Simultaneous assessment of energy, charge state and angular distribution for medium energy ions interacting with ultra-thin self-supporting targets: a time-of-flight approach
R. Holeňák, S. Lohmann, F. Sekula, D. Primetzhofer
We demonstrate simultaneous measurements of the charge state, energy and angular distribution of keV ions in transmission experiments through self-supporting foils. Using a time-of-flight approach we have introduced an electrostatic deflection apparatus as an extension to existing medium energy ion scattering (MEIS) instrumentation. Different positive, neutral and negative charge states have been discriminated and quantified for initially singly charged beams of He, N, O and Ne in the energy range from 25 to 250 keV. In parallel, the ion energy after interaction with the target has been assessed for all detected particles, while particles can be discriminated by deflection angle. Self-supporting thin carbon foils were used as samples to benchmark our experiments with literature data where available.
A Monte Carlo code based on Geant 3.21 has been used for simulations of energy losses and angular scattering in a time-of-flight Suprathermal Ion Telescope (SIT) on the Solar-Terrestrial Relations Observatory (STEREO). A hemispherical isotropic particle distribution, a monoenergetic or power law in energy is used in these simulations. The impact of scattering, energy losses and system noise on the instrument mass resolution is discussed.
Accurately accounting for effects on times-of-flight caused by finite field-transition times during the ejection of ions from a storage trap: A study for TOF and MRTOF mass spectrometry
Time-Of-Flight (TOF) methods are very effective to detect particles accelerated in laser-plasma interactions, but they shows significant limitations when used in experiments with high energy and intensity lasers, where both high-energy ions and remarkable levels of ElectroMagnetic Pulses (EMPs) in the radiofrequency-microwave range are generated. Here we describe a novel advanced diagnostic method for the characterization of protons accelerated by intense matter interactions with high-energy and high-intensity ultra-short laser pulses up to the femtosecond and even future attosecond range. The…
We present a method to measure the kinetic energy of electrons emitted upon ion impact via their time-of-flight. Pulsed beams of H$^{+}$, D$_2^{+}$, He$^{+}$ and Ne$^{+}$ ions with velocities between 0.4 and 3.5 a.u. are transmitted through thin, self-supporting carbon and gold foils. Transmitted ions and secondary electrons are detected with a position-sensitive detector behind the sample and their respective energies are determined via their flight times. A coincidence criterium can be applied in the acquisition software. Measured electron energies range between 10 and 400 eV. Above ion velo…
Energy spectra of backscattered and transmitted ions with primary energies of 50 keV and 100 keV interacting with self-supporting foils were recorded with a Time-of-Flight Medium-Energy Ion Scattering setup in a single experiment. Self-supporting Au and W foils without backing material were used. For He ions transmitted through Au the spectrum of detected particles shows two distinct components corresponding to different energy losses in the film, whereas for protons no such phenomenon was observed. To determine the origin of these different contributions, measurements for different angles of …
Isochronous mass spectrometry (IMS) in storage rings is a powerful tool for mass measurements of exotic nuclei with very short half-lives down to several tens of microseconds, using a multicomponent secondary beam separated in-flight without cooling. However, the inevitable momentum spread of secondary ions limits the precision of nuclear masses determined by using IMS. Therefore, the momentum measurement in addition to the revolution period of stored ions is crucial to reduce the influence of the momentum spread on the standard deviation of the revolution period, which would lead to a much im…
Trapping molecular ions that have been sympathetically cooled with laser-cooled atomic ions is a useful platform for exploring cold ion chemistry. We designed and characterized a new experimental apparatus for probing chemical reaction dynamics between molecular cations and neutral radicals at temperatures below 1 K. The ions are trapped in a linear quadrupole radio-frequency trap and sympathetically cooled by co-trapped, laser-cooled, atomic ions. The ion trap is coupled to a time-of-flight mass spectrometer to readily identify product ion species, as well as to accurately determine trapped i…
Plastic scintillation detectors for Time-of-Flight (TOF) measurements are almost essential for event-by-event identification of relativistic rare isotopes. In this work, a pair of plastic scintillation detectors of 50 $\times$ 50 $\times$ 3$^{t}$ mm$^3$ and 80 $\times$ 100 $\times$ 3$^{t}$ mm$^3$ have been set up at the external target facility (ETF), Institute of Modern Physics. Their time, energy and position responses are measured with $^{18}$O primary beam at 400 MeV/nucleon. After the off-line walk-effect and position corrections, the time resolution of the two detectors are determined to…
A novel detector based on a polycrystalline diamond sensor is here employed in an advanced Time-Of-Flight scheme for the characterization of energetic ions accelerated during laser-matter interactions. The optimization of the detector and of the advanced TOF methodology allow to obtain signals characterized by high signal-to-noise ratio and high dynamic range even in the most challenging experimental environments, where the interaction of high-intensity laser pulses with matter leads to effective ion acceleration, but also to the generation of strong Electromagnetic Pulses (EMPs) with intensit…
We introduce a new concomitant referencing mode for operating a multi-reflection time-of-flight mass spectrograph (MRTOF-MS), wherein the reference and analyte ions are interleaved on a cycle by cycle bases. Using this mode, we demonstrate an improved technique for performing wide bandwidth mass measurements via MRTOF-MS. This new technique offers a simplified analysis and high-accuracy.
Time-Of-Flight (TOF) technique coupled with semiconductor detectors is a powerful instrument to provide real-time characterization of ions accelerated because of laser-matter interactions. Nevertheless, the presence of strong electromagnetic pulses (EMPs) generated during the interactions, can severely hinder its employment. For this reason, the diagnostic system must be designed to have high EMP shielding. Here we present a new advanced prototype of detector, developed at ENEA-Centro Ricerche Frascati (Italy), with a large area (15 mm x 15 mm) polycrystalline diamond sensor having 150 microns…
The Isochronous Mass Spectrometry (IMS) is a powerful tool for mass measurements of exotic nuclei with half-lives as short as several tens of micro-seconds in storage rings. In order to improve the mass resolving power while preserving the acceptance of the storage ring, the IMS with two Time-Of-Flight (TOF) detectors has been implemented at the storage ring CSRe in Lanzhou, China. Additional velocity information beside the revolution time in the ring can be obtained for each of the stored ions by using the double TOF detector system. In this paper, we introduced a new method of using a 658 nm…
We have performed laser cooling of Mg ions confined in a Penning trap. The externally produced ions were captured in flight, stored and laser cooled. Laser-induced fluorescence was observed perpendicular to the cooling laser axis. Optical detection down to the single ion level together with electronic detection of the ion oscillations inside the Penning trap have been used to acquire information on the ion storage time, ion number and ion temperature. Evidence for formation of ion crystals has been observed. These investigations are an important prerequisite for sympathetic cooling of simultan…
A radiofrequency quadrupole ion trap system for use with a multi-reflection time-of-flight mass spectrograph (MRTOF) for short-lived nuclei has been developed. The trap system consists of two different parts, an asymmetric taper trap and a flat trap. The ions are cooled to a sufficient small bunch for precise mass measurement with MRTOF in only 2 ms cooling time in the flat trap, then orthogonally ejected to the MRTOF for mass analysis. A trapping efficiency of ~27% for 23Na+ and ~5.1% for 7Li+ has been achieved.
In this work, we report on the timing performances of the Time-Of-Flight (TOF) apparatus of the FRACAS large acceptance mass spectrometer designed to measure the fragmentation cross sections of a $^{12}$C beam in hadrontherapy. The TOF system is composed of a Parallel Plate Avalanche Counter and scintillating detectors to create so-called $Δ$E---TOF maps used in the fragment charge identification process. From tests with an alpha source and a $^{12}$C beam experiment, we measured a coincidence resolving time for the apparatus below 300 ps. Those results should lead in the final design to the i…
In this paper we prove that the choice of a suitable treatment of the scintillator surfaces, along with suitable photodetectors electronics and specific algorithms for raw data analysis, allow to achieve an optimal tradeoff between energy, time and DOI resolution, thus strongly supporting the feasibility of a prostate TOF- PET probe, MRI compatible, with the required features and performance. In numbers this means a detector element of 1.5mm x 1.5mm x 10mm, achieving at the same time energy resolution around 11.5%, time-of- flight resolution around 150 ps and DOI resolution even below 1 mm. We…
The layout of a new instrument designed to study the interaction of highly charged ions with surfaces, which consists of an ion source, a beamline including charge separation and a target chamber, is presented here. By varying the charge state and impact velocity of the projectiles separately, the dissipation of potential and kinetic energy at or below the surface can be studied independently. The target chamber offers the use of tunable metal-insulator-metal devices as detectors for internal electronic excitation, a timeof-flight system to study the impact induced particle emission and the po…
The concept of isochronous mass spectrometry (IMS) applying two time-of-flight (TOF) detectors originated many years ago at GSI. However, the corresponding method for data analysis has never been discussed in detail. Recently, two TOF detectors have been installed at CSRe and the new working mode of the ring is under test. In this paper, a data analysis method for this mode is introduced and tested with a series of simulations. The results show that the new IMS method can significantly improve mass resolving power via the additional velocity information of stored ions. This improvement is espe…
A newly constructed apparatus at the National Institute of Standards and Technology (NIST) is designed for the isolation, manipulation, and study of highly charged ions. Highly charged ions are produced in the NIST electron-beam ion trap (EBIT), extracted through a beamline that selects a single mass/charge species, then captured in a compact Penning trap. The magnetic field of the trap is generated by cylindrical NdFeB permanent magnets integrated into its electrodes. In a room-temperature prototype trap with a single NdFeB magnet, species including Ne10+ and N7+ were confined with storage ti…
In typical nuclear physics experiments with radioactive ion beams (RIBs) selected by the in-flight separation technique, Si detectors or ionization chambers are usually equipped for the charge determination of RIBs. The obtained charge resolution relies on the performance of these detectors for energy loss determination, and this affects the particle identification capability of RIBs. We present an approach on improving the resolution of charge measurement for heavy ions by using the abundant energy loss information from different types of existing detectors along the beam line. Without alteri…
Spectrometers based on the magnetic adiabatic collimation followed by an electrostatic filter (MAC-E-filter) principle combine high angular acceptance with an excellent energy resolution. These features make MAC-E-filters very valuable for experiments where the kinetic energy of ions or electrons from rare processes has to be measured with utmost sensitivity and precision. Examples are direct neutrino mass experiments like KATRIN which investigate the energy of electrons in the endpoint region of the tritium $β$-spectrum. However, the MAC-E-filter is a very sharp energy high-pass filter but no…
An electrostatic time-of-flight detector named E-MCP has been developed for quick diagnostics of circulating beam and timing measurement in mass spectrometry at the Rare-RI Ring in RIKEN. The E-MCP detector consists of a conversion foil, potential grids, and a microchannel plate. Secondary electrons are released from the surface of the foil when a heavy ion hits it. The electrons are accelerated and deflected by 90$^\circ$ toward the microchannel plate by electrostatic potentials. A thin carbon foil and a thin aluminum-coated mylar foil were used as conversion foils. We obtained time resolutio…
Nuclear fusion in ultra-dense deuterium D(-1) induced by 0.2 J pulses with 5 ns pulse length ejects ions with energies in the MeV range. The ns-resolved signal to a collector can be observed directly on an oscilloscope, showing ions arriving with energies in the range 2-14 MeV u-1 at flight times 12-100 ns, mainly protons from the fusion process and deuterons ejected by proton collisions. Electrons and photons give almost no contribution to the fast signal. The observed signal at several mA peak current corresponds to 1x10^13 particles released per laser shot and to an energy release > 1 J ass…
A newly assembled multi-reflection time-of-flight mass spectrograph (MRTOF-MS) at RIKEN's RIBF facility became operational for the first time in spring 2020; further modifications and performance tests using stable ions were completed in early 2021. By using a pulsed-drift-tube technique to modify the ions' kinetic energy in a wide range, we directly characterize the dispersion function of the system for use in a new procedure for optimizing the voltages applied to the electrostatic mirrors. Thus far, a mass resolving power of $R_m > 1\,000\,000$ is reached within a total time-of-flight of onl…
The Gamma-Ray Imager/Polarimeter for Solar flares (GRIPS) is a balloon-borne telescope designed to study solar-flare particle acceleration and transport. We describe GRIPS's first Antarctic long-duration flight in Jan 2016 and report preliminary calibration and science results. Electron and ion dynamics, particle abundances and the ambient plasma conditions in solar flares can be understood by examining hard X-ray (HXR) and gamma-ray emission (20 keV to 10 MeV) with enhanced imaging, spectroscopy and polarimetry. GRIPS is specifically designed to answer questions including: What causes the spa…
