Angle resolved photoemission spectroscopy (ARPES) studies of the overdoped cuprate superconductor La$_{2-x}$Sr$_x$CuO$_4$ find only small changes in the near nodal electron self energy over a spectral range of several hundred meV as the doping increases from x=0.2 to x=0.3 and the superconducting transition temperature T_c decreases from 32K to 0K. These measurements put constraints on the structure of the electron-electron interaction. Here we show that a spin-fluctuation interaction leads to behavior which is consistent with these experimental results.
Evidence for the presence of high energy magnetic excitations in overdoped La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) has raised questions regarding the role of spin-fluctuations in the pairing mechanism. If they remain present in overdoped LSCO, why does $T_c$ decrease in this doping regime? Here, using results for the dynamic spin susceptibility ${\rm Im}χ(q,ω)$ obtained from a determinantal quantum Monte Carlo (DQMC) calculation for the Hubbard model we address this question. We find that while high energy magnetic excitations persist in the overdoped regime, they lack the momentum to scatter pairs bet…
We investigate the pairing symmetry in heavily overdoped Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$ based on the spin-fluctuation mechanism. The exotic octet nodes of the superconducting gap and the unusual evolution of the gap with doping observed by the recent experiments are well explained in a unified manner. We demonstrate that the scatterings of electrons on the Fermi patches is mainly responsible for the incommensurate spin fluctuations and consequently the Fermi-surface-dependent multi-gap structure, since the Fermi level is close to the flat band. In addition, we find that a $d$-wave pairing s…
We propose a theoretical description of the superconducting state of under- to overdoped cuprates, based on the short coherence length of these materials and the associated strong pairing fluctuations. The calculated $T_c$ and the zero temperature excitation gap $Δ(0)$, as a function of hole concentration $x$, are in semi-quantitative agreement with experiment. Although the ratio $T_c/Δ(0)$ has a strong $x$ dependence, different from the universal BCS value, and $Δ(T)$ deviates significantly from the BCS prediction, we obtain, quite remarkably, quasi-universal behavior, for the normalized supe…
Cooper's one pair problem is investigated for a 2D lattice in the background of both passive and active Fermi sea in a weakly correlated environment. Boson exchange mechanisms involving excitons as well as phonons are invoked for pairing in the s- wave channel. The important quantities calculated are pairing energy and coherence length as functions of bosonic energy, attracted coupling constant and band filling factor. Comparison of our theoretical results with those from experiments on overdoped cuprate superconductors and other type of theoretical calculations show electronic mechanism to be…
Studying the disappearance of superconductivity at the end of the overdoped region of the cuprate phase diagram offers a different approach for investigating the interaction which is responsible for pairing in these materials. In the underdoped region this question is complicated by the presence of charge and stripe ordered phases as well as the pseudogap. In the overdoped region the situation appears simpler with only a normal phase, a superconducting phase and impurity scattering. Here, for the overdoped region, we report the results of a combined dynamic cluster approximation (DCA) and a we…
We present a theoretical framework for understanding the behavior of the normal and superconducting states of overdoped cuprate high temperature superconductors in the vicinity of the doping-tuned quantum superconductor-to-metal transition. The key ingredients on which we focus are d-wave pairing, a flat antinodal dispersion, and disorder. Even for homogeneous disorder, these lead to effectively granular superconducting correlations and a superconducting transition temperature determined in large part by the superfluid stiffness rather than the pairing scale.
Overdoped high-temperature cuprate superconductors have been widely believed to be described by the physics of d-wave BCS-like superconductivity. However, recent measurements indicate that as the doping is increased, the superfluid density decreases smoothly to zero rather than increasing as expected by BCS theory in the absence of disorder. Here, we combine time-domain THz spectroscopy with kHz range mutual inductance measurements on the same overdoped La$_{2-x}$Sr$_{x}$CuO$_{4}$ films to determine both the superfluid and the uncondensed carrier density as a function of doping. A significant …
Evidence is presented from the scaling of the Knight shift, entropy and transport properties together with the sharp peaking of condensation energy, critical currents, superfluid density and a variety of other physical properties for the occurrence of a common critical doping point in lightly overdoped high-Tc superconductors (HTS). This critical doping lies at the point where the doping-dependent normal-state pseudogap energy, Eg, falls to zero and bears a strong, though incomplete, resemblance to a quantum critical point (QCP). A QCP scenario could lead directly to an explanation of the non-…
The spin dynamics in single crystal, electron-doped Ba(Fe1-xCox)2As2 has been investigated by inelastic neutron scattering over the full range from undoped to the overdoped regime. We observe damped magnetic fluctuations in the normal state of the optimally doped compound (x=0.06) that share a remarkable similarity with those in the paramagnetic state of the parent compound (x=0). In the overdoped superconducting compound (x=0.14), magnetic excitations show a gap-like behavior, possibly related to a topological change in the hole Fermi surface (Lifshitz transition), while the imaginary part of…
We report in-plane Cu(63) Nuclear Magnetic Resonance measurements for a series of fully enriched Ca(0.1)La(0.9)Ba(1.65)La(0.35)Cu(3)O(y) powder samples, which belong to the YBCO family, but the doping could vary from very underdoped to extremely overdoped. From these measurements we determine the average nuclear quadrupole resonance frequency ν_Q, and its second moment Δ(ν_Q), both set by the in-plane hole density, n, as a function of oxygen level, y. We find that in the overdoped side n is saturated, but Δ(ν_Q) rapidly increases with increasing y. The relevance of these results to the increas…
Cooper's formalism for fermionic pairing has been revisited considering upto 3rd neighbour hopping terms, firstly with a Fermi liquid like background on a square lattice keeping in mind the overdopped cuprates. Then the whole scheme is repeated with a Marginal Fermi liquid- like background, taking into account the self energy correction of the mobile electrons to include a more realitic density of states in the calculation. Detailed comparison of our theoretical results with those from experiments strongly supports the Marginal Fermi liquid- like character of the normal phase with exciton medi…
Photoexcited quasiparticle relaxation dynamics in overdoped Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ ($T_{c}$=65~K, hole doping $p$=0.22) single crystal is investigated as a function of temperature. We provide evidence of a $\sim$22~meV pseudogap ($T^{\ast}$$\approx$100~K) at this doping level. Our data support the scenario where both the superconducting gap and pseudogap coexist in the superconducting state. Our results also suggest an increased scattering rate between electrons and spin fluctuations as the sample enters the pseudogap phase.
The thermoelectric power S(T) of single-layer Bi2Sr2CuO6+d is studied as a function of oxygen doping in the strongly overdoped region of the phase diagram (T, d). As other physical properties in this region, diffusion thermopower Sdiff(T) also shows an important deviation from conventional Fermi liquid behaviour. This departure from T-linear S(T) dependence together with the results of susceptibility on the same samples suggest that the origin of the observed non-metallic behaviour is the existence of a singularity in the density of states near the Fermi level. The doping and temperature depen…
We successfully tuned an underdoped ultrathin YBa2Cu3O7-x film into the overdoped regime by means of electrostatic doping using an ionic liquid as a dielectric material. This process proved to be reversible. Transport measurements showed a series of anomalous features compared to chemically doped bulk samples and a different two-step doping mechanism for electrostatic doping was revealed. The normal resistance increased with carrier concentration on the overdoped side and the high temperature (180 K) Hall number peaked at a doping level of p$\sim$0.15. These anomalous behaviors suggest that th…
Motivated by the presence of an extremely small electron pocket in the electronic band structure of infinite-layer (IL) nickelate superconductors, we systematically explore the superconducting (SC) properties of a two-dimensional Hubbard model influenced by an additional conduction band with small occupancy (dry Fermi sea). Our dynamic cluster quantum Monte Carlo calculations demonstrated the unusual impact of this additional dry metallic layer, which shifts the SC dome of the correlated Hubbard layer towards the overdoped regime, namely the $d$-wave SC can be enhanced (suppressed) in the over…
Electronic anisotropy was studied for overdoped (Y,Ca)Ba2Cu3O7-d with various doping levels (p). It was found that the pseudogap-like behavior in the resistivity disappear when p exceeds 0.17, independent of the oxygen deficiency. The anisotropy ratio (g) estimated from upper critical fields showed a rapid decrease at around p = 0.18, approaching g = 3 for p > 0.20.
We consider a model self-energy consisting of an isotropic Fermi liquid term and a Marginal Fermi liquid term which is anisotropic over the Fermi surface, vanishing in the same directions as the superconducting gap and the pseudogap. This model self-energy gives a consistent description of experimental results from Angle-Dependent Magneto-Resistance (ADMR), specific heat, de Haas-van Alphen, and measurements of the quasi-particle dispersion near the Fermi surface from photoemission. In particular, we reconcile the strongly doping dependent anomalous scattering rate observed in ADMR with the al…
A d-wave, Eliashberg analysis of break junction and STM tunneling spectra on BiSrCaCuO (Bi2212) reveals that a spectral dip feature is directly linked to strong electronic coupling to a narrow boson spectrum, evidenced by a large peak in the boson spectral weight. The tunneling dip feature remains robust in the overdoped regime of Bi2212 with bulk Tc values of 56 K-62 K. This is contrary to recent optical conductivity measurements of the self-energy that suggest the narrow boson spectrum disappears in overdoped Bi2212 and therefore cannot be essential for the pairing mechanism. The discrepancy…
Using self consistent mean field and functional renormalization group approaches we show that s-wave pairing symmetry is robust in the heavily electron-doped iron chalcogenides $(\text{K, Cs}) \text{Fe}_{2-x}\text{Se}_2 $. This is because in these materials the leading antiferromagnetic (AFM) exchange coupling is between next-nearest-neighbor (NNN) sites while the nearest neighbor (NN) magnetic exchange coupling is ferromagnetic (FM). This is different from the iron pnictides, where the NN magnetic exchange coupling is AFM and leads to strong competition between s-wave and d-wave pairing in th…
We report an angular quantum oscillation study of Tl_2Ba_2CuO_{6+delta} for two different doping levels (Tc = 10K and 26 K) and determine the Fermi surface size and topology in considerable detail. Our results show that Fermi liquid behavior is not confined to the edge of the superconducting dome and is robust up to at least T_c^{max}/3.5. Superconductivity is found to survive up to a larger doping p_c = 0.31 than in La_{2-x}Sr_xCuO_4. Our data imply that electronic inhomogeneity does not play a significant role in the loss of superconductivity and superfluid density in overdoped cuprates, and…
We demonstrated experimentally a direct way to probe a hidden propensity to the formation of spin density wave (SDW) in a non-magnetic metal with strong Fermi surface nesting. Substituting Fe for a tiny amount of Cu (1%) induced an incommensurate magnetic order below 20 K in heavily-overdoped La2-xSrxCuO4 (LSCO). Elastic neutron scattering suggested that this order cannot be ascribed to the localized spins on Cu or doped Fe. Angle-resolved photoemission spectroscopy (ARPES), combined with numerical calculations, revealed a strong Fermi surface nesting inherent in the pristine LSCO that likely …
We present low-temperature thermal conductivity measurements on the cuprate Tl_2Ba_2CuO_{6+delta} throughout the overdoped regime. In the T -> 0 limit, the thermal conductivity due to d-wave nodal quasiparticles provides a bulk measurement of the superconducting gap, Delta. We find Delta to decrease with increasing doping, with a magnitude consistent with spectroscopic measurements (photoemission and tunneling). This argues for a pure and simple d-wave superconducting state in the overdoped region of the phase diagram, which appears to extend into the underdoped regime down to a hole concentra…
Hall coefficient $R_H$ and thermoelectric power TEP are studied systematically in the single crystals $Nd_{2-x}Ce_xCuO_{4+δ}$ (NCCO) with different x from underdoped to overdoped regime. With increasing doping level, both $R_H$ and TEP decrease and change their sign from negative to positive. A striking feature is that the temperature dependence of the Hall angle follows a $T^4$ behavior in the underdoped regime, while a $T^2$ in the overdoped regime. These behaviors are closely related to the evolution of Fermi surface with doping level observed by ARPES.
The doping of charge carriers into the CuO2 planes of copper oxide Mott insulators causes a gradual destruction of antiferromagnetism and the emergence of high-temperature superconductivity. Optimal superconductivity is achieved at a doping concentration p beyond which further increases in doping cause a weakening and eventual disappearance of superconductivity. A potential explanation for this demise is that ferromagnetic fluctuations compete with superconductivity in the overdoped regime. In this case a ferromagnetic phase at very low temperatures is predicted to exist beyond the doping conc…
The evolution of the thermoelectric power S(T) with doping, p, of single-layer Bi2Sr2CuO6+d ceramics in the strongly overdoped region is studied in detail. Analysis in term of drag and diffusion contributions indicates a departure of the diffusion from the T-linear metallic behavior. This effect is increased in the strongly overdoped range (p~0.2-0.28) and should reflect the proximity of some topological change.
The doping dependence of the themopower, in-plane resistivity rho_ab(T), out-of-plane resistivity rho_c(T), and susceptibility has been systematically measured for high-quality single crystal Bi2Sr2Ca2Cu3O10+delta. We found that the transition temperature Tc and pseudogap formation temperature T_rho_c*, below which rho_c shows a typical upturn, do not change from their optimum values in the "overdoped" region, even though doping actually proceeds. This suggests that, in overdoped region, the bulk $T_c$ is determined by the always underdoped inner plane, which have a large superconducting gap, …
We report Raman scattering spectra for single crystals of overdoped Tl2Ba2CuO6+d (Tl-2201) at low temperatures. It was observed that the pair-breaking peaks in A1g and B1g spectra radically shift to lower energy with carrier doping. We interpret it as s-wave component mixing into d-wave, although the crystal structure is tetragonal. Since similar phenomena were observed also in YBa2Cu3Oy and Bi2Sr2CaCu2Oz, we conclude that s-wave mixing is a common property for overdoped high-Tc superconductors.
We present the ab-plane optical conductivity of four single crystals of Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+δ}$ (Bi2212) with different carrier doping levels from the strongly underdoped to the strongly overdoped range with $T_c$=66, 88, 77, and 67 K respectively. We focus on the redistribution of the low frequency optical spectral weight (SW) in the superconducting and normal states. The temperature dependence of the low-frequency spectral weight in the normal state is significantly stronger in the overdoped regime. In agreement with other studies, the superconducting order is marked by an increa…
We use scanning tunneling microscopy to investigate Bi2Sr2Ca2Cu3O10+δ trilayer cuprates from the optimally doped to overdoped regime. We find that the two distinct superconducting gaps from the inner and outer CuO2 planes both decrease rapidly with doping, in sharp contrast to the nearly constant Tc. Spectroscopic imaging reveals the absence of quasiparticle interference in the antinodal region of overdoped samples, showing an opposite trend to that in single- and double-layer compounds. We propose that the existence of two types of inequivalent CuO2 planes and the intricate interaction betwee…
Using angle-resolved photoemission spectroscopy, we studied the electronic structure of NaFe$_{1-x}$Co$_x$As from an optimally doped superconducting compound ($x=0.028$) to a heavily overdoped non-superconducting one ($x=0.109$). Similar to the case of "122" type iron pnictides, our data suggest that Co dopant in NaFe$_{1-x}$Co$_x$As supplies extra charge carriers and shifts the Fermi level accordingly. In the $x=0.109$ compound, the hole-like bands around the zone center $Γ$ move to deeper binding energies and an electron pocket appears instead. The overall band renormalization remains basica…
We analyze the two-orbital (with $d_{x^2-y^2}$ and $d_{3z^2-r^2}$ orbitals) analogue of the $t$-$J$-$U$ model as applied to the description of the copper-oxide monolayer deposited on the Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ substrate (CuO$_2$/BSCCO). We show, that an $extended$ $s$-$wave$ superconducting dome appears in the heavily hole overdoped regime of the model, with dominant contribution to the pairing coming from the $d_{3z^2-r^2}$ orbitals. Also, the lower critical doping for the appearance of the SC state concurs with the Lifshitz Transition after which the hole-like Fermi pockets are create…
A recent article suggested that the saturation of low energy spectral weight observed by X-ray absorption spectroscopy in the cuprates at high hole doping could be explained within the single-band Hubbard model. We show that this result is an artifact of inappropriate integration limits.
The superconducting transition temperature, Tc, of bilayers comprising underdoped La2-xSrxCuO4 films capped by a thin heavily overdoped metallic La1.65Sr0.35CuO4 layer, is found to increase with respect to Tc of the bare underdoped films. The highest Tc is achieved for x = 0.12, close to the 'anomalous' 1/8 doping level, and exceeds that of the optimally-doped bare film. Our data suggest that the enhanced superconductivity is confined to the interface between the layers. We attribute the effect to a combination of the high pairing scale in the underdoped layer with an enhanced phase stiffness …
We show that low-energy spectral features in the cuprates can be separated into different components by the measurement of the recombination dynamics of different low-energy excitations in real-time using femtosecond laser spectroscopy. Quasiparticle (QP) recombination across the gap and intra-gap localized state relaxation processes exhibit qualitatively different time- and temperature-dependences. The relaxation measurements also show the existence of two distinct coexisting energy gaps near optimum doping and in the overdoped region, one more or less temperature independent (which exists ab…
The ab plane optical spectra of two single crystals of La(2-x)Sr(x)Cu(4), one overdoped and one underdoped, were investigated. We observe a gap-like depression of the effective scattering rate below 700 cm(-1) in both systems. This feature persists up to 300 K in the underdoped sample with the concentration of Sr x=0.14 but loses prominance at temperatures above 300 K in the overdoped regime (x=0.22). Below 700 cm(-1) the scattering rate is temperature dependent and superlinear in frequency for both samples. Above this frequency the effective scattering rate becomes linear in frequency and is …
We report on a study of the influence of defects introduced in the CuO$_{2}$ planes of cuprates in a wide range of hole dopings n. T$_{c}$ and electrical resistivity $ρ(T)$ measurements have been performed on electron irradiated YBa$_{2}$Cu$_{3}$O$_{7-δ}$ and Tl$_{2}$Ba$_{2}$CuO$_{6+x}$ single crystals. A universal scaling between the decrease in T$_{c}$ and $\UNICODE[m]{0x394}ρ_{2D}\UNICODE[m]{0xd7}n$, where $\UNICODE[m]{0x394}ρ_{2D}$ is the increase of the 2D-resistance induced by the defects, is found for all the samples investigated here. This demonstrates that n is the relevant parameter …
According to a generic temperature vs. carrier-doping (T-p) phase diagram of high-temperature superconductors it has been proposed that as doping increases to the overdoped region they approach gradually a conventional (canonical) Fermi Liquid. However, Hall effect measurements in several systems reported by different authors show a still strong \emph{T}-dependence in overdoped samples. We report here electrical transport measurements of Y_{1-x}Ca_{x}Ba_{2}Cu_{3}O_{7-delta} thin films presenting a temperature dependence of the Hall constant, R_H, which does not present a gradual transition tow…
In high-temperature cuprate superconductors, the anti-ferromagnetic spin fluctuations are thought to have a very important role in naturally producing an attractive interaction between the electrons in the $d$-wave channel. The connection between superconductivity and spin fluctuations is expected to be especially consequential at the overdoped end point of the superconducting dome. In some materials, that point seems to coincide with a Lifshitz transition, where the Fermi surface changes from the hole-like centered at ($π, π$) to the electron-like, centered at the $Γ$ point causing a loss of …
We have performed angle-resolved photoemission spectroscopy on the overdoped Ba$_{0.3}$K$_{0.7}$Fe$_2$As$_2$ superconductor ($T_c$ = 22 K). We demonstrate that the superconducting (SC) gap on each Fermi surface (FS) is nearly isotropic whereas the gap value varies from 4.4 to 7.9 meV on different FSs. By comparing with under- and optimally-doped Ba$_{1-x}$K$_x$Fe$_2$As$_2$, we find that the gap value on each FS nearly scales with $T_c$ over a wide doping range (0.25 $\textyen leq$ $x$ $\textyen leq$ 0.7). Although the FS volume and the SC gap magnitude are strongly doping dependent, the multip…
We consider the implications of a phenomenological model self-energy for the charge transport properties of the metallic phase of the overdoped cuprate superconductors. The self-energy is the sum of two terms with characteristic dependencies on temperature, frequency, location on the Fermi surface, and doping. The first term is isotropic over the Fermi surface, independent of doping, and has the frequency and temperature dependence characteristic of a Fermi liquid. The second term is anisotropic over the Fermi surface (vanishing at the same points as the superconducting energy gap), strongly v…
By partially doping Pb to effectively suppress the superstructure in single-layered cuprate Bi2Sr2CuO6+δ(Pb-Bi2201) and annealing them in vacuum or in high pressure oxygen atmosphere, a series of high quality Pb-Bi2201 single crystals are obtained with Tc covering from 17 K to non-supercondcuting in the overdoped region. High resolution angle resolved photoemission spectroscopy (ARPES) measurements are carried out on these samples to investigate the evolution of the Fermi surface topology with doping in the normal state. Clear and complete Fermi surface are observed and quantitatively analyzed…
We study the electronic structure and superconductivity in CuO$_2$ monolayer grown recently on $d$-wave cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$. Density functional theory calculations indicate significant charge transfer across the interface such that the CuO$_2$ monolayer is heavily overdoped into the hole-rich regime yet inaccessible in bulk cuprates. We show that both the Cu $d_{x^2-y^2}$ and $d_{3z^2-r^2}$ orbitals become important and the Fermi surface contains one electron and one hole pocket associated with the two orbitals respectively. Constructing a minimal correlated tw…
Single crystals of the optimally doped, moderately and strongly overdoped high temperature superconductor Tl2Ba2CuO6+x (Tl-2201) with Tc=80, 56 and 30K, respectively, have been investigated by polarized Raman scattering. By taking the peak position of the B_1g component of electronic Raman scattering as 2Delta_0 we found that the reduced gap value (2Delta_0/k_BT_c) strongly decreases with increasing doping. The behavior of the low frequency scattering for the B_1g and B_2g scattering components is similar for optimally doped and overdoped crystals and can be described by a w^3 - and w -law, re…
Based on an improved U(1) slave-boson approach to the t-J Hamiltonian, we invest igate a relationship between the superfluid weight $n_s/m^*$(the superconducting charge carrier density/the effective mass of the charge carrier) and the superc onducting temperature $T_c$. From the present study we find a linear increase of $n_s/m^*$ with $T_c$ with th e doping concentration in the underdoped region, a saturation around the optimal doping and a decrease in both $n_s/m^*$ and $T_c$ in the overdoped region. Such a trend of the `boomerang' shaped locus in $n_s/m^*$ vs. $T_c$ with increas ing doping …
The single-site two-electron exchange amplitude J_sd between the Cu 4s and Cu 3d_{x^2-y^2} states is found to be the pairing mechanism of high-T_c overdoped cuprates. The noninteracting part of the Hamiltonian spans the copper Cu 4s, Cu 3d_{x^2-y^2} and oxygen O 2p_x and O 2p_y states. Within the standard BCS treatment an explicit expression for the momentum dependence of the gap Delta_p is derived and shown to fit the angle-resolved photoemission spectroscopy (ARPES) data. The basic thermodynamic and electrodynamic properties of the model (specific heat C(T), London penetration depth lambda(T…
Strange metals possess highly unconventional transport characteristics, such as a linear-in-temperature ($T$) resistivity, an inverse Hall angle that varies as $T^2$ and a linear-in-field ($H$) magnetoresistance. Identifying the origin of these collective anomalies has proved profoundly challenging, even in materials such as the hole-doped cuprates that possess a simple band structure. The prevailing dogma is that strange metallicity in the cuprates is tied to a quantum critical point at a doping $p*$ inside the superconducting dome. Here, we study the high-field in-plane magnetoresistance of …
Electronic band dispersions in copper oxide superconductors have kinks around 70 meV that are typically attributed to coupling of electrons to a bosonic mode. We performed angle resolved photoemission spectroscopy (ARPES) experiments on overdoped cuprate high temperature superconductors to test the relationship between the superconducting transition temperature and electron-bosonic mode coupling. Remarkably, the kinks remain strong in the heavily overdoped region of the doping phase diagram of LSCO, even when the superconductivity completely disappears. This unexpected observation is incompati…
Magnetotransport measurements on the overdoped cuprate La_{1.7}Sr_{0.3}CuO_4 are fitted using the Ong construction and band parameters inferred from angle-resolved photoemission. Within a band picture, the low temperature Hall data can only be fitted satisfactorily by invoking strong basal-plane anisotropy in the mean-free-path $\ell$. This violation of the isotropic-$\ell$ approximation supports a picture of dominant small-angle elastic scattering in cuprates due to out-of-plane substitutional disorder. We show that both band anisotropy and anisotropy in the elastic scattering channel strongl…
Despite often being dismissively described as exhibiting conventional Fermi-liquid-like behaviour, heavily overdoped high-Tc cuprates sport several unexpected features. Thermodynamic properties expected to be roughly constant with doping decrease towards zero, signalling that a growing fraction of carriers remain in the normal state below Tc. Near Tc, the superconducting energy gap fills in with temperature, contrary to the expectations of BCS theory. Most recently a transition in the Hall number of some cuprates was found to extend to a very high doping (x~0.27), far beyond the pseudogap crit…
We report magnetic susceptibility performed on overdoped Bi2Sr2CuO6+d powders as a function of oxygen doping d and temperature T. The decrease of the spin susceptibility with increasing T is confirmed. At sufficient high temperature, the spin susceptibility Chi_s presents an unusual linear temperature dependence Chi_s ~ Chi_s0 -Chi_1 T. Moreover, a linear correlation between Chi_1 and Chi_s0 for increasing hole concentration is displayed. A temperature Tchi, independent of hole doping characterizes this scaling. Comparison with other cuprates of the literature(LSCO, Tl-2201 and Bi-2212), over …
Low-temperature specific heat (SH) is measured on Ba(Fe$_{1-x}$Co$_{x}$)$_2$As$_2$ single crystals in a wide doping region under different magnetic fields. For the overdoped sample, we find the clear evidence for the presence of $T^2$ term in the data, which is absent both for the underdoped and optimal doped samples, suggesting the presence of line nodes in the energy gap of the overdoped samples. Moreover, the field induced electron specific heat coefficient $Δγ(H)$ increases more quickly with the field for the overdoped sample than the underdoped and optimal doped ones, giving another suppo…
Correlation between the strength of low-temperature T-linear normal-state resistivity and $T_{\rm c}$ in overdoped electron-doped cuprate superconductors
本文在动能驱动超导框架内，揭示了过掺杂电子掺杂型铜氧化物超导体中由自旋激发同时介导的电子umklapp散射与电子配对，自然导致了低温T线性正常态电阻率强度与超导转变温度$T_{\ m c}$之间的内在关联。
Hall effect and quantum oscillation measurements on high temperature cuprate superconductors show that underdoped compositions have a small Fermi surface pocket whereas when heavily overdoped, the pocket increases dramatically in size. The origin of this change in electronic structure has been unclear, but may be related to the high temperature superconductivity. Here we show that the clean overdoped single-layer cuprate Tl2Ba2CuO6+x (Tl2201) displays CDW order with a remarkably long correlation length $ξ\approx 200$ Å which disappears above a hole concentration p_CDW ~ 0.265. We show that the…
We study oxygen K-edge x-ray absorption spectroscopy (XAS) and investigate the validity of the Zhang-Rice singlet (ZRS) picture in overdoped cuprate superconductors. Using large-scale exact diagonalization of the three-orbital Hubbard model, we observe the effect of strong correlations manifesting in a dynamical spectral weight transfer from the upper Hubbard band to the ZRS band. The quantitative agreement between theory and experiment highlights an additional spectral weight reshuffling due to core-hole interaction. Our results confirm the important correlated nature of the cuprates and eluc…
We report on semiclassical angle-dependent magnetoresistance oscillations (AMRO) and the Shubnikov-de Haas effect in the electron-overdoped cuprate superconductor Nd$_{2-x}$Ce$_x$CuO$_4$. Our data provide convincing evidence for magnetic breakdown in the system. This shows that a reconstructed multiply-connected Fermi surface persists, at least at strong magnetic fields, up to the highest doping level of the superconducting regime. Our results suggest an intimate relation between translational symmetry breaking and the superconducting pairing in the electron-doped cuprate superconductors.
Critical current measurements were made on thin films of YBa2Cu3O7-delta and Y0.8Ca0.2Ba2Cu3O7-delta produced by sol-gel and pulsed laser deposition, respectively. Both samples have high critical currents at low temperatures and the critical current, Jc, is largest in the overdoped Y0.8Ca0.2Ba2Cu3O7-delta thin film. Annealing studies show a large increase in Jc with increasing hole concentration and suggests that the maximum Jc should occur for overdoped samples. The very overdoped region of the superconducting phase diagram was probed by studying bulk ceramic Y0.8Ca0.2Ba2Cu3O7-delta samples, …
In the present work, we report the new findings on the doping level dependence of the phase coherence between superconducting Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ (Bi-2212) grains. The experimental results from the strongly underdoped and overdoped regimes deviated from the expectation based on the doping level dependence of the superfluid density at $T$ = 0 K. These findings appear to be governed by interplay between competing orders inside the superconducting dome of cuprate superconductors. Two quantum critical points are likely to exist at the underdoped and overdoped regimes beneath the supercon…
