Effect of an electric field on liquid helium scintillation produced by fast electrons
N. S. Phan, V. Cianciolo, S. M. Clayton, S. A. Currie, R. Dipert, T. M. Ito, S. W. T. MacDonald, C. M. O'Shaughnessy, J. C. Ramsey, G. M. Seidel, E. Smith, E. Tang, Z. Tang, W. Yao
The dependence on applied electric field ($0 - 40$ kV/cm) of the scintillation light produced by fast electrons and $α$ particles stopped in liquid helium in the temperature range of 0.44 K to 3.12 K is reported. For both types of particles, the reduction in the intensity of the scintillation signal due to the applied field exhibits an apparent temperature dependence. Using an approximate solution of the Debye-Smoluchowski equation, we show that the apparent temperature dependence for electrons can be explained by the time required for geminate pairs to recombine relative to the detector signal integration time. This finding indicates that the spatial distribution of secondary electrons with respect to their geminate partners possesses a heavy, non-Gaussian tail at larger separations, and has a dependence on the energy of the primary ionization electron. We discuss the potential application of this result to pulse shape analysis for particle detection and discrimination.
We present a measurement of scintillation efficiency for a few tens of keV nuclear recoils (NR) with a liquid argon time projection chamber under electric fields ranging from $0$ to $3\ {\rm kV/cm}$. The calibration data are taken with $^{252}{\rm Cf}$ radioactive source. Observed scintillation and electroluminescence spectra are simultaneously fit with spectra derived from Geant4-based Monte Carlo simulation and an NR model. The scintillation efficiency extracted from the fit is reported as a function of recoil energy and electric field. This result can be used for designing the detector and …
Superfluid $^4$He is a promising target material for direct detection of light ($<$ 1 GeV) dark matter. Possible signal channels available for readout in this medium include prompt photons, triplet excimers, and roton and phonon quasiparticles. The relative yield of these signals has implications for the sensitivity and discrimination power of a superfluid $^4$He dark matter detector. Using a 16~cm$^3$ volume of 1.75~K superfluid $^4$He read out by six immersed photomultiplier tubes, we measured the scintillation from electronic recoils ranging between 36.3 and 185 keV$_\mathrm{ee}$, yielding …
A multi-cell He gas-scintillator active target, designed for the measurement of photoreaction cross sections, is described. The target has four main chambers, giving an overall thickness of 0.103 $\mathrm{g/cm^{2}}$ at an operating pressure of 2 MPa. Scintillations are read out by photomultiplier tubes and the addition of small amounts of $\mathrm{N}_{2}$ to the He, to shift the scintillation emission from UV to visible, is discussed. First results of measurements at the MAX IV Laboratory tagged-photon facility show that the target has good timing resolution and can cope well with a high-flux …
The interpretation of the DAMA seasonal variation pattern as a Dark Matter (DM) effect rests on the assumption that all sources of variable background have been excluded from the measurement. We have identified an overlooked background that mimics the DM signature -- a large, patently existing effect that has nothing to do with detection within the scintillators. This process takes place exclusively within the individual photomultiplier tubes (PMTs), with two familiar actors (thermionic electrons and helium atoms), two familiar processes (helium penetration of glass and ion afterpulsing), and …
We have measured the scintillation and ionization yield of recoiling nuclei in liquid argon as a function of applied electric field by exposing a dual-phase liquid argon time projection chamber (LAr-TPC) to a low energy pulsed narrow band neutron beam produced at the Notre Dame Institute for Structure and Nuclear Astrophysics. Liquid scintillation counters were arranged to detect and identify neutrons scattered in the TPC and to select the energy of the recoiling nuclei. We report measurements of the scintillation yields for nuclear recoils with energies from 10.3 to 57.3 keV and for median ap…
Molecular structure, electric property, and scintillation and quenching of liquid scintillators
Tsinghua University（清华大学）；Department of Engineering Physics, Tsinghua University（清华大学工程物理系）；Center for High Energy Physics, Tsinghua University（清华大学高能物理中心）；Key Laboratory of Particle & Radiation Imaging (Tsinghua University), Ministry of Education（教育部粒子与辐射成像重点实验室（清华大学））
We are developing a novel high-brightness atomic beam, comprised of a two-body exotic atom called muonium (M $ = μ^+ + e^-$), for next-generation atomic physics and gravitational interaction measurements. This M source originates from a thin sheet of superfluid helium (SFHe), hence diagnostics and later measurements require a detection system which is operational in a dilution cryostat at temperatures below 1 K. In this paper, we describe the operation and characterization of silicon photomultipliers (SiPMs) at ultra-low temperatures in SFHe targets. We show the temperature dependence of the s…
The angular dependence of the columnar recombination in xenon gas, if observed for low energy nuclear tracks, can be used for a direction-sensitive dark matter search. We measured both scintillation and ionization to study columnar recombination for 5.4 MeV alpha particles in a high pressure gas detector filled with 8 atm xenon. Since the recombination photons are emitted several~$μ$s after de-excitation emission, scintillation photons are separated to the fast and slow components. The fast component does not show dependence on the track angle relative to the drift electric field, on the other…
Dual phase xenon detectors are widely used in experimental searches for galactic darkmatter particles. The origin of single electron backgrounds following prompt scintillation and proportional scintillation signals in these detectors is not fully understood, although there has been progress in recent years. In this paper, we describe single electron backgrounds in ${}^{83m}Kr$ calibration events and their correlation with drift and extraction fields, using the Particle Identification in Xenon at Yale (PIXeY) dual-phase xenon time projection chamber. The single electron background induced by th…
TetraPhenyl Butadiene is the wavelength shifter most widely used in combination with liquid Argon. The latter emits scintillation photons with a wavelength of 127 nm that need to be downshifted to be detected by photomultipliers with glass or quartz windows. TetraPhenyl Butadiene has been demonstrated to have an extremely high conversion efficiency, possibly higher than 100 % for 127 nm photons, while there is no precise information about the time dependence of its emission. It is usually assumed to be exponentially decaying with a characteristic time of the order of one ns, as an extrapolatio…
Liquid argon is used as active medium in a variety of neutrino and Dark Matter experiments thanks to its excellent properties of charge yield and transport and as a scintillator. Liquid argon scintillation photons are emitted in a narrow band of 10~nm centered around 127 nm and with a characteristic time profile made by two components originated by the decay of the lowest lying singlet and triplet state of the excimer Ar$_2^*$ to the dissociative ground state. A model is proposed which takes into account the quenching of the long lived triplet states through the self-interaction with other tri…
Prompt scintillation signals from $^{83m}$Kr calibration sources are a useful metric to calibrate the spatial variation of light collection efficiency and electric field magnitude of a two phase liquid-gas xenon time projection chamber. Because $^{83m}$Kr decays in two steps, there are two prompt scintillation pulses for each calibration event, denoted S1a and S1b. We study the ratio of S1b to S1a signal sizes in the Particle Identification in Xenon at Yale (PIXeY) experiment and its dependence on the time separation between the two signals ($Δt$), notably its increase at low $Δt$. In PIXeY da…
Experiments searching for weak interacting massive particles with noble gases such as liquid argon require very low detection thresholds for nuclear recoils. A determination of the scintillation efficiency is crucial to quantify the response of the detector at low energy. We report the results obtained with a small liquid argon cell using a monoenergetic neutron beam produced by a deuterium-deuterium fusion source. The light yield relative to electrons was measured for six argon recoil energies between 11 and 120 keV at zero electric drift field.
Understanding liquid xenon scintillation and ionization processes is of great interest to improve analysis methods in current and future detectors. In this paper, we investigate the dynamics of the scintillation process for excitation by $\mathcal{O}$(10 keV) electrons from a $^{83m}$Kr source and $\mathcal{O}$(6 MeV) $α$-particles from a $^{222}$Rn source, both mixed with the xenon target. The single photon sampling method is used to record photon arrival times in order to obtain the corresponding time distributions for different applied electric fields between about 0.8 V/cm to 1.2 kV/cm. En…
Liquid xenon-based direct detection dark matter experiments have recently expanded their searches to include high-energy nuclear recoil events as motivated by effective field theory dark matter and inelastic dark matter interaction models, but few xenon recoil calibrations above 100 keV are currently available. In this work, we measured the scintillation and ionization yields of xenon recoils up to 426 keV. The experiment uses 14.1 MeV neutrons to scatter off xenon in a compact liquid xenon time projection chamber and produce quasi-monoenergetic xenon recoils between 39 keV and 426 keV. We rep…
Measurements were made of scintillation light yield of alpha particles from the $^{222}$Rn decay chain within the DarkSide-50 liquid argon time projection chamber. The light yield was found to increase as the applied electric field increased, with alphas in a 200 V/cm electric field exhibiting a 2% increase in light yield compared to alphas in no field.
We performed a time-resolved spectroscopic study of the VUV/UV argon scintillation as a function of pressure and electric field, by means of a wavelength sensitive detector operated with different radioactive sources. Our work conveys new evidence of distinctive features of the argon light which are in contrast with the general assumption that, for particle detection purposes, the scintillation can be considered to be largely monochromatic at 128 nm (second continuum). The wavelength and the time-resolved analysis of the photon emission reveal that the dominant component of the argon scintilla…
A small-scale, two-phase (liquid/gas) xenon time projection chamber (Xurich II) was designed, constructed and is under operation at the University of Zurich. Its main purpose is to investigate the microphysics of particle interactions in liquid xenon at energies below 50 keV, which are relevant for rare event searches using xenon as target material. Here we describe in detail the detector, its associated infrastructure, and the signal identification algorithm developed for processing and analysing the data. We present the first characterisation of the new instrument with calibration data from …
We have constructed an apparatus to study DC electrical breakdown in liquid helium at temperatures as low as 0.4 K and at pressures between the saturated vapor pressure and $\sim$600 torr. The apparatus can house a set of electrodes that are 12 cm in diameter with a gap of $1-2$ cm between them, and a potential up to $\pm 50$ kV can be applied to each electrode. Initial results demonstrated that it is possible to apply fields exceeding 100 kV/cm in a 1 cm gap between two electropolished stainless steel electrodes 12 cm in diameter for a wide range of pressures at 0.4 K. We also measured the cu…
We present measurements of the scintillation pulse shape in liquid xenon for nuclear recoils (NR) and electronic recoils (ER) at electric fields of 0 to 0.5 kV/cm for energies $<$ 15 keV and $<$ 70 keV electron-equivalent, respectively. The average pulse shapes are well-described by an effective model with two exponential decay components, where both decay times are fit parameters. We find significant broadening of the pulse for ER due to delayed luminescence from the recombination process. In addition to the effective model, we fit a model describing the recombination luminescence for ER at z…
Experimental data shows that both ionization charge and scintillation light in LAr depend on the deposited energy density ($dE/dx$) and electric field ($\mathcal{E}$). Moreover, free ionization charge and scintillation light are anticorrelated, complementary at a given ($dE/dx$, $\mathcal{E}$) pair. We present LArQL, a phenomenological model that provides the anticorrelation between light and charge and its dependence on the deposited energy as well as on the electric field applied. It modifies the Birks' charge model considering the contribution from the escape electrons at null and low elect…
We measure the liquid argon scintillation response to electronic recoils in the energy range of $2.82$ to $1274.6~{\rm keV}$ at null electric field. The single-phase detector with a large optical coverage used in this measurement yields $12.8 \pm 0.3 ~ (11.2 \pm 0.3)~{\rm photoelectron/keV}$ for $511.0$-${\rm keV}$ $γ$-ray events based on a photomultiplier tube single photoelectron response modeling with a Gaussian plus an additional exponential term (with only a Gaussian term). It is exposed to a variety of calibration sources such as $^{22}{\rm Na}$ and $^{241}{\rm Am}$ $γ$-ray emitters, and…
Scintillation pulse characterization with spectrum-inspired temporal neural networks: case studies on particle detector signals
PLAC, Key Laboratory of Quark and Lepton Physics (MOE)（PLAC，夸克与轻子物理国家重点实验室）；Central China Normal University（中部师范大学）；Hubei Provincial Engineering Research Center of Silicon Pixel Chip & Detection Technology（湖北省硅像素芯片与探测技术工程研究中心）；Key Laboratory of Particle and Radiation Imaging (MOE), Department of Engineering Physics（粒子与辐射成像国家重点实验室，工程物理系）；Tsinghua University（清华大学）
We describe a method for dark matter detection based on the evaporation of helium atoms from a cold surface and their subsequent detection using field ionization. When a dark matter particle scatters off a nucleus of the target material, elementary excitations (phonons or rotons) are produced. Excitations which have an energy greater than the binding energy of helium to the surface can result in the evaporation of helium atoms. We propose to detect these atoms by ionizing them in a strong electric field. Because the binding energy of helium to surfaces can be below 1~meV, this detection scheme…
Detection of the vacuum ultraviolet (VUV) scintillation light produced by liquid noble elements is a central challenge in order to fully exploit the available timing, topological, and calorimetric information in detectors leveraging these media. In this paper, we characterize a novel, windowless amorphous selenium based photodetector with direct sensitivity to VUV light. We present here the manufacturing and experimental setup used to operate this detector at low transport electric fields (2.7-5.2 V/$μ$m) and across a wide range of temperatures (77K-290K). This work shows that the first proof-…
High pressure xenon Time Projection Chambers (TPC) based on secondary scintillation (electroluminescence) signal amplification are being proposed for rare event detection such as directional dark matter, double electron capture and double beta decay detection. The discrimination of the rare event through the topological signature of primary ionisation trails is a major asset for this type of TPC when compared to single liquid or double-phase TPCs, limited mainly by the high electron diffusion in pure xenon. Helium admixtures with xenon can be an attractive solution to reduce the electron diffu…
Strontium iodide doped with europium is a new scintillator material being developed as an alternative to lanthanum bromide doped with cerium for use in high energy astrophysical detectors. As with all scintillators, the issue of nonproportionality is important because it affects the energy resolution of the detector. In this study, we investigate how the nonproportionality of strontium iodide doped with europium changes as a function of temperature 16 deg. C to 60 deg. C by heating the strontium iodide doped with europium scintillator separate from the photomultiplier tube. In a separate exper…
We present evidence of non-excimer-based secondary scintillation in gaseous xenon, obtained using both the NEXT-White TPC and a dedicated setup. Detailed comparison with first-principle calculations allows us to assign this scintillation mechanism to neutral bremsstrahlung (NBrS), a process that has been postulated to exist in xenon that has been largely overlooked. For photon emission below 1000 nm, the NBrS yield increases from about 10$^{-2}$ photon/e$^{-}$ cm$^{-1}$ bar$^{-1}$ at pressure-reduced electric field values of 50 V cm$^{-1}$ bar$^{-1}$ to above 3$\times$10$^{-1}$ photon/e$^{-}$ …
We present measurements of light and charge signals in a dual-phase time projection chamber at electric fields varying from 10 V/cm up to 500 V/cm and at zero field using 511 keV gamma rays from a $^{22}$Na source. We determine the drift velocity, electron lifetime, diffusion constant, and light and charge yields at 511 keV as a function of the electric field. In addition, we fit the scintillation pulse shape to an effective exponential model, showing a decay time of 43.5 ns at low field that decreases to 25 ns at high fields.
Liquid xenon (LXe) is employed in a number of current and future detectors for rare event searches. We use the EXO-200 experimental data to measure the absolute scintillation and ionization yields generated by $γ$ interactions from $^{228}$Th (2615~keV), $^{226}$Ra (1764~keV) and $^{60}$Co (1332~keV and 1173~keV) calibration sources, over a range of electric fields. The $W$-value that defines the recombination-independent energy scale is measured to be $11.5~\pm~0.5$~(syst.)~$\pm~0.1$~(stat.) eV. These data are also used to measure the recombination fluctuations in the number of electrons and …
