We propose and analyze a mechanism for Bose-Einstein condensation of stationary dark-state polaritons. Dark-state polaritons (DSPs) are formed in the interaction of light with laser-driven 3-level Lambda-type atoms and are the basis of phenomena such as electromagnetically induced transparency (EIT), ultra-slow and stored light. They have long intrinsic lifetimes and in a stationary set-up with two counterpropagating control fields of equal intensity have a 3D quadratic dispersion profile with variable effective mass. Since DSPs are bosons they can undergo a Bose-Einstein condensation at a critical temperature which can be many orders of magnitude larger than that of atoms. We show that thermalization of polaritons can occur via elastic collisions mediated by a resonantly enhanced optical Kerr nonlinearity on a time scale short compared to the decay time. Finally condensation can be observed by turning stationary into propagating polaritons and monitoring the emitted light.
A quantum model of Bose-Einstein condensation based on processes involving polaritons excited in an intracavity absorbing cell with resonance atoms, which is manifested in the spectral characteristics of the system, is considered. It is shown that the spectral 'condensation' appears which is directly related to the degeneracy of a weakly interacting gas of polaritons resulting in quasi-condensation at room temperature. The possibility of obtaining polariton condensation as a new phase state by using the confinement of polaritons in an atomic optical harmonic trap is discussed.
We consider a new approach for storing quantum information by macroscopic atomic excitations of two level atomic system. We offer the original scheme of quantum cloning of optical field into the cavity polaritons containing the phase insensitive parametrical amplifier and atomic cell placed in the cavity. The high temperature quasi-condensation (and/or condensation) phenomenon for polaritons arising in the cavity under the certain conditions is proposed for the first time.
Analysis of exciton-polariton condensation under different pumping schemes for 1D and 2D microcavities including the effect of strong correlation between polaritons
We show that superradiant emission (SR) in semiconductor laser diode structures is governed by the master equation of the form of Ginzburg-Landau equation or Gross-Pitaevskii equation for a phase transition to coherent matter state. We conjectured condensation of one-dimensional longitudinal lower polaritons with effective mass of 10$^{-11}$ the mass of free electron. Two different regimes of SR emission and polariton condensation are predicted, one of which exhibits some characteristic features of the Dicke superradiance in atomic gases. The predictions of analytic model are confirmed by the …
Two-photon absorption (TPA) allows accessing dark states of matter otherwise inaccessible to light, which serve as important building blocks for quantum information processing. In a semiconductor microcavity, TPA driven condensation of strongly-coupled light-matter exciton-polaritons can enable new solid-state quantum simulations of dark state-condensate interactions, and was predicted to stimulate THz emission. Here, we report the first observation of two-photon pumped polariton condensation, demonstrated by angle-resolved photoluminescence in a GaAs-based microcavity. TPA is evidenced in the…
We present a reaction/diffusion model for the formation of a lower polariton condensate in a micro cavity containing an organic semiconducting molecular crystalline film. Our model--based upon an anthracene film sandwiched between two reflecting dielectric mirrors--consists of three coupled fields corresponding to a gas of excitons created by an external driving pulse, a reservoir of vibron states formed by the coupling between a ground-state vibrational model and a cavity photon, and a lower polariton condensate. We show that at finite temperature, the presence of the vibron reservoir can aug…
We study Frenkel exciton-polariton Bose-Einstein condensation in a two-dimensional defect-free triangular photonic crystal with an organic semiconductor active medium containing bound excitons with dipole moments oriented perpendicular to the layers. We find photonic Bloch modes of the structure and consider their strong coupling regime with the excitonic component. Using the Gross- Pitaevskii equation for exciton polaritons and the Boltzmann equation for the external exciton reservoir, we demonstrate the formation of condensate at the points in reciprocal space where photon group velocity equ…
Exciton-polaritons in semiconductor microcavities have been used to demonstrate quantum effects such as Bose-Einstein condensation, superfluity, and quantized vortices. However, in these experiments, the polaritons have not reached thermal equilibrium when they undergo the transition to a coherent state. This has prevented the verification of one of the canonical predictions for condensation, namely the phase diagram. In this work, we have created a polariton gas in a semiconductor microcavity in which the quasiparticles have a lifetime much longer than their thermalization time. This allows t…
We put forward and discuss in detail a scheme to achieve Bose-Einstein condensation of stationary-light dark-state polaritons with dipolar interaction. To this end we have introduced a diamond-like coupling scheme in a vapor of Rydberg atoms under the frozen gas approximation. To determine the system's dynamics we employ normal modes and identify the dark-state polariton corresponding to one of the modes. We show that in contrast to atomic dipolar ultra-cold vapors dark-state polariton Bose-Einstein condensates proposed here can be stable for a negative dipolar interaction constant.
We show that polaritons in an array of interacting micro-cavities with strong atom-photon coupling can form a two-component Bose-Hubbard model. Both polariton species are thereby protected against spontaneous emission as their atomic part is stored in two ground states of the atoms. The parameters of the effective model can be tuned via the driving strength of external lasers. We also describe a method to measure the number statistics in one cavity for each polariton species independently.
Exciton-polaritons can condense to a macroscopic quantum state through a non-equilibrium process of pumping and decay. In recent experiments, polariton condensates are used to observe, for a short time, nonlinear Josephson phenomena by coupling two condensates. However, it is still not clear how these phenomena are affected by the pumping and decay at long times and how the coupling alters the polariton condensation. Here, we consider a polariton Josephson junction pumped on one side and study its dynamics within a mean-field theory. The Josephson current is found to give rise to multi-stabili…
We study the spontaneous emission of a partially excited Bose-Einstein condensate composed of two-level atoms. The formation of polaritons induced by the ground-state part of the condensate leads to an avoided crossing in the photon spectrum. This avoided crossing acts similarly to a photonic band gap and modifies the spontaneous emission rate.
The dynamics of spatial coherence and momentum distribution of polaritons in the regime of Bose-Einstein condensation are investigated in a GaAs microcavity with embedded quantum wells under nonresonant excitation with picosecond laser pulses. It is shown that the onset of the condensate first order sparial coherence is accompanied by narrowing of the polariton momentum distribution. At the same time, at sufficiently high excitation densities, there is significant qualitative discrepancy between the dynamic behavior of the width of the polariton momentum distribution determined from direct mea…
Room-temperature Bose--Einstein condensates (BECs) of exciton polaritons have been realized in organic molecular systems owing to the strong light--matter interaction, strong exciton binding energy, and low effective mass of a polaritonic particle. These molecular-exciton-polariton BECs have demonstrated their potential in nonlinear optics and optoelectronic applications. In this study, we demonstrate that molecular-polariton BECs can be utilized for Bose enhancement of excitation-energy transfer (EET) in a molecular system with an exciton donor coupled to a group of exciton acceptors that are…
We examine the possibility of observing Bose condensation of a confined two-dimensional polariton gas in an organic quantum well. We deduce a suitable parameterization of a model Hamiltonian based upon the cavity geometry, the biexciton binding energy, and similar spectroscopic and structural data. By converting the sum-over-states to a semiclassical integration over $d$-dimensional phase space, we show that while an ideal 2-D Bose gas will not undergo condensation, an interacting gas with the Bogoliubov dispersion $H(p)\approx s p$ close to $p=0$ will undergo Bose condensation at a given crit…
We propose a scheme which can realize an extended two-component Bose-Hubbard model using polaritons confined in an array of optical cavities. In addition to the density-dependent interactions, this model also contains nonlinear coupling terms between the two components of the polariton. Using a mean-field calculation, we obtain the phase diagram which shows how these terms affect the transition between the Mott insulator and the superfluid phase. In addition, we employ both a perturbation approach and an exact diagonalization method to gain more insights into the phase diagram.
We develop a theory for the dynamics of the density matrix describing a multimode polariton condensate. In such a condensate several single-particle orbitals become highly occupied, due to stimulated scattering from reservoirs of high-energy excitons. A generic few-parameter model for the system leads to a Lindblad equation which includes saturable pumping, decay, and condensate interactions. We show how this theory can be used to obtain the population distributions, and the time-dependent first- and second-order coherence functions, in such a multimode condensate. As a specific application, w…
In this letter, we give an analytical quantum description of a non-equilibrium polariton Bose-Einstein condensate (BEC) based on the solution of the master equation for the full polariton density matrix in the limit of fast thermalization. We find the density matrix of a non-equilibrium BEC, that takes into account quantum correlations between all polariton states. We show that the formation of BEC is accompanied by the build-up of cross-correlations between the ground state and the excited states reaching their highest values at the condensation threshold. Despite the non-equilibrium nature o…
Phase transitions, where observable properties of a many-body system change discontinuously, can occur in both open and closed systems. Ultracold atoms have provided an exemplary model system to demonstrate the physics of closed-system phase transitions, confirming many theoretical models and results. Our understanding of dissipative phase transitions in quantum systems is less developed, and experiments that probe this physics even less so. By placing cold atoms in optical cavities, and inducing strong coupling between light and excitations of the atoms, one can experimentally study phase tra…
A novel, optimized numerical method of modeling of an exciton-polariton superfluid in a semiconductor microcavity was proposed. Exciton-polaritons are spin-carrying quasiparticles formed from photons strongly coupled to excitons. They possess unique properties, interesting from the point of view of fundamental research as well as numerous potential applications. However, their numerical modeling is challenging due to the structure of nonlinear differential equations describing their evolution. In this paper, we propose to solve the equations with a modified Runge--Kutta method of 4th order, fu…
Improving the measurement precision of temperature is very important and challenging, especially in the low temperature range. Based on the existence of invariant subspaces during the polariton thermalization, we propose a new way to enhance the measurement precision of the low temperature and obtain Landau bound to avoid that the measurement uncertainty of the temperature diverges as the temperature approaches zero. The measurement precision of the low temperature increases significantly with the number of polariton states. In order to resist the dissipation, the incoherent pumping is necessa…
We study a model of a photon mode dipole-coupled to a medium of two-level oscillators in a microcavity in the presence of dephasing processes introduced by coupling to external baths. Decoherence processes can be classified as pair-breaking or non-pair-breaking in analogy with magnetic or non-magnetic impurities in superconductors. In the absence of dephasing, the ground state of the model is a polariton condensate with a gap in the excitation spectrum. Increase of the pair-breaking parameter $γ$ reduces the gap, which becomes zero at a critical value $γ_{C1}$; for large $γ$, the conventional …
We propose a method to enhance the spatial coupling between ballistic exciton-polariton condensates in a semiconductor microcavity based on available spatial light modulator technologies. Our method, verified by numerically solving a generalized Gross-Pitaevskii model, exploits the strong nonequilibrium nature of exciton-polariton condensation driven by localized nonresonant optical excitation. Tailoring the excitation beam profile from a Gaussian into a polygonal shape results in refracted and focused radial streams of outflowing polaritons from the excited condensate which can be directed to…
We investigate a chain of superconducting stripline resonators, each interacting with a transmon qubit, that are capacitively coupled in a row. We show that the dynamics of this system can be described by a Bose-Hubbard Hamiltonian with attractive interactions for polaritons, superpositions of photons and qubit excitations. This setup we envisage constitutes one of the first platforms where all technological components that are needed to experimentally study chains of strongly interacting polaritons have already been realized. By driving the first stripline resonator with a microwave source an…
Motivated by recent experiments on cold atomic gases in ultra high finesse optical cavities, we consider the problem of a two-band Bose--Hubbard model coupled to quantum light. Photoexcitation promotes carriers between the bands and we study the non-trivial interplay between Mott insulating behavior and superfluidity. The model displays a global U(1) X U(1) symmetry which supports the coexistence of Mott insulating and superfluid phases, and yields a rich phase diagram with multicritical points. This symmetry property is shared by several other problems of current experimental interest, includ…
A full quantum theory beyond the mean-field regime is developed for an exciton polariton condensate, to gain a complete understanding of quantum fluctuations. We find analytical solution for the polariton density matrix, showing the polariton nonlinearity causing fast relaxation correlated with the pump so as to yield the condensation at threshold. Increasing the pump intensity, a nonequilibrium phase transition towards the condensation of lower polaritons emerges, with a statistics transiting from a thermal, through a super-Poissonian and to a nonclassical distribution beyond the understandin…
A spatial potential trap is formed in a 6.0 μm Al(Ga)N nanowire by varying the Al composition along its length during epitaxial growth. The polariton emission characteristics of a dielectric microcavity with the single nanowire embedded in-plane has been studied at room temperature. Excitation is provided at the Al(Ga)N end of the nanowire and polariton emission is observed from the lowest bandgap GaN region of the nanowire. Comparison of the results with those measured in an identical microcavity with an uniform GaN nanowire and having an identical exciton-photon detuning suggests evaporative…
It is shown, that Bose-Einstein statistical distributions can occur not only in quantum system, but in classical systems as well. The coherent dynamics of the system, or equivalently autocatalytic dynamics in momentum space of the system is the main reason for the Bose-Einstein condensation. A coherence is possible in both quantum and classical systems, and in both cases can lead to Bose-Einstein statistical distribution.
We propose a novel mechanism for a nonequilibrium phase transition in a $U(1)$-broken phase of an electron-hole-photon system, from a Bose-Einstein condensate of polaritons to a photon laser, induced by the non-Hermitian nature of the condensate. We show that a (uniform) steady state of the condensate can always be classified into two types, namely, arising either from lower or upper-branch polaritons. We prove (for a general model) and demonstrate (for a particular model of polaritons) that an exceptional point where the two types coalesce marks the endpoint of a first-order-like phase bounda…
We show that Bose-Einstein condensate can be created in quasi-one-dimensional systems in a purely geometrical way, namely by bending or other suitable deformation of a tube.
It is shown, that Bose-Einstein condensation can occur not only in spatially extended equilibrium systems, but also in the systems far from thermal equilibrium, which show order-disorder phase transition. The investigation is performed by solving the Complex Ginzburg-Landau equation, a universal model for nonequilibrium order-disorder phase transitions.
