We study the propagation of strongly interacting Rydberg polaritons through an atomic medium in a one-dimensional optical lattice. We derive an effective single-band Hubbard model to describe the dynamics of the dark state polaritons under realistic assumptions. Within this model, we analyze the driven-dissipative transport of polaritons through the system by considering a coherent drive on one side and by including the spontaneous emission of the metastable Rydberg state. Using a variational approch to solve the many-body problem, we find strong antibunching of the outgoing photons despite the losses from the Rydberg state decay.
We demonstrate hybridization of optical cavity photons with atomic Rydberg excitations using electromagnetically induced transparency (EIT). The resulting dark state Rydberg polaritons exhibit a compressed frequency spectrum and enhanced lifetime indicating strong light-matter mixing. We study the coherence properties of cavity Rydberg polaritons and identify the generalized EIT linewidth for optical cavities. Strong collective coupling suppresses polariton losses due to inhomogeneous broadening, which we demonstrate by using different Rydberg levels with a range of polarizabilities. Our resul…
Interfacing light and matter at the quantum level is at the heart of modern atomic and optical physics and enables new quantum technologies involving the manipulation of single photons and atoms. A prototypical atom-light interface is electromagnetically induced transparency, in which quantum interference gives rise to hybrid states of photons and atoms called dark-state polaritons. We have observed individual dark-state polaritons as they propagate through an ultracold atomic gas involving Rydberg states. Strong long-range interactions between Rydberg atoms give rise to an effective interacti…
We experimentally study the effects of the anisotropic Rydberg-interaction on $D$-state Rydberg polaritons slowly propagating through a cold atomic sample. In addition to the few-photon nonlinearity known from similar experiments with Rydberg $S$-states, we observe the interaction-induced dephasing of Rydberg polaritons at very low photon input rates into the medium. We develop a model combining the propagation of the two-photon wavefunction through our system with nonperturbative calculations of the anisotropic Rydberg-interaction to show that the observed effect can be attributed to pairwise…
Electromagnetically-induced transparency (EIT) with Rydberg atoms enables strong interactions between atoms to be controlled and measured by pulses of light. Consequently, Rydberg dark polaritons are a promising platform for quantum simulations. Of particular interest are simulations of one-dimensional systems, known to exhibit unique properties compared to their higher-dimensional counterparts. One limitation of standard EIT is that reducing the polariton group velocity to bring the dark polaritons to rest also implies activating strong Rydberg interactions. To achieve independent control of …
We propose a scheme for realizing fractional quantum Hall states of light. In our scheme, photons of two polarizations are coupled to different atomic Rydberg states to form two flavors of Rydberg polaritons that behave as an effective spin. An array of optical cavity modes overlapping with the atomic cloud enables the realization of an effective spin-1/2 lattice. We show that the dipolar interaction between such polaritons, inherited from the Rydberg states, can be exploited to create a flat, topological band for a single spin-flip excitation. At half filling, this gives rise to a photonic (o…
We analyze the fidelity of a deterministic quantum phase gate for two photons counterpropagating as polaritons through a cloud of Rydberg atoms under the condition of electromagnetically induced transparency (EIT). We provide analytical results for the phase shift of the quantum gate, and provide an estimation for all processes leading to a reduction to the gate fidelity. Especially, the influence of losses form the intermediate level, dispersion of the photon wave packet, scattering into additional polariton channels, finite lifetime of the Rydberg state, as well as effects of transverse size…
We present a pulsed four-wave mixing (FWM) scheme via a Rydberg state to create, store and retrieve collective Rydberg polaritons. The storage medium consists of a gas of thermal Rb atoms confined in a 220 μm thick cell, which are heated above room temperature. The experimental sequence consists of a pulsed excitation of Rydberg polaritons via the D1 line, a variable delay or storage time, and a final retrieval pulse via the D2 line. The lifetime of the Rydberg polaritons is around 1.2 ns, almost entirely limited by the excitation bandwidth and the corresponding motional dephasing of the atoms…
We present a driven dissipative protocol for creating an optical analog of the Laughlin state in a system of Rydberg polaritons in a twisted optical cavity. We envision resonantly driving the system into a 4-polariton state by injecting photons in carefully selected modes. The dissipative nature of the polariton-polariton interactions leads to a decay into a two-polariton analog of the Laughlin state. Generalizations of this technique could be used to explore fractional statistics and anyon based quantum information processing. We also model recent experiments that attempt to coherently drive …
We investigate theoretically the deterministic generation of quantum states with negative Wigner functions, by using giant non-linearities due to collisional interactions between Rydberg polaritons. The state resulting from the polariton interactions may be transferred with high fidelity into a photonic state, which can be analyzed using homodyne detection followed by quantum tomography. Besides generating highly non-classical states of the light, this method can also provide a very sensitive probe for the physics of the collisions involving Rydberg states.
We provide a theoretical framework describing slow-light polaritons interacting via atomic Rydberg states. We use a diagrammatic method to analytically derive the scattering properties of two polaritons. We identify parameter regimes where polariton-polariton interactions are repulsive. Furthermore, in the regime of attractive interactions, we identify multiple two-polariton bound states, calculate their dispersion, and study the resulting scattering resonances. Finally, the two-particle scattering properties allow us to derive the effective low-energy many-body Hamiltonian. This theoretical p…
We study a system of three photons in an atomic medium coupled to Rydberg states near the conditions of electromagnetically induced transparency. Based on the analytical analysis of the microscopic set of equations in the far-detuned regime, the effective three-body interaction for these Rydberg polaritons is derived. For slow light polaritons, we find a strong three-body repulsion with the remarkable property that three polaritons can become essentially non-interacting at short distances. This analysis allows us to derive the influence of the three-body repulsion on bound states and correlati…
We investigate a hybrid quantum system that consists of a superatom coupled to a surface phonon-polariton. We apply this hybrid quantum system to subtract individual photons from a beam of light. Rydberg atom blockade is used to attain absorption of a single photon by an atomic microtrap. Surface phonon-polariton coupling to the superatom then triggers the transfer of the excitation to a storage state, a single Rydberg atom. The approach utilizes the interaction between a superatom and a Markovian bath that acts as a controlled decoherence mechanism to irreversibly project the superatom state …
We present an extension of our recent paper [Bienias et al., Phys. Rev. A 90, 053804 (2014)] in which we demonstrated the scattering properties and bound-state structure of two Rydberg polaritons, as well as the derivation of the effective low-energy many-body Hamiltonian. Here, we derive a microscopic Hamiltonian describing the propagation of Rydberg slow light polaritons in one dimension. We describe possible decoherence processes within a Master equation approach, and derive equations of motion in a Schroedinger picture by using an effective non-Hermitian Hamiltonian. We illustrate diagramm…
We proposed utilizing a medium with a high optical depth (OD) and a Rydberg state of low principal quantum number, $n$, to create a weakly-interacting many-body system of Rydberg polaritons, based on the effect of electromagnetically induced transparency (EIT). We experimentally verified the mean field approach to weakly-interacting Rydberg polaritons, and observed the phase shift and attenuation induced by the dipole-dipole interaction (DDI). The DDI-induced phase shift or attenuation can be viewed as a consequence of the elastic or inelastic collisions among the Rydberg polaritons. Using a w…
We propose a novel scheme for coupling a Rydberg state to a stationary light polariton, based on a dual-V level scheme. We investigate the properties of the resulting stationary Rydberg polariton, and show that its form and its quadratic dispersion relation closely resemble that of the stationary light polariton of the underlying dual-V scheme. We consider the influence of a Rydberg impurity on the system and find strong interaction-induced absorption of the involved probe field. The proposed scheme for a stationary Rydberg polariton might find applications for realizing interacting polaritons…
We develop an effective field theory (EFT) to describe the few- and many-body propagation of one dimensional Rydberg polaritons. We show that the photonic transmission through the Rydberg medium can be found by mapping the propagation problem to a non-equilibrium quench, where the role of time and space are reversed. We include effective range corrections in the EFT and show that they dominate the dynamics near scattering resonances in the presence of deep bound states. Finally, we show how the long-range nature of the Rydberg-Rydberg interactions induces strong effective $N$-body interactions…
We use a microwave field to control the quantum state of optical photons stored in a cold atomic cloud. The photons are stored in highly excited collective states (Rydberg polaritons) enabling both fast qubit rotations and control of photon-photon interactions. Through the collective read-out of these pseudo-spin rotations it is shown that the microwave field modifies the long-range interactions between polaritons. This technique provides a powerful interface between the microwave and optical domains, with applications in quantum simulations of spin liquids, quantum metrology and quantum netwo…
We study the propagation of Rydberg slow light polaritons through an atomic medium for intermediate interactions. Then, the dispersion relation for the polaritons is well described by the slow light velocity alone, which allows for an analytical solution for arbitrary shape of the atomic cloud. We demonstrate the connection of Rydberg polaritons to the behavior of a conventional Kerr nonlinearity for weak interactions, and determine the leading quantum corrections for increasing interactions. We propose an experimental setup which allows one to measure the effective two-body interaction potent…
The combination of high optical nonlinearity in the electromagnetically induced transparency (EIT) effect and strong electric dipole-dipole interaction (DDI) among the Rydberg-state atoms can lead to important applications in quantum information processing and many-body physics. One can utilize the Rydberg-EIT system in the strongly-interacting regime to mediate photon-photon interaction or qubit-qubit operation. One can also employ the Rydberg-EIT system in the weaklyinteracting regime to study the Bose-Einstein condensation of Rydberg polaritons. Most of the present theoretical models dealt …
We study the non-equilibrium steady state arising from the interplay between coherent and dissipative dynamics in strongly interacting Rydberg gases using a recently introduced variational method [H. Weimer, Phys. Rev. Lett. 114, 040402 (2015)]. We give a detailed discussion of the properties of this novel approach, and we provide a comparison with methods related to the Bogoliubov-Born-Green-Kirkwood-Yvon hierarchy. We find that the variational approach offers some intrinsic advantages, and we also show that it is able to explain the experimental results obtained in an ultracold Rydberg gas o…
The combination of electromagnetically induced transparency (EIT) with the nonlinear interaction between Rydberg atoms provides an effective interaction between photons. In this paper, we investigate the storage of optical pulses as collective Rydberg atomic excitations in a cold atomic ensemble. By measuring the dynamics of the stored Rydberg polaritons, we experimentally demonstrate that storing a probe pulse as Rydberg polaritons strongly enhances the Rydberg mediated interaction compared to the slow propagation case. We show that the process is characterized by two time scales. At short st…
We study interactions between polaritons, arising when photons strongly couple to collective excitations in an array of two-level atoms trapped in an optical lattice inside a cavity. We consider two types of interactions between atoms: Dipolar forces and atomic saturability, which ranges from hard-core repulsion to Rydberg blockade. We show that, in spite of the underlying repulsion in the subsystem of atomic excitations, saturability induces a broadband bunching of photons for two-polariton scattering states. We interpret this bunching as a result of interference, and trace it back to the mis…
We study the dissipative propagation of quantized light in interacting Rydberg media under the conditions of electromagnetically induced transparency (EIT). Rydberg blockade physics in optically dense atomic media leads to strong dissipative interactions between single photons. The regime of high incoming photon flux constitutes a challenging many-body dissipative problem. We experimentally study in detail for the first time the pulse shapes and the second-order correlation function of the outgoing field and compare our data with simulations based on two novel theoretical approaches well-suite…
We propose a technique for engineering momentum-dependent dissipation in Bose-Einstein condensates with non-local interactions. The scheme relies on the use of momentum-dependent dark-states in close analogy to velocity-selective coherent population trapping. During the short-time dissipative dynamics, the system is driven into a particular finite-momentum phonon mode, which in real space corresponds to an ordered structure with non-local density-density correlations. Dissipation-induced ordering can be observed and studied in present-day experiments using cold atoms with dipole-dipole or off-…
We study the photon statistics of weak coherent pulses propagating through a cold Rydberg atomic ensemble in the regime of Rydberg electromagnetically induced transparency. We show experimentally that the value of the second-order autocorrelation function of the transmitted light strongly depends on the position within the pulse and heavily varies during the transients of the pulse. In particular, we show that the falling edge of the transmitted pulse displays much lower values than the rest of the pulse. We derive a theoretical model that quantitatively predicts our results and explains the p…
We study the non-equilibrium many-body dynamics of a cold gas of ground state alkali atoms weakly admixed by Rydberg states with laser light. On a timescale shorter than the lifetime of the dressed states, effective dipole-dipole or van der Waals interactions between atoms can lead to the formation of strongly correlated phases, such as atomic crystals. Using a semiclassical approach, we study the long-time dynamics where decoherence and dissipative processes due to spontaneous emission and blackbody radiation dominate, leading to heating and melting of atomic crystals as well as particle loss…
Coupling light to Rydberg states of atoms under conditions of electromagnetically induced transparency (EIT) leads to the formation of strongly interacting quasi-particles, termed Rydberg polaritons. We derive a one-dimensional model describing the time evolution of these polaritons under paraxial propagation conditions, which we verify by numerical two-excitation simulations. We determine conditions allowing for a description by an effective Hamiltonian of a single-species polariton, and calculate ground-state correlations by use of the density matrix renormalization group (DMRG). Under typic…
A time-dependent periodical field can be utilized to efficiently modify the Rabi coupling of system, exhibiting nontrivial dynamics. We propose a scheme to show that this feature can be applied for speeding up the formation of dissipative steady entanglement based on Rydberg anti-blockade mechanism in a simplified configuration, fundamentally stemming from a frequency match between the external-field modulation frequency and the systematic characteristic frequency. In the presence of an optimal modulation frequency that is exactly equal to the central frequency of driving field, it enables a s…
We study two-photon excitation of Rydberg states of atoms under stimulated adiabatic passage with delayed laser pulses. We find that the combination of strong interaction between the atoms in Rydberg state and the spontaneous decay of the intermediate exited atomic state leads to the Rydberg excitation of precisely one atom within the atomic ensemble. The quantum Zeno effect offers a lucid interpretation of this result: the Rydberg blocked atoms repetitively scattering photons effectively monitor a randomly excited atom which therefore remains in the Rydberg state. This system can be used for …
We study resonant optical excitations of strongly-interacting Rydberg states of atoms in the presence of relaxations. We employ the quantum stochastic (Monte Carlo) wavefunctions to simulate the dissipative dynamics of tens of atoms in two-dimensional lattices. We show that under typical experimental conditions involving slow Rydberg state decay and sizable relaxation of atomic coherences, on the time scale of several microseconds the atomic ensemble approaches a stationary state in which much of the quantum correlations between the atoms have decayed away. The steady state, however, exhibits …
We demonstrate a multiphoton Rydberg dark resonance where a Lambda-system is coupled to a Rydberg state. This N-type level scheme combines the ability to slow and store light pulses associated with long lived ground state superpositions, with the strongly interacting character of Rydberg states. For the nd_{5/2} Rydberg state in 87Rb (with n=26 or 44) and a beam size of 1 mm we observe a resonance linewidth of less than 100 kHz in a room temperature atomic ensemble limited by transit-time broadening. The resonance is switchable with an electric field of order 1 V/cm. We show that, even when ph…
We propose and analyze an approach for preparation of high fidelity entanglement and antiferromagnetic states using Rydberg mediated interactions with dissipation. Using asymmetric Rydberg interactions the two-atom Bell singlet is a dark state of the Rydberg pumping process. Master equation simulations demonstrate Bell singlet preparation fidelity $\mcF=0.998$. Antiferromagnetic states are generated on a four spin plaquette in agreement with results found from diagonalization of the transverse field Ising Hamiltonian.
We consider a one-dimensional lattice of atoms with laser excitation to a Rydberg state and spontaneous emission. The atoms are coupled due to the dipole-dipole interaction of the Rydberg states. This driven-dissipative system has a broad range of non-equilibrium phases, such as antiferromagnetic ordering and bistability. Using the quantum trajectory method, we calculate the spatial correlation function throughout the parameter space for up to 20 lattice sites. We show that bistability significantly strengthens the spatial correlations and entanglement.
Scheme to prepare three-dimensional entangled state between a pair of Rydberg atoms is proposed via dissipative dynamics and Electromagnetic Induced Transparency (EIT) associated with the single-atom dark state. The prepared entangled state is the dark state of the whole system. The schemes are feasible no matter the system initially in arbitrary purity or mixed states and do not have accurate requirements on evolution time. In contrast to most of the former Rydberg-atombased dissipative schemes, the Rydberg-Rydberg interaction (RRI) strength do not need to satisfy a certain relation with lase…
We examine the dynamics of Rydberg polaritons with dipolar interactions that propagate in multiple spatial modes. The dipolar excitation exchange between different Rydberg states mediates an effective exchange between polaritons that enables photons to hop across different spatial channels. Remarkably, the efficiency of this photon exchange process can increase with the channel distance and becomes optimal at a finite rail separation. Based on this mechanism, we design a simple photonic network that realizes a two photon quantum gate with a robust $π$-phase, protected by the symmetries of the …
We investigate the dipole mediated transport of Rydberg impurities through an ultracold gas of atoms excited to an auxiliary Rydberg state. In one experiment we continuously probe the system by coupling the auxiliary Rydberg state to a rapidly decaying state which realizes a dissipative medium. In-situ imaging of the impurities reveals diffusive spreading controlled by the intensity of the probe laser. By preparing the same density of hopping partners but then switching off the dressing fields the spreading is effectively frozen. This is consistent with numerical simulations which indicate the…
We show that the dynamics of a laser driven Rydberg gas in the limit of strong dephasing is described by a master equation with manifest kinetic constraints. The equilibrium state of the system is uncorrelated but the constraints in the dynamics lead to spatially correlated collective relaxation reminiscent of glasses. We study and quantify the evolution towards equilibrium in one and two dimensions, and analyze how the degree of glassiness and the relaxation time are controlled by the interaction strength between Rydberg atoms. We also find that spontaneous decay of Rydberg excitations leads …
We present an experimental study of cavity assisted Rydberg atom electromagnetically induced transparency (EIT) using a high-finesse optical cavity ($F \sim 28000$). Rydberg atoms are excited via a two-photon transition in a ladder-type EIT configuration. A three-peak structure of the cavity transmission spectrum is observed when Rydberg EIT is generated inside the cavity. The two symmetrically spaced side peaks are caused by bright-state polaritons, while the central peak corresponds to a dark-state polariton. Anti-crossing phenomenon and the effects of mirror adsorbate electric fields are st…
Recently, the creation of photonic Landau levels in a twisted cavity has been demonstrated in Nature \textbf{534}, 671 (2016). Here we propose a scheme to adiabatically transfer flux quanta in multiples of $3\hbar$ simultaneously to all cavity photons by coupling the photons through flux-threaded cones present in such cavity setup. The flux transfer is achieved using external light fields with orbital angular momentum and a near-resonant dense atomic medium as mediator. Furthermore, coupling the cavity fields to a Rydberg state in a configuration supporting electromagnetically induced transpar…
A steady-state superradiant laser can be used to generate ultranarrow-linewidth light, and thus has important applications in the fields of quantum information and precision metrology. However, the light produced by such a laser is still essentially classical. Here, we show that the introduction of a Rydberg medium into a cavity containing atoms with a narrow optical transition can lead to the steady-state superradiant emission of ultranarrow-linewidth $nonclassical$ light. The cavity nonlinearity induced by the Rydberg medium strongly modifies the superradiance threshold, and leads to a Mollo…
Experimentally observed quantum few-body dynamics of neutral atoms excited to a Rydberg state are numerically analyzed with Lindblad master equation formalism. For this, up to five rubidium atoms are trapped with optical tweezers, arranged in various two-dimensional configurations, and excited to Rydberg 67S state in the nearest-neighbor blockade regime. Their coherent evolutions are measured with time-varying ground-state projections. The experimental results are analyzed with a model Lindblad equation with the homogeneous and inhomogeneous dampings determined by systematic and statistical er…
Dense Rydberg gases are out-of-equilibrium systems where strong density-density interactions give rise to effective kinetic constraints. They cause dynamic arrest associated with highly-constrained many-body configurations, leading to slow relaxation and glassy behavior. Multi-component Rydberg gases feature additional long-range interactions such as excitation-exchange. These are analogous to particle swaps used to artificially accelerate relaxation in simulations of atomistic models of classical glass formers. In Rydberg gases, however, swaps are real physical processes, which provide dynami…
In the last twenty years, Rydberg atoms have become a versatile and much studied system for implementing quantum many-body systems in the framework of quantum computation and quantum simulation. However, even in the absence of coherent evolution Rydberg systems exhibit interesting and non-trivial many-body phenomena such as kinetic constraints and non-equilibrium phase transitions that are relevant in a number of research fields. Here we review our recent work on such systems, where dissipation leads to incoherent dynamics and also to population decay. We show that those two effects, together …
A quantum-feedback-based scheme is proposed for generating multipartite entanglements of Rydberg atoms in a dissipative optical cavity. The Rydberg blockade mechanism efficiently prevents double excitations of the system, which is further exploited to speed up the stabilization of an entangled state with a single Rydberg state excitation. The corresponding feedback operations are greatly simplified, since only one regular atom needs to be controlled during the whole process, irrespective of the number of particles. The form of entangled state is also adjustable via regulating the Rabi frequenc…
The coupling of weak light fields to Rydberg states of atoms under conditions of electromagnetically induced transparency (EIT) leads to the formation of Rydberg polaritons which are quasi-particles with tunable effective mass and long-range interactions. Confined to one spatial dimension their low energy physics is that of a moving-frame Luttinger liquid which due to the long-range character of the repulsive interaction can form a Wigner crystal. We calculate the Luttinger $K$ parameter using density-matrix renormalization group (DMRG) simulations and find that under typical slow-light condit…
To facilitate quantum simulation of open quantum systems at finite temperatures, an important ingredient is to achieve thermalization on a given time-scale. We consider a Rydberg aggregate (an arrangement of Rydberg atoms that interact via long-range interactions) embedded in a laser-driven atomic environment. For the smallest aggregate (two atoms), suitable laser parameters can be found by brute force scanning of the four tunable laser parameters. For more atoms, however, such parameter scans are too computationally costly. Here we apply Gaussian processes to predict the thermalization perfor…
We extend the recent result of bipartite Bell singlet [Carr and Saffman, Phys. Rev. Lett. {\bf111}, (2013)] to a stationary three-dimensional entanglement between two-individual neutral Rydberg atoms. This proposal makes full use of the coherent dynamics provided by Rydberg mediated interaction and the dissipative factor originating from the spontaneous emission of Rydberg state. The numerical simulation of the master equation reveals that both the target state negativity ${\cal N}(\hatρ_{\infty})$ and fidelity ${\cal F}(\hatρ_{\infty})$ can exceed 99.90%. Furthermore, a steady three-atom sing…
