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arXiv 2203.04542cond-mat.str-elcond-mat.mtrl-sci
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光驱动电荷有序Dirac电子系统的动力学相变

Dynamical phase transitions in the photodriven charge-ordered Dirac-electron system

Yasuhiro Tanaka, Masahito Mochizuki

摘要:

以有机盐$α$ -(BEDT-TTF)$_2$ I $_3$为例,对电荷有序基态的Dirac-电子相互作用体系的光致相变和电荷动力学进行了理论研究.通过分析这种化合物的扩展哈伯德模型,使用基于含时薛定谔方程和Floquet理论的数值模拟相结合的方法,我们观察到连续的动态相变从电荷有序绝缘体到无隙狄拉克半金属,并最终到陈氏绝缘体相照射下的圆偏振光。这些相变的发生是圆偏振光的两个主要效应的结果,即,通过熔化电荷有序来关闭电荷间隙,通过破坏狄拉克点处的时间反演对称性来打开拓扑间隙。我们证明,这些光诱导现象是受驱动的相关狄拉克电子的电荷动力学。

英文摘要:

Photoinduced phase transitions and charge dynamics in the interacting Dirac-electron system with a charge-ordered ground state are theoretically studied by taking an organic salt $α$-(BEDT-TTF)$_2$I$_3$. By analysing the extended Hubbard model for this compound using a combined method of numerical simulations based on the time-dependent Schrödinger equation and the Floquet theory, we observe successive dynamical phase transitions from the charge-ordered insulator to a gapless Dirac semimetal and, eventually, to a Chern insulator phase under irradiation with circularly polarized light. These phase transitions occur as a consequence of two major effects of circularly polarized light, i.e., closing of the charge gap through melting the charge order and opening of the topological gap by breaking the time reversal symmetry at the Dirac points. We demonstrate that these photoinduced phenomena are governed by charge dynamics of driven correlated Dirac electrons.

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