We consider a two-dimensional extension of the 1D waveguide quantum electrodynamics and investigate the nature of linear excitations in two-dimensional arrays of qubits coupled to networks of chiral waveguides. We show that the combined effects of chirality and long-range photon mediated qubit-qubit interactions lead to the emergence of the two-dimensional flat bands in the polaritonic spectrum, corresponding to slow strongly correlated light.
We investigate polariton-phonon hybrid excitations, which describe the collective excitations of emitter-photon polaritons and vibrational phonons, in a periodic array of vibrating two-level emitters interacting with waveguide photons. We demonstrate the emergence of an interaction-induced quasiperiodic structure caused by the interplay between phonon scatterings and waveguide-mediated long-range couplings. This quasiperiodicity fundamentally changes the excitation characteristics in the subradiant regime, which feature an appearance of topological edge states and a transition between ergodic …
We investigate the phenomena of Brillouin induced opacity in nanoscale linear waveguides and Brillouin induced transparency in nanoscale ring waveguides. The concept of phonon-polariton is required in order to get a deep understanding of such phenomena. Phonon-polaritons are coherent superposition of photons and phonons obtained in the strong coupling regime induced through stimulated Brillouin scattering in the presence of a pump field. The formation of phonon-polaritons can be observed via linear optical spectra that are calculated here using the input-output formalism. For a linear waveguid…
We experimentally demonstrate the propagation of long-range surface plasmon-polaritons in a nobel metal stripe waveguide at an optical wavelength of 780 nm. To minimize propagation damping the lithographically structured waveguide is produced from a thin gold stripe embedded in a dielectric polymer. Our waveguide geometry supports a symmetric fundamental and anti-symmetric first order mode. For the fundamental mode we measure a propagation loss of $(6.12^{+0.66} _{-0.54})$ dB/mm, in good agreement with numerical simulations using a vectorial eigenmode solver. Our results are a promising starti…
Exciton-polaritons are hybrid light-matter excitations arising from the non-perturbative coupling of a photonic mode and an excitonic resonance. Behaving as interacting photons, they show optical third-order nonlinearities providing effects such as optical parametric oscillation or amplification. It has been suggested that polariton-polariton interactions can be greatly enhanced by inducing aligned electric dipoles in their excitonic part. However direct evidence of a true particle-particle interaction, such as superfluidity or parametric scattering is still missing. In this work, we demonstra…
Single surface plasmon polaritons are excited using photons generated via spontaneous parametric down-conversion. The mean excitation rates, intensity correlations and Fock state populations are studied. The observed dependence of the second order coherence in our experiment is consistent with a linear uncorrelated Markovian environment in the quantum regime. Our results provide important information about the effect of loss for assessing the potential of plasmonic waveguides for future nanophotonic circuitry in the quantum regime.
Boosting self hybridized exciton polaritons with metal clad WS2 waveguides
Institute of Experimental and Applied Physics, Kiel University（基尔大学实验与应用物理研究所）；Ruprecht Haensel Laboratory, Deutsches Elektronen-Synchrotron DESY（德国电子同步加速器研究所鲁普雷希特·亨塞尔实验室）
We investigate how the dynamical Casimir effect can entangle quantum systems in different coupling regimes of circuit quantum electrodynamics, and show the robustness of such entanglement generation against dissipative effects with current technology. We consider two qubit-resonator systems, which are coupled by a SQUID driven with an external magnetic field, and explore the entire range of coupling regimes between each qubit and its respective resonator. In this scheme, we derive a semianalytic explanation for the entanglement generation between both superconducting qubits when they are coupl…
Microscopic theory of exciton-polariton model involving multiple molecules: Macroscopic quantum electrodynamics formulation and essence of direct intermolecular interactions
Architectures based on waveguide quantum electrodynamics have emerged as promising candidates for quantum networks. In this paper, we analyze the propagation of single-photons in disordered many-atom waveguides. We pay special attention to the influence of chirality (directionality of photon transport) on the formation of localized photonic states, considering separately the cases of the disorder in the atomic positions and in the atomic transition frequencies.
Quantum correlations between distant particles remain enigmatic since the birth of quantum mechanics. Here we predict a novel kind of bound quantum state in the simplest one-dimensional setup of two interacting particles in a box. Paradoxically, two entangled particles become localized at the opposite edges of the box even though their interactions at large distance should seemingly play no role. Such states could be realized in the waveguide quantum electrodynamics platform, where an array of superconducting qubits or cold atoms is coupled to a waveguide. We demonstrate how long-range wavegui…
Coherent light-matter interaction at the single photon and electronic qubit level promises the remarkable potential for nonclassical information processing. Against the efforts of improving the figure of merit of the cavities, here we demonstrate strong anharmonicity in the polariton dressed states via dark state resonances in a highly dissipative cavity. It is shown that vacuum Rabi oscillation occurs for a single quantum emitter inside a cavity even with bosonic decay-to-interaction rate ratio exceeding $10^{2}$, when the photon field is coupled to an auxiliary high-$Q$ cavity. Moreover, pho…
We identify a general connection between the physics of exceptional points in non-Hermitian systems and the few-photon bound states in waveguide quantum electrodynamics (QED) systems. We show that, in waveguide QED systems where the local quantum system exhibits an exceptional point, the tightest-bound few-photon bound state occurs at the exceptional point. We illustrate this connection with an explicit computation on a waveguide QED system in which a waveguide is coupled to a Jaynes-Cummings system. Our result provides a quantum signature of the exceptional point physics and indicates that th…
While the theoretical studies in waveguide quantum electrodynamics predominate with single-photon and two-photon Fock state (photon number states) input, the experiments are primarily carried out using a faint coherent light. We create a theoretical toolbox to compare and contrast linear and nonlinear light scattering by a two-level or a three-level emitter embedded in an open waveguide carrying Fock state or coherent state inputs. We identify rules to compare light transport properties, the Kerr, and cross-Kerr nonlinearities of the medium for the two types of inputs. A generalized descriptio…
The requirement for optical-electrical-optical conversion of signals in optical technologies is often one of the majors bottleneck in terms of speed and energy consumption. The use of dressed photons (also called polaritons), that allows for intrinsic sizable interactions, could significantly improve the performances of optical integrated elements such as switches or optical gates. In this work we demonstrate the ultrafast switch of a laser coupled into a polaritonic waveguide triggered by an optical pulse resonant with the same dispersion but at a lower energy. Our experiments show two effect…
We consider the quantum electrodynamics of a binary array of chiral waveguides, each containing many atoms. We show that the one-photon amplitude of a single-excitation state obeys a two-dimensional Dirac equation. Using this result, we develop the scattering theory for the Dirac equation in this setting and illustrate our results with numerical simulations.
In this review we present the theoretical foundations and first principles frameworks to describe quantum matter within quantum electrodynamics (QED) in the low-energy regime. Having a rigorous and fully quantized description of interacting photons, electrons and nuclei/ions, from weak to strong light-matter coupling regimes, is pivotal for a detailed understanding of the emerging fields of polaritonic chemistry and cavity materials engineering. The use of rigorous first principles avoids ambiguities and problems stemming from using approximate models based on phenomenological descriptions of …
Photons strongly coupled to material systems constitute a novel system for studying the dynamics of non-equilibrium quantum many-body systems. We give a fully analytical description of the dynamics of photons coupled to a one-dimensional array of two-level atoms. The description incorporates input, scattering inside the medium, and the ejection of photons from the array. We show that inelastic collisions, previously identified in small systems, also occur in infinite systems and elucidate the physics behind this effect. The developed theory constitutes an effective field theory for the dynamic…
Unidirectional reflectionlessness is investigated in a waveguide quantum electrodynamics system that consists of a cavity and a $Λ$-type three-level quantum dot coupled to a one-dimensional plasmonic waveguide. Analytical expressions of transmission and reflection coefficients are derived and discussed for both resonant and off-resonant couplings. By appropriately modulating the coupling strength, phase shift and Rabi frequency, unidirectional reflectionlessness is observed at the exceptional points. And unidirectional coherent perfect absorption is exhibited at the vicinity of exceptional poi…
We study single photon transport in a one-dimensional disordered lattice of three-level atoms coupled to an optical waveguide. In particular, we study atoms of Λ-type that are capable of exhibiting electromagnetically induced transparency (EIT) and separately consider disorder in the atomic positions and transition frequencies. We mainly address the question of how preferential emission into waveguide modes (chirality) can influence the formation of spatially localized states. Our work has relevance to experimental studies of cold atoms coupled to nanoscale waveguides and has possible applicat…
A lattice of trapped atoms strongly coupled to a one-dimensional nanophotonic waveguide is investigated in exploiting the concept of polariton as the system natural eigenstate. We apply a bosonization procedure, which was presented separately by P. W. Anderson and V. M. Agranovich, to transform excitation spin-half operators into interacting bosons, and which shown here to confirm the hard-core boson model. We derive polariton-polariton kinematic interactions and study them by solving the scattering problem. In using the excitation-photon detuning as a control parameter, we examine the regime …
We present the general structure of two-photon S matrix for a waveguide coupled to a local quantum system that supports multiple ground states. The presence of the multiple ground states results in a non-commutative aspect of the system with respect to the exchange of the orders of photons. Consequently, the two-photon S matrix significantly differs from the standard form as described by the cluster decomposition principle in the quantum field theory.
We theoretically predict the formation of two-photon bound states in a two-dimensional waveguide network hosting a lattice of two-level atoms. The properties of these bound pairs and the exclusive domains of the parameter space where they emerge due to the interplay between the on-site photon blockade and peculiar shape of polariton dispersion resulting from the long-range radiative couplings between the qubits are investigated in detail. In addition, we analyze the effect of the finite-size system on localization characteristics of these excitations.
We study the coherent properties of plasmon polaritons optically excited on periodic nanostructures. The gold grains are coupled to a single mode photonic waveguide which exhibits a dramatically reduced transmission originating from the derived quantum interference. With a nonequilibrium description of Floquet-dressed polaritons we demonstrate the switching of light transmission through the waveguide due to sheer existence of intraband transitions in gold from right above the Fermi level driven by the external laser light.
It has been proved that surface plasmon polariton (SPP) can well conserve and transmit the quantum nature of entangled photons. Therefore, further utilization and manipulation of such quantum nature of SPP in a plasmonic chip will be the next task for scientists in this field. In quantum logic circuits, the controlled-NOT (CNOT) gate is the key building block. Here, we implement the first plasmonic quantum CNOT gate with several-micrometer footprint by utilizing a single polarization-dependent beam-splitter (PDBS) fabricated on the dielectric-loaded SPP waveguide (DLSPPW). The quantum logic fu…
We examine the propagation of single photons in periodic and disordered dimer chains coupled to one-dimensional chiral and bidirectional waveguides. Each dimer is composed of two dipole-coupled atoms. In the disordered setting, we separately treat two types of position disorder, namely in dimer length and in dimer separation. The focus of this study is to understand in what ways the interplay between dipole-dipole interactions and directionality of photon emission can impact the transport of single photons. Cold atoms trapped near optical fibers can serve as an experimentally realizable platfo…
Realizing a fully connected network of quantum processors requires the ability to distribute quantum entanglement. For distant processing nodes, this can be achieved by generating, routing, and capturing spatially entangled itinerant photons. In this work, we demonstrate the deterministic generation of such photons using superconducting transmon qubits that are directly coupled to a waveguide. In particular, we generate two-photon N00N states and show that the state and spatial entanglement of the emitted photons are tunable via the qubit frequencies. Using quadrature amplitude detection, we r…
This review describes the emerging field of waveguide quantum electrodynamics (WQED) concerned with the interaction of photons propagating in a waveguide with localized quantum emitters. The collective emitter-photon interactions can lead to both enhanced and suppressed coupling compared to the case of independent emitters. Here, we focus on guided photons and ordered arrays, leading to super- and sub-radiant states, bound photon states and quantum correlations with promising quantum information applications. We highlight recent groundbreaking experiments performed with different quantum platf…
We study the collective decay rates of multi-dimensional quantum networks in which one-dimensional waveguides form an intersecting hyper-rectangular lattice, with qubits located at the lattice points. We introduce and motivate the \emph{dimensional reduction of poles} (DRoP) conjecture, which identifies all collective decay rates of such networks via a connection to waveguides with a one-dimensional topology (e.g. a linear chain of qubits). Using DRoP, we consider many-body effects such as superradiance, subradiance, and bound-states in continuum in multi-dimensional quantum networks. We find …
We propose a robust and broadband integrated terahertz (THz) coupler based on the in-plane surface plasmon polaritons (SPPs) waveguides, conducted with the quantum coherent control -- Stimulated Raman Adiabatic Passage (STIRAP). Our coupler consists of two asymmetric specific curved corrugated metallic structures working as the input and output SPPs waveguides, and one straight corrugated metallic structure functioning as the middle SPPs waveguide. From the theoretical and simulated results, we demonstrate that the SPPs can be efficiently transfered from the input to the output waveguides. Our…
While designing the energy-momentum relation of photons is key to many linear, non-linear, and quantum optical phenomena, a new set of light-matter properties may be realized by employing the topology of the photonic bath itself. In this work we investigate the properties of superconducting qubits coupled to a metamaterial waveguide based on a photonic analog of the Su-Schrieffer-Heeger model. We explore topologically-induced properties of qubits coupled to such a waveguide, ranging from the formation of directional qubit-photon bound states to topology-dependent cooperative radiation effects.…
We investigate the behavior of two quantum emitters (two-level atoms) embedded in a linear waveguide, in a quasi-one-dimensional configuration. Since the atoms can emit, absorb and reflect radiation, the pair can spontaneously relax towards an entangled bound state, under conditions in which a single atom would instead decay. We analyze the properties of these bound states, which occur for resonant values of the interatomic distance, and discuss their relevance with respect to entanglement generation. The stability of such states close to the resonance is studied, as well as the properties of …
We study theoretically driven quantum dynamics in periodic arrays of two-level qubits coupled to the waveguide. We demonstrate, that strongly subradiant eigenstates of the master equation for the density matrix emerge under strong coherent driving for arrays with the anti-Bragg periods $d=λ/4,3λ/4$... This happens even though are no such states at low driving powers. Thus, our findings show that in the quantum nonlinear regime the domain of existence of subradiant states expands beyond conventional subwavelength structures. These driven states are directly manifested in long-living quantum cor…
We propose a novel quantum electrodynamics (QED) platform where quantum emitters interact with a Hofstadter-ladder waveguide. We demonstrate several intriguing phenomena stemming from the exotic dispersion relation and vacuum mode properties led by the effective spin-orbit coupling, which have no analog in other QED setups. First, by assuming emitter's frequency to be resonant with the lower band, we find that the spontaneous emission is chiral with most photonic field decaying unidirectionally. Both numerical and analytical results indicate that the Hofstadter-ladder waveguide can be engineer…
Dark state spectroscopy in nonlinear waveguide quantum electrodynamics
Andrew and Erna Viterbi Department of Electrical & Computer Engineering, Technion - Israel Institute of Technology（安德鲁和埃尔纳·维特比电气与计算机工程系，以色列理工学院）；Helen Diller Quantum Center, Technion - Israel Institute of Technology（海伦·迪勒量子中心，以色列理工学院）
We provide the first classification of three-photon eigenstates in a finite periodic array of two-level atoms coupled to a waveguide. We focus on the strongly subwavelength limit and show the hierarchical structure of the eigenstates in the complex plane. The main characteristic eigenstates are explored using entanglement entropy as a distinguishing feature. We show that the rich interplay of effects from order, chaos to localisation found in two-photon systems extends naturally to three-photon systems. There also exist interaction-induced localised states unique to three-photon systems such a…
We study theoretically subradiant states in the array of atoms coupled to photons propagating in a one-dimensional waveguide focusing on the strongly interacting many-body regime with large excitation fill factor $f$. We introduce a generalized many-body entropy of entanglement based on exact numerical diagonalization followed by a high-order singular value decomposition. This approach has allowed us to visualize and understand the structure of a many-body quantum state. We reveal the breakdown of fermionized subradiant states with increase of $f$ with emergence of short-ranged dimerized antif…
Non-Markovian time-evolution of quantum systems is a challenging problem, often mitigated by employing numerical methods or making simplifying assumptions. In this work, we address this problem in waveguide QED by developing a diagrammatic approach, which performs fully analytical non-Markovian time evolution of single-photon states. By revisiting Fermi's two atom problem, we tackle the impeding question of whether rotating-wave approximation violates causality in single-photon waveguide QED. Afterward, we introduce and prove the \emph{no upper half-plane poles (no-UHP) theorem}, which connect…
We explore amplification and cross-Kerr nonlinearity by a three-level emitter (3LE) embedded in a waveguide and driven by two light beams. The coherent amplification and cross-Kerr nonlinearity were demonstrated in recent experiments, respectively, with a V and a ladder-type 3LE coupled to an open superconducting transmission line carrying two microwave fields. Here, we consider $Λ$, V, and ladder-type 3LE, and compare the efficiency of coherent and incoherent amplification as well as the magnitude of the cross-Kerr phase shift in all three emitters. We apply the Heisenberg-Langevin equations …
Phonon interactions are inevitable in cavity quantum electrodynamical systems based on solid-state emitters or fluorescent molecules, where vibrations of the lattice or chemical bonds couple to the electronic degrees of freedom. Due to the non-Markovian response of the vibrational environment, it remains a significant theoretical challenge to describe such effects in a computationally efficient manner. This is particularly pronounced when the emitter-cavity coupling is comparable to or larger than the typical phonon energy range, and polariton formation coincides with vibrational dressing of t…
We study the dynamics of a general multi-emitter system coupled to the squeezed vacuum reservoir and derive a master equation for this system based on the Weisskopf-Wigner approximation. In this theory, we include the effect of positions of the squeezing sources which is usually neglected in the previous studies. We apply this theory to a quasi-one-dimensional waveguide case where the squeezing in one dimension is experimentally achievable. We show that while dipole-dipole interaction induced by ordinary vacuum depends on the emitter separation, the two-photon process due to the squeezed vacuu…
The embedding of tunable quantum emitters in a photonic bandgap structure enables the control of dissipative and dispersive interactions between emitters and their photonic bath. Operation in the transmission band, outside the gap, allows for studying waveguide quantum electrodynamics in the slow-light regime. Alternatively, tuning the emitter into the bandgap results in finite range emitter-emitter interactions via bound photonic states. Here we couple a transmon qubit to a superconducting metamaterial with a deep sub-wavelength lattice constant ($λ/60$). The metamaterial is formed by periodi…
Loss resilience of driven-dissipative remote entanglement in chiral waveguide quantum electrodynamics
University of Illinois Urbana-Champaign（伊利诺伊大学厄巴纳-香槟分校）；Pritzker School of Molecular Engineering, University of Chicago（芝加哥大学普里茨克分子工程学院）；Department of Physics, University of Chicago（芝加哥大学物理系）
Quantum information is typically encoded in the state of a qubit that is decoupled from the environment. In contrast, waveguide quantum electrodynamics studies qubits coupled to a mode continuum, exposing them to a loss channel and causing quantum information to be lost before coherent operations can be performed. Here we restore coherence by realizing a dark state that exploits symmetry properties and interactions between four qubits. Dark states decouple from the waveguide and are thus a valuable resource for quantum information but also come with a challenge: they cannot be controlled by th…
