This paper is devoted to the study of a degradation of CsI(Tl)crystals scintillation characteristics under irradiation with gamma-quanta at the uniformly distributed absorbed dose up to 3700 rad. The sample set consisted of 25 crystals of 30 cm long having a truncated pyramid shape and 30 rectangular crystals of the same length. A large difference in the light output deterioration caused by the radiation was observed for the samples of the same shape. A substantial dependence of the average light output loss from the sample shape is seen as well. On the other hand, the crystals from the same ingot behave very similarly under irradiation.
Noble gases and liquids are excellent scintillators and this opens a unique opportunity to directly detect the primary scintillation light produced in these media by photons or particles. This signal can be used for several purposes, for example as a start signal for TPCs or for particles identification. Usually photomultipliers (PMs) are used for the detection of the scintillation light. In our previous work we have demonstrated that costly PMs could be replaced by gaseous detectors with CsI photocathodes . Such detectors have the same quantum efficiency as the best PMs but at the same time a…
We have investigated scintillation light distribution in BaF$_{2}$ and pure CsI crystals with dimensions 3x3x20 cm$^{3}$ using the Geant4 toolkit. The diffuse wrapping material is selected as coating for the crystals. The simulated cosmic muons and 105 MeV electrons are used as beam particles. The optical attenuation along the crystals is explored with the simulation data. We have demonstrated the impact of the crystal surface finish on the light distribution at the crystal end, optical photon arrival time, incidence angle distributions, and optical attenuation for the studied crystals.
Scintillation at cryogenic temperatures can give rise to detectors with particle discrimination for rare-event searches such as dark matter detection. We present time-resolved scintillation studies of Caesium Iodide (CsI) under excitation of both alpha and gamma particles over a long acquisition window of 1 ms to fully capture the scintillation decay between room temperature and 4 K. This allows a measurement of the light yield independent of any shaping time of the pulse. We find the light yield of CsI to increase up to two orders of magnitude from that of room temperature at cryogenic temper…
Caesium iodide is one of the more extensively studied scintillators. Here we present X-ray luminescence spectra, scintillation light output and decay curves as function of temperature, from room temperature down to below 10 K. Features of the observed intrinsic luminescence are explained in terms of radiative recombination of on- and off-centre STE. A model permitting interpretation of the dynamics of luminescence changes in CsI with temperature is suggested. This model includes adiabatic potential energy surfaces (APES) associated with singlet and triplet states of self-trapped excitons (STE)…
Scintillation characteristics of an undoped CsI crystal at low-temperature for dark matter search
University of Science and Technology (UST)（韩国科学技术院）；Institute for Basic Science (IBS)（基础科学研究院）；Jeju National University（济州国立大学）；Kyungpook National University（庆北国立大学）
Monte Carlo simulations are increasingly used in scintigraphic imaging to model imaging systems and to develop and assess tomographic reconstruction algorithms and correction methods for improved image quantitation. GATE (GEANT 4 Application for Tomographic Emission) is a new Monte Carlo simulation platform based on GEANT4 dedicated to nuclear imaging applications. This paper describes the GATE simulation of a prototype of scintillation camera dedicated to small animal imaging and consisting of a CsI(Tl) crystal array coupled to a position sensitive photomultiplier tube. The relevance of GATE …
We present results of several measurements of CsI[Na] scintillation response to 3-60 keV energy nuclear recoils performed by the COHERENT collaboration using tagged neutron elastic scattering experiments and an endpoint technique. Earlier results, used to estimate the coherent elastic neutrino-nucleus scattering (CEvNS) event rate for the first observation of this process achieved by COHERENT at the Spallation Neutron Source (SNS), have been reassessed. We discuss corrections for the identified systematic effects and update the respective uncertainty values. The impact of updated results on fu…
Scintillation response of cryogenic CsI to few-keV and sub-keV nuclear recoils
University of Chicago（芝加哥大学）；Donostia International Physics Center (DIPC)（多诺西亚国际物理中心）；Ikerbasque, Basque Foundation for Science（伊克尔巴斯基克，巴斯克科学基金会）；Instituto de Física Corpuscular, CSIC & Universitat de València（粒子物理研究所，西班牙国家科学研究委员会与瓦伦西亚大学）
This paper presents the results of the fast neutron irradiation (E$_n$ > 0.5MeV) of an EJ-276 scintillator performed in the MARIA research reactor with fluence up to 5.3$\times$10$^{15}$ particles/cm$^2$. In our work, four samples with size $ϕ$25.4~mm$\times$5~mm were tested. The changes in the light yield, emission and absorption spectrum and neutron/gamma discrimination using PuBe source before and after irradiation are presented. The figure of merit in neutron/gamma discrimination based on the charge integration method for different neutron fluences and different short gate integration time…
We have examined long term changes in signal amplitude gain, energy resolution and detection efficiency for the active components of the PIBETA detector system. Beam defining plastic scintillation counters were operated in a ~1 MHz stopped $π^+$ beam for a period of 297 days, accumulating radiation doses of up to 2 Mrad. Detectors in the charged particle tracking system--a pair of cylindrical multi-wire proportional chambers and a thin plastic scintillation barrel-shaped hodoscope array--were irradiated during the same running period with an average dose of ~40 krad. Individual CsI(undoped cry…
The responds of different common alkali halide crystals to alpha-rays and gamma-rays are tested in our research. It is found that only CsI(Na) crystals have significantly different waveforms between alpha and gamma scintillations, while others have not this phenomena. It is suggested that the fast light of CsI(Na) crystals arises from the recombination of free electrons with self-trapped holes of the host crystal CsI. Self-absorption limits the emission of fast light of CsI(Tl) and NaI(Tl) crystals.
The bright scintillation of pure CsI operated at liquid-nitrogen temperature makes of this material a promising dark matter and neutrino detector. We present the first measurement of its quenching factor for nuclear recoils. Our findings indicate it is indistinguishable from that for sodium-doped CsI at room temperature. Additional properties such as light yield, afterglow, scintillation decay properties for electron and nuclear recoils, and energy proportionality are studied over the \mbox{108-165 K} temperature range, confirming the vast potential of this medium for rare-event searches.
Measurements of the degradation in performance of 30 cm long CsI(Tl) scintillation crystals exposed to 1 MeV photon doses of 2, 10, 35, 100 and 1000 Gy are presented. The light yield, light yield longitudinal non-uniformity, scintillation decay times, energy resolution and timing resolution of a set of spare crystals from the BABAR and Belle experiments are studied as a function of these doses. In addition, a model that describes the plateau observed in the light output loss as a function of dose in terms of increase in concentrations of absorption centres with irradiation is presented.
Pulse shape discrimination using CsI(Tl) scintillators to perform neutral hadron particle identification is explored with emphasis towards application at high energy electron-positron collider experiments. Through the analysis of the pulse shape differences between scintillation pulses from photon and hadronic energy deposits using neutron and proton data collected at TRIUMF, it is shown that the pulse shape variations observed for hadrons can be modelled using a third scintillation component for CsI(Tl), in addition to the standard fast and slow components. Techniques for computing the hadron…
The detection of primary scintillation light in combination with the charge or secondary scintillation signals is an efficient technique to determine the events t=0 as well as particle / photon separation in large mass TPC detectors filled with noble gases and/or condensed noble gases. The aim of this work is to demonstrate that costly photo-multipliers could be replaced by cheap novel photosensitive gaseous detectors: wire counters, GEMs or glass capillary tubes coupled with CsI photocathodes. We have performed systematic measurements with Ar, Kr and Xe gas at pressures in the range of 1-50 a…
We will discuss an imaging measurement with a single photon sensitive and low noise camera aiming to a new paradigm in the optical readout of scintillation detectors. The features of the single photon sensitive camera will be characterized and demonstrated with a measurement on double-slit Young's interference in single photon mode. An imaging test on CsI(Tl) crystal and alpha source will be performed further for preliminary measurements on the noise level and sensitivity of the system with a 1/2", f/1.4 lens, which reaches an sensitivity on light intensity around 1/10 of the 3-inch PMT and sh…
Presented here are first tests of a Gaseous Photomultiplier based on a cascade of Thick GEM structures intended for gamma-ray position reconstruction in liquid Argon. The detector has a MgF$_2$ window, transparent to VUV light, and a CsI photocathode deposited on the first THGEM. A gain of $8\cdot10^{5}$ per photoelectron and $\sim100\%$ photoelectron collection efficiency are measured at stable operation settings. The excellent position resolution capabilities of the detector (better than 100 $μ$m) at 100 kHz readout rate, is demonstrated at room temperature. Structural integrity tests of the…
GAGG(Ce) is a novel scintillator with a fast response and high light output without a hygroscopic nature. It is expected to be a useful detector for charged particles at high-counting rates. However, the response of the GAGG(Ce) scintillator to charged particles has not been fully examined. In the present work, the light output and energy resolution of the GAGG(Ce) scintillator were measured for protons and alpha particles at $E_{p}=5$-68 MeV and $E_α=8$-54 MeV as well as gamma rays at $E_γ=662$ keV from a $^{137}$Cs source. The results were compared with those of the CsI(Tl) scintillator. The…
Scintillators play an important role in radiation detection and imaging. Thallium-doped cesium iodide (CsI:Tl) and sodium iodide (NaI:Tl) are two of the major scintillators that have been used for many applications for many decades. In this paper we will present an improved scintillation performance of Bridgman method grown CsI(Tl) and NaI(Tl) crystals developed by Xtallized Intelligence, Inc. (XI, Inc.) and we will compare the performance with commercially available CsI:Tl and NaI:Tl. In a preliminary testing using MicroFJ-60035-TSV silicon photomultipliers (ON Semiconductor), the newly devel…
Previous studies showed that CsI(Na) crystals have significantly different waveforms between alpha and gamma scintillations. In this work, the light yield and PSD capability of CsI(Na) scintillators as a function of the temperature down to 80 K has been studied. As temperature drops, the fast component rises and the slow component decreases. By cooling the CsI(Na) crystals, the light yield of high ionization events are enhanced significantly, while the light yield of background gamma events are suppressed. At 110 K, CsI(Na) crystal achieves the optimal balance between low threshold and good ba…
We have studied channeling effects in a Cesium Iodide (CsI) crystal that is similar in composition to the ones being used in a search for Weakly Interacting Massive Particles (WIMPs) dark matter candidates, and measured its energy-dependent quenching factor, the relative scintillation yield for electron and nuclear recoils. The experimental results are reproduced with a GEANT4 simulation that includes a model of the scintillation efficiency as a function of electronic stopping power. We present the measured and simulated quenching factors and the estimated effects of channeling.
This paper describes the implementation and performance of CsI(Tl) pulse shape discrimination for the Belle II electromagnetic calorimeter, representing the first application of CsI(Tl) pulse shape discrimination for particle identification at an electron-positron collider. The pulse shape characterization algorithms applied by the Belle II calorimeter are described. Control samples of $γ$, $μ^+$, $π^\pm$, $K^\pm$ and $p/\bar{p}$ are used to demonstrate the significant insight into the secondary particle composition of calorimeter clusters that is provided by CsI(Tl) pulse shape discrimination…
The Mu2e calorimeter is composed by 1400 un-doped CsI crystals coupled to large area UV extended Silicon Photomultipliers arranged in two annular disks. This calorimeter has to provide precise information on energy, timing and position. It should also be fast enough to handle the high rate background and it must operate and survive in a high radiation environment. Simulation studies estimated that, in the hottest regions, each crystal will absorb a dose of 300 Gy and will be exposed to a neutron fluency of 6 x 10^{11} n/cm^2 in 3 years of running. Test of un-doped CsI crystals irradiated up to…
A light yield of 20.4 $\pm$ 0.8 photoelectrons/keV was achieved with an undoped CsI crystal coupled directly to a photomultiplier tube at 77 Kelvin. This is by far the largest yield in the world achieved with CsI crystals. An energy threshold that is several times lower than the current dark matter experiments utilizing CsI(Tl) crystals may be achievable using this technique. Together with novel CsI crystal purification methods, the technique may be used to improve the sensitivities of dark matter and coherent elastic neutrino-nucleus scattering experiments. Also measured were the scintillatio…
As a novel approach on visual photon imaging by a single photon sensitive camera and PMTs, this work is trying to measure and identify muon tracks from the 2-D images of CsI(Tl) crystal (scintillator detectors). It is possible that muon tracks can be seen directly with a good signal-to-noise ratio neither with further amplification nor external light, which provides an evolution method for particle measurement in the photon-starved regime of scintillation detectors. The setup of the crystal and camera testing system and the identification algorithm of muon track will be discussed in detail inc…
The electromagnetic calorimeter of PANDA at the FAIR facility will rely on an operation of lead tungstate (PWO) scintillation crystals at temperatures near -25 deg.C to provide sufficient resolution for photons in the energy range from 8 GeV down to 10 MeV. Radiation hardness of PWO crystals was studied at the IHEP (Protvino) irradiation facility in the temperature range from room temperature down to -25 deg.C. These studies have indicated a significantly different behaviour in the time evolution of the damaging processes well below room temperature. Different signal loss levels at the same do…
LYSO scintillation crystals, due to their significant characteristics such as high light yield, fast decay time, small Moliére radius, and good radiation hardness, are proposed to be used for the electromagnetic calorimeter section of the Turkish Accelerator Center Particle Factory (TAC-PF) detector. In this work, the center of gravity technique was used to determine the impact coordinates of an electron initiating an electromagnetic shower in the LYSO array, the calorimeter module contains nine crystals, each 25 mm$\times$25 mm in cross-section and 200 mm in length. The response of the calori…
ZnO-based scintillation ceramics for application in HENPA LENPA analyzers have been investigated. The following ceramic samples have been prepared: undoped ones (ZnO), an excess of zinc in stoichiometry (ZnO:Zn), doped with gallium (ZnO:Ga) and lithium (ZnO:Li). Optical transmission, x-ray excited emission, scintillation decay and pulse height spectra were measured and analyzed. Ceramics have reasonable transparency in visible range (up to 60% for 0.4 mm thickness) and energy resolution (14.9% at 662 keV Cs137 gamma excitation). Undoped ZnO shows slow (1.6 μs) luminescence with maximum at 2.37…
Pulse shape discrimination with pure CsI scintillators is investigated as a method for separating energy deposits by energetic neutrons and photons at particle physics experiments. Using neutron data collected near the European XFEL XS1 beam window the pulse shape discrimination capabilities of pure CsI are studied and compared to CsI(Tl) using near-identical detector setups, which were operated in parallel. The inelastic interactions of 100MeV neutrons are observed to produce a slower scintillation emission in pure CsI relative to energy deposits from cosmic muons. By employing a charge-ratio…
The Mu2e experiment is constructing a calorimeter consisting of 1,348 undoped CsI crystals in two disks. Each crystal has a dimension of 34 x 34 x 200 mm, and is readout by a large area silicon PMT array. A series of technical specifications was defined according to physics requirements. Preproduction CsI crystals were procured from three firms: Amcrys, Saint-Gobain and Shanghai Institute of Ceramics. We report the quality assurance on crystal's scintillation properties and their radiation hardness against ionization dose and neutrons. With a fast decay time of 30 ns and a light output of more…
Investigated in this work were sensitivities of a prototype detector for the detection of low-mass dark matter particles produced at the Spallation Neutron Source at the Oak Ridge National Laboratory in two years of data taking. The presumed prototype consisted of 10 kg undoped CsI or NaI scintillation crystals directly coupled with SiPM arrays operated at 77 K. Compared to the COHERENT CsI(Na) detector, a much higher light yield was assumed for the prototype. An experiment with a cylindrical 1~kg undoped CsI crystal coupled directly to two photomultiplier tubes at about 77~K was conducted as …
Characterization and Optimization of a Cryogenic Pure CsI Detector with Remarkable Light Yield and Unprecedented Energy Resolution for CLOVERS Experiment
The Belle II experiment is presently in phase-2 operation at the SuperKEKB electron-positron collider in KEK (Tsukuba, Japan). The detector is an upgrade of the Belle experiment at the KEKB collider and it is optimized for the study of rare B decays, being also sensitive to signals of New Physics beyond the Standard Model. The Electromagnetic Calorimeter (ECL) is based on CsI(Tl) scintillation crystals. It splits in a barrel and two annular end-cap regions, these latter named Forward and Backward, according to the asymmetric design of the collider. CsI(Tl) crystals deliver a high light output …
Investigated in this work are sensitivities to non-standard neutrino interactions (NSI) of a prototype detector placed about 20 meters away from the Spallation Neutron Source at the Oak Ridge National Laboratory in two years of data taking. The presumed prototype consists of 10 kg undoped CsI scintillation crystals directly coupled with SiPM arrays operated at 77 K. Compared to the COHERENT CsI(Na) detector, a much higher light yield is assumed for the prototype. An experiment with a cylindrical undoped CsI crystal coupled directly to a photomultiplier tube at about 77 K was conducted to verif…
This Thesis present the process of development very low sensitivity to background radiation n-g scintillation detectors with close to 100% efficiency to corpuscular diagnostic of thermonuclear plasma. The detectors developed using this methodology were installed in two major Neutral Particle Analyzers for the JET tokamak (Gemma-2M and ISEP) and they operated successfully for many years. The configuration for such detectors is based on the growing of very thin scintillators of CsI(Tl) on top of quartz supporters and then glued to photomultipliers by keeping the thickness of the supporter and th…
To study an alternative to BaF2, as the crystal choice for the Mu2e calorimeter, thirteen pure CsI crystals from Opto Materials and ISMA producers have been characterized by determining their light yield (LY) and longitudinal response uniformity (LRU), when read with a UV extended PMT. The crystals show a LY of ~ 100 p.e./MeV (~ 150 p.e./MeV) when wrapped with Tyvek and coupled to the PMT without (with) optical grease. The LRU is well represented by a linear slope that is on average around -0.6 %/cm. The timing performances of the Opto Materials crystal, read with a UV extended MPPC, have been…
Pulse-shape discrimination (PSD) is usually achieved using the different fast and slow decay components of inorganic scintillators, such as BaF2, CsI:Tl, etc. However, LaBr3:Ce is considered to not possess different components at room temperature, but has been proved to have the capability of discriminating γ and α events using fast digitizers. In this paper, ionization-density-dependent transport and rate equations are used to quantitatively model the competing processes in a particle track. With one parameter set, the model reproduces the nonproportionality response of electrons or α particl…
A high sensitivity Cardiac SPECT system using curved crystals with pinhole collimation was proposed previously (Dey, IEEE TNS 2012, Bhusal et al, Med. Phys. 2019). Here, we hypothesize that a high curvature hemi-ellipsoid detector results in measurable differences in light distribution from events at different depths in the crystal. This was tested by analyzing the scintillation light in hemi-ellipsoid detector using Monte-Carlo (Geant4) and evaluation of both the localization error at detector and the back-projected errors in object-space. We used Geant4 to simulate the propagation of scintil…
Ensuring the radiation hardness of PbWO4 crystals was one of the main priorities during the construction of the electromagnetic calorimeter of the CMS experiment at CERN. The production on an industrial scale of radiation hard crystals and their certification over a period of several years represented a difficult challenge both for CMS and for the crystal suppliers. The present article reviews the related scientific and technological problems encountered.
Future HEP experiments present stringent challenges to inorganic scintillators in both fast timing response and radiation tolerance. This paper reports recent progress in developing ultrafast inorganic scintillators with sub-ns decay time for future precision timing detectors and high-rate experiments. Performance of fast and ultrafast crystals with mass production capability are compared to CsI crystals which are used for the Mu2e calorimeter. Examples are LYSO:Ce, BaF2 and BaF2:Y, which are considered for Mu2e-II. Crystal radiation hardness against gamma-rays and hadrons is reported. Current…
Super Tau-Charm Facility (STCF) is a next-generation high luminosity electron-positron collider facility and is currently one of the major options for accelerator-based particle physics experiment in China. The crystal-based electromagnetic calorimeter (EMC) with undoped CsI is a major sub-system of the STCF spectrometer. To fulfill the increasing physics requirements on measurement precision and the suffering of radiation, improving the detected light yield is an important task of STCF EMC R&D. This paper studies a "wavelength shifting in propagation" scheme for STCF EMC using the nanostructu…
The CMS detector at the LHC requires a major upgrade to cope with the higher instantaneous luminosity and the elevated radiation levels. The active media of the forward backing hadron calorimeters is projected to be radiation-hard, high light yield scintillation materials or similar alternatives. In this context, we have studied various radiation-hard scintillating materials such as Polyethylene Terephthalate (PET), Polyethylene Naphthalate (PEN), High Efficiency Mirror (HEM) and quartz plates with various coatings. The quartz plates are pure Cerenkov radiators and their radiation hardness has…
Development of Ultrafast and Radiation-Hard GAGG for the Next-Generation of High-Energy Physics Calorimeters
European Organization for Nuclear Research (CERN)（欧洲核子研究组织（CERN））；University Claude Bernard Lyon1（里昂第一大学克洛德·贝尔纳）；University of Strasbourg（斯特拉斯堡大学）；Crytur, Ltd（Crytur有限公司）；Institute of Physics of the Academy of Sciences of the Czech Republic (FZU)（捷克科学院物理研究所（FZU））
