We consider a new approach for storing quantum information by macroscopic atomic excitations of two level atomic system. We offer the original scheme of quantum cloning of optical field into the cavity polaritons containing the phase insensitive parametrical amplifier and atomic cell placed in the cavity. The high temperature quasi-condensation (and/or condensation) phenomenon for polaritons arising in the cavity under the certain conditions is proposed for the first time.
A quantum model of Bose-Einstein condensation based on processes involving polaritons excited in an intracavity absorbing cell with resonance atoms, which is manifested in the spectral characteristics of the system, is considered. It is shown that the spectral 'condensation' appears which is directly related to the degeneracy of a weakly interacting gas of polaritons resulting in quasi-condensation at room temperature. The possibility of obtaining polariton condensation as a new phase state by using the confinement of polaritons in an atomic optical harmonic trap is discussed.
We propose and analyze a mechanism for Bose-Einstein condensation of stationary dark-state polaritons. Dark-state polaritons (DSPs) are formed in the interaction of light with laser-driven 3-level Lambda-type atoms and are the basis of phenomena such as electromagnetically induced transparency (EIT), ultra-slow and stored light. They have long intrinsic lifetimes and in a stationary set-up with two counterpropagating control fields of equal intensity have a 3D quadratic dispersion profile with variable effective mass. Since DSPs are bosons they can undergo a Bose-Einstein condensation at a cri…
We show that superradiant emission (SR) in semiconductor laser diode structures is governed by the master equation of the form of Ginzburg-Landau equation or Gross-Pitaevskii equation for a phase transition to coherent matter state. We conjectured condensation of one-dimensional longitudinal lower polaritons with effective mass of 10$^{-11}$ the mass of free electron. Two different regimes of SR emission and polariton condensation are predicted, one of which exhibits some characteristic features of the Dicke superradiance in atomic gases. The predictions of analytic model are confirmed by the …
Analysis of exciton-polariton condensation under different pumping schemes for 1D and 2D microcavities including the effect of strong correlation between polaritons
We present a reaction/diffusion model for the formation of a lower polariton condensate in a micro cavity containing an organic semiconducting molecular crystalline film. Our model--based upon an anthracene film sandwiched between two reflecting dielectric mirrors--consists of three coupled fields corresponding to a gas of excitons created by an external driving pulse, a reservoir of vibron states formed by the coupling between a ground-state vibrational model and a cavity photon, and a lower polariton condensate. We show that at finite temperature, the presence of the vibron reservoir can aug…
Two-photon absorption (TPA) allows accessing dark states of matter otherwise inaccessible to light, which serve as important building blocks for quantum information processing. In a semiconductor microcavity, TPA driven condensation of strongly-coupled light-matter exciton-polaritons can enable new solid-state quantum simulations of dark state-condensate interactions, and was predicted to stimulate THz emission. Here, we report the first observation of two-photon pumped polariton condensation, demonstrated by angle-resolved photoluminescence in a GaAs-based microcavity. TPA is evidenced in the…
We study Frenkel exciton-polariton Bose-Einstein condensation in a two-dimensional defect-free triangular photonic crystal with an organic semiconductor active medium containing bound excitons with dipole moments oriented perpendicular to the layers. We find photonic Bloch modes of the structure and consider their strong coupling regime with the excitonic component. Using the Gross- Pitaevskii equation for exciton polaritons and the Boltzmann equation for the external exciton reservoir, we demonstrate the formation of condensate at the points in reciprocal space where photon group velocity equ…
In the paper we consider a new approach for storage and cloning of quantum information by three level atomic (molecular) systems in the presence of the electromagnetically induced transparency (EIT) effect. For that, the various schemes of transformation into the bright and dark polaritons for quantum states of optical field in the medium are proposed. Physical conditions of realization of quantum nondemolition (QND) storage of quantum optical state are formulated for the first time. We have shown that the best storage and cloning of can be achieved with the atomic ensemble in the Bose-Einstei…
Exciton-polaritons can condense to a macroscopic quantum state through a non-equilibrium process of pumping and decay. In recent experiments, polariton condensates are used to observe, for a short time, nonlinear Josephson phenomena by coupling two condensates. However, it is still not clear how these phenomena are affected by the pumping and decay at long times and how the coupling alters the polariton condensation. Here, we consider a polariton Josephson junction pumped on one side and study its dynamics within a mean-field theory. The Josephson current is found to give rise to multi-stabili…
Exciton-polaritons in semiconductor microcavities have been used to demonstrate quantum effects such as Bose-Einstein condensation, superfluity, and quantized vortices. However, in these experiments, the polaritons have not reached thermal equilibrium when they undergo the transition to a coherent state. This has prevented the verification of one of the canonical predictions for condensation, namely the phase diagram. In this work, we have created a polariton gas in a semiconductor microcavity in which the quasiparticles have a lifetime much longer than their thermalization time. This allows t…
The dynamics of spatial coherence and momentum distribution of polaritons in the regime of Bose-Einstein condensation are investigated in a GaAs microcavity with embedded quantum wells under nonresonant excitation with picosecond laser pulses. It is shown that the onset of the condensate first order sparial coherence is accompanied by narrowing of the polariton momentum distribution. At the same time, at sufficiently high excitation densities, there is significant qualitative discrepancy between the dynamic behavior of the width of the polariton momentum distribution determined from direct mea…
We examine the possibility of observing Bose condensation of a confined two-dimensional polariton gas in an organic quantum well. We deduce a suitable parameterization of a model Hamiltonian based upon the cavity geometry, the biexciton binding energy, and similar spectroscopic and structural data. By converting the sum-over-states to a semiclassical integration over $d$-dimensional phase space, we show that while an ideal 2-D Bose gas will not undergo condensation, an interacting gas with the Bogoliubov dispersion $H(p)\approx s p$ close to $p=0$ will undergo Bose condensation at a given crit…
Phase transitions, where observable properties of a many-body system change discontinuously, can occur in both open and closed systems. Ultracold atoms have provided an exemplary model system to demonstrate the physics of closed-system phase transitions, confirming many theoretical models and results. Our understanding of dissipative phase transitions in quantum systems is less developed, and experiments that probe this physics even less so. By placing cold atoms in optical cavities, and inducing strong coupling between light and excitations of the atoms, one can experimentally study phase tra…
We develop a theory for the dynamics of the density matrix describing a multimode polariton condensate. In such a condensate several single-particle orbitals become highly occupied, due to stimulated scattering from reservoirs of high-energy excitons. A generic few-parameter model for the system leads to a Lindblad equation which includes saturable pumping, decay, and condensate interactions. We show how this theory can be used to obtain the population distributions, and the time-dependent first- and second-order coherence functions, in such a multimode condensate. As a specific application, w…
We study a model of a photon mode dipole-coupled to a medium of two-level oscillators in a microcavity in the presence of dephasing processes introduced by coupling to external baths. Decoherence processes can be classified as pair-breaking or non-pair-breaking in analogy with magnetic or non-magnetic impurities in superconductors. In the absence of dephasing, the ground state of the model is a polariton condensate with a gap in the excitation spectrum. Increase of the pair-breaking parameter $γ$ reduces the gap, which becomes zero at a critical value $γ_{C1}$; for large $γ$, the conventional …
We propose a method to enhance the spatial coupling between ballistic exciton-polariton condensates in a semiconductor microcavity based on available spatial light modulator technologies. Our method, verified by numerically solving a generalized Gross-Pitaevskii model, exploits the strong nonequilibrium nature of exciton-polariton condensation driven by localized nonresonant optical excitation. Tailoring the excitation beam profile from a Gaussian into a polygonal shape results in refracted and focused radial streams of outflowing polaritons from the excited condensate which can be directed to…
A full quantum theory beyond the mean-field regime is developed for an exciton polariton condensate, to gain a complete understanding of quantum fluctuations. We find analytical solution for the polariton density matrix, showing the polariton nonlinearity causing fast relaxation correlated with the pump so as to yield the condensation at threshold. Increasing the pump intensity, a nonequilibrium phase transition towards the condensation of lower polaritons emerges, with a statistics transiting from a thermal, through a super-Poissonian and to a nonclassical distribution beyond the understandin…
In the first part of this thesis I study the intermediate regime between ordinary lasing and a BEC of exciton polaritons. I take into account the fermionic structure of polaritons, treating the excitons as two-level systems coupled to a single mode in a microcavity. I introduce decoherence and dissipation processes to this system. Employing many-body Green function techniques, similar to those used by Abrikosov and Gor'kov in their theory of gapless superconductivity, I provide a mathematical structure that unifies models of lasers with models of condensates. This allows me to study the stabil…
In this letter, we give an analytical quantum description of a non-equilibrium polariton Bose-Einstein condensate (BEC) based on the solution of the master equation for the full polariton density matrix in the limit of fast thermalization. We find the density matrix of a non-equilibrium BEC, that takes into account quantum correlations between all polariton states. We show that the formation of BEC is accompanied by the build-up of cross-correlations between the ground state and the excited states reaching their highest values at the condensation threshold. Despite the non-equilibrium nature o…
Semiconductor microcavity systems strongly coupled to quantum wells are now receiving a great deal of attention because of their ability to efficiently generate coherent light by the Bose-Einstein condensation (BEC) of an exciton-polariton gas. Since the exciton polaritons are composite quasi-bosonic particles, many fundamental features arise from their original constituents, i.e., electrons, holes and photons. As a result, not only equilibrium phases typified by the BEC but also nonequilibrium lasing phases can be achieved. In this contribution, we describe a framework which can treat such eq…
Bose-Einstein condensation is a remarkable manifestation of quantum statistics and macroscopic quantum coherence. Superconductivity and superfluidity have their origin in Bose-Einstein condensation. Ultracold quantum gases have provided condensates close to the original ideas of Bose and Einstein, while condensation of polaritons and magnons have introduced novel concepts of non-equilibrium condensation. Here, we demonstrate a Bose-Einstein condensate (BEC) of surface plasmon polaritons in lattice modes of a metal nanoparticle array. Interaction of the nanoscale-confined surface plasmons with …
When molecular transitions strongly couple to photon modes, they form hybrid light-matter modes called polaritons. Collective vibrational strong coupling is a promising avenue for control of chemistry, but this can be deterred by the large number of quasi-degenerate dark modes. The macroscopic occupation of a single polariton mode by excitations, as observed in Bose-Einstein condensation, offers promise for overcoming this issue. Here we theoretically investigate the effect of vibrational polariton condensation on the kinetics of electron transfer processes. Compared with excitation with infra…
Magnetic control of an exciton-polariton condensate in a van der Waals magnet
University of Regensburg（雷根斯堡大学）；Technical University of Munich（慕尼黑工业大学）；University of Chemistry and Technology Prague（布拉格化工大学）；Regensburg Center for Ultrafast Nanoscopy（雷根斯堡超快纳米学中心）；Université Paris Cité（巴黎西岱大学）
Exciton-polaritons are hybrid elementary excitations of light and matter that, thanks to their nonlinear properties, enable a plethora of physical phenomena ranging from room temperature condensation to superfluidity. While polaritons are usually exploited in high density regime, evidence of quantum correlations at the level of few excitations has been recently reported, thus suggesting the possibility of using these systems for quantum information purposes. Here we show that integrated circuits of propagating single polaritons can be arranged to build deterministic quantum logic gates in whic…
