The generalized Rabi model (gRM) with both one- and two-photon coupling terms has been successfully implemented in circuit quantum electrodynamics systems. In this paper, we examine theoretically multiphoton resonances in the gRM and derive their effective Hamiltonians. With different detunings in the system, we show that all three- to six-photon resonances can be achieved by involving two intermediate states. Furthermore, we study the interplay between multiphoton resonance and chiral transport of photon Fock states in a resonator junction with broken time-reversal symmetry. Depending on the qubit-photon interaction and photon-hopping amplitude, we find that the system can demonstrate different short-time dynamics.
We present an analytical approach to the problem of the multiphoton absorption and Rabi oscillations in an armchair graphene nanoribbon (AGNR) in the presence of a time-oscillating strong electric field induced by a light wave directed parallel to the ribbon axis. The two-dimensional Dirac equation for the massless electron subject to the ribbon confinement is employed. In the resonant approximation the electron-hole pair production rate, associated with the electron transitions between the valence and conduction size-quantized subbands, the corresponding multiphoton absorption coefficient and…
In the framework of the non-secular perturbation theory based on the Bogoliubov averaging method, the coherent dynamics of multiphoton Raman transitions in a two-level spin system driven by an amplitude-modulated microwave field is studied. Closed-form expressions for the Rabi frequencies of these transitions have been obtained beyond the rotating wave approximation for the low-frequency driving component. It is shown that spin states dressed by the high-frequency component of the driving field are shifted due to the Bloch-Siegert-like effect caused by antiresonant interactions with the strong…
When an atom is strongly coupled to a cavity, the two systems can exchange a single photon through a coherent Rabi oscillation. This process enables precise quantum-state engineering and manipulation of atoms and photons in a cavity, which play a central role in quantum information and measurement. Recently, a new regime of cavity QED has been reached experimentally where the strength of the interaction between light and artificial atoms (qubits) becomes comparable to the atomic transition frequency or the resonance frequency of the cavity mode. Here we show that this regime can strongly modif…
We investigate the quantum noise properties of a weakly nonlinear Duffing resonator in the deep quantum regime, where only few quanta are excited. This regime is dominated by the appearance of coherent multiphoton resonances in the nonlinear response of the resonator to the modulation. We determine simple expressions for the photon noise spectrum and find that the multiphoton resonances also induces a multiple peak structure in that noise. When the corresponding multiphoton Rabi oscillations are underdamped, zero temperature quantum fluctuations determine comparable populations of all quasiene…
We introduce an exact mapping between the Dirac equation in (1+1)-dimensional curved spacetime (DCS) and a multiphoton quantum Rabi model (QRM). A background of a (1+1)-dimensional black hole requires a QRM with one- and two-photon terms that can be implemented in a trapped ion for the quantum simulation of Dirac particles in curved spacetime. We illustrate our proposal with a numerical analysis of the free fall of a Dirac particle into a (1+1)-dimensional black hole, and find that the Zitterbewegung effect, measurable via the oscillatory trajectory of the Dirac particle, persists in the prese…
Nonlinear dynamics of establishment of electron-hole coherent superpositions states in graphene by multiphoton resonant excitation of interband transitions in laser fields is considered. The single-particle time dependent density matrix for such a quantized system is calculated in the multiphoton resonant approximation. The dependence of Rabi oscillations of Fermi-Dirac sea in graphene on the time, momentum, and photon number at multiphoton laser-excitation is analyzed.
We study Rabi oscillations of the second-order Raman transition realized on dressed states of a qubit excited by an amplitude-modulated microwave field. The co-rotating component of the ultrastrong low-frequency modulation field excites virtual multiple photon processes between the dressed states and forms the Rabi frequency in the so-called rotating wave approximation (RWA). The counter-rotating modulation component also gives a significant contribution to the Rabi frequency owing to the Bloch--Siegert effect. It is shown that for properly chosen parameters of the modulation field and qubit, …
Rabi frequencies for multiphoton absorption by atoms or molecules that can be characterized as two- or three-level systems are obtained in the cases of single and double laser perturbations. If the ambiguity in the origin of absolute energy is conveniently gauged off in the three-level model, there appears an additional non linear frequency which is originated from the separate evolution of a relative-frequency component induced in the whole system by the simultaneous action of the two perturbations.
We present a study of manipulating the multiphoton blockade phenomenon in a single mode cavity with two ladder-type three-level atoms. Combining the cavity QED with electromagnetically induced transparency technique, we show that it is possible to actively manipulate the photon blockade when two atoms are in phase radiations. As a result, the two-photon blockade can be changed to three-photon blockade by changing the control field Rabi frequency. In the case of out-phase radiations, we show that the three-photon blockade can be improved with enhanced mean photon number. In addition, we show th…
We investigate the multiphoton quantum dynamics of a leaking single-mode quantized cavity field coupled with a resonantly driven two-level system possessing permanent dipoles. The frequencies of the interacting subsystems are being considered very different, e.g., microwave ranges for the cavity and optical domains for the frequency of the two-level emitter, respectively. In this way, the emitter couples to the resonator mode via its diagonal dipole moments only. Furthermore, the generalized Rabi frequency resulting form the external coherent driving of the two-level subsystem is assumed as we…
The interplay of interactions, symmetries and gauge fields usually leads to intriguing quantum many-body phases. To explore the nature of emerging phases, we study a quantum Rabi triangle system as an elementary building block for synthesizing an artificial magnetic field. We develop an analytical approach to study the rich phase diagram and the associated quantum criticality. Of particular interest is the emergence of a chiral-coherent phase, which breaks both the $\mathbb{Z}_2$ and the chiral symmetry. In this chiral phase, photons flow unidirectionally and the chirality can be tuned by the …
The light propagation of a probe field pulse in a four-level double-lambda type system driven by laser fields that form a closed interaction loop is studied. Due to the finite frequency width of the probe pulse, a time-independent analysis relying on the multiphoton resonance assumption is insufficient. Thus we apply a Floquet decomposition of the equations of motion to solve the time-dependent problem beyond the multiphoton resonance condition. We find that the various Floquet components can be interpreted in terms of different scattering processes, and that the medium response oscillating in…
There are well-known dark states in the even-qubit Dicke models, which are the products of the two-qubit singlets and a Fock state, where the qubits are decoupled from the photon field. These spin singlets can be used to store quantum correlations since they preserve entanglement even under dissipation, driving and dipole-dipole interactions. One of the features for these dark states is that their eigenenergies are independent of the qubitphoton coupling strength. We have obtained a novel kind of dark-like states for the multi-qubit and multi-photon Rabi models, whose eigenenergies are also co…
We present a new tractable quantum Rabi model for $N$-level atoms by extending the $\mathbb Z_2$ symmetry of the two-state Rabi model. The Hamiltonian is $\mathbb Z_N$ symmetric and allows the parameters in the level separation terms to be complex while remaining hermitian. This latter property means that the new model is {\em chiral}, which makes it differ from any existing $N$-state Rabi models in the literature. The $\mathbb Z_N$ symmetry provides partial diagonalization of the general Hamiltonian. The exact isolated (i.e. exceptional) energies of the model have the Rabi-like form but are $…
Unwanted multiphoton emission commonly reduces the degree of entanglement of photons generated by non-classical light sources and, in turn, hampers their exploitation in quantum information science and technology. Quantum emitters have the potential to overcome this hurdle but, so far, the effect of multiphoton emission on the quality of entanglement has never been addressed in detail. Here, we tackle this challenge using photon pairs from a resonantly-driven quantum dot and comparing quantum state tomography and second-order coherence measurements as a function of the excitation power. We obs…
We map a quantum Rabi ring, consisting of $N$ cavities arranged in a ring geometry, into an effective magnetic model containing the XY exchange and the Dzyaloshinskii Moriya (DM) interactions. The analogue of the latter is induced by an artificial magnetic field, which modulates photon hopping between nearest-neighbor cavities with a phase. The mean-field behavior of both systems is almost identical, facilitating the description of the different phases in the quantum optical model through simple arguments of competing magnetic interactions. For the square geometry ($N=4$) the rich phase diagra…
A highly-efficient method for optical detection and separation of left- and right-handed chiral molecules is presented. The method utilizes a closed-loop three-state system in which the population dynamics depends on the phases of the three couplings. Due to the different signs of the coupling between two of the states for the opposite chiralities and the phase sensitivity of the scheme, the population dynamics is chirality-dependent. By using concepts from the `shortcuts to adiabaticity' approach, one can achieve 100\% contrast in state population transfer between the two enantiomers, which c…
Comparison of the standard and dressed-picture master equations for the quantum Rabi model in the ultrastrong coupling regime
Institute of Physics, University of Brasília（巴西利亚大学物理研究所）；International Center of Physics, Institute of Physics, University of Brasília（巴西利亚大学物理研究所国际物理中心）
Applied Physics Graduate Program, Smalley-Curl Institute, Rice University（莱斯大学斯莫利-卡尔研究所应用物理研究生项目）；Department of Electrical and Computer Engineering, Rice University（莱斯大学电气与计算机工程系）；Smalley–Curl Institute, Rice University（莱斯大学斯莫利-卡尔研究所）；Department of Physics, Graduate School of Engineering Science, Yokohama National University（横滨国立大学工学研究科物理系）；Institute for Multidisciplinary Sciences, Yokohama National University（横滨国立大学跨学科学术院）；Department of Physics and Astronomy, Rice University（莱斯大学物理与天文学系）；Department of Materials Science and NanoEngineering, Rice University（莱斯大学材料科学与纳米工程系）；Department of Physics, Indiana University（印第安纳大学物理系）；Department of Physics, Harvard University（哈佛大学物理系）；Department of Physics, Villanova University（维拉诺瓦大学物理系）
Nonlinear cascaded quantum network with giant emitters
Shaanxi Province Key Laboratory of Quantum Information and Quantum Optoelectronic Devices, School of Physics, Xi’an Jiaotong University（西安交通大学物理学院）；Center for Quantum Computing, RIKEN（理化学研究所量子计算中心）；Center for Quantum Sciences and School of Physics, Northeast Normal University（东北师范大学物理学院）；Department of Microtechnology and Nanoscience, Chalmers University of Technology（查尔姆斯理工大学微技术与纳米科学系）；School of Physics and Optoelectronics, South China University of Technology（华南理工大学物理与光电工程学院）；Physics Department, The University of Michigan（密歇根大学物理系）
Cavity quantum electrodynamics studies light-matter interactions at single quanta level. Chiral photon-emitter coupling in photonic structures is characterized as unidirectional propagation locked by the local polarization of light. However, to realize the strong interaction of photon-emitter with direction-locked propagation, which will bring novel applications in nonreciprocal quantum devices, has not been reported yet. Here, we propose the coupled photonic crystal and metallic nanoparticle structure, where through strong local field with high helicity, the rate of circularly polarized photo…
We consider a generalized Jaynes-Cummings model of a two-level atom interacting with a multimode nondegenerate coherent field. The sum of the mode frequencies is equal to the two-level transition frequency, creating the resonance condition. The intermediate levels associated with the multi-photon process are adiabatically eliminated using the non-resonant conditions for these transitions. Under such general conditions, the infinite atom-multiphoton interaction is effectively mapped onto an equivalent reduced \textit{2}$\times$\textit{2} bipartite qubit system that facilitates the study of the …
Cavity quantum electrodynamics, which explores the granularity of light by coupling a resonator to a nonlinear emitter, has played a foundational role in the development of modern quantum information science and technology. In parallel, the field of condensed matter physics has been revolutionized by the discovery of underlying topological robustness in the face of disorder, often arising from the breaking of time-reversal symmetry, as in the case of the quantum Hall effect. In this work, we explore for the first time cavity quantum electrodynamics of a transmon qubit in the topological vacuum…
A quantum particle in a slowly-changing potential well $V(x,t)=V(x-x_0(εt))$, periodically shaken in time at a slow frequency $ε$, provides an important quantum mechanical system where the adiabatic theorem fails to predict the asymptotic dynamics over time scales longer than $ \sim 1 / ε$. Specifically, we consider a double-well potential $V(x)$ sustaining two bound states spaced in frequency by $ω_0$ and periodically-shaken in complex plane. Two different spatial displacements $x_0(t)$ are assumed: the real spatial displacement $x_0(εt)=A \sin (εt)$, corresponding to ordinary Hermitian shaki…
Geometric mechanisms enabling spin- and enantio-sensitive observables in one photon ionization of chiral molecules
Max-Born-Institut（马克斯·玻恩研究所）；Insitute of Physics, Humboldt University zu Berlin（柏林洪堡大学物理研究所）；Technion - Israel Institute of Technology（以色列理工学院）；Department of Physics, Imperial College London（帝国理工学院物理系）；Department of Physics, Freie Universität Berlin（柏林自由大学物理系）；Technische Universität Berlin（柏林工业大学）
Huzhou University（湖州大学）；Shenzhen University（深圳大学）；Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area (Guangdong)（粤港澳大湾区量子科学中心（广东））；Henan Normal University（河南师范大学）；Gannan Normal University（赣南师范大学）；Hunan Normal University（湖南师范大学）；National University of Defense Technology（国防科技大学）
Quantum dynamics of few-photon pulsed waveguide-QED with a single artificial atom: frequency-dependent scattering theory and time-dependent matrix product states
