The Rabi model describes the simplest nontrivial interaction between a few-level system and a bosonic mode, featuring in multiple seemingly unrelated systems of importance to quantum science and technology. While exact expressions for the energies of this model and its few-mode extensions have been obtained, they involve roots of transcendental functions and are thus cumbersome and unintuitive. Utilizing the symmetric generalized rotating wave approximation (S-GRWA), we develop a family of approximations to the energies of the two-mode two-photon Rabi model. The simplest elements of the family are analytically tractable, providing good approximations in regimes of interest such as ultra- and deep-strong coupling. Higher-order approximate energies can be used if more accuracy is required.
The interaction between an atom and a one mode external driving field is an ubiquitous problem in many branches of physics and is often modeled using the Rabi Hamiltonian. In this paper we present a series of analytically solvable Hamiltonians that approximate the Rabi Hamiltonian and compare our results to the Jaynes-Cummings model which neglects the so-called counter-rotating term in the Rabi Hamiltonian. Through a unitary transformation that diagonlizes the Jaynes-Cummings model, we transform the counter-rotating term into separate terms representing several different physical processes. By…
We report on multi-photon Rabi oscillations and controlled tuning of a multi-level system at room temperature (S=5/2 for Mn2+:MgO) in and out of a quasi-harmonic level configuration. The anisotropy is much smaller than the Zeeman splittings, such as the six level scheme shows only a small deviation from an equidistant diagram. This allows us to tune the spin dynamics by either compensating the cubic anisotropy with a precise static field orientation, or by microwave field intensity. Using the rotating frame approximation, the experiments are very well explained by both an analytical model and …
Controllable interaction between photons and distant spins via vacuum Rabi oscillations
QuTech and Kavli Institute of Nanoscience, Delft University of Technology（代尔夫特理工大学量子纳米科学卡弗里研究所）；Netherlands Organization for Applied Scientific Research (TNO)（荷兰应用科学研究组织）
We study a cavity-QED setup consisting of a two-level system coupled to a single cavity mode with two-photon relaxation. The system dynamics is modeled via a Lindblad master equation consisting of the Rabi Hamiltonian and a two-photon dissipator. We show that an even-photon relaxation preserves the $Z_2$ symmetry of the Rabi model, and provide a framework to study the corresponding non-Hermitian dynamics in the number-parity basis. We discuss the role of different terms in the two-photon dissipator and show how one can extend existing results for the closed Rabi spectrum to the open case. Furt…
A double rephasing photon echo is analyzed for inversion-free photon echo-based quantum memories using controlled Rabi flopping, where the Rabi flopping is used for phase control of atom coherence. Unlike the rephasing-caused pi-phase shift in a single rephasing scheme, the control Rabi flopping between the excited state and an auxiliary third state induces coherence inversion. Thus, the absorptive photon echo in a double rephasing scheme can be manipulated to be emissive via the controlled Rabi flopping. Here we present a quantum coherence control of atom phases in a double rephasing photon e…
The analytically exact solutions to the two-photon Rabi-Stark model are given by using the Bogoliubov operators approach. Transcendental functions responsible for the exact solutions are derived. The zeros of the transcendental functions reproduce completely the regular spectra. The first-order quantum phase transitions are also detected by the pole structure of the derived transcendental functions, similar to the one-photon Rabi-Stark model, different from the two-photon Rabi model where the energy levels for the ground-state and the first excited state do not cross. The spectra collapse char…
The generalized Rabi model (gRM) with both one- and two-photon coupling terms has been successfully implemented in circuit quantum electrodynamics systems. In this paper, we examine theoretically multiphoton resonances in the gRM and derive their effective Hamiltonians. With different detunings in the system, we show that all three- to six-photon resonances can be achieved by involving two intermediate states. Furthermore, we study the interplay between multiphoton resonance and chiral transport of photon Fock states in a resonator junction with broken time-reversal symmetry. Depending on the …
Quantum multi--photon spin--boson model is considered. We solve an operator Riccati equation associated with that model and present a candidate for a generalized parity operator allowing to transform spin--boson Hamiltonian to a block diagonal form what indicates an existence of the related symmetry of the model.
We investigate the quantum phase transition in the dissipative anisotropic quantum Rabi model in the framework of quantum dressed master equation. From perspectives of both numerical and analytical analysis, we unravel the implication of the giant photon-bunching feature on the first-order quantum phase transition. The observed two-photon statistics can be well described analytically within a few lowest eigenstates at the low temperature. Moreover, such significant photon-bunching peak is generally exhibited at the deep-strong qubit-photon coupling, which is however lacking in the dissipative …
We predict large cooperative effect involving two atom two photon vacuum Rabi oscillations in a high quality cavity. The two photon emission occurs as a result of simultaneous de-excitation of both atoms with two photon resonance condition $ω_1+ω_2\approx ω_a+ω_b$, where $ω_1$, $ω_2$ are the atomic transition frequencies and $ω_a$, $ω_b$ are the frequencies of the emitted photons. The actual resonance condition depends on the vacuum Rabi couplings. The effect can be realized either with identical atoms in a bimodal cavity or with nonidentical atoms in a single mode cavity.
We present an interaction scheme that exhibits a dynamical consequence of virtual photons carried by a vacuum-field dressed two-level atom in the ultrastrong coupling regime. We show that, with the aid of an external driving field, virtual photons provide a transition matrix element that enables the atom to evolve coherently and reversibly to an auxiliary level accompanied by the emission of a real photon. The process corresponds to a type of vacuum Rabi oscillation, and we show that the effective vacuum Rabi frequency is proportional to the amplitude of a single virtual photon in the ground s…
We demonstrate that four-wave mixing processes in high-quality non-linear resonators can lead to Rabi-like oscillations in photon occupation numbers and second-order correlation functions, being a characteristic feature of the presence of entangled photon pairs in the optical signal. In the case of a system driven by a continuous coherent pump, the oscillations occur in the transient regime. We show that driving the system with pulsed coherent pumping would generate strongly anti-bunched photon states.
The two-photon Rabi Hamiltonian is a simple model describing the interaction of light with matter, with the interaction being mediated by the exchange of two photons. Although this model is exactly soluble in the rotating-wave approximation, we work with the full Hamiltonian, maintaining the non-integrability of the model. We demonstrate that, despite this non-integrability, there exist isolated, exact solutions for this model analogous to the so-called Juddian solutions found for the single-photon Rabi Hamiltonian. In so doing we use a Bogoliubov transformation of the field mode, as described…
A coherent coupling among different energy photons provided by nonlinear optical interaction is regarded as a photonic version of the Rabi oscillation. Cavity enhancement of the nonlinearity reduces energy requirement significantly and pushes the scalability of the frequency-encoded photonic circuit based on the photonic Rabi oscillation. However, confinement of the photons in the cavity severely limits the number of interactable frequency modes. Here we demonstrate a wide-bandwidth and efficient photonic Rabi oscillation achieving full-cycle oscillation based on a cavity-enhanced nonlinear op…
We determine the Rabi oscillations for coherent and squeezed coherent states via one- and two-photon atomic transitions in two- and three-level atoms, respectively. The effect of squeezing coherent states is to reduce the large number of photons of mesoscopic scale to fewer photons and so be able to use numerical solutions with the aid of the Jaynes-Cummings model. We maximize the squeezing of the coherent state by minimizing the ratio of the photon number variance to photon number, thus narrowing the region where revival occurs.
Two-photon Rabi splitting in a cavity-dot system provides a basis for multi-qubit coherent control in quantum photonic network. Here we report on two-photon Rabi splitting in a strongly coupled cavity-dot system. The quantum dot was grown intentionally large in size for large oscillation strength and small biexciton binding energy. Both exciton and biexciton transitions couple to a high quality factor photonic crystal cavity with large coupling strengths over 130 $μ$eV. Furthermore, the small binding energy enables the cavity to simultaneously couple with two exciton states. Thereby two-photon…
There are well-known dark states in the even-qubit Dicke models, which are the products of the two-qubit singlets and a Fock state, where the qubits are decoupled from the photon field. These spin singlets can be used to store quantum correlations since they preserve entanglement even under dissipation, driving and dipole-dipole interactions. One of the features for these dark states is that their eigenenergies are independent of the qubitphoton coupling strength. We have obtained a novel kind of dark-like states for the multi-qubit and multi-photon Rabi models, whose eigenenergies are also co…
We propose a superconducting circuit to implement a two-photon quantum Rabi model in a solid-state device, where a qubit and a resonator are coupled by a two-photon interaction. We analyze the input-output relations for this circuit in the strong coupling regime and find that fundamental quantum optical phenomena are qualitatively modified. For instance, two-photon interactions are shown to yield single- or two-photon blockade when a pumping field is either applied to the cavity mode or to the qubit, respectively. In addition, we derive an effective Hamiltonian for perturbative ultrastrong two…
Tho-photon Rabi oscillations hold potential for quantum computing and quantum information processing, because during a Rabi cycle a pair of entangled photons may be created. We theoretically investigate the onset of this phenomenon in a heterodimer comprising a semiconductor quantum dot strongly coupled to a metal nanoparticle. Two-photon Rabi oscillations in this system occur due to a coherent two-photon process involving the ground-to-biexciton transition in the quantum dot. The presence of a metal nanoparticle nearby the quantum dot results in a self-action of the quantum dot via the metal …
General solutions to the quantum Rabi model involve subspaces with unbounded number of photons. However, for the multiqubit multimode case, we find special solutions with at most one photon for arbitrary number of qubits and photon modes. Unlike the Juddian solution, ours exists for arbitrary single qubit-photon coupling strength with constant eigenenergy. This corresponds to a horizontal line in the spectrum, while still being a qubit-photon entangled state. As a possible application, we propose an adiabatic scheme for the fast generation of arbitrary single-photon multimode W states with non…
Within the framework of exact quantum electrodynamics in dispersing and absorbing media, we have studied the emission from an initially in the upper state prepared emitter in a high quality cavity in the case, when there are two cavity modes that resonantly interact with the emitter. In particular, when one of the modes is in resonance with the emitter transition and the other mode is tuned to the frequency equal to the Rabi splitting of the first mode, the effect of Rabi resonance is observed.
Exact spectrum of the two-photon Rabi Hamiltonian is found, proceeding in full analogy with the solution of standard (one-photon) Rabi Hamiltonian, published by Braak in Phys. Rev. Lett. 107, 100401 (2011). The Hamiltonian is rewritten as a set of two differential equations. Symmetries that get hidden after further treatment are found. One can plainly see, how the Hilbert space splits into four disjunct subspaces, categorized by four values of the symmetry parameter $c=\pm1,\pm i$. There were only two values $\pm1$ for the standard Rabi model. Four analytic functions are introduced by a recurr…
A generalized quantum Rabi Hamiltonian with both one- and two-photon terms has emerged in the circuit quantum electrodynamics system for a decade. The usual parity symmetry is broken naturally in the simultaneous presence of both couplings, which complicates analytical treatments, even in the rotating wave approximations. In this paper, we propose an adiabatic approximation to this generic model by using Bogoliubov operators, and obtain a very concise analytical solution for both eigenvalues and eigenstates. Although the adiabatic approximation is only exact in the vanishing limit of the qubit…
Quantum emitters with a $Λ$-type level structure enable numerous protocols and applications in quantum science and technology. Understanding and controlling their dynamics is, therefore, one of the central research topics in quantum optics. Here, we drive two-photon Rabi oscillations between the two ground states of cesium atoms and observe the associated oscillatory Raman gain and absorption that stems from the atom-mediated coherent photon exchange between the two drive fields. The atoms are efficiently and homogeneously coupled with the probe field by means of a nanofiber-based optical inte…
It is shown that the (driven) quantum Rabi model and its 2-photon and 2-mode generalizations possess a hidden $sl(2)$-algebraic structure which explains the origin of the quasi-exact solvability of these models. It manifests the first appearance of a hidden algebraic structure in quantum spin-boson systems without $U(1)$ symmetry.
The true level crossings in a subspace of the asymmetric two-photon quantum Rabi model (tpQRM) have been observed when the bias parameter of qubit is an even multiple of the renormalized cavity frequency. Generally, such level crossings imply the existence of the hidden symmetry because the bias term breaks the obvious symmetry exactly. In this work, we propose a Bogoliubov operator approach (BOA) for the asymmetric tpQRM to derive the symmetry operators associated with the hidden symmetry hierarchically. The explicit symmetry operators consisting of Lie algebra at low biases can be easily obt…
Spectral collapse, the transition from discrete to continuous spectrum, is a characteristic in quantum Rabi models. We explore this phenomenon in the two-photon quantum Rabi model in optical phase space and find that, in the so-called degenerate qubit regime, the collapse is similar to that happening in the transition from a quantum harmonic to an inverted quadratic potential with the free-partical potential as transition point. In this regime, it is possible to construct Dirac-normalizable eigenfunctions for the model that show well defined parity. In the general model, we use parity to diago…
We study numerically the dynamics of the Rabi Hamiltonian, describing the interaction of a single cavity mode and a two-level atom without the rotating wave approximation, subjected to damping and dephasing reservoirs included via usual Lindblad superoperators in the master equation. We show that the combination of the antirotating term and the atomic dephasing leads to linear asymptotic photons generation from vacuum. We reveal the origins of the phenomenon and estimate its importance in realistic situations.
The collective dynamics of two non-interacting two-level emitters, which are coupled to a structured wave guide that supports two-photon bound states, is investigated. Tuning the energy of the two emitters such that they are in resonance with the two-photon bound state energy band, we identify parameter regimes where the system displays fractional populations and essentially undamped Rabi oscillations. The Rabi oscillations, which have no analog in the single-emitter dynamics, are attributed to the existence of a collective polaron-like photonic state that is induced by the emitter-photon coup…
We propose a robust realization of the two-photon quantum Rabi model in a trapped-ion setting based on a continuous dynamical decoupling scheme. In this manner the magnetic dephasing noise, which is identified as the main obstacle to achieve long time coherent dynamics in ion-trap simulators, can be safely eliminated. More specifically, we investigate the ultrastrong coupling regime of the two-photon quantum Rabi model whose realization in trapped ions involves second-order sideband processes. Hence, the resulting dynamics becomes unavoidably slow and more exposed to magnetic noise requiring a…
We investigate the population dynamics of the three-level system in the two-photon absorption (TPA) process, mainly focusing the influence of pulse width and Rabi frequency on the population dynamics of the system. We observe the dependency of the population with the Rabi frequency and the pulse width. We also show that the arbitrary superposition state consisted in two states, upper state and lower state, is possible by controlling the pulse width and Rabi frequency. The results obtained can be used to the case of more complex multilevel system and they can be valuable for coherent quantum co…
By applying the Bogoliubov transformations and through the introduction of the Bargmann-Hilbert spaces, we obtain analytic representations of solutions to the driven Rabi model without ${\cal Z}_2$ symmetry, and the 2-photon and two-mode quantum Rabi models. In each case, transcendental function is analytically derived whose zeros give the energy spectrum of the model. The zeros can be numerically found by standard root-search techniques.
We study the Two Photon Quantum Rabi Model by way of its spectral functions and survival probabilities. This approach allows numerical precision with large truncation numbers, and thus exploration of the spectral collapse. We provide independent checks and calibration of the numerical results by studying an exactly solvable case and comparing the essential qualitative structure of the spectral functions. We stress that the large time limit of the survival probability provides us with an indicator of spectral collapse, and propose a technique for the detection of this signal in the current and …
A Rabi dimer is used to model a recently reported circuit quantum electrodynamics system composed of two coupled transmission-line resonators with each coupled to one qubit. In this study, a phonon bath is adopted to mimic the multimode micromechanical resonators and is coupled to the qubits in the Rabi dimer. The dynamical behavior of the composite system is studied by the Dirac-Frenkel time-dependent variational principle combined with the multiple Davydov D$_{2}$ ansätze. Initially all the photons are pumped into the left resonator, and the two qubits are in the down state coupled with the …
We consider the generalized quantum Rabi model with the so-called $A^{2}$-term in the light of the Hepp-Lieb-Preparata quantum phase transition. We investigate the dressed photon in its ground state when the atom-light coupling strength is in the deep-strong coupling regime. We show how the dressed photon appears in the ground state. We dedicate this paper to Pavel Exner and Herbert Spohn on the occasion of their 70th birthdays, and Klaus Hepp on the occasion of his 80th birthday.
We study the solvability of the time-independent matrix Schrödinger differential equations of the quantum Rabi model and its 2-photon and two-mode generalizations in Bargmann Hilbert spaces of entire functions. We show that the Rabi model and its 2-photon and two-mode analogs are quasi-exactly solvable. We derive the exact, closed-form expressions for the energies and the allowed model parameters for all the three cases in the solvable subspaces. Up to a normalization factor, the eigenfunctions for these models are given by polynomials whose roots are determined by systems of algebraic equatio…
We discuss a cavity-QED scheme to deterministically generate entangled photons pairs by using a three-level atom successively coupled to two single longitudinal mode high-Q cavities presenting polarization degeneracy. The first cavity is prepared in a well defined Fock state with two photons with opposite circular polarizations while the second cavity remains in the vacuum state. A half-of-a-resonant Rabi oscillation in each cavity transfers one photon from the first to the second cavity, leaving the photons entangled in their polarization degree of freedom. The feasibility of this implementat…
Recent progress on qubit manipulation allows application of periodic driving signals on qubits. In this study, a harmonic driving field is added to a Rabi dimer to engineer photon and qubit dynamics in a circuit quantum electrodynamics device. To model environmental effects, qubits in the Rabi dimer are coupled to a phonon bath with a sub-Ohmic spectral density. A non-perturbative treatment, the Dirac-Frenkel time-dependent variational principle together with the multiple Davydov D$_2$ {\it Ansatz} is employed to explore the dynamical behavior of the tunable Rabi dimer. In the absence of the p…
An implicit formula for the spectrum of the two-photon Rabi model was presented by Travenec in Phys. Rev. A 85, 043805 (2012) in analogy to the method of Braak [Phys. Rev. Lett. 107, 100401 (2011)]. The spectrum is given by common zeros of four functions $G_c(z, E)$ taken with a fixed value of $z\in\mathbb{C}$. We point out that all the $G_c(z,E)$ functions defined by Travenec are identically zero, thus the spectrum is not in fact given by their roots.
Photon-based strongly-correlated lattice models like the Jaynes-Cummings and Rabi lattices differ from their more conventional relatives like the Bose-Hubbard model by the presence of an additional tunable parameter: the frequency detuning between the pseudo-spin degree of freedom and the harmonic mode frequency on each site. Whenever this detuning is large compared to relevant coupling strengths, the system is said to be in the dispersive regime. The physics of this regime is well-understood at the level of a single Jaynes-Cummings or Rabi site. Here, we extend the theoretical description of …
This paper presents a proof of the existence of novel bound states of the two-photon quantum Rabi model at the collapse point. The two-photon Rabi model is interesting not only for its important role on non-linear light-matter interaction, but also for the exhibition of many-energy-levels degenerating process called the "spectral collapse". The squeezing property of the two-photon annihilation and creation operators is the origin for this phenomenon which is well studied without the energy-slitting term $ω_0$. However, many numerical studies have pointed out that with the presence of $ω_0$ , s…
We investigate a one-dimensional Rabi-Hubbard type of model, arranged such that a qdot is sandwiched between every cavity. The role of the qdot is to transmit photons between neighboring cavities, while simultaneously acting as a photon non-linearity. We consider three-level qdots in the $Λ$ configuration, where the left and right leg couples exclusively to the left or right cavity. This non-commuting interaction leads to two highly entangled incompressible phases, separated by a second order quantum phase transition: the qdot degrees-of-freedom act as a dynamical lattice for the photons and a…
In this paper, we uncover the elusive level crossings in a subspace of the asymmetric two-photon quantum Rabi model (tpQRM) when the bias parameter of qubit is an even multiple of the renormalized cavity frequency. Due to the absence of any explicit symmetry in the subspace, this double degeneracy implies the existence of the hidden symmetry. The non-degenerate exceptional points are also given completely. It is found that the number of the doubly degenerate crossing points in the asymmetric tpQRM is comparable to that in asymmetric one-photon QRM in terms of the same order of the constrained …
By mapping the Hamiltonians of the two-mode and 2-photon Rabi models to differential operators in suitable Hilbert spaces of entire functions, we prove that the two models possess entire and normalizable wavefunctions in the Bargmann-Hilbert spaces only if the frequency $ω$ and coupling strength $g$ satisfy certain constraints. This is in sharp contrast to the quantum Rabi model for which entire wavefunctions always exist. For model parameters fulfilling the aforesaid constraints we determine transcendental equations whose roots give the regular energy eigenvalues of the models. Furthermore, w…
We study the ground state phase diagram of a nonlinear two-photon Rabi-Hubbard (RH) model in one dimension using quantum Monte Carlo (QMC) simulations and density matrix renormalization group (DMRG) calculations. Our model includes a nonlinear photon-photon interaction term. Absent this term, the RH model has only one phase, the normal disordered phase, and suffers from spectral collapse at larger values of the photon-qubit interaction or inter-cavity photon hopping. The photon-photon interaction, no matter how small, stabilizes the system which now exhibits {\it two} quantum phase transitions…
An infinite family of exact solutions of the two-photon Rabi model was found by investigating the differential algebraic properties of the Hamiltonian. This family corresponds to energy level crossings not covered by the Juddian class, which is given by elemetary functions. In contrast, the new states are expressible in terms of parabolic cylinder or Bessel functions. We discuss three approaches for discovering this hidden structure: factorization of differential equations, Kimura transformation, and a doubly-infinite, transcendental basis of the Bargmann space.
We have found the algebraic structure of the two-qubit quantum Rabi model behind the possibility of its novel quasi-exact solutions with finite photon numbers by analyzing the Hamiltonian in the photon number space. The quasi-exact eigenstates with at most $1$ photon exist in the whole qubit-photon coupling regime with constant eigenenergy equal to single photon energy \hbarω, which can be clear demonstrated from the Hamiltonian structure. With similar method, we find these special "dark states"-like eigenstates commonly exist for the two-qubit Jaynes-Cummings model, with $E=N\hbarω$ (N=-1,0,1…
We explore the spectral problem of the two photon Rabi model from the point of view of complex differential equations in the Bargmann representation. The wave-functions are automatically entire but to ensure finite norm one has to effectively construct asymptotic expansions. This is achieved by means of the Mellin transformation and convergent factorial series, which allow direct computation of the spectral determinant. By further analysing the differential equation satisfied by the Mellin transform, we obtain a new form of the spectral conditions -- in terms of holonomy matrices and contour i…
