Parallel dark soliton pair in a bistable 2D exciton-polariton superfluid
Giovanni Lerario, Sergei V. Koniakhin, Anne Maître, Dmitry Solnyshkov, Alessandro Zilio, Quentin Glorieux, Guillaume Malpuech, Elisabeth Giacobino, Simon Pigeon, Alberto Bramati
Collective excitations, such as vortex-antivortex and dark solitons, are among the most fascinating effects of macroscopic quantum states. However, 2D dark solitons are unstable and collapse into vortices due to snake instabilities. Making use of the optical bistability in exciton-polariton microcavities, we demonstrate that a pair of dark solitons can be formed in the wake of an obstacle in a polariton flow resonantly supported by a homogeneous laser beam. Unlike the purely dissipative case where the solitons are grey and spatially separate, here the two solitons are fully dark, rapidly align at a specific separation distance and propagate parallel as long as the flow is in the bistable regime. Remarkably, the use of this regime allows to avoid the phase fixing arising in resonant pumping regime and to circumvent the polariton decay. Our work opens very wide perspectives of studying new classes of phase-density defects which can form in driven-dissipative quantum fluids of light.
Microcavity exciton polaritons are promising candidates to build a new generation of highly nonlinear and integrated optoelectronic devices. Such devices range from novel coherent light emitters to reconfigurable potential landscapes for electro-optical polariton-lattice based quantum simulators as well as building blocks of optical logic architectures. Especially for the latter, the strongly interacting nature of the light-matter hybrid particles has been used to facilitate fast and efficient switching of light by light, something which is very hard to achieve with weakly interacting photons.…
Motivated by recent experiments, we theoretically analyze the flow past an obstacle of a one-dimensional "quantum fluid of light" which is resonantly driven, and exhibits bistability. The flow is found to abruptly change several times when the fluid velocity or the obstacle potential strength are increased. In contrast to the cases of usual fluids and superfluids, the transitions take place between stationary states. They involve the fluid bistability in an essential way. Remarkably, at the transitions points, the fluid in the obstacle wake lies in the unstable intermediate density state.
In this work, we implement a new experimental configuration which exploits the specific properties of the optical bistability exhibited by the polariton system and we demonstrate the generation of a superfluid turbulent flow in the wake of a potential barrier. The propagation and direction of the turbulent flow are sustained by a support beam on distances an order of magnitude longer than previously reported. This novel technique is a powerful tool for the controlled generation and propagation of quantum turbulences and paves the way to the study of the hydrodynamic of quantum turbulence in dr…
The general theory of dark solitons relies on repulsive interactions and therefore predicts the impossibility to form dark-soliton bound states. One important exception to this prediction is the observation of bound solitons in non-local nonlinear media. Here, we report that exciton-polariton superfluids can also sustain dark-soliton molecules although the interactions are fully local. With a novel all optical technique, we create two dark solitons and bind them to each other to form an unconventional dark-soliton molecule. We demonstrate that the stability of this structure and the separation…
In resonantly pumped polariton superfluids we recently explored a new regime based on the bistability of the polariton system to enhance the propagation of polariton fluids up to macroscopic distances. This technique together with an all-optical imprinting method allowed the generation and control of various topological excitations such as quantized vortices and dark solitons. The flexibility and scalability of the new experimental scheme opens the way to the systematic study of quantum turbulence in driven dissipative quantum fluids of light. In this article we review the basic working princi…
We report the formation of a macroscopic coherent state emerging from colliding polariton fluids. Four lasers with random relative phases, arranged in a square, pump resonantly a planar microcavity, creating four coherent polariton fluids propagating toward each other. When the density (interactions) increases, the four fluids synchronise and the topological excitations (vortex or soliton) disappear to form a single superfluid.
We present a simple method to compensate for losses in a polariton superfluid. Based on a weak support field, it allows for an extended propagation of a resonantly driven polariton superfluid at a minimal energetic cost. Moreover, this setup based on optical bistability, leads to a significant release of the phase constraint imposed by the resonant driving. This release, together with the macroscopic polariton propagation, offers a unique opportunity to study the hydrodynamics of topological excitations of polariton superfluids such as quantized vortices and dark solitons. We numerically study…
We report the experimental investigation and theoretical modeling of a rotating polariton superfluid relying on an innovative method for the injection of angular momentum. This novel, multi-pump injection method uses four coherent lasers arranged in a square, resonantly creating four polariton populations propagating inwards. The control available over the direction of propagation of the superflows allows injecting a controllable non-quantized amount of optical angular momentum. When the density at the center is low enough to neglect polariton-polariton interactions, optical singularities, ass…
We theoretically study Hawking radiation processes from an analog acoustic black hole in a flowing superfluid of exciton-polaritons in a one-dimensional semiconductor microcavity. Polaritons are coherently injected into the microcavity by a laser pump with a suitably tailored spot profile. An event horizon with a large analog surface gravity is created by inserting a defect in the polariton flow along the cavity plane. Experimentally observable signatures of the analog Hawking radiation are identified in the scattering of phonon wavepackets off the horizon, as well as in the spatial correlatio…
We study the Berezinskii-Kosterlitz-Thouless mechanism for vortex-antivortex pair formation in two-dimensional superfluids for nonequilibrium condensates. Our numerical study is based on a classical field model for driven-dissipative quantum fluids that is applicable to polariton condensates. We investigate the critical noise needed to create vortex-antivortex pairs in the systems, starting from a state with uniform phase. The dependence of the critical noise on the nonequilibrium and energy relaxation parameters is analyzed in detail.
We develop a theory for the interaction of light with superfluid optical media, describing the motion of quantum impurities that are created and dragged through the liquid by propagating photons. It is well known that a mobile impurity suffers dissipation due to phonon emission as soon as it moves faster than the speed of sound in the superfluid - Landau's critical velocity. Surprisingly we find that in the present hybrid light-matter setting, polaritonic impurities can be protected against environmental decoherence and be allowed to propagate well above the Landau velocity without jeopardizin…
The dynamics of an exciton-polariton superfluid resonantly pumped in a semiconductor microcavity are investigated by mean-field theory. Modulational instability develops into crystalline order and then ordered and disordered states alternately form. A supersolid-like state is also found, in which superflow coexists with crystalline order at rest.
Steady states reached in a coherently pumped exciton-polariton superfluid are investigated. As the pump parameter is changed, the translational symmetry of the uniform system is spontaneously broken, and various steady patterns of quantized vortices are formed. This is peculiar to nonequilibrium dissipative systems with continuous pumping.
We study the necessary condition under which a resonantly driven exciton polariton superfluid flowing against an obstacle can generate turbulence. The value of the critical velocity is well estimated by the transition from elliptic to hyperbolic of an operator following ideas developed by Frisch, Pomeau, Rica for a superfluid flow around an obstacle, though the nature of equations governing the polariton superfluid is quite different. We find analytical estimates depending on the pump amplitude and on the pump energy detuning, quite consistent with our numerical computations.
Due to their driven-dissipative nature, photonic quantum fluids present new challenges in understanding superfluidity. Some associated effects have been observed, and notably the report of nearly dissipationless flow for coherently driven microcavity-polaritons was taken as a smoking gun for superflow. Here we show that the superfluid response --- the difference between responses to longitudinal and transverse forces --- is zero for coherently driven polaritons. This is a consequence of the gapped excitation spectrum caused by external phase locking. Furthermore, while a normal component exist…
We report the formation of a ring-shaped array of vortices after injection of angular momentum in a polariton superfluid. The angular momentum is injected by a $\ell= 8$ Laguerre-Gauss beam, whereas the global rotation of the fluid is hindered by a narrow Gaussian beam placed at its center. In the linear regime a spiral interference pattern containing phase defects is visible. In the nonlinear (superfluid) regime, the interference disappears and the vortices nucleate as a consequence of the angular momentum quantization. The radial position of the vortices evolves freely in the region between …
The experimental investigation of spontaneously created vortices is of utmost importance for the understanding of quantum phase transitions towards a superfluid phase, especially for two dimensional systems that are expected to be governed by the Berezinski-Kosterlitz-Thouless physics. By means of time resolved near-field interferometry we track the path of such vortices, created at random locations in an exciton-polariton condensate under pulsed non-resonant excitation, to their final pinning positions imposed by the stationary disorder. We formulate a theoretical model that successfully repr…
Rotation of a container holding a viscous fluid forms a vortex which grows with increasing angular velocity. A superfluid, however, is intrinsically different from these normal fluids because its rotation is quantized. Even if a container of superfluid is rotating, the fluid itself remains still until a critical velocity is reached. Beyond the critical velocity, all the particles conspire to suddenly pick up an angular momentum of $\hbar$ each and forms a quantized vortex. As a result, a superfluid is known to increase its rotation by a total angular momentum of $N\hbar$. In this letter, we sh…
The dynamics of an exciton--polariton superfluid resonantly injected into a semiconductor microcavity are investigated numerically. The results reveal that a Bénard--von Kármán vortex street is generated in the wake behind an obstacle potential, in addition to the generation of quantized vortex dipoles and dark solitons. The vortex street is shown to be robust against a disorder potential in a sample and it can be observed even in time-integrated measurements.
Superfluidity---the suppression of scattering in a quantum fluid at velocities below a critical value---is one of the most striking manifestations of the collective behaviour typical of Bose-Einstein condensates. This phenomenon, akin to superconductivity in metals, has until now only been observed at prohibitively low cryogenic temperatures. For atoms, this limit is imposed by the small thermal de Broglie wavelength, which is inversely related to the particle mass. Even in the case of ultralight quasiparticles such as exciton-polaritons, superfluidity has only been demonstrated at liquid heli…
We study non-equilibrium polariton superfluids in the optical parametric oscillator (OPO) regime using a two-component Gross-Pitaevskii equation with pumping and decay. We identify a regime above OPO threshold, where the system undergoes spontaneous symmetry breaking and is unstable towards vortex formation without any driving rotation. Stable vortex solutions differ from metastable ones; the latter can persist in OPO superfluids but can only be triggered externally. Both spontaneous and triggered vortices are characterised by a generalised healing length, specified by the OPO parameters only.
We study the properties of propagating polariton wave-packets and their connection to the stability of doubly charged vortices. Wave-packet propagation and related photoluminescence spectra exhibit a rich behaviour dependent on the excitation regime. We show that, because of the non-quadratic polariton dispersion, doubly charged vortices are stable only when initiated in wave-packets propagating at small velocities. Vortices propagating at larger velocities, or those imprinted directly into the polariton optical parametric oscillator (OPO) signal and idler are always unstable to splitting.
We study the properties of a binary microcavity polariton superfluid coherently injected by two lasers. The crossover from the supersonic to subsonic regime, where motion is frictionless, is described by evaluating the Bogoliubov spectra. We show that according to the Landau criteria, the coupling between the two components precludes the existence of superfluidity just for one component but not for the other. By analysing the drag force exerted on a defect, we give a recipe to experimentally address the crossover from the supersonic to the subsonic regime.
Exciton-polariton condensate in semiconductor microcavities constitute a novel kind of non-equilibrium superfluid. In a recent experiment [P. Stepanov, {\it et. al.,} Nat. Commun. {\bf 10}, 1038 (2019)], the dispersion relation of collective excitations in a polariton condensate under the resonant pumping has been investigated with the emphasis on the role of reservoir of long-lived excitons in determining the superfluidity. Inspired by such an experimental advance, we study the superfluidity of a exciton-polaritonn condensate under non-resonant pumping by calculating the drag force exerted on…
Exciton-polaritons are quasi-particles arising from the strong coupling regime between excitons and photons. In planar microcavitites, phenomena such as superfluidity or Bose-Einstein condensation can be observed. Those systems have demonstrated to be very efficient in the hydrodynamic generation of topological excitations, such as vortex-antivortex pairs or dark solitons. However, the lifetime and motion of those excitations were limited by the driven dissipative nature of the system. In this thesis, we present a rich variety of results about the generation and control of such topological exc…
Quantum effects of fields on curved spacetimes may be studied in the laboratory thanks to quantum fluids. Here we use a polariton fluid to study the Hawking effect, the correlated emission from the quantum vacuum at the acoustic horizon. We show how out-of-equilibrium physics affects the dispersion relation, and hence the emission and propagation of correlated waves: the fluid properties on either side of the horizon are critical to observing the Hawking effect. We find that emission may be optimised by supporting the phase and density of the fluid upstream of the horizon in a regime of optica…
Quantum fluids of light are an emerging platform for energy efficient signal processing, ultra-sensitive interferometry and quantum simulators at elevated temperatures. Here we demonstrate the optical control of the topological excitations induced in a large polariton condensate, realising the bosonic analog of a long Josephson junction and reporting the first observation of bosonic Josephson vortices. When a phase difference is imposed at the boundaries of the condensate, two extended regions become separated by a sharp $π$-slippage of the phase and a solitonic depletion of the density, formi…
We consider the possible phases of microcavity polaritons tuned near a bipolariton Feshbach resonance. We show that, as well as the regular polariton superfluid phase, a "molecular" superfluid exists, with (quasi-)long-range order only for pairs of polaritons. We describe the experimental signatures of this state. Using variational approaches we find the phase diagram (critical temperature, density and exciton-photon detuning). Unlike ultracold atoms, the molecular superfluid is not inherently unstable, and our phase diagram suggests it is attainable in current experiments.
A quantum fluid passing an obstacle behaves differently from a classical one. When the flow is slow enough, the quantum gas enters a superfluid regime and neither whirlpools nor waves form around the obstacle. For higher flow velocities, it has been predicted that the perturbation induced by the defect gives rise to the turbulent emission of quantised vortices and to the nucleation of solitons. Using an interacting Bose gas of exciton-polaritons in a semiconductor microcavity, we report the transition from superfluidity to the hydrodynamic formation of oblique dark solitons and vortex streets …
The dark solitons observed in a large variety of nonlinear media are unstable against the modulational (snake) instabilities and can break in vortex streets. This behavior has been investigated in nonlinear optical crystals and ultracold atomic gases. However, a deep characterization of this phenomenon is still missing. In a resonantly pumped 2D polariton superfluid, we use an all-optical imprinting technique together with the bistability of the polariton system to create dark solitons in confined channels. Due to the snake instabilities, the solitons are unstable and break in arrays of vortex…
In this paper we discuss, within the Gross--Pitaevskii framework, superfluidity, soliton nucleation, and instabilities in a non-equilibrium polariton fluid injected by a spatially localized and continuous-wave coherent pump and flowing against a defect located outside the pump spot. In contrast to equilibrium condensates, the steady-state solutions of the driven-dissipative equations in this specific geometry hardly show a clean superfluid flow around the defect and rather feature a crossover from shallow to deep soliton-like perturbation. This is explained in terms of the properties of one-di…
Fluids of exciton-polaritons, excitations of two dimensional quantum wells in optical cavities, show collective phenomena akin to Bose condensation. However, a fundamental difference from standard condensates stems from the finite life-time of these excitations, which necessitate continuous driving to maintain a steady state. A basic question is whether a two dimensional condensate with long range algebraic correlations can exist under these non-equilibrium conditions. Here we show that such driven two-dimensional Bose systems cannot exhibit algebraic superfluid order except in low-symmetry, a…
Recently, exciton-polaritons in a semiconductor microcavity were found to condense into a coherent ground state much like a Bose-Einstein condensate and a superfluid. They have become a unique testbed for generating and manipulating quantum vortices in a driven-dissipative superfluid. Here, we generate exciton-polariton condensate with non-resonant Laguerre-Gaussian (LG) optical beam and verify the direct transfer of light's orbital angular momentum to exciton-polariton quantum fluid. Quantized vortices are found in spite of large energy relaxation involved in non-resonant pumping. We identifi…
We study the spin vortices and skyrmions coherently imprinted into an exciton-polariton condensate on a planar semiconductor microcavity. We demonstrate that the presence of a polarization anisotropy can induce a complex dynamics of these structured topologies, leading to the twist of their circuitation on the Poincaré sphere of polarizations. The theoretical description of the results carries the concept of generalized quantum vortices in two-component superfluids, which are conformal with polarization loops around an arbitrary axis in the pseudospin space.
Superfluidity, the ability of a liquid or gas to flow with zero viscosity, is one of the most remarkable implications of collective quantum coherence. In equilibrium systems like liquid 4He and ultracold atomic gases, superfluid behaviour conjugates diverse yet related phenomena, such as persistency of metastable flow in multiply connected geometries and the existence of a critical velocity for frictionless flow when hitting a static defect. The link between these different aspects of superfluid behaviour is far less clear in driven-dissipative systems displaying collective coherence, such as …
The study of superfluid and Berezinskii-Kosterlitz-Thouless phases in exciton-polaritons requires an understanding of vortex dynamics in a dissipative unconfined condensate. In this article we study the motion of dynamic vortex-antivortex pairs and show that vortex pair stability defined as ordered motion as opposed to rapid separation or recombination is the result of balance between dissipative velocities in the condensate and interaction with thermal polaritons. The addition of a trapping potential is further shown to considerably enhance the lifetime of a single vortex pair in this system.…
We study the quantum hydrodynamical features of exciton-polaritons flowing circularly in a ring-shaped geometry. We consider a resonant-excitation scheme in which the spinor polariton fluid is set into motion in both components by spin-to-orbital angular momentum conversion. We show that this scheme allows to control the winding number of the fluid, and to create two circulating states differing by two units of the angular momentum. We then consider the effect of a disorder potential, which is always present in realistic nanostructures. We show that a smooth disorder is efficiently screened by…
Singly quantized vortices have been already observed in many systems including the superfluid helium, Bose Einstein condensates of dilute atomic gases, and condensates of exciton polaritons in the solid state. Two dimensional superfluids carrying spin are expected to demonstrate a different type of elementary excitations referred to as half quantum vortices characterized by a pi rotation of the phase and a pi rotation of the polarization vector when circumventing the vortex core. We detect half quantum vortices in an exciton-polariton condensate by means of polarization resolved interferometry…
We propose a method to achieve photon pair propagation in an array of three-level superconducting circuits. Assuming experimentally accessible three-level artificial atoms with strong anharmonicity coupled via microwave transmission lines in both one and two dimensions we analyze the circuit Quantum Electrodynamics(QED) of the system. We explicitly show that for a suitable choice of the coupling ratio between different levels, the single photon propagation is suppressed and the propagation of photon pairs emerges. This propagation of photon pairs leads to the pair superfluid of polaritons asso…
A novel, optimized numerical method of modeling of an exciton-polariton superfluid in a semiconductor microcavity was proposed. Exciton-polaritons are spin-carrying quasiparticles formed from photons strongly coupled to excitons. They possess unique properties, interesting from the point of view of fundamental research as well as numerous potential applications. However, their numerical modeling is challenging due to the structure of nonlinear differential equations describing their evolution. In this paper, we propose to solve the equations with a modified Runge--Kutta method of 4th order, fu…
We use a one-dimensional polariton fluid in a semiconductor microcavity to explore the rich nonlinear dynamics of counter-propagating interacting Bose fluids. The intrinsically driven-dissipative nature of the polariton fluid allows to use resonant pumping to impose a phase twist across the fluid. When the polariton-polariton interaction energy becomes comparable to their kinetic energy, linear interference fringes transform into a train of solitons. A novel type of bistable behavior controlled by the phase twist across the fluid is experimentally evidenced.
We investigate the possibility of creating X-waves, or localized wave packets, in resonantly excited exciton-polariton superfluids. We demonstrate the existence of X-wave traveling solutions in the coupled exciton-photon system past the inflection point, where the effective mass of lower polaritons is negative in the direction perpendicular to the wavevector of the pumping beam. Contrary to the case of bright solitons, X-waves do not require nonlinearity for sustaining their shape. Nevertheless, we show that nonlinearity is important for their dynamics, as it allows for their spontaneous forma…
We study a two-dimensional incoherently pumped exciton-polariton condensate described by an open-dissipative Gross-Pitaevskii equation for the polariton dynamics coupled to a rate equation for the exciton density. Adopting a hydrodynamic approach, we use multiscale expansion methods to derive several models appearing in the context of shallow water waves with viscosity. In particular, we derive a Boussinesq/Benney-Luke type equation and its far-field expansion in terms of Kadomtsev-Petviashvili-I (KP-I) equations for right- and left-going waves. From the KP-I model, we predict the existence of…
In a homogeneous two-dimensional system at non-zero temperature, although there can be no ordering of infinite range, a superfluid phase is predicted for a Bose liquid. The stabilization of phase in this superfluid regime is achieved by the formation of bound vortex-antivortex pairs. It is believed that several different systems share this common behaviour, when the parameter describing their ordered state has two degrees of freedom, and the theory has been tested for some of them. However, there has been no direct experimental observation of the phase stabilization mechanism by a bound pair. …
The spontaneous formation of lattice structure of quantized vortices is a characteristic feature of superfluidity in closed systems under thermal equilibrium. In exciton-polariton Bose-Einstein condensate, which is a typical example of macroscopic quantum state in open systems, spontaneous vortex lattices have also been proposed by not yet observed. Here, we take into account the finite decay rate of exciton reservoir, and theoretically investigate the vortex structures in circularly pumped polariton Bose-Einstein condensate. Our results show that a decreasing reservoir decay rate can reduce t…
We report an experimental study of superfluid hydrodynamic effects in a one-dimensional polariton fluid flowing along a laterally patterned semiconductor microcavity and hitting a micron-sized engineered defect. At high excitation power, superfluid propagation effects are observed in the polariton dynamics, in particular, a sharp acoustic horizon is formed at the defect position, separating regions of sub- and super-sonic flow. Our experimental findings are quantitatively reproduced by theoretical calculations based on a generalized Gross-Pitaevskii equation. Promising perspectives to observe …
The appearance of quantised vortices in the classical ``rotating bucket'' experiments of liquid helium and ultracold dilute gases provides the means for fundamental and comparative studies of different superfluids. Here, we realize the ``rotating bucket'' experiment for optically trapped quantum fluid of light based on exciton-polariton Bose-Einstein condensate in semiconductor microcavity. We utilise the beating note of two frequency-stabilized single-mode lasers to generate an asymmetric time-periodic rotating, non-resonant excitation profile that both injects and stirs the condensate throug…
I calculate the superfluid density of a non-equilibrium steady state condensate of particles with finite lifetime. Despite the absence of a simple Landau critical velocity, a superfluid response survives, but dissipation reduces the superfluid fraction. I also suggest an idea for how the superfluid density of an example of such a system, i.e. microcavity polaritons, might be measured.
Recent experiments on thin-film microcavities give evidence of Bose condensation of exciton-polariton states. Inspired by these observations, we consider the possibility that such exotic "half-light/half matter" states could be observed in thin-film organic semiconductors where the oscillator strength is generally stronger than in inorganic systems. Here we present a theoretical model and simulations of macroscopic exciton-polartiton condensates in thracene thin films sandwiched within a micro-meter scale resonant cavity and establish criteria for the conditions under which BEC could be achiev…
The phenomenon of stable persistent currents is central to the studies of superfluidity in a range of physical systems. While all of the previous theoretical studies of superfluid flows in annular geometries concentrated on conservative systems, here we extend the stability analysis of persistent currents to open-dissipative exciton-polariton superfluids. By considering an exciton-polariton condensate in an optically-induced annular trap, we determine stability conditions for an initially imposed flow with a non-zero orbital angular momentum. We show, theoretically and numerically, that the sy…
Besides being superfluids, microcavity exciton-polariton condensates are capable of spontaneous pattern formation due to their forced-dissipative dynamics. Their macroscopic and easily detectable response to small perturbations can be exploited to create sensitive devices. We show how controlled pumping in the presence of a peak-dip shaped potential can be used to detect small externally applied velocities which lead to the formation of traveling holes in one dimension and vortex pairs in two dimensions. Combining an annulus geometry with a weak link, the set up that we describe can be used to…
We investigate the process of coarsening via annihilation of vortex-antivortex pairs, following the quench to the condensate phase in a nonresonantly pumped polariton system. We find that the late-time dynamics is an example of universal phase ordering kinetics, characterized by scaling of correlation functions in time. Depending on the parameters of the system, the evolution of the characteristic length scale L(t) can be the same as for the two-dimensional XY model, described by a power law with the dynamical exponent z \aprox 2 and a logarithmic correction, or z \aprox 1 which agrees with pr…
BEC of exciton-polaritons and related effects such as superfluidity1,2, spontaneous symmetry breaking3,4 and quantised vortices5,6 open way to creation of novel light sources7 and optical logic elements8. Remarkable observations of exciton-polariton BEC in microcavities9-12 have been reported in the recent ten years. Very recently, thermalisation and subsequent condensation of cavity photons in a dye-filled microcavity have been observed13. Here we show that BEC of both exciton-polaritons and photons can be created in the same system under different optical excitation conditions. A dynamic pha…
