Motivated by the superconductivity of $M_x$Bi$_2$Se$_3$, we study topological excitations in a nematic superconductor using Ginzburg-Landau theory. An isolated excitation at low field is shown to be either a distorted phase vortex or a tightly-bounded pair of half quantum vortices. Close to upper critical field $H_{c2}$, the vortex lattice is shown to be always hexagonal in the extreme type-II limit. Due to the different symmetries of the vortex lattice states, at least two phase transitions must take place when the external field is lowered from $H_{c2}$.
Electronic nematicity is ubiquitous in Fe-based superconductors, but what the primary nematic order is and how the various nematic phenomena correlate with each other are still elusive. In this manuscript we study the physical consequence of the orbital nematic order on the spin correlations. We find that the orbital nematic order can drive a significant spin nematicity and can enhance the integrated intensity of the spin fluctuations. Our study shows that the orbital nematic order has strong effect on the spin correlations and it can not be taken as an unimportant secondary effect of the nema…
In this work we explore the interplay between superconductivity and nematicity in the framework of a Ginzburg Landau theory with a nematic order parameter coupled to the superconductor order parameter, often used in the description of superconductivity of Fe based materials. In particular, we focus on the study of the vortex-vortex interaction in order to determine the way nematicity affects its attractive or repulsive character. To do so, we use a dynamical method based on the solutions of the Time Dependent Ginzburg Landau equations in a bulk superconductor. An important contribution of our …
Unconventional mixed state in the nematic superconductor LiFeAs
CNR-SPIN（意大利国家研究委员会自旋物理研究所）；Division of Mathematics, University of Dundee（邓迪大学数学系）；Maxwell Institute, University of Edinburgh（爱丁堡大学麦克斯韦研究所）；School of Mathematics, University of Leeds（利兹大学数学学院）；Leibniz-Institute for Solid State and Materials Research, IFW-Dresden（德累斯顿IFW莱布尼茨固体与材料研究所）；PSI Center for Neutron and Muon Sciences CNM（瑞士保罗谢尔研究所中子与缪子科学中心）；Laboratorium für Festkörperphysik, ETH Zürich（苏黎世联邦理工学院凝聚态物理实验室）
We study topological excitations in two-component nematic superconductors, with a particular focus on Cu$_x$Bi$_2$Se$_3$ as a candidate material. We find that the lowest-energy topological excitations are coreless vortices: a bound state of two spatially separated half-quantum vortices. These objects are nematic Skyrmions, since they are characterized by an additional topological charge. The inter-Skyrmion forces are dipolar in this model, i.e. attractive for certain relative orientations of the Skyrmions, hence forming multi-Skyrmion bound states.
The nematic susceptibility of hole-doped Ba1-xKxFe2As2 and electron-doped Ba(Fe1-xCox)2As2 iron-based superconductors is obtained from measurements of the elastic shear modulus using a three-point bending setup in a capacitance dilatometer. Nematic fluctuations, although weakened by doping, extend over the whole superconducting dome in both systems, suggesting their close tie to superconductivity. Evidence for quantum critical behavior of the nematic susceptibility is, surprisingly, only found for Ba(Fe1-xCox)2As2, the system with the lower maximal Tc value.
We derive the effective action for the collective spin modes in iron-based superconductors. We show that, due to the orbital-selective nature of spin fluctuations, the magnetic and nematic instabilities are controlled by the degrees of orbital nesting between electron and hole pockets. Within a prototypical three-pockets model the hole-electron orbital mismatch is found to boost spin-nematic order. This explains the enhancement of the nematic order in FeSe as compared to 122 compounds, and its suppression under pressure, where the emergence of the second hole pocket compensates the orbital mis…
In recent years, there have been increasing experimental evidence suggesting the existence of an electronic nematic state in a number of unconventional $d$-wave superconductors. Interestingly, it is expected that the long-range nematic order can coexist with $d$-wave superconductivity. We analyze the in-plane upper critical field $H_{c2}$ after taking the influence of nematic state into account, and find that the four-fold oscillation of angle-dependent $H_{c2}$ in a pure $d$-wave superconducting state is turned into a novel two-fold oscillation pattern by a weak nematic order. Moreover, such …
The nematic-superconductor state is an example of a quantum liquid crystal that breaks gauge as well as rotation invariance. It was conjectured to exist in the pseudogap regime of the cuprates high $T_c$ superconductors. The nematic-superconductor state is characterized by two complex order parameters: one of them is related with superconductivity and the other one describes a nematic order. It supports two main classes of topological defects: half-vortices and disclinations. In this paper we present a Ginzburg-Landau approach to study the structure of these topological defects. Due to a geome…
We review our recent experimental results on the electronic nematic phase in electron- and hole-doped BaFe$_2$As$_2$ and FeSe. The nematic susceptibility is extracted from shear-modulus data (obtained using a three-point-bending method in a capacitance dilatometer) using Landau theory and is compared to the nematic susceptibility obtained from elastoresistivity and Raman data. FeSe is particularly interesting in this context, because of a large nematic, i.e., a structurally distorted but paramagnetic, region in its phase diagram. Scaling of the nematic susceptibility with the spin lattice rela…
Studies of the copper-based superconductors demonstrate how their phase diagram becomes more complex as experimental probes improve, able to distinguish among subtly different electronic phases. One of those phases, nematicity, has become the matter of great interest also in the iron-based superconductors, where it is detected deep in the tetragonal state. Here we present the evolution of the in-plane Nernst effect anisotropy in the strain detwinned Ca(Fe1-xCox)2As2 single crystals, whose behaviour can be explained within the approach developed to describe the nematic order parameter in liquid…
We investigate the states of triplet pairing in a candidate nematic superconductor versus typical material parameters, using the mean field theory for two- and three-dimensional tight-binding models with local triplet pairing in the $E_u$ representation. In the two-dimensional model, the system favors the fully gapped chiral state for weaker warping or lower filling level, while a nodal and nematic $Δ_{4x}$ state is favorable for stronger warping or higher filling, with the $d$-vector aligned along the principle axis. In the presence of lattice distortion, relative elongation along one of the …
We report theoretical results for the stability of half-quantum vortices (HQVs) in the superfluid phases of $^3$He confined in highly anisotropic Nafen aerogel. Superfluidity of $^3$He confined in Nafen is the realization of a "nematic superfluid" with Cooper pairs condensed into a single p-wave orbital aligned along the anisotropy axis of the Nafen aerogel. In addition to the nematic phase, we predict a second "chiral" phase that onsets at a lower transition temperature. This chiral phase spontaneously breaks time-reversal symmetry and is a topological superfluid. Both superfluid phases are e…
We demonstrate that in iron-based superconductors, the extended S_{+-} SC state coexists with the d_{x^2-y^2} state under generic conditions. The mixed S_{+-} + d_{x^2-y^2} SC is a natural nematic state in which the tetragonal symmetry C_4 is broken to C_2 explaining puzzling findings of nematic SC in FeSe films [Science 332, 1410 (2011)]. Moreover, we report the possibility of a first order transition at low-T from the nematic S_{+-} + d_{x^2-y^2} state to the pure d_{x^2-y^2} state induced by the Zeeman magnetic field proposing an original experimental strategy for identifying our mixed nema…
We employ polarization-resolved Raman spectroscopy to study critical nematic fluctuations in Ba(Fe$_{1-x}$Au$_x$)$_2$As$_2$ superconductors above and across well separated tetragonal to orthorhombic phase transition at temperature $T_S(x)$ and the Néel transition at $T_N(x)$. The static Raman susceptibility in $XY$ symmetry channel increases upon cooling from room temperature following the Curie-Weiss law, with Weiss temperature $T_θ(x)$ several tens of degrees lower than $T_S(x)$. Data reveals a hidden nematic quantum critical point at $x_{c} = 0.031$ when the system becomes superconducting, …
The new development in sublattice-phase-resolved imaging of electronic structure now allow for the visualisation of the nematic-order state characteristic energy of cuprate superconductors in a wide doping regime. However, it is still unclear how this characteristic energy of the nematic-order state is correlated with the enhancement of superconductivity. Here the doping dependence of the nematic-order state characteristic energy in cuprate superconductors and of its possible connection to the enhancement of superconductivity is investigated within the framework of the kinetic-energy-driven su…
We study the effects of the Lifshitz transition from closed to open Fermi surface in dirty topological insulators with the nematic superconductivity near the critical temperature. We solve linearized Gor'kov equations and find that the nematic superconductor with an open Fermi surface has a lower critical temperature and more susceptible to the disorder than the superconductor with the closed Fermi surface. We propose that correspondence between the critical temperature and stability against the disorder is the general feature of the superconductivity. We investigate the effects of the Lifshit…
Nematic superconductivity with spontaneously broken rotation symmetry has recently been reported in doped topological insulators, $M_x$Bi$_2$Se$_3$ ($M$=Cu, Sr, Nb). Here we show that the electromagnetic (EM) response of these compounds provides a spectroscopy for bosonic excitations that reflect the pairing channel and the broken symmetries of the ground state. Using quasiclassical Keldysh theory, we find two characteristic bosonic modes in nematic superconductors: the nematicity mode and the chiral Higgs mode. The former corresponds to the vibrations of the nematic order parameter associated…
Electronic nematic states with broken rotational symmetry often emerge in correlated materials. In most iron-based superconductors, the nematic anisotropy is oriented in the Fe-Fe direction of the iron square lattice. Recently, a novel type of nematicity along the diagonal Fe-As direction has been suggested in heavily hole-doped $A$Fe$_2$As$_2$ ($A=$ Rb or Cs). However, the transport studies focusing on the fluctuations of such nematicity have provided controversial results regarding the presence of diagonal nematic order. Here we report high-resolution heat capacity measurements under in-plan…
Motivated by the recent experiment indicating that superconductivity in the doped topological insulator Cu$_x$Bi$_2$Se$_3$ has an odd-parity pairing symmetry with rotational symmetry breaking, we study the general class of odd-parity superconductors with two-component order parameters in trigonal and hexagonal crystal systems. In the presence of strong spin-orbit interaction, we find two possible superconducting phases below $T_c$, a time-reversal-breaking (i.e., chiral) phase and an anisotropic (i.e., nematic) phase, and determine their relative energetics from the gap function in momentum sp…
Chuang et al (Reports, 8th of January 2010, p. 181)1 report quasiparticle interference (QPI) imaging that shows pronounced C2 asymmetry. They interpreted this result as indication of an electronic nematic phase with an electron band dispersive only along the b-axis of this orthorhombic material. We argue that this asymmetry is consistent with the underlying long range magnetic order and that LDA electronic structure provides a better description of the QPI images than the 1D band structure conjectured by Chuang et al.
Electronic nematicity in iron pnictide materials has been extensively studied by various experimental techniques, yet its heat capacity anomaly at the phase transition has not been examined quantitatively. In this work we review the thermodynamic description of nematicity in $Ba(Fe_{1-x}Co_{x})_{2}As_{2}$ using the Landau free energy, which defines the behavior of three thermodynamic quantities: the structural orthorhombicity that develops below the nematic transition, the softening shear modulus above the transition, and the discontinuous heat capacity at the transition. We derive a quantitat…
We investigate the response of a doped topological insulator Bi$_2$Se$_3$ with spin-triplet nematic superconductivity to external magnetization. We calculate the Zeeman part of magnetic susceptibility for nematic and chiral superconducting phases near T$_c$ in Ginzburg-Landau formalism. Superconducting order parameter from $E_u$ representation has non-trivial coupling with the transversal Zeeman field that results in a paramagnetic response to a magnetization. The topology of a Fermi surface has a strong influence on magnetic susceptibility. Lifshitz transition from closed to open Fermi surfac…
We study the dc conductivity of iron-based superconductors within the orbital-selective spin fluctuation scenario. Within this approach, the anisotropy of spin fluctuations below the spin-nematic transition at T$_S$ is also responsible for the orbital ordering, induced by nematic self-energy corrections to the quasiparticle dispersion. As a consequence, the anisotropy of the dc conductivity below T$_S$ is determined not only by the anisotropy of the scattering rates as expected within a spin-nematic scenario, but also by the modification of the Fermi velocity due to the orbital reconstruction.…
It is shown that the electric charge of vortices can result in a helical instability of straight vortex lines in layered superconductors, particularly Bi-based cuprates or organic superconductors. This instability may result in a phase transition to a uniformly twisted vortex state, which could be detected by torque magnetometry, neutron diffraction, electromagnetic or calorimetric measurements.
We have extended Brandt's method for accurate, efficient calculations within Ginzburg-Landau theory for periodic vortex lattices at arbitrary mean induction to lattices of "doubly quantized" vortices.
Electrical resistivity measurements of detwinned single crystals of the representative iron arsenide Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ reveal a dramatic in-plane anisotropy associated with the tetragonal-to-orthorhombic structural transition that precedes the onset of long-range antiferromagnetic order. These results indicate that the structural transition in this family of compounds is fundamentally electronic in origin.
We investigate the dynamics of magnetic vortices in type II superconductors with normal state pinning sites using the Ginzburg-Landau equations. Simulation results demonstrate hopping of vortices between pinning sites, influenced by external magnetic fields and external currents. The system is highly nonlinear and the vortices show complex nonlinear dynamical behaviour.
We report controlled local manipulation of single vortices by low temperature magnetic force microscope (MFM) in a thin film of superconducting Nb. We are able to position the vortices in arbitrary configurations and to measure the distribution of local depinning forces. This technique opens up new possibilities for the characterization and use of vortices in superconductors.
The nature of the pseudogap and its relationship with superconductivity are one of the central issues of cuprate superconductors. Recently, a possible scenario has been proposed that the pseudogap state is a distinct phase characterized by spontaneous rotational symmetry breaking called "nematicity" based on transport and magnetic susceptibility measurements, where the symmetry breaking was observed below the pseudogap temperature $T^*$. Here, we report a temperature-dependent ARPES study of nematicity in slightly overdoped Bi${}_{1.7}$Pb${}_{0.5}$Sr${}_{1.9}$CaCu${}_2$O${}_{8+δ}$ triggered by…
Observability of half-quantum vortices and skyrmions in p-wave superconductors is an outstanding open question. Under the most common conditions, fractional flux vortices are not thermodynamically stable in bulk samples. Here we show that in chiral p-wave superconductors, there is a regime where, in contrast lattices of integer flux vortices are not thermodynamically stable. Instead skyrmions made of spatially separated half-quantum vortices are the topological defects produced by an applied external field.
We derive the exact modified London equation for the two-gap superconductor, compare it with its single-gap counterpart. We show that the vortices in the two-gap superconductor are soft (or continuous) core vortices. In particular, we discuss the topological structure of the finite energy vortices (Abrikosov-like vortices), and find that they can be viewed as the incarnation of the baby skyrmion stretched in the third direction. Besides, we point out that the knot soliton in the two-gap superconductor is the twisted Abrikosov-like vortex with its two periodic ends connected smoothly. The relat…
We study the pinning of vortices in thin film superconductors by magnetic dots in the London approximation. A single dot is in general able to pin multiple field-induced vortices, up to a saturation number n_s, which can be much larger than one. However, the magnetic field of the dot also creates intrinsic vortices and anti-vortices, which must be accounted for. In a ferromagnetic dot array, the intrinsic anti-vortices are pinned only interstitially. Much stronger pinning effect is expected of an antiferromagnetic dot array. Possible realizations of various magnetic configurations are discusse…
Fit-Free Optical Determination of Electronic Thermalization Time in Nematic Iron-Based Superconductors
Department of Physics, University of Puerto Rico（波多黎各大学物理系）；Department of Materials Science and Engineering, University of Wisconsin–Madison（威斯康星大学麦迪逊分校材料科学与工程系）
The iron-based superconductors are characterized by multiple-orbital physics where all the five Fe 3$d$ orbitals get involved. The multiple-orbital nature gives rise to various novel phenomena like orbital-selective Mott transition, nematicity and orbital fluctuation that provide a new route for realizing superconductivity. The complexity of multiple-orbital also asks to disentangle the relationship between orbital, spin and nematicity, and to identify dominant orbital ingredients that dictate superconductivity. The bulk FeSe superconductor provides an ideal platform to address these issues be…
The electronic nematic phase is characterized as an ordered state of matter with rotational symmetry breaking, and has been well studied in the quantum Hall system and the high-$T_c$ superconductors, regardless of cuprate or pnictide family. The nematic state in high-$T_c$ systems often relates to the structural transition or electronic instability in the normal phase. Nevertheless, the electronic states below the superconducting transition temperature is still an open question. With high-resolution scanning tunneling microscope measurements, direct observation of vortex core in FeSe thin film…
In systems combining type-II superconductivity and magnetism the non-stationary magnetic field of moving Abrikosov vortices may excite spin waves, or magnons. This effect leads to the appearance of an additional damping force acting on the vortices. By solving the London and Landau-Lifshitz-Gilbert equations we calculate the magnetic moment induced force acting on vortices in ferromagnetic superconductors and superconductor/ferromagnet superlattices. If the vortices are driven by a dc force, magnon generation due to the Cherenkov resonance starts as the vortex velocity exceeds some threshold v…
Charge-$4e$ superconductivity as a novel phase of matter remains elusive so far. Here we show that charge-$4e$ phase can arise as a vestigial order above the nematic superconducting transition temperature in time-reversal-invariant nematic superconductors. On the one hand, the nontrivial topological defect -- nematic vortex -- is energetically favored over the superconducting phase vortex when the nematic stiffness is less than the superfluid stiffness; consequently the charge-$4e$ phase emerges by proliferation of nematic vortices upon increasing temperatures. On the other hand, the Ginzburg-…
Nematicity plays an important role in the physics of iron-based superconductors (IBS). Its microscopic origin and in particular its importance for the mechanism of high-temperature superconductivity itself are highly debated. A crucial knowledge in this regard is the degree to which the nematic order influences the electronic structure of these materials. Earlier angle-resolved photoemission spectroscopy (ARPES) studies found that the effect is dramatic in three families of IBS including 11, 111 and 122 compounds: energy splitting reaches 70 meV and Fermi surface becomes noticeably distorted. …
Nematic superconductors are characterized by an apparent crystal symmetry breaking that results in the anisotropy of the in-plane upper critical magnetic field $H_{c2}$. The symmetry breaking is usually attributed to the strain of the crystal lattice. The nature and the value of the strain are debatable. We perform systematic measurements of the $H_{c2}$ anisotropy in the high-quality Sr$_x$Bi$_2$Se$_3$ single crystals in the temperature range 1.8~K$<T<T_c\approx 2.7$~K using temperature stabilization with an accuracy of 0.0001 K. We observe that in all tested samples the anisotropy is weakly …
Magnetic flux structures in single crystals of the layered spin triplet superconductor Sr$\_{2}$RuO$\_{4}$ are studied by scanning micro SQUID Force microscopy. Vortex chains appear as the applied field is tilted along the in-plane direction of the superconductor. The vortex chains align along the direction of the in-plane component of the applied magnetic field. The decoration of in-plane vortices by crossing Abrikosov vortices is observed: two vortex orientations are apparent simultaneously, one along the layers and the other perpendicular to the layers. The crossing vortices appear preferen…
A theory of superconductivity in the iron-based materials requires an understanding of the phase diagram of the normal state. In these compounds, superconductivity emerges when stripe spin density wave (SDW) order is suppressed by doping, pressure or atomic disorder. This magnetic order is often pre-empted by nematic order, whose origin is yet to be resolved. One scenario is that nematic order is driven by orbital ordering of the iron 3d-electrons that triggers stripe SDW order. Another is that magnetic interactions produce a spin-nematic phase, which then induces orbital order. In this articl…
We discuss the main features of Hall tunneling of pancake vortices in superclean high-$T_{c}$ superconductors. The general formalism for the calculation of the lifetime of a vortex pinned in a metastable configuration is described. The results are applied to the problem of quantum tunneling of a pancake vortex from a columnar defect in the limit of a small driving current.
By using the time-dependent Ginzburg-Landau theory, we show that extremely diverse experimental data on flux-flow resistivity in multiband superconductors can be qualitatively explained by a composite nature of Abrikosov vortices consisting of elementary fractional vortices in different bands. In composite vortices, the ratio of a core size to electric field relaxation length is found to vary in wide limits depending on system parameters. As a result, the flux-flow magneto-resistance can strongly exceed the single-component Bardeen-Stephen estimation provided that moving vortices generate elec…
We take account of normal currents that emerge when vortices move. Moving Abrikosov vortices in the bulk and Pearl vortices in thin films are considered. Velocity dependent distributions of both normal and persistent currents are studied in the frame of time-dependent London equations. In thin films near the Pearl vortex core, these distributions are intriguing in particular.
The cuprate superconductors are characterized by numerous ordering tendencies, with the nematic order being the most distinct form of order. Here the intertwinement of the electronic nematicity with superconductivity in cuprate superconductors is studied based on the kinetic-energy-driven superconductivity. It is shown that the optimized Tc takes a dome-like shape with the weak and strong strength regions on each side of the optimal strength of the electronic nematicity, where the optimized Tc reaches its maximum. This dome-like shape nematic-order strength dependence of Tc indicates that the …
We discuss the problem of broken time reversal symmetry near grain boundaries in a d-wave superconductor based on a Ginzburg-Landau theory. It is shown that such a state can lead to fractional vortices on the grain boundary. Both analytical and numerical results show the structure of this type of state.
A nematic superconductor can in principle support a vestigial order phase above its superconducting transition temperature, with rotational symmetry spontaneously broken while remain nonsuperconducting. We examine the condition for this vestigial nematic order to occur, within a Ginzburg-Landau theory with order parameter fluctuations included. Contrary to prior theoretical results, we found that this vestigial order actually requires very stringent conditions to be met: the material must be sufficiently deep in the nematic regime (i.e. far away from the boundary separating the nematic and chi…
Electronic nematicity is often found in unconventional superconductors, suggesting its relevance for electronic pairing. In the strongly hole-doped iron-based superconductors, the symmetry channel and strength of the nematic fluctuations, as well as the possible presence of long-range nematic order, remain controversial. Here, we address these questions using transport measurements under elastic strain. By decomposing the strain response into the appropriate symmetry channels, we demonstrate the emergence of a giant in-plane symmetric contribution, associated with the growth of both strong ele…
We use large-scale Monte-Carlo simulations to study thermal fluctuations in chiral $p$-wave superconductors in an applied magnetic field in three dimensions. We consider the thermal stability of previously predicted unusual double-quanta flux-line lattice ground states in such superconductors. In previous works it was shown that, neglecting thermal fluctuations, a chiral $p$-wave superconductor forms an hexagonal lattice of doubly-quantized vortices, except extremely close to the vicinity of $H_{c2}$ where double-quanta vortices split apart. We find dissociation of double-quanta vortices drive…
We investigate chiral superconductivity which occurs in the electronic nematic state. A vortex state in a $c$-axis magnetic field is studied on the basis of the two-component Ginzburg-Landau model for nematic-chiral superconductors. It is shown that various vortex lattice structures are stabilized by nontrivial cooperation of nematicity and chirality in superconductors. In particular, the vortex lattice structural transition occurs when a square anisotropy parameter $ν$ is positive (negative) and the nematicity is induced along the [110] axis ([100] axis). We discuss nematic-chiral superconduc…
We investigated the form of the orbital ordering in the electronic nematic phase of the Iron-based superconductors by applying a group theoretical analysis on a realistic five-band model. We find the orbital order can be either of the inter-orbital s-wave form or the intra-orbital d-wave form. From the comparison with existing ARPES measurements of band splitting, we find the orbital ordering in the 122 system is dominated by an intra-orbital d-wave component, while that in the 111 system is dominated by an inter-orbital s-wave component. We find both forms of orbital order are strongly entang…
The angular-dependent magnetoresistance (AMR) of the ab plane is measured on the single crystals of FeSe1-xSx (x = 0, 0.07, 0.13 and 1) and FeSe1-yTey (y = 0.06, 0.61 and 1) at various temperatures under fields up to 9 T. A pronounced twofold-anisotropic carrier-scattering effect is identified by AMR, and attributed to a magnetic-field-induced spin nematicity that emerges from the tetragonal normal-state regime below a characteristic temperature Tsn. This magnetically polarized spin nematicity is found to be ubiquitous in the isoelectronic FeSe1-xSx and FeSe1-yTey systems, no matter whether th…
A key prediction of the SO(5) theory is the antiferromagnetic vortex state. Recent neutron scattering experiment on LSCO superconductors revealed enhanced antiferromagnetic order in the vortex state. Here we review theoretical progress since the original proposal and present a theory of static and dynamic antiferromanetic vortices in LSCO superconductors. It is shown that the antiferromagnetic region induced by the vortices can be greater than the coherence length, due to the light effective mass of the dynamic antiferromagnetic fluctuations at optimal doping, and close promixity to the antife…
