Andrew Smith, Kemal Sobotkiewich, Amanatullah Khan, Eric A. Montoya, Liu Yang, Zheng Duan, Tobias Schneider, Kilian Lenz, Jürgen Lindner, Kyongmo An, Xiaoqin Li, Ilya N. Krivorotov
Auto-oscillations of magnetization driven by direct spin current have been previously observed in multiple quasi-zero-dimensional (0D) ferromagnetic systems such as nanomagnets and nanocontacts. Recently, it was shown that pure spin Hall current can excite coherent auto-oscillatory dynamics in quasi-one-dimensional (1D) ferromagnetic nanowires but not in quasi-two-dimensional (2D) ferromagnetic films. Here we study the 1D to 2D dimensional crossover of current-driven magnetization dynamics in wire-based Pt/$\mathrm{Ni}_{80}\mathrm{Fe}_{20}$ bilayer spin Hall oscillators via varying the wire width. We find that increasing the wire width results in an increase of the number of excited auto-oscillatory modes accompanied by a decrease of the amplitude and coherence of each mode. We also observe a crossover from a hard to a soft onset of the auto-oscillations with increasing the wire width. The amplitude of auto-oscillations rapidly decreases with increasing temperature suggesting that interactions of the phase-coherent auto-oscillatory modes with incoherent thermal magnons plays an important role in suppression of the auto-oscillatory dynamics. Our measurements set the upper limit on the dimensions of an individual spin Hall oscillator and elucidate the mechanisms leading to suppression of coherent auto-oscillations with increasing oscillator size.
The distribution of the Hall voltage induced by low-frequency AC current is studied theoretically in the incoherent linear transport of quantum Hall systems. It is shown that the Hall-voltage distribution makes a crossover from the uniform distribution to a concentrated-near-edges distribution as the frequency is increased or the diagonal conductivity is decreased. This crossover is also reflected in the frequency dependence of AC magnetoresistance.
We report the observation of the crossover between the extrinsic and intrinsic spin Hall effect induced by alloying. We found that the spin Hall angle, the ratio of the spin Hall conductivity to the electric conductivity, changes drastically by tuning the composition of Au-Cu alloy. The spin Hall angle changes the sign only in a limited range of the Cu concentration due to the extrinsic skew scattering, while the intrinsic contribution becomes dominant with increasing the Cu concentration. This observation provides essential information for fundamental understanding of spin-orbit physics.
In this paper, we study topological properties and Hall conductivities in PbC/MnSe heterostructure under the illumination of a circularly polarized light. At high frequency regime, energy gap, Chern numbers, and Hall conductivities are studied based on the Floquet theory and Green's function formalism, respectively. The interplay between spin orbit coupling and light leads to topological phase transition between anomalous Hall states and spin Hall states, which is related to the emission and absorption of two virtual photons. The anomalous Hall conductivities are dependent on polarization of l…
We theoretically study the crossover between spin Hall effect and spin swapping, a recently predicted phenomenon that consists in the interchange between the current flow and its spin polarization directions [Lifshits and Dyakonov, Phys. Rev. Lett. 103, 186601 (2009)]. Using a tight-binding model with spin-orbit coupled disorder, spin Hall effect, spin relaxation and spin swapping are treated on equal footing. We demonstrate that spin Hall effect and spin swapping present very different dependences as a function of the spin-orbit coupling and disorder strengths. As a consequence, we show that …
We propose a new theory of the topological Hall effect (THE) in systems with chiral magnetization vortices such as magnetic skyrmions. We solve the problem of electron scattering on a magnetic skyrmion exactly, for an arbitrary strength of exchange interaction and the skyrmion size. We report the existence of different regimes of THE and resolve the apparent contradiction between the adiabatic Berry phase theoretical approach and the perturbation theory for THE. We traced how the topological charge Hall effect transforms into the spin Hall effect upon varying the exchange interaction strength …
Recent reports of spin-orbit coupling enhancement in chemically modified graphene have opened doors to studies of the spin Hall effect with massless chiral fermions. Here, we theoretically investigate the interaction and impurity density dependence of the extrinsic spin Hall effect in spin-orbit coupled graphene. We present a nonperturbative quantum diagrammatic calculation of the spin Hall response function in the strong-coupling regime that incorporates skew scattering and anomalous impurity density-independent contributions on equal footing. The spin Hall conductivity dependence on Fermi en…
Suspended graphene nano-ribbons formed during current annealing of suspended graphene flakes have been investigated experimentally. Transport measurements show the opening of a transport gap around charge neutrality due to the formation of "Coulomb islands", coexisting with quantum Hall conductance plateaus appearing at moderate values of magnetic field $B$. Upon increasing $B$, the transport gap is rapidly suppressed, and is taken over by a much larger energy gap due to electronic correlations. Our observations show that suspended nano-ribbons allow the investigation of phenomena that could n…
We determine the composition of intrinsic as well as extrinsic contributions to the anomalous Hall effect (AHE) in the isoelectronic L1o FePd and FePt alloys. We show that the AHE signal in our 30 nm thick epitaxially deposited films of FePd is mainly due to extrinsic side-jump, while in the epitaxial FePt films of the same thickness and degree of order the intrinsic contribution is dominating over the extrinsic mechanisms of the AHE. We relate this crossover to the difference in spin-orbit strength of Pt and Pd atoms and suggest that this phenomenon can be used for tuning the origins of the A…
We have proposed a method to synchronize multiple spin-transfer torque oscillators based on spin pumping, inverse spin Hall, and spin Hall effects. The proposed oscillator system consists of a series of nano-magnets in junction with a normal metal with high spin-orbit coupling, and an accumulative feedback loop. We conduct simulations to demonstrate the effect of modulated charge currents in the normal metal due to spin pumping from each nano-magnet. We show that the interplay between the spin Hall effect and inverse spin Hall effect results in synchronization of the nano-magnets.
We investigate the crossover regime from three dimensional topological insulators $Bi_2Te_3$ and $Bi_2Se_3$ to two dimensional topological insulators with quantum spin Hall effect when the layer thickness is reduced. Using both analytical models and first-principles calculations, we find that the crossover occurs in an oscillatory fashion as a function of the layer thickness, alternating between topologically trivial and non-trivial two dimensional behavior.
We experimentally study spin-Hall nano-oscillators based on [Co/Ni] multilayers with perpendicular magnetic anisotropy. We show that these devices are capable of single-frequency auto-oscillations at current densities comparable to those in the in-plane magnetized oscillators. The demonstrated oscillators exhibit large magnetization precession amplitudes, and their oscillation frequency is highly tunable by the electric current. These features make them promising for applications in high-speed integrated microwave circuits.
This paper reviews the state of the art in spin-torque and spin Hall effect driven nano-oscillators. After a brief introduction to the underlying physics, the authors discuss different implementations of these oscillators, their functional properties in terms of frequency range, output power, phase noise, and modulation rates, and their inherent propensity for mutual synchronization. Finally, the potential for these oscillators in a wide range of applications, from microwave signal sources and detectors to neuromorphic computation elements, is discussed together with the specific electronic ci…
We report on the observation of quantum transport and interference in a graphene device that is attached with a pair of split gates to form an electrostatically-defined quantum point contact (QPC). In the low magnetic field regime, the resistance exhibited Fabry-Pérot (FP) resonances due to np'n (pn'p) cavities formed by the top gate. In the quantum Hall (QH) regime with a high magnetic field, the edge states governed the phenomena, presenting a unique condition where the edge channels of electrons and holes along a p-n junction acted as a solid-state analogue of a monochromatic light beam. We…
An array of spin torque oscillators (STOs) for practical applications such as pattern recognition was recently proposed, where several STOs are connected by a common nonmagnet. In this structure, in addition to the electric and/or magnetic interactions proposed in previous works, the STOs are spontaneously coupled to each other through the nonmagnetic connector, due to the injection of spin current. Solving the Landau-Lifshitz-Gilbert equation numerically for such system consisting of three STOs driven by the spin Hall effect, it is found that both in-phase and antiphase synchronization of the…
We report transport studies of Mn-doped Bi2Te3 topological insulator (TI) films with accurately controlled thickness grown by molecular beam epitaxy. We find that films thicker than 5 quintuple-layer (QL) exhibit the usual anomalous Hall effect for magnetic TIs. When the thickness is reduced to 4 QL, however, characteristic features associated with the topological Hall effect (THE) emerge. More surprisingly, the THE vanishes again when the film thickness is further reduced to 3 QL. Theoretical calculations demonstrate that the coupling between the top and bottom surface states at the dimension…
Spin Hall nano-oscillators (SHNOs) are promising candidates for new microwave oscillators with high durability due to a small driving current. However, conventional SHNOs with an in-plane precession (IPP) mode require a bias field for stable oscillations which is not favored in certain applications such as neuromorphic computing. Here, we propose and theoretically analyze a bias-field-free SHNO with an in-plane hard axis and an out-of-plane precession (OPP) mode by solving the Landau-Lifshitz-Gilbert (LLG) equation analytically and numerically. We derive formulas for driving currents and prece…
This paper introduces a novel oscillator that combines the tunability of spin Hall-driven nano oscillators with the high quality factor (Q) of high overtone bulk acoustic wave resonators (HBAR), integrating both reference and tunable oscillators on the same chip with CMOS. In such magneto acoustic spin Hall (MASH) oscillators, voltage oscillations across the magnetic tunnel junction (MTJ) that arise from a spin-orbit torque (SOT) are shaped by the transmission response of the HBAR that acts as a multiple peak-bandpass filter and a delay element due to its large time constant, providing delayed…
Near-zero effective magnetization enabling ultra-low threshold currents in spin Hall micro-oscillators
Rheinland-Pfälzische Technische Universität Kaiserslautern-Landau（莱茵兰-普法尔茨技术大学凯泽斯劳滕-兰道）；University College London（伦敦大学学院）；Tohoku University（东北大学）；Japan Atomic Energy Agency（日本原子能机构）；CNRS, Université Paris-Saclay（法国国家科学研究中心，巴黎萨克雷大学）
We experimentally study the dynamical modes excited by spin current in Spin Hall nano-oscillators based on the Pt/[Co/Ni] multilayers with perpendicular magnetic anisotropy. Both propagating spin wave and localized solitonic modes of the oscillation are achieved and controlled by varying the applied magnetic field and current. At room temperature, the generation linewidth broadening associated with mode hopping was observed at currents close to the transition between different modes and in the mode coexistence regimes. The mode hopping was suppressed at cryogenic temperatures, confirming that …
We experimentally demonstrate that both quasi-linear and nonlinear self-localized bullet modes of magnetization auto-oscillation can be excited by dc current in the nano-gap spin Hall nano-oscillator, by utilizing the geometry with an extended gap. The quasi-linear mode is stable at low driving currents, while the bullet mode is additionally excited at larger currents, and becomes increasingly dominant with increasing current. Time-resolved measurements show that the formation of the bullet mode is delayed relative to the quasi-linear mode by up to 100 nanoseconds, demonstrating that the mecha…
We show how the two-dimensional (2D) topological insulator evolves, by stacking, into a strong or weak topological insulator with different topological indices, proposing a new conjecture that goes beyond an intuitive picture of the crossover from quantum spin Hall to the weak topological insulator. Studying the conductance under different boundary conditions, we demonstrate the existence of two conduction regimes in which conduction happens through either surface- or edge-conduction channels. We show that the two conduction regimes are complementary and exclusive. Conductance maps in the pres…
A strategy for a scalable synchronization of an array of spin-Hall oscillators (SHOs) is illustrated. In detail, we present micromagnetic simulations of two and five SHOs realized by means of couples of triangular golden contacts on the top of a Pt/CoFeB/Ta trilayer. Results highlight that the synchronization occurs for the whole current region that gives rise to the excitation of self-oscillations. This is linked to the role of the magnetodipolar coupling, which is the phenomenon driving the synchronization when the distance between oscillators is not too large. Synchronization turns out to b…
The Ising machine is an unconventional computing architecture that can be used to solve NP-hard combinatorial optimization problems more efficiently than traditional von Neumann architectures. Fast, compact oscillator networks which provide programmable connectivities among arbitrary pairs of nodes are highly desirable for the development of practical oscillator-based Ising machines. Here we propose using an electrically coupled array of GHz spin Hall nano-oscillators to realize such a network. By developing a general analytical framework that describes injection locking of spin Hall oscillato…
We report the experimental results from a dark study and a photo-excited study of the high mobility GaAs/AlGaAs system at large filling factors, $ν$. At large-$ν$, the dark study indicates several distinct phase relations ("Type-1", "Type-2", and "Type-3") between the oscillatory diagonal- and Hall- resistances, as the canonical Integral Quantum Hall Effect (IQHE) is manifested in the "Type-1" case of approximately orthogonal diagonal- and Hall resistance- oscillations. Surprisingly, the investigation indicates quantum Hall plateaus also in the "Type-3" case characterized by approximately "ant…
We study the quantum Hall plateau transition on rectangular tori. As the aspect ratio of the torus is increased, the two-dimensional critical behavior, characterized by a subthermodynamic number of topological states in a vanishing energy window around a critical energy, changes drastically. In the thin-torus limit, the entire spectrum is Anderson-localized; however, an extensive number of states retain a Chern number $C\neq 0$. We resolve this apparent paradox by mapping the thin-torus quantum Hall system onto a disordered Thouless pump, where the Chern number corresponds to the winding numbe…
We investigate magnetization dynamics in a spin-Hall oscillator using a direct current measurement as well as conventional microwave spectrum analysis. When the current applies an anti-damping spin-transfer torque, we observe a change in resistance which we ascribe to the excitation of incoherent exchange magnons. A simple model is developed based on the reduction of the effective saturation magnetization, quantitatively explaining the data. The observed phenomena highlight the importance of exchange magnons on the operation of spin-Hall oscillators.
We study the impact of spin wave damping ($α$) on the auto-oscillation properties of nano-constriction based spin Hall nano-oscillators (SHNOs). The SHNOs are based on a 5 nm Pt layer interfaced to a 5 nm Py$_{100-x-y}$Pt$_{x}$Ag$_{y}$ magnetic layer, where the Pt and Ag contents are co-varied to keep the saturation magnetization constant (within 10 %), while $α$ varies close to a factor of three. We systematically investigate the influence of the Gilbert damping on the magnetodynamics of these SHNOs by means of electrical microwave measurements. Under the condition of a constant field, the th…
Spin Hall oscillators (SHO) are promising candidates for the generation, detection and amplification of high frequency signals, that are tunable through a wide range of operating frequencies. They offer to be read out electrically, magnetically and optically in combination with a simple bilayer design. Here, we experimentally study the spatial dependence and spectral properties of auto-oscillations in SHO devices based on Pt(7 nm)/\ Ni$_{\mathrm{80}}$Fe$_{\mathrm{20}}$(5 nm) tapered nanowires. Using Brillouin light scattering microscopy, we observe two individual self-localized spin-wave bulle…
We demonstrate a combined frequency and time domain investigation of injection-locked, constriction-based spin Hall nano-oscillators by Brillouin light scattering (BLS) and time-resolved magneto-optical Kerr effect (TR-MOKE). This was achieved by applying an alternating current in the GHz regime in addition to the direct current which drives auto-oscillations in the constriction. In the frequency domain, we analyze the width of the locking range, the increase in intensity and reduction in linewidth as a function of the applied direct current. Then we show that the injection locking of the auto…
When a three-dimensional (3D) ferromagnetic topological insulator thin film is magnetized out-of-plane, conduction ideally occurs through dissipationless, one-dimensional (1D) chiral states that are characterized by a quantized, zero-field Hall conductance. The recent realization of this phenomenon - the quantum anomalous Hall effect - provides a conceptually new platform for studies of edge-state transport, distinct from the more extensively studied integer and fractional quantum Hall effects that arise from Landau level formation. An important question arises in this context: how do these 1D…
Spin-Hall nano-oscillators (SHNOs) are promising spintronic devices to realize current controlled GHz frequency signals in nanoscale devices for neuromorphic computing and creating Ising systems. However, traditional SHNOs -- devices based on transition metals -- have high auto-oscillation threshold currents as well as low quality factors and output powers. Here we demonstrate a new type of hybrid SHNO based on a permalloy (Py) ferromagnetic-metal nanowire and low-damping ferrimagnetic insulator, in the form of epitaxial lithium aluminum ferrite (LAFO) thin films. The superior characteristics …
Current-driven spin-orbit torques are investigated in a heterostructure composed of a ferromagnet deposited on top of a three dimensional topological insulator using the linear response formalism. We develop a tight-binding model of the heterostructure adopting a minimal interfacial hybridization scheme that promotes induced magnetic exchange on the topological surface states, as well as induced Rashba-like spin-orbit coupling in the ferromagnet. Therefore, our model accounts for spin Hall effect from bulk states together with inverse spin galvanic and magnetoelectric effects at the interface …
Spin torque oscillators placed onto a nonmagnetic heavy metal show synchronized auto-oscillations due to the coupling originating from spin Hall magnetoresistance effect. Here, we study a system having two spin torque oscillators under the effect of the spin Hall torque, and show that switching the external current direction enables us to control the phase difference of the synchronization between in-phase and antiphase.
Nano-constriction spin-Hall nano-oscillators (NC-SHNOs) are one of the most promising alternatives among the microwave spintronics devices. They can provide highly coherent and widely tuneable microwave signals and can be fabricated at low temperatures, which makes them compatible with back-end-of-the-line CMOS processing. For its applications, the frequency stability of each device is crucial, in particular for synchronization of oscillator arrays. In this work, we focus on the influence of a realistic grain structure on the SHNO frequency stability using both measurements as well as micromag…
Tunable inter-edge interactions in a bilayer graphene quantum Hall antidot
Institute of Physics, École Polytechnique Fédérale de Lausanne (EPFL)（洛桑联邦理工学院物理研究所）；Research Center for Functional Materials, National Institute for Materials Science（国立材料研究所功能材料研究中心）；International Center for Materials Nanoarchitectonics, National Institute for Materials Science（国立材料研究所国际纳米材料架构中心）；Institute of Experimental and Applied Physics and Halle-Berlin-Regensburg Cluster of Excellence CCE, University of Regensburg（雷根斯堡大学实验与应用物理研究所及哈勒-柏林-雷根斯堡卓越集群CCE）；Center for Quantum Science and Engineering (QSE Center), École Polytechnique Fédérale de Lausanne (EPFL)（洛桑联邦理工学院量子科学与工程中心）
We experimentally study the auto-oscillating spin-wave modes in NiFe/$β-$W constriction-based spin Hall nano-oscillators as a function of bias current, in-plane applied field strength, and azimuthal field angle, in the low-field range of 40-80 mT. We observe two different spin-wave modes: i) a linear-like mode confined to the minima of the internal field near the edges of the nanoconstriction, with weak frequency dependencies on the bias current and the applied field angle, and ii) a second, lower frequency mode that has significantly higher threshold current and stronger frequency dependencie…
This letter studies the dynamical behavior of spin-Hall nanoscillators from a micromagnetic point of view. The model parameters have been identified by reproducing recent experimental data quantitatively. Our results indicate that a strongly localized mode is observed for in-plane bias fields such as in the experiments, while predict the excitation of an asymmetric propagating mode for large enough out-of plane bias field similarly to what observed in spin-torque nanocontact oscillators. Our findings show that spin-Hall nanoscillators can find application as spin-wave emitters for magnonic app…
