimulate THz emission. Here, we report the first observation of two-photon pumped polariton condensation, demonstrated by angle-resolved photoluminescence in a GaAs-based microcavity. TPA is evidenced in the…
For molecular polaritons, disorder and phonon timescales control the activation of dark states in the thermodynamic limit
University of Colorado Boulder（科罗拉多大学博尔德分校）；Institute of Chemistry, Chinese Academy of Sciences（中国科学院化学研究所）；University of Chinese Academy of Sciences（中国科学院大学）
A full quantum theory beyond the mean-field regime is developed for an exciton polariton condensate, to gain a complete understanding of quantum fluctuations. We find analytical solution for the polariton density matrix, showing the polariton nonlinearity causing fast relaxation correlated with the pump so as to yield the condensation at threshold. Increasing the pump intensity, a nonequilibrium phase transition towards the condensation of lower polaritons emerges, with a statistics transiting from a thermal, through a super-Poissonian and to a nonclassical distribution beyond the understandin…
Strong coupling between cavity photons and various excitations in condensed matters boosts the field of light-matter interaction and generates several exciting sub-fields, such as cavity optomechanics and cavity magnon polariton. Axion quasiparticles, emerging in topological insulators, were predicted to strongly couple with the light and generate the so-called axion polariton. Here, we demonstrate that there arises a gapless level attraction in cavity axion polariton of antiferromagnetic topological insulators, which originates from a nonlinear interaction between axion and the odd-order reso…
Strong light-matter interactions in hybrid polaritonic systems
Umeå University（于默奥大学）；Politecnico di Milano（米兰理工大学）；Rice University（莱斯大学）；University of Padova（帕多瓦大学）；University of Rome Tor Vergata（罗马托尔维加塔大学）；University of Milan（米兰大学）；University of Bologna（博洛尼亚大学）；Elettra Sincrotrone Trieste（的里雅斯特同步辐射中心）；Scuola Normale Superiore（比萨高等师范学院）；Istituto Nanoscienze – CNR（国家研究委员会纳米科学研究所）
Room-temperature Bose--Einstein condensates (BECs) of exciton polaritons have been realized in organic molecular systems owing to the strong light--matter interaction, strong exciton binding energy, and low effective mass of a polaritonic particle. These molecular-exciton-polariton BECs have demonstrated their potential in nonlinear optics and optoelectronic applications. In this study, we demonstrate that molecular-polariton BECs can be utilized for Bose enhancement of excitation-energy transfer (EET) in a molecular system with an exciton donor coupled to a group of exciton acceptors that are…
Superposition states of circular currents of exciton-polaritons mimic the superconducting flux qubits. The phase of a polariton fluid must change by an integer number of $2π$, when going around the ring. If one introduces a $π$-phase delay line in the ring, the fluid is obliged to propagate a clockwise or anticlockwise circular current to reduce the total phase gained over one round-trip to zero or to build it up to $2π$. We show that such a $π$-delay line can be provided by a dark soliton pinned to a potential well created by a C-shape non-resonant pump-spot. The resulting split-ring polarito…
