Bi $_2$ Sr $_{2-x}$ La PDMATHAAC CuO $_{6+δ}$角分辨光电发射中表观费米面穴的结构起源
Structural origin of apparent Fermi surface pockets in angle-resolved photoemission of Bi$_2$Sr$_{2-x}$La$_x$CuO$_{6+δ}$
P. D. C. King, J. A. Rosen, W. Meevasana, A. Tamai, E. Rozbicki, R. Comin, G. Levy, D. Fournier, Y. Yoshida, H. Eisaki, K. M. Shen, N. J. C. Ingle, A. Damascelli, F. Baumberger
We observe apparent hole pockets in the Fermi surfaces of single-layer Bi-based cuprate superconductors from angle-resolved photoemission (ARPES). From detailed low-energy electron diffraction measurements and an analysis of the ARPES polarization-dependence, we show that these pockets are not intrinsic, but arise from multiple overlapping superstructure replicas of the main and shadow bands. We further demonstrate that the hole pockets reported recently from ARPES [Meng et al, Nature 462, 335 (2009)] have a similar structural origin, and are inconsistent with an intrinsic hole pocket associated with the electronic structure of a doped CuO$_2$ plane. The nature of the Fermi surface topology in the enigmatic pseudogap phase therefore remains an open question.
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Comment on arXiv:1012.1484v1 Structural origin of apparent Fermi surface pockets in angle-resolved photoemission of Bi_2Sr_{2-x}La_xCuO_{6+δ} by King et al
Two pseudogaps with different energy scales at the antinode of the high-temperature Bi$_2$Sr$_2$CuO$_6$ superconductor using angle-resolved photoemission spectroscopy
我们已经进行了高分辨率角分辨光电子能谱的单层铜酸盐Bi $_2$ Sr $_2$ CuO $_6$澄清的赝能隙的起源。通过使用不同的光子能量,我们已经成功地直接观察到两个不同的赝能隙与两个不同的能量尺度共存的波腹区域:一个反映了$d_{x^2-y^2}$波配对强度,而另一个具有较大的能量尺度,表明起源不同于超导。观察到的双赝能隙行为提供了一个关键,以充分理解赝能隙现象的铜酸盐。
Anisotropic dressing of charge-carriers in the electron-doped cuprate superconductor Sm(1.85)Ce(0.15)CuO(4) from angle-resolved photoemission measurements
Identification of Nodal Kink in Electron-Doped (Nd$_{1.85}$Ce$_{0.15}$)CuO$_4$ Superconductor from Laser-Based Angle-Resolved Photoemission Spectroscopy
对电子掺杂的(Nd $_{1.85}$ Ce $_{0.15}$)CuO $_4$高温超导体进行了高分辨激光角分辨光电子能谱测量。我们揭示了一个明确的扭结在$\sim$ 60毫电子伏的色散沿(0,0)-($π$,$π$)节方向,伴随着峰-谷-驼峰功能的光电子能谱。这表明,在电子掺杂的超导体中,节点电子与集体激发(玻色子)耦合,声子是最有可能的玻色子候选者。这一发现建立了一个普遍性的节点电子耦合在空穴和电子掺杂的高温铜氧化物超导体。
The superconductivity of high transition temperature (Tc) occurs in copper oxides with carrier-doping to an antiferromagnetic (AF) Mott insulator. This discovery more than thirty years ago immediately led to a prediction about the formation of a small Fermi pocket. This structure, however, has not yet been detected, while it could be a key element in relating high-Tc superconductivity to Mott physics. To address this long-standing issue, we investigate the electronic structure of a five-layered Ba2Ca4Cu5O10(F,O)2 with inner CuO2 planes demonstrated to be cleanest ever in cuprates. Most surpris…
Electronic Structure of Ce-Doped and -Undoped Nd$_2$CuO$_4$ Superconducting Thin Films Studied by Hard X-ray Photoemission and Soft X-ray Absorption Spectroscopy
Persistent Fermi Pockets and Robust Electron Pairing in Lightly Doped CuO$_2$ Planes of Cuprate Superconductors
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所凝聚态物理国家实验室);University of Chinese Academy of Sciences(中国科学院大学);Max Planck Institute for Solid State Research(马克斯·普朗克固体研究研究所);Technical Institute of Physics and Chemistry, Chinese Academy of Sciences(中国科学院理化技术研究所);Songshan Lake Materials Laboratory(松山湖材料实验室);Beijing Academy of Quantum Information Sciences(北京量子信息科学研究院)
Monotonic d-wave Superconducting Gap in Optimally-Doped Bi$_2$Sr$_{1.6}$La$_{0.4}$CuO$_6$ Superconductor by Laser-Based Angle-Resolved Photoemission Spectroscopy
利用超高分辨激光角分辨光电子能谱研究了最佳掺杂Bi $_2$ Sr $_{1.6}$ La $_{0.4}$ CuO $_6$超导体的超导能隙和赝能隙随动量和温度的变化关系。在超导状态下测得的能隙表现出标准的{ \it d}-波形。赝能隙在T $_c$以上的费米面的很大一部分打开,在结区附近形成“费米弧”。在“费米弧”以外的区域,赝能隙具有与超导态类似的能隙大小和动量依赖性,能隙随温度变化很小,在T_PDMATHABMR上没有突变。这些观测结果表明赝能隙和超导能隙是密切相关的,并支持赝能隙是超导能隙的先驱的观点。
Superconducting gap symmetry of Ba0.6K0.4Fe2As2 studied by angle-resolved photoemission spectroscopy
我们对最佳掺杂的Ba $_{0.6}$ K $_{0.4}$ Fe $_2$ As $_2$化合物进行了高分辨角分辨光电子能谱研究,并精确地测定了四个费米面片中超导能隙的动量依赖关系,其中包括一个新发现的M点外电子袋。在这个口袋上的SC间隙几乎是各向同性的,其幅度($Δ$ $\sim$ 11 meV)与内部电子和空穴口袋($\sim$ 12 meV)相当,尽管它比外部空穴口袋($\sim$ 6 meV)大得多。SC能隙值的费米面依赖性基本上与扩展s波对称性所期望的$Δ$($k$)= $Δ$ $_0$ cos $k_x$ cos $k_y$公式一致。观察到的与简单公式的有限偏差表明了多轨道效应的重要性。
Superconductivity distorted by the coexisting pseudogap in the antinodal region of Bi$_{1.5}$Pb$_{0.55}$Sr$_{1.6}$La$_{0.4}$CuO$_{6+δ}$: A photon-energy-dependent angle-resolved photoemission study
超导电性和赝能隙之间的相互作用是铜氧化物物理的一个重要方面。然而,赝能隙的性质仍然存在争议,部分原因是不同的实验提出了不同的能隙函数。本文采用光子能量依赖角分辨光电子能谱(ARPES)研究了Bi $_{1.5}$ Pb $_{0.55}$ Sr $_{1.6}$ La $_{0.4}$ CuO $_{6+δ}$ .我们发现,在低光子能量的反节ARPES谱是由背景信号,这可能会导致一个错误的评估的光谱间隙的大小占主导地位。一旦背景是适当的占,独立的光子能量,在不同的能量下,主要归因于赝能隙和超导性,以及偏离一个简单的d-波形式的整体光谱间隙的波腹光谱鲁棒地显示两个共存的功能。这些结果支持了赝能隙和超导性之间的竞争导致能隙畸变的观点。
Occurrence of Fermi Pockets without Pseudogap Hypothesis and Clarification of the Energy Distribution Curves of Angle-Resolved Photoemission Spectroscopy in Underdoped Cuprate Superconductors
Reaffirming the $d_{x^2-y^2}$ superconducting gap using the auto-correlation angle-resolved photoemission spectroscopy of Bi$_{1.5}$Pb$_{0.55}$Sr$_{1.6}$La$_{0.4}$CuO$_{6+δ}$
Electronic structure of heavily electron-doped BaFe$_{1.7}$Co$_{0.3}$As$_2$ studied by angle-resolved photoemission
我们对重电子掺杂非超导BaFe $_{1.7}$ Co $_{0.3}$ As $_2$进行了高分辨角分辨光电子能谱研究。我们发现在空穴掺杂的超导体Ba $_{0.6}$ K $_{0.4}$ Fe $_2$ As $_2$中观察到的两个空穴费米面口袋在该化合物中不存在或非常小,而在M点处的两个电子口袋由于Co替代的电子掺杂而显著膨胀。非SC和SC样品的费米面的比较表明,通过反铁磁波矢连接的空穴和电子口袋的共存是实现铁基超导体的超导性机制的必要条件。
Angle-resolved photoemission spectroscopy of Na-doped Ca2CuO2Cl2 single crystals: Fingerprints of a magnetic insulator in a heavily underdoped superconductor
To reconcile the two experimental findings on La_{2-x}Sr_{x}CuO_4, namely, Fermi surface (FS) observed by angle-resolved photoemission spectroscopy and sharp incommensurate magnetic peaks by neutron scattering, we propose a picture that a quasi-one-dimensional FS (q-1dFS) is realized in each CuO_{2} plane whose q-1d direction alternates along the c-axis.
We performed an optical spectroscopy study on single crystals of Pr$_{0.85}$LaCe$_{0.15}$CuO$_{4-δ}$ (PLCCO) to revisit the electron-hole asymmetry, which has been understood as a fundamental property of cuprates. Four differently annealed samples - as-grown, reduced, optimally oxygenated, and over-oxygenated samples - were prepared, which have superconducting transition temperatures, $T_c$ = 0, 15, 24, and 18 K, respectively. We observed that low-energy quasiparticle spectral weights of all the PLCCO samples are significantly small in comparison with those of other electron-doped cuprate fami…
Hard X-ray Cu $2p$ Core-Level Photoemission of High-$T_c$ Cuprate Superconductors
用硬X射线光电子能谱(HX-PES)对单层La $_{2-x}$ Sr $_{x}$ CuO $_{4}$、La掺杂Bi $_2$ Sr $_{1.6}$ La $_{0.4}$ CuO $_{6+δ}$(Bi 2201)和双层Bi $_2$ Sr $_{2}$ CaCu $_{2}$ O $_{8+δ}$(Bi 2212)高温超导体中Cu $2p$芯能级谱进行了详细的研究.我们鉴定了Cu $^{2+}$衍生的(i)Zhang-Rice单线态(ZRS)特征,(ii)$d^{n+1}\underline{L}$(配体屏蔽)特征,(iii)$d^{n}$卫星特征,以及主峰中空穴掺杂衍生的高结合能特征。在Bi基铜酸盐中,与La $_{2-x}$ Sr $_{x}$ CuO $_{4}$相比,$d^{n}$卫星特征的强度似乎强烈增强。从X射线光子能量相关的测量,它表明,在卫星区域的强度增加与Bi $4s$核心水平的光谱强度。修正后的$d^{n}$卫星强度与Cu-O层的掺杂含量或层数无关。我们的研究结果表明,相关的ZRS功能和空穴掺杂引起的高结合能谱的主峰与超导电性的变化的相对强度。
In order to study the possible superconductivity at the polar surfaces of 1111-type iron-based superconductors, which is doped with a large amount of holes in spite of the electron doping in bulk materials, we have performed angle-resolved photoemission spectroscopy (ARPES) studies on superconducting PrFeAsO$_{1-y}$~crystals. We have indeed observed the opening of a superconducting gap on surface-derived hole pockets as well as on a bulk-derived hole pocket. The superconducting gap is found to open on the surface-derived hole pockets below the bulk $T_c$, which suggests that the surface superc…
Doping evolution of the electronic structure in the single-layer cuprates Bi$_2$Sr$_{2-x}$La$_x$CuO$_{6+δ}$: Comparison with other single-layer cuprates
我们已经进行了角分辨光电子能谱和芯层X射线光电子能谱研究的单层铜酸盐Bi $_2$ Sr $_{2-x}$ La $_x$ CuO $_{6+δ}$(Bi 2201),并揭示了掺杂的电子结构的演变从轻掺杂到最佳掺杂区域。我们已经观察到的色散准粒子带的形成,费米“弧”的费米面的演变和化学势的移动与空穴掺杂在其他铜酸盐。Bi 2201中的掺杂演变类似于Ca $_{2-x}$ Na $_{x}$ CuO $_{2}$ Cl $_2$(Na-CCOC)中的掺杂演变,其中已经观察到朝向母绝缘体的较低哈伯德带的快速化学势偏移,但是与La $_{2-x}$ Sr $_{x}$ CuO $_{4}$(LSCO)中的掺杂演变完全不同,其中化学势不偏移,而色散带和费米弧/表面已经在轻掺杂区中的费米能级周围形成。利用紧束缚拟合定量分析了费米面形状和能带色散,推导出的次近邻跳跃积分$t'$也证实了与Na-CCOC的相似性和与LSCO的不同.
We present a comprehensive study of the low-energy band structure and Fermi surface (FS) topology of $A$Co$_2$As$_2$ ($A=$ Ca, Sr, Ba, Eu) using high-resolution angle-resolved photoemission spectroscopy. The experimental FS topology and band dispersion data are compared with theoretical full-potential linearized augmented-plane-wave (FP-LAPW) calculations, which yielded reasonably good agreement. We demonstrate that the FS maps of $A$Co$_2$As$_2$ are significantly different from those of the parent compounds of Fe-based high-temperature superconductors. Further, the FSs of CaCo$_2$As$_2$ do no…
We performed angle-resolved photoemission spectroscopy with micro-focused beam on a topological line-nodal compound CaSb2 which undergoes a superconducting transition at the onset Tc~1.8 K, to clarify the Fermi-surface topology relevant to the occurrence of superconductivity. We found that a three-dimensional hole pocket at the G point is commonly seen for two types of single-crystalline samples fabricated by different growth conditions. On the other hand, the carrier-doping level estimated from the position of the chemical potential was found to be sensitive to the sample fabrication conditio…
Nodeless high-T$_c$ superconductivity in highly-overdoped monolayer CuO$_2$
本文研究了最近在$d$波铜氧化物超导体Bi $_2$ Sr $_2$ CaCu $_2$ O $_{8+δ}$上生长的CuO $_2$单层的电子结构和超导电性。密度泛函理论的计算表明,显着的电荷转移的界面,使CuO $_2$单层是严重过掺杂到空穴丰富的制度,但无法在散装铜酸盐。我们发现Cu的$d_{x^2-y^2}$和$d_{3z^2-r^2}$轨道都变得重要,费米面分别包含一个电子和一个空穴口袋。构建一个最小的相关的两轨道模型的$e_g$复杂的,我们表明,自旋轨道交换相互作用产生的无节点超导体扩展$s$波配对对称性和配对能隙相媲美的散装$d$波间隙,与最近的实验一致。研究结果指出了在臭氧生长的过渡金属氧化物单层异质结构中实现新的高$T_c$超导体的方向。