我们探讨了成功的各种版本的一个频带的t-J模型在解释角分辨光电发射光谱的原型，准二维，tetraxis，反铁磁绝缘体$Sr_2CuO_2Cl_2$的全光谱功能。在提出证明我们从实验数据中提取$A(k,ω)$的理由后，我们依赖于一个正方形32位晶格的研究的精确对角化结果，这是目前可用的最大的簇，以进行这种比较。我们的工作使我们相信：（1）一个包括三位自旋相关跳跃和三位三近邻跳跃的单带模型，不仅能解释色散关系，而且能解释准粒子寿命--只有在$k = (π/2,0)$附近我们才发现不一致;（ii）能量依赖的加宽函数$Γ(E) = Γ_0 + A E$在解释对光谱函数的非相干贡献方面是重要的。
英文摘要：
We explore the success of various versions of the one-band t-J model in explaining the full spectral functions found in angle-resolved photoemission spectra for the prototypical, quasi two-dimensional, tetragonal, antiferromagnetic insulator $Sr_2CuO_2Cl_2$. After presenting arguments justifying our extraction of $A(k,ω)$ from the experimental data, we rely on exact-diagonalization results from studies of a square 32-site lattice, the largest cluster for which such information is presently available, to perform this comparison. Our work leads us to believe that (i) a one-band model that includes hopping out to third-nearest neighbours, as well three-site, spin-dependent hopping, can indeed explain not only the dispersion relation, but also the quasiparticle lifetimes -- only in the neighbourhood of $k = (π/2,0)$ do we find disagreement; (ii) an energy-dependent broadening function, $Γ(E) = Γ_0 + A E$, is important in accounting for the incoherent contributions to the spectral functions.
The electron dynamics in the CuO chains has been elusive in Y-Ba-Cu-O cuprate systems by means of standard angle-resolved photoemission spectroscopy (ARPES); cleaved sample exhibits areas terminated by both CuO-chain or BaO layers, and the size of a typical beam results in ARPES signals that are superposed from both terminations. Here, we employ spatially-resolved ARPES with submicrometric beam (nano-ARPES) to reveal the surface-termination-dependent electronic structures of the double CuO chains in YBa$_2$Cu$_4$O$_8$. We present the first observation of sharp metallic dispersions and Fermi su…
Polycrystalline CuO samples with Co doping were prepared by solid state method with flowing oxygen condition and examined their structural and multiferroic properties. Structural studies have confirmed single phase monoclinic crystal structure of all samples, however, in Co doped samples a decrease in volume with an increase in monoclinic distortion is found. For pristine sample, temperature dependent magnetization has confirmed two antiferromagnetic (AFM) transitions at 213 K and 230 K and frequency independent dielectric peaks at these AFM transitions suggesting the ferroelectric nature. Mag…
The magnetic properties of CuO encompass several contemporary themes in condensed matter physics, including quantum magnetism, magnetic frustration, magnetically-induced ferroelectricity and orbital currents. Here we report polarized and unpolarized neutron inelastic scattering measurements which provide a comprehensive map of the cooperative spin dynamics in the low temperature antiferromagnetic (AFM) phase of CuO throughout much of the Brillouin zone. At high energies ($E \gtrsim 100$\,meV) the spectrum displays continuum features consistent with the des Cloizeax--Pearson dispersion for an i…
Hybridization of Bogoliubov-quasiparticles between adjacent CuO$_2$ layers in the triple-layer cuprate Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ studied by ARPES
An intact CuO$_2$ plane is widely believed to be a prerequisite for the high-$T_c$ superconductivity in cuprate superconductors. However, an exception may exist in the superconducting Ba$_2$CuO$_{3+δ}$ materials where CuO chains play a more important role. From first-principles density functional theory calculations, we have studied the electronic and magnetic structures of Ba$_2$CuO$_{3+δ}$. The stoichiometric Ba$_2$CuO$_3$ and Ba$_2$CuO$_4$ contain quasi-one-dimensional CuO chains and intact two-dimensional CuO$_2$ planes, respectively. In comparison with the nonmagnetic metal Ba$_2$CuO$_4$,…
Reaffirming the $d_{x^2-y^2}$ superconducting gap using the auto-correlation angle-resolved photoemission spectroscopy of Bi$_{1.5}$Pb$_{0.55}$Sr$_{1.6}$La$_{0.4}$CuO$_{6+δ}$
Angle-resolved photoemission spectroscopy (ARPES) has revealed peculiar properties of mobile dopants in correlated anti-ferromagnets (AFMs). But describing them theoretically, even in simplified toy models, remains a challenge. Here we study ARPES spectra of a single mobile hole in the $t-J$ model. Recent progress in the microscopic description of mobile dopants allows us to use a geometric decoupling of spin and charge fluctuations at strong couplings, from which we conjecture a one-to-one relation of the one-dopant spectral function and the spectrum of a constituting spinon in the \emph{undo…
CE-antiferromagnetic electronic structure in LaSr$_2$Mn$_2$O$_7$ revealed by micro-focused angle-resolved photoemission spectroscopy and tight-binding models
Tokyo University of Science（东京科学大学）；Japan Atomic Energy Agency（日本原子力机构）；Sophia University（上智大学）；National Institutes for Quantum Science and Technology (QST)（量子科学技术研究机构）；Institute of Materials Structure Science, High Energy Accelerator Research Organization (KEK)（高能加速器研究机构物质结构科学研究所）
Strength of the phonon-coupling mode in $La_{2-x}Sr_{x}CuO_{4}$, $Bi_{2}Sr_{2}CaCu_{2}O_{8+x}$ and $YBa_{2}Cu_{3}O_{6+x}$: An estimation from the ARPES-nodal measurements
We have studied the superexchange interaction $J_{ij}$ in doped $2D$ cuprates. The AFM interaction strongly depends on the state of the lattice of a CuO$_2$ layer surrounded by two LaO rock salt layers. In a static $U$ and $D$ stripe nanostructure, the homogeneous AFM interaction is impossible due to the $U/D/U...$ periodic stripe sequence and $T_N=0$. In a dynamic stripe nanostructure, the ideal CuO$_2$ layer with nonlocal effects and the homogeneous AFM interaction are restored. However the interaction $J_{ij}$ decreases by the exponential factor due to partial dynamic quenching. The meaning…
Understanding the complex phase diagram of cuprate superconductors is an outstanding challenge. The most actively studied questions surround the nature of the pseudogap and strange metal states and their relationship to superconductivity. In contrast, there is general agreement that the low energy physics of the Mott insulating parent state is well captured by a two-dimensional spin $S$ = 1/2 antiferromagnetic (AFM) Heisenberg model. However, recent observations of a large thermal Hall conductivity in several parent cuprates appear to defy this simple model and suggest proximity to a magneto-c…
Angle-resolved photoemission spectroscopy (ARPES) measurements have established the phenomenon of kink in band dispersion of high-$T_{\rm c}$ cuprate superconductors. However, systematic studies of the kink in electron-doped cuprates are still lacking experimentally. We performed $in$-$situ$ ARPES measurements on ${\rm La}_{2-x}{\rm Ce}_x{\rm CuO}_{4\pmδ}$ (LCCO) thin films over a wide electron doping ($n$) range from 0.05 to 0.23. While the nodal kink is nearly invisible, an antinodal kink around 45 meV, surviving above 200 K, is observed for $n\sim0.05-0.19$, whose position is roughly indepe…
Superconductivity distorted by the coexisting pseudogap in the antinodal region of Bi$_{1.5}$Pb$_{0.55}$Sr$_{1.6}$La$_{0.4}$CuO$_{6+δ}$: A photon-energy-dependent angle-resolved photoemission study
超导电性和赝能隙之间的相互作用是铜氧化物物理的一个重要方面。然而，赝能隙的性质仍然存在争议，部分原因是不同的实验提出了不同的能隙函数。本文采用光子能量依赖角分辨光电子能谱（ARPES）研究了Bi $_{1.5}$ Pb $_{0.55}$ Sr $_{1.6}$ La $_{0.4}$ CuO $_{6+δ}$ .我们发现，在低光子能量的反节ARPES谱是由背景信号，这可能会导致一个错误的评估的光谱间隙的大小占主导地位。一旦背景是适当的占，独立的光子能量，在不同的能量下，主要归因于赝能隙和超导性，以及偏离一个简单的d-波形式的整体光谱间隙的波腹光谱鲁棒地显示两个共存的功能。这些结果支持了赝能隙和超导性之间的竞争导致能隙畸变的观点。
Extremely Correlated Fermi Liquid Description of Normal State ARPES in Cuprates
用角分辨光电子能谱学（ARPES）测量的高温超导铜氧化物正常态单粒子谱函数，被认为是反常的，也是理解的关键。在这里，我们表明，一个前所未有的详细描述的数据所产生的光谱函数的极其相关的费米液态的t-J模型最近提出的Shastry。本说明书包括关于最佳掺杂的Bi $_2$ Sr $_2$ CaCu $_2$ O $_{8+δ}$的激光和常规同步加速器ARPES数据，以及关于La $_{1.85}$ Sr $_{0.15}$ CuO $_4$材料的常规同步加速器ARPES数据。{ \em它适用于具有相同物理参数值的所有数据集}，满足粒子求和规则，并成功解决了色散中两个广泛讨论的“扭结”异常。
Recent angle resolved photoemission spectrascope (ARPES) experiments on strongly underdoped Bi$_2$Sr$_{2-x}$La$_x$CuO$_{6+δ}$ cuprates have reported an unusual gap in the nodal direction. Transport experiments on these cuprates found variable range hopping behavior observed. These cuprates have both electron and hole doping which has led to proposals that this cuprate is analogous to a partially compensated semiconductors. The nodal gap then corresponds to the Efros-Schklovskii(ES) gap in such semiconductors. We calculate the doping dependence and temperature dependence of a ES gap model and f…
We report an experimental study of the magnetic order and electronic structure and transport of the layered pnictide EuMnSb$_2$, performed using neutron diffraction, angle-resolved photoemission spectroscopy (ARPES), and magnetotransport measurements. We find that the Eu and Mn sublattices display antiferromagnetic (AFM) order below $T_\mathrm{N}^\mathrm{Eu} = 21(1)$ K and $T_\mathrm{N}^\mathrm{Mn} = 350(2)$ K respectively. The former can be described by an A-type AFM structure with the Eu spins aligned along the $c$ axis (an in-plane direction), whereas the latter has a C-type AFM structure w…
The layered MnBi2nTe3n+1 family represents the first intrinsic antiferromagnetic topological insulator (AFM TI, protected by a combination symmetry ) ever discovered, providing an ideal platform to explore novel physics such as quantum anomalous Hall effect at elevated temperature and axion electrodynamics. Recent angle-resolved photoemission spectroscopy (ARPES) experiments on this family have revealed that all terminations exhibit (nearly) gapless topological surface states (TSSs) within the AFM state, violating the definition of the AFM TI, as the surfaces being studied should be -breaking …
We show how an accurate first-principles treatment of the antiferromagnetic (AFM) ground state of La$_2$CuO$_4$ can be obtained without invoking any free parameters such as the Hubbard $U$. The magnitude and orientation of our theoretically predicted magnetic moment of $0.495 μ_{B}$ on Cu-sites along the (100) direction are in excellent accord with experimental results. The computed values of the band gap (1.00 eV) and the exchange-coupling (-138 meV) match the corresponding experimental values. We identify interesting band splittings below the Fermi energy, including an appreciable Hund's spl…
We use high-resolution, tunable angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) calculations to study the electronic properties of single crystals of MnBi2Te4, a material that was predicted to be the first intrinsic antiferromagnetic (AFM) topological insulator. We observe both bulk and surface bands in the electronic spectra, in reasonable agreement with the DFT calculations results. In striking contrast to the earlier literatures showing a full gap opening between two surface band manifolds along (0001) direction, we observed a gapless Dirac cone remain …
Based on first-principles calculations and symmetry analysis, we propose that EuIn$_2$As$_2$ is a long awaited axion insulator with antiferromagnetic (AFM) long range order. Characterized by the parity-based invariant $\mathbb Z_4=2$, the topological magneto-electric effect is quantized with $θ=π$ in the bulk, with a band gap as large as 0.1 eV. When the staggered magnetic moment of the AFM phase is along $a/b$ axis, it's also a TCI phase. Gapless surface states emerge on (100), (010) and (001) surfaces, protected by mirror symmetries (nonzero mirror Chern numbers). When the magnetic moment is…
Studies of the electronic spectral function in cuprates by Angle-Resolved Photo-Emission Spectroscopy reveal unusual features in the pseudogap phase that persist in the superconducting phase. We address here these observations based on the recently proposed idea that the pseudogap is due to the fractionalization of modulated particle-particle pairs (a Pair Density Wave) into uniform particle-particle and modulated particle-hole pairs. The constraint that appears between these two types of pairs can be seen has an amplitude for the pseudogap energy scale. This constraint directly modify the ele…
利用扫描隧道显微镜（STM）研究了高温超导体$_2$ O $_2$的解理面，发现一维CuO链中存在电荷密度波（CDW）调制.在同一时间，没有签名的CDW已被报道的光谱功能的链带先前研究的光电发射。我们使用软X射线角分辨光电子能谱（SX-ARPES）来检测在以前的工作中没有检测到的链衍生的表面带。发现新表面带的$2k_\textup{F}$为0.55 π，ε $^{-1}$，这与STM在直接空间中观察到的CDW波矢量相匹配。这揭示了费米面嵌套的相关性的CuO链中的CDW的形成在YBa $_2$ Cu $_2$ O $_{7-δ}$。与CDW顺序的短程性质的协议，新检测到的表面带表现出赝能隙，其能量尺度也对应于STM观察到的。
