The polariton, a quasiparticle formed by strong coupling of a photon to a matter excitation, is a fundamental ingredient of emergent photonic quantum systems ranging from semiconductor nanophotonics to circuit quantum electrodynamics. Exploiting the interaction between polaritons has led to the realization of superfluids of light as well as of strongly correlated phases in the microwave domain, with similar efforts underway for microcavity exciton-polaritons. Here, we develop an ultracold-atom analogue of an exciton-polariton system in which interacting polaritonic phases can be studied with full tunability and without dissipation. In our optical-lattice system, the exciton is replaced by an atomic excitation, while an atomic matter wave is substituted for the photon under a strong dynamical coupling. We access the band structure of the matter-wave polariton spectroscopically by coupling the upper and lower polariton branches, and explore polaritonic many-body transport in the superfluid and Mott-insulating regimes, finding quantitative agreement with our theoretical expectations. Our work opens up novel possibilities for studies of polaritonic quantum matter.
Quantum nonlinear optics is a quickly growing field with large technological promise, at the same time involving complex and novel many-body phenomena. In the usual scenario, optical nonlinearities originate from the interactions between polaritons, which are hybrid quasi-particles mixing matter and light degrees of freedom. Here we introduce a type of polariton which is intrinsically nonlinear and emerges as the natural quasi-particle in presence quantum degenerate fermionic matter. It is a composite object made of a fermion trapped inside an optical soliton forming a topological defect in a …
Exciton-polaritons have been shown to be an optimal system in order to investigate the properties of bosonic quantum fluids. We report here on the observation of dark solitons in the wake of engineered circular obstacles and their decay into streets of quantized vortices. Our experiments provide a time-resolved access to the polariton phase and density, which allows for a quantitative study of instabilities of freely evolving polaritons. The decay of solitons is quantified and identified as an effect of disorder-induced transverse perturbations in the dissipative polariton gas.
Polariton condensation can be regarded as a self-organization phenomenon, where phase ordering is established among particles in the system. In such condensed systems, further ordering can possibly occur in the particle density distribution, under particular experimental conditions. In this work we report on spontaneous pattern formation in a polariton condensate under non-resonant optical pumping. The slightly elliptical ring-shaped excitation laser we employ is such to force condensation to occur in a single-energy state with periodic boundary conditions, giving rise to a multi-lobe standing…
Optically pumping high quality semiconductor microcavities allows for the spontaneous formation of polariton condensates, which can propagate over distances of many microns. Tightly focussed pump spots here are found to produce expanding incoherent bottleneck polaritons which coherently amplify the ballistic polaritons and lead to the formation of unusual ring condensates. This quantum liquid is found to form a remarkable sunflower-like spatial ripple pattern which arises from self interference with Rayleigh-scattered coherent polariton waves in the Cerenkov regime.
The spontaneous formation of lattice structure of quantized vortices is a characteristic feature of superfluidity in closed systems under thermal equilibrium. In exciton-polariton Bose-Einstein condensate, which is a typical example of macroscopic quantum state in open systems, spontaneous vortex lattices have also been proposed by not yet observed. Here, we take into account the finite decay rate of exciton reservoir, and theoretically investigate the vortex structures in circularly pumped polariton Bose-Einstein condensate. Our results show that a decreasing reservoir decay rate can reduce t…
Dynamics of exciton-polariton multistability is theoretically investigated. Phase portraits are used as a tool to enlighten the microscopic phenomena which influence spin multistability of a confined polariton field as well as ultrafast reversible spin switching. The formation of a non-radiative reservoir, due to polariton pairing into biexcitons is found to play the lead role in the previously reported spin switching experiments. Ways to tailor this reservoir formation are discussed in order to obtain optimal spin switching reliability.
We present numerical analysis of steady states in a two-component (spinor) driven-dissipative quantum fluid formed by condensed exciton-polaritons in an annular optically induced trap. We demonstrate that an incoherent ring-shaped optical pump creating the exciton-polariton confinement supports the existence of stationary and rotating azimuthon steady states with azimuthally modulated density. Such states can be imprinted by coherent light pulses with a defined orbital angular momentum, as well as generated spontaneously in the presence of thermal noise.
We study the spontaneous formation of exciton polariton vortices in an all-optical non-resonantly excited annular trap, which is formed by ring-shaped subpicosecond laser pulses. Since the light emitted by these vortices carries orbital angular momentum (OAM) corresponding to their topological charge, we apply a dedicated OAM spectroscopy technique to detect the OAM of the measurement signal with picosecond time resolution. This allows us to identify the formation of OAM modes and investigate the dynamics of the vortex formation process. We also study the power dependence of this process and h…
Second-order time correlation measurements with a temporal resolution better than 3 ps were performed on a CdTe microcavity where spontaneous Bose-Einstein condensation is observed. After the laser pulse, the nonresonantly excited thermal polariton population relaxes into a coherent polariton condensate. Photon statistics of the light emitted by the microcavity evidences a clear phase transition from the thermal state to a coherent state, which occurs within 3.2 ps after the onset of stimulated scattering. Following this very fast transition, we show that the emission possesses a very high coh…
An exciton-polariton microcavity that incorporates magnetic ions can exhibit a spontaneous self-trapping phenomenon which is an analog of the classical polaron effect. We investigate in detail the full model of a polariton condensate that includes pumping and losses, the spin degree of freedom, external magnetic field and energy relaxation. In the quasi-one-dimensional case, we show that the polaron effect can give rise to a spontaneous lattice of perfectly arranged polarization domains in an antiferromagnetic configuration. We find that partial polarization of the condensate at moderate magne…
We consider linear periodic chains of exciton-polariton condensates formed by pumping polaritons non-resonantly into a linear network. To the leading order, such a sequence of condensates establishes relative phases as to minimize a classical one-dimensional XY Hamiltonian with nearest and next to nearest neighbors. We show that the low energy states of polaritonic linear chains demonstrate various classical regimes: ferromagnetic, antiferromagnetic and frustrated spiral phases, where quantum or thermal fluctuations are expected to give rise to a spin liquid state. At the same time nonlinear i…
Soliton formation in a bound state in the continuum GaN waveguide polariton laser
Laboratoire Charles Coulomb, Université de Montpellier, CNRS（蒙彼利埃大学查尔斯·库隆实验室）；Institut Pascal, PHOTON-N2, Université Clermont Auvergne, CNRS, Clermont INP（克莱蒙奥弗涅大学帕斯卡尔研究所）；B. Verkin Institute for Low Temperature Physics and Engineering of the National Academy of Sciences of Ukraine（乌克兰国家科学院B.维尔金低温物理与工程研究所）；Naturwissenschaftlich-Technische Fakultät, Universität Siegen（锡根大学自然科学技术学院）；CRHEA, Université Cote d’Azur, CNRS（蔚蓝海岸大学CRHEA研究中心）；Centre de Nanosciences et de Nanotechnologies, CNRS, Université Paris-Saclay（巴黎萨克雷大学纳米科学和纳米技术研究中心）
The polaronic system consisting of an impurity in a dilute Bose-Einstein condensate is considered in the presence of a narrow Feshbach resonance. For this purpose a coupled-channel model is used, which at the mean field level predicts the formation of quasiparticles that are a superposition of the impurity and the molecular states. The impurity-boson interactions and the coupling between the open and closed channels are then considered weak and a perturbative calculation of the corrections to the mean field results is presented. This allows to examine the properties of the quasiparticles, such…
The regime of ultrastrong light-matter interaction has been investigated theoretically and experimentally, using zero-dimensional electromagnetic resonators coupled with an electronic transition between two confined states of a semiconductor quantum well. We have measured a splitting between the coupled modes that amounts to 48% of the energy transition, the highest ratio ever observed in a light-matter coupled system. Our analysis, based on a microscopic quantum theory, shows that the nonlinear polariton splitting, a signature of this regime, is a dynamical effect arising from the self-intera…
Formation of oblique solitons by a flow of polariton condensate past an obstacle is considered. The flow is non-uniform due to a finite life-time of polaritons what changes drastically the conditions of formation of oblique solitons compared with the atomic condensate case. The theory shows that the polariton solitons can be generated by a subsonic flow in agreement with the recent experiment [A. Amo {\it et al.}, Science, {\bf 332,} 1167 (2011)]. Geometric form of oblique solitons and other their parameters are calculated analytically and analytical results are confirmed by numerical simulati…
Quasiparticles in semiconductors -- such as microcavity polaritons -- can form condensates in which the steady-state density profile is set by the balance of pumping and decay. By taking account of the polarization degree of freedom for a polariton condensate, and considering the effects of an applied magnetic field, we theoretically discuss the interplay between polarization dynamics, and the spatial structure of the pumped decaying condensate. If spatial structure is neglected, this dynamics has attractors that are linearly polarized condensates (fixed points), and desynchronized solutions (…
Besides being superfluids, microcavity exciton-polariton condensates are capable of spontaneous pattern formation due to their forced-dissipative dynamics. Their macroscopic and easily detectable response to small perturbations can be exploited to create sensitive devices. We show how controlled pumping in the presence of a peak-dip shaped potential can be used to detect small externally applied velocities which lead to the formation of traveling holes in one dimension and vortex pairs in two dimensions. Combining an annulus geometry with a weak link, the set up that we describe can be used to…
Two-photon absorption (TPA) allows accessing dark states of matter otherwise inaccessible to light, which serve as important building blocks for quantum information processing. In a semiconductor microcavity, TPA driven condensation of strongly-coupled light-matter exciton-polaritons can enable new solid-state quantum simulations of dark state-condensate interactions, and was predicted to stimulate THz emission. Here, we report the first observation of two-photon pumped polariton condensation, demonstrated by angle-resolved photoluminescence in a GaAs-based microcavity. TPA is evidenced in the…
Recent experiments in exciton-polariton systems have provided high-precision measurements of the value of the polariton-polariton interaction constant, which is a key parameter that governs the nonlinear dynamics of polariton condensates and potentially enables quantum correlated polaritons. Yet, until now, this parameter has only been addressed theoretically using perturbative treatments or approximations that do not include the composite nature of the excitons. Here, we use a recently developed microscopic description of polaritons involving electrons, holes, and photons, where the interacti…
We report the formation of a macroscopic coherent state emerging from colliding polariton fluids. Four lasers with random relative phases, arranged in a square, pump resonantly a planar microcavity, creating four coherent polariton fluids propagating toward each other. When the density (interactions) increases, the four fluids synchronise and the topological excitations (vortex or soliton) disappear to form a single superfluid.
Cavity quantum electrodynamics (QED) manipulates the coupling of light with matter, and allows for several emitters to couple coherently with one light mode. However, even in a many-body system, the light-matter coupling mechanism was so far restricted to one body processes. Leveraging cavity QED for the quantum simulation of complex, many-body systems has thus far relied on multi-photon processes, scaling down the light-matter interaction to the low energy and slow time scales of the many-body problem. Here we report on cavity QED experiments using molecular transitions in a strongly interact…
Polaritons are an emerging platform for exploration of synthetic materials [1] and quantum information processing [2] that draw properties from two disparate particles: a photon and an atom. Cavity polaritons are particularly promising, as they are long-lived and their dispersion and mass are controllable through cavity geometry [3]. To date, studies of cavity polaritons have operated in the mean-field regime, using short-range interactions between their matter components [4]. Rydberg excitations have recently been demonstrated as a promising matter-component of polaritons [5], due to their st…
The self-trapping of exciton-polariton condensates is demonstrated and explained by the formation of a new polaron-like state. Above the polariton lasing threshold, local variation of the lattice temperature provides the mechanism for an attractive interaction between polaritons. Due to this attraction, the condensate collapses into a small bright spot. Its position and momentum variances approach the Heisenberg quantum limit. The self-trapping does not require either a resonant driving force or a presence of defects. The trapped state is stabilized by the phonon-assisted stimulated scattering…
Following experimental realizations of room temperature polariton lasing with organic molecules, we present a microscopic model that allows us to explore the crossover from weak to strong matter-light coupling. We consider a non-equilibrium Dicke-Holstein model, including both strong coupling to vibrational modes and strong matter-light coupling, providing the phase diagram of this model in the thermodynamic limit. We discuss the mechanism of polariton lasing, uncovering a process of self-tuning, and identify the relation and distinction between regular dye lasers and organic polariton lasers.
Polariton condensates have proved to be model systems to investigate topological defects, as they allow for direct and non-destructive imaging of the condensate complex order parameter. The fundamental topological excitations of such systems are quantized vortices. In specific configurations, further ordering can bring the formation of vortex lattices. In this work we demonstrate the spontaneous formation of ordered vortical states, consisting in geometrically self-arranged vortex-antivortex pairs. A mean-field generalized Gross-Pitaevskii model reproduces and supports the physics of the obser…
The appearance of quantised vortices in the classical ``rotating bucket'' experiments of liquid helium and ultracold dilute gases provides the means for fundamental and comparative studies of different superfluids. Here, we realize the ``rotating bucket'' experiment for optically trapped quantum fluid of light based on exciton-polariton Bose-Einstein condensate in semiconductor microcavity. We utilise the beating note of two frequency-stabilized single-mode lasers to generate an asymmetric time-periodic rotating, non-resonant excitation profile that both injects and stirs the condensate throug…
Mass-anisotropy driven stripe pattern formation and directional modulational instability in polariton condensate
Indian Institute of Technology Kharagpur（印度理工学院卡拉格普尔分校）；Indian Institute of Technology Gandhinagar（印度理工学院甘地纳加尔分校）；Max Planck Institute for the Physics of Complex Systems（马克斯·普朗克复杂系统物理研究所）；Department of Physics, Virginia Tech（弗吉尼亚理工大学物理系）
Strong light matter coupling between excitons and microcavity photons, as described in the framework of cavity quantum electrodynamics, leads to the hybridization of light and matter excitations. The regime of collective strong coupling arises, when various excitations from different host media are strongly coupled to the same optical resonance. This leads to a well-controllable admixture of various matter components in three hybrid polariton modes. Here, we study a cavity device with four embedded GaAs quantum wells hosting excitons that are spectrally matched to the A-valley exciton resonanc…
We develop a theory for light propagating in an atomic Bose-Einstein condensate in the presence of strong interactions. The resulting many-body correlations are shown to have profound effects on the optical properties of this interacting medium. For weak atom-light coupling, there is a well-defined quasiparticle, the polaron-polariton, supporting light propagation with spectral features differing significantly from the noninteracting case. The damping of the polaron-polariton depends nonmonotonically on the light-matter coupling strength, initially increasing and then decreasing. This gives ri…
Two-dimensional semiconductors inside optical microcavities have emerged as a versatile platform to explore new hybrid light-matter quantum states. The strong light-matter coupling leads to the formation of exciton-polaritons, which in turn interact with the surrounding electron gas to form quasiparticles called polaron-polaritons. Here, we develop a general microscopic framework to calculate the properties of these quasiparticles such as their energy and the interactions between them. From this, we give microscopic expressions for the parameters entering a Landau theory for the polaron-polari…
We present a theoretical study on polaritons in highly doped semiconductor microcavities. In particular, we focus on a cavity mode that is resonant with the absorption threshold (`Fermi edge'). In agreement with experimental results, the strong light-matter coupling is maintained under very high doping within our ladder diagram approximation. While the lower polariton is qualitatively unaltered, it acquires a finite lifetime due to relaxation of the valence band hole if the electron density exceeds a certain critical value. On the other hand the upper polariton has a finite lifetime for all de…
Atomically thin crystals of transition metal dichalcogenides are ideally suited to study the interplay of light-matter coupling, polarization and magnetic field effects. In this work, we investiagte the formation of exciton-polaritons in a MoSe2 monolayer, which is integrated in a fully-grown, monolithic microcavity. Due to the narrow linewidth of the polaritonic resonances, we are able to directly investigate the emerging valley Zeeman splitting of the hybrid light-matter resonances in the presence of a magnetic field. At a detuning of -54.5 meV (13.5 % matter constituent of the lower polarit…
The interplay between strong light-matter interactions and charge doping represents an important frontier in the pursuit of exotic many-body physics and optoelectronics. Here, we consider a simplified model of a two-dimensional semiconductor embedded in a microcavity, where the interactions between electrons and holes are strongly screened, allowing us to develop a diagrammatic formalism for this system with an analytic expression for the exciton-polariton propagator. We apply this to the scattering of spin-polarized polaritons and electrons, and show that this is strongly enhanced compared wi…
We investigate the process of condensation of exciton-polaritons in a one-dimensional nanowire, predicting spontaneous formation of domains of uncondensed excitons and condensed polaritons. We demonstrate a universal scaling law for the density of domains, which results from the competition between characteristic timescales present in the system. However, we find that the system does not follow the standard Kibble-Żurek scenario of a nonequilibrium phase transition.
We predict that spatially modulated Zeeman splitting resulting in the formation of Zeeman lattice can be used for creation of localized self-sustained excitations in spinor polariton condensates with dominant repulsive interactions. In such lattices, the phenomenon of TE-TM splitting, playing the role of effective spin-orbit interaction, leads to the emergence of the stripe phase and formation of stable gap-stripe solitons with complex intrinsic structure resulting from the presence of two characteristic spatial scales, one of which is set by the period of Zeeman lattice, while other is set by…
The key to understanding the universal behaviour of systems driven away from equilibrium lies in the common description obtained when particular microscopic models are reduced to order parameter equations. Universal order parameter equations written for complex matter fields are widely used to describe systems as different as Bose-Einstein condensates of ultra cold atomic gases, thermal convection, nematic liquid crystals, lasers and other nonlinear systems. Exciton-polariton condensates recently realised in semiconductor microcavities are pattern forming systems that lie somewhere between equ…
Optical microcavities supporting exciton-polariton quasi-particles offer one of the most powerful platforms for investigation of rapidly developing area of topological photonics in general, and of photonic topological insulators in particular. Energy bands of the microcavity polariton graphene are readily controlled by magnetic field and influenced by the spin-orbit coupling effects, a combination leading to formation of linear unidirectional edge states in polariton topological insulators as predicted very recently. In this work we depart from the linear limit of non-interacting polaritons an…
We study the formation of topological defects (quantum vortices) during the formation of a 2D polariton condensate at the $Γ$ point of a honeycomb lattice via the Kibble-Zurek mechanism. The lattice modifies the single-particle dispersion. The typical interaction energies at the quench time correspond to the linear part of the dispersion. The resulting scaling exponent for the density of topological defects is numerically found as $0.95\pm0.05$. This value differs from the one expected for 2D massive particles (1/2), but is indeed compatible with the one expected for a linear dispersion. We mo…
Transition metal dichalcogenides represent an ideal testbed to study excitonic effects, spin-related phenomena and fundamental light-matter coupling in nanoscopic condensed matter systems. In particular, the valley degree of freedom, which is unique to such direct band gap monolayers with broken inversion symmetry, adds fundamental interest in these materials. Here, we implement a Tamm-plasmon structure with an embedded MoSe2 monolayer and study the formation of polaritonic quasi-particles. Strong coupling conditions between the Tamm-mode and the trion resonance of MoSe2 are established, yield…
Microcavity polaritons are composite half-light half-matter quasi-particles, which have recently been demonstrated to exhibit rich physical properties, such as non-equilibrium Bose-Einstein condensation, parametric scattering and superfluidity. At the same time, polaritons have some important advantages over photons for information processing applications, since their excitonic component leads to weaker diffraction and stronger inter-particle interactions, implying, respectively, tighter localization and lower powers for nonlinear functionality. Here we present the first experimental observati…
