Photonic scattering materials, such as biological tissue and white paper, are made of randomly positioned nanoscale inhomogeneities in refractive index that lead to multiple scattering of light. Typically these materials, both naturally-occurring or man-made, are formed through self assembly of the scattering inhomogeneities, which imposes challenges in tailoring the disorder and hence the optical properties. Here, We report on the nanofabrication of photonic scattering media using direct laser writing with deterministic design. These deterministic scattering media consist of submicron thick polymer nanorods that are randomly oriented within a cubic volume. We study the total transmission of light as a function of the number density of rods and of the sample thickness to extract the scattering and transport mean free paths using radiative transfer theory. Such photonic scattering media with deterministic and controllable properties are model systems for fundamental light scattering in particular with strong anisotropy and offer new applications in solid-state lighting and photovoltaics.
We show the designs of one- and two-dimensional photonic negative index metamaterials around telecom wavelengths. Designed bulk structures are inherently connected, which render their fabrication feasible by direct laser writing and chemical vapor deposition.
We present the blueprint for a novel negative-index metamaterial. This structure is fabricated via three-dimensional two-photon direct laser writing and silver shadow evaporation. The comparison of measured linear optical spectra with theory shows good agreement and reveals a negative real part of the refractive index at around 3.85 micrometer wavelength - despite the fact that the metamaterial structure is bi-anisotropic due to the lack of inversion symmetry along its surface normal.
We demonstrate the first buried optical waveguides in diamond using focused femtosecond laser pulses. The properties of nitrogen vacancy centers are preserved in the waveguides, making them promising for diamond-based magnetometers or quantum information systems.
Multiple controllable spiking patterns are obtained in a 1310 nm Vertical Cavity Surface Emitting Laser (VCSEL) in response to induced perturbations and for two different cases of polarized optical injection, namely parallel and orthogonal. Achievement of reproducible spiking responses in VCSELs operating at the telecom wavelengths offers great promise for future uses of these devices in ultrafast neuromorphic photonic systems for non-traditional computing applications.
We present here our recent progress in the three-dimensional (3D) direct laser writing (DLW) of step-index core waveguides inside diverse technologically relevant dielectric substrates, with specific emphasis on the demonstration of DLW mid-infrared waveguiding in the whole transparency range of these materials.
Infrared optical photonic crystals fabricated using direct laser writing, which is based on the two-photon polymerization of suitable monomers, have received substantial interest since the emergence of this process. Two-photon polymerization could be a disruptive technology for the fabrication of all-dielectric photonic crystals in the infrared spectral range, as it allows the synthesis of large scale arrays of uniform structures with arbitrary geometries and arrangements. However, all-dielectric photonic crystals that provide birefringent optical responses in the infrared spectral range have …
In the present article we substantially expand on our recent study about the fabrication of mesoscale polymeric templates of disordered photonic network materials. We present a detailed analysis and discussion of important technical aspects related to the fabrication and characterization of these fascinating materials. Compared to our initial report we were able to reduce the typical structural length scale of the seed pattern from $a=3.3μm$ to $a=2μm$, bringing it closer to the technologically relevant fiber-optic communications wavelength range around $λ\sim 1.5 μm$. We have employed scannin…
Anderson localization is a ubiquitous interference phenomenon in which waves fail to propagate in a disordered medium. Unlike in a classical resonator, satisfying the favorable condition for the interference in a disordered medium is truly a statistical problem in physics. Recent progress in realizing Anderson localization is mainly limited to the iterative method for optimizing the disordered medium. Availability of an in-situ, active control for optimization surely paves the way of realizing the Anderson localization and its applications. In this letter, we have proposed an electro-optic con…
We propose supercritical xenon in a hollow-core photonic bandgap fiber as a highly nonlinear medium, and demonstrate 200 nm control over the guidance window of the fiber as the xenon goes through its supercritical phase transition. The large optical polarizability and monoatomic nature of xenon are predicted to allow large optical nonlinearity, on the same order as that of fused silica, while maintaining greatly reduced Raman scattering, offering benefits for nonlinear and quantum optics.
In this paper we present a systematic study of photonic bandgap engineering using aperiodic lattices (ALs). Up to now ALs have tended to be defined by specific formulae (e.g. Fibonacci, Cantor), and theories have neglected other useful ALs along with the vast majority of non-useful (random) ALs. Here, we present a practical and efficient Fourier space-based general theory to identify all those ALs having useful band properties, which are characterized by well-defined Fourier (i.e. lattice momentum) components. Direct control of field localization comes via control of the Parseval strength comp…
We show the possibility to periodically modulate refractive index in atomic medium in space or/and time while simultaneously keeping vanishing absorption/gain. Such modulation is based on periodic resonant enhancement of refractive index, controlled by an external optical field, and opens a way to produce coherently controllable photonic structures. We suggest possible implementation of the proposed scheme in rare-earth doped crystals with excited state absorption.
Increasing any degree of freedom of light beam may open a wide application area of this special light beam. Vortex beam with a dimension of orbital angular momentum (OAM) as a useful light source has been widely applied in many fields. Here, unique multicolor concentric ultrafast vortex beams (MUCU-VBs), which are also named ultrafast photonic rainbow, with controllable orbital angular momentum are firstly generated using cascaded four-wave mixing (CFWM) in an yttrium aluminum garnet (YAG) plate. Up to 9 multicolor concentric annular ultrafast vortex sidebands are generated simultaneously. The…
Vortices are whirling disturbances commonly found in nature ranging from tremendously small scales in Bose-Einstein condensates to cosmologically colossal scales in spiral galaxies. An optical vortex, generally associated with a spiral phase, can carry orbital angular momentum (OAM). The optical OAM can either be in the longitudinal direction if the spiral phase twists in the spatial domain or in the transverse direction if the phase rotates in the spatiotemporal domain. In this article, we demonstrate the intersection of spatiotemporal vortices and spatial vortices in a wave packet. As a resu…
Today, it is well known that light possesses a linear momentum which is along the propagation direction. Besides, scientists also discovered that light can possess an angular momentum (AM), a spin angular momentum (SAM) associated with circular polarization and an orbital angular momentum (OAM) owing to the azimuthally dependent phase. Even though such angular momenta are longitudinal in general, a SAM transverse to the propagation has opened up a variety of key applications [1]. In contrast, investigations of the transverse OAM are quite rare due to its complex nature. Here we demonstrate a s…
We report resonant features of novel controllable reflectarray which consists of meander-like graphene strips placed on a metal-backed dielectric substrate. The structure manifests two kinds of resonances appeared as sharp deeps of reflectivity. The first one exists because the strips of periodic cells of the structure have resonant sizes for induced surface plasmon-polaritons. The second kind of resonances is defined by excitation of TM eigenwaves of the whole structure as a plane photonic crystal. The latter resonances do not depend on whether the strips of the unit cells have resonant sizes…
Photonic molecules can be used to realize complex optical energy states and modes, analogous to those found in molecules, with properties useful for applications like spectral engineering and quantum optics. It is desirable to implement photonic molecules using high quality factor photonic integrated ring resonators due to their narrow atom-like spectral resonance, tunability, and the ability to scale the number of resonators on a photonic circuit. However, to take full advantage of molecule spectral complexity and tuning degree of freedom, resonator structures should have full symmetry in ter…
Coupled semiconductor lasers are systems possessing complex dynamics that are interesting for numerous applications in photonics. In this work, we investigate the existence and the stability of asymmetric phase-locked states of the fundamental active photonic dimer consisting of two coupled lasers. We show that stable phase-locked states of arbitrary asymmetry exist for extended regions of the parameter space of the system and that their field amplitude ratio and phase difference can be dynamically controlled by appropriate current injection. The model includes the important role of carrier de…
We show that by using a perturbed photonic Dirac-cone, one can realize ultra-narrow and finite Q-factor peak in the wavevector space, with both the peak value and the width separately tunable. We also discuss a lower bound in the minimal viable width given a peak Q-value while maintaining sufficient Q differentiation among modes. The strong angular and frequency Q-selection finds applications in optical devices where strong angle- and frequency-selection is needed.
Highly directional and lossless surface wave has significant potential applications in the two-dimensional photonic circuits and devices. Here we experimentally demonstrate a selective Dyakonov surface wave coupling at the interface between a transparent polycarbonate material and nematic liquid crystal 5CB. By controlling the anisotropy of the nematic liquid crystal with an applied magnetic field, a single ray at a certain incident angle from a diverged incident beam can be selectively coupled into surface wave. The implementation of this property may lead to a new generation of on-chip integ…
We report the fabrication of single mode buried channel waveguides for the whole mid-infrared transparency range of chalcogenide sulphide glasses by means of direct laser writing. We have explored the potential of this technology by fabricating a prototype three-dimensional three-beam combiner for future application in stellar interferometry, which delivers a monochromatic interference visibility of 99.89% at 10.6 \mum, and an ultrahigh bandwidth (3-11 \mum) interference visibility of 21.3%. These results demonstrate that it is possible to harness the whole transparency range offered by chalco…
Currently, direct-write waveguide fabrication is probably the most widely studied application of femtosecond laser micromachining in transparent dielectrics. Devices such as buried waveguides, power splitters, couplers, gratings and optical amplifiers have all been demonstrated. Waveguide properties depend critically on the sample material properties and writing laser characteristics. In this paper we discuss the challenges facing researchers using the femtosecond laser direct-write technique with specific emphasis being placed on the suitability of fused silica and phosphate glass as device h…
We report on controllable production of nanostructures embedded in a porous glass substrate by femtosecond laser direct writing. We show that a hollow nano-void with a lateral size of ~40 nm and an axial size of ~1500 nm can be achieved by manipulating the peak intensity and polarization of the writing laser beam. Our finding enables direct construction of 3D nanofluidics inside glass.
Nonlinear topological photonics has been attracting increasing research interest, as it provides an exciting photonic platform that combines the advantages of active all-optical control offered by nonlinear optics with the unique features of topological photonic systems, such as topologically-protected defect-immune light propagation. In this paper, we demonstrate that topological interface modes and trivial edge modes of a specially designed graphene metasurface can be coupled in a tunable and optically controllable manner, thus providing an efficient approach to transfer optical power to top…
Quill effect, one of the intriguing phenomena in ultrafast laser writing, to our knowledge, has not been studied in low-loss-waveguide (LLW) writing regime yet, probably due to its invisibility under conventional white-light microscope in that regime. In this report, with help of adaptive third harmonic generation microscopy we reveal the quill effect in LLW writing regime and study its influences on the properties of written photonic integrated components in term of polarization-related properties in fused silica and beam-splitting ratio of three-waveguide-coupler in borosilicate glass.
Photonic lattices have emerged as a promising approach to localize light in space, for example, through topologically protected edge states and Aharonov-Bohm caging. They are of particular importance in the study of flat band systems via the associated nondiffracting compact localized states. However, such states typically appear static, thus not allowing adaptive or evolutionary features of light localization. Here we report on the first experimental realization of an oscillating compact localized state (OCLS). We observe an oscillatory intensity beating during propagation in a two-dimensiona…
We demonstrated fabrication of waveguide and directional coupler in bulk glass-ceramics Zerodur, through femtosecond laser direct-writing. Waveguide propagation loss of no more than 1.5 dB/cm was achieved. We expect this will lead to the deployment of Zerodur integrated photonics in fields like space-borne astronomy, quantum technology and fundamental physics, for both economic and technical benefits.
We report on femtosecond laser writing of single mode optical waveguides in chalcogenide Gallium Lanthanum Sulphide (GLS) glass. A multiscan fabrication process was employed to create waveguides with symmetric single mode guidance and low insertion losses at 800 nm wavelength, compatible with Ti:Sapphire ultrafast lasers. μRaman and X-Ray microanalysis were used to elucidate the origin of the laser-induced refractive index change in GLS. Nonlinear refractive index measurements of the waveguides were performed by finding the optical switching parameters of a directional coupler, demonstrating t…
Dense and efficient circuits with component sizes approaching the physical limit is the hallmark of high performance integration. However, current fabrication technology is mostly constraint to 2D lithography, and thermal energy dissipation induced by switching electronic signal lines presents a fundamental challenge for truly 3D electronic integration. Photonics reduces this problem, and direct laser writing of a photoresin is a promising high-resolution tool for 3D photonic integration. Here, we combine one and two-photon polymerization (TPP) for waveguide integration for the first time, dra…
Femtosecond laser writing is a powerful technique that allows rapid and cost-effective fabrication of photonic integrated circuits with unique three-dimensional geometries. In particular, the possibility to reconfigure such devices by thermo-optic phase shifters represents a paramount feature, exploited to produce adaptive and programmable circuits. However, the scalability is strongly limited by the flaws of current thermal phase shifters, which require hundreds of milliwatts to operate and exhibit large thermal crosstalk. In this work, thermally-insulating three-dimensional microstructures a…
Hyperuniform disordered networks belong to a peculiar class of structured materials predicted to possess partial and complete photonic bandgaps for relatively moderate refractive index contrasts. The practical realization of such photonic designer materials is challenging however, as it requires control over a multi-step fabcrication process on optical length scales. Here we report the direct-laser writing of hyperuniform polymeric templates followed by a silicon double inversion procedure leading to high quality network structures made of polycrystalline silicon. We observe a pronounced gap i…
Photonic molecules, named by analogy with chemical molecules, are clusters of closely located electromagnetically interacting microcavities or "photonic atoms". As two or several microcavities are brought close together, their optical modes interact, and a rich spectrum of photonic molecule supermodes emerges, which depends both on geometrical and material properties of individual cavities and on their mutual interactions. Here, we discuss ways of controllable manipulation of photonic molecule supermodes, which improve or add new functionalities to microcavity-based optical components. We pres…
We report on the experimental realization of an optical analogue of a quantum geometric potential for light wave packets constrained on thin dielectric guiding layers fabricated in silica by the femtosecond laser writing technology. We further demonstrate the optical version of a topological crystal, with the observation of Bloch oscillations and Zener tunneling of purely geometric nature.
We present the experimental implementation and theoretical model of a controllable dephasing quantum channel using photonic systems. The channel is implemented by coupling the polarization and the spatial distribution of light, that play, in the perspective of Open Quantum Systems, the role of quantum system and environment, respectively. The capability of controlling our channel allows us to visualize its effects in a quantum system. Differently from standard dephasing channels, our channel presents an exotic behavior in the sense that the evolution of a state, from a pure to a mixed state, s…
This paper considers the refraction and diffraction of waves in three-dimensional crystals formed by anisotropically scattering centers. The partial wave expansion method is used to consider the effect of multiple rescattering of waves by centers composing a crystal. The expression for the refractive index of a crystal is derived. It is shown that instead of the diagonal elements of the scattering matrix $\mathbf{T}$, appearing in the expression for the refractive index of a chaotic medium, the derived expression includes the diagonal elements of the reaction matrix $\mathbf{K}$. This fact is …
Femtosecond laser writing is applied to form Bragg grating waveguides in the diamond bulk. Type II waveguides are integrated with a single pulse point-by-point periodic laser modification positioned towards the edge of the waveguide core. These photonic devices, operating in the telecommunications band, allow for simultaneous optical waveguiding and narrowband reflection from a 4th order grating. This fabrication technology opens the way towards advanced 3D photonic networks in diamond for a range of applications.
We present the controllability capabilities for the limit cycles of an extremely tunable photonic oscillator, consisting of two coupled semiconductor lasers. We show that this system supports stable limit cycles with frequencies ranging from a few to more than a hundred GHz that are characterized by a widely varying degree of asymmetry between the oscillations of the two lasers. These dynamical features are directly controllable via differential pumping as well as optical frequency detuning of the two lasers, suggesting a multi-functional oscillator for chip-scale radio-frequency photonics app…
Self-organized semiconductor quantum dots represent almost ideal two-level systems, which have strong potential to applications in photonic quantum technologies. For instance, they can act as emitters in close-to-ideal quantum light sources. Coupled quantum dot systems with significantly increased functionality are potentially of even stronger interest since they can be used to host ultra-stable singlet-triplet spin qubits for efficient spin-photon interfaces and for a deterministic photonic 2D cluster-state generation. We realize an advanced quantum dot molecule (QDM) device and demonstrate e…
We propose and experimentally demonstrate femtosecond direct laser writing with Bessel beams for the fabrication of photonic crystals with spatial filtering functionality. Such filters are mechanically stable, of small (of order of millimeter) size, do not require direct access to the far-field domain, and therefore are excellent candidates for intracavity spatial filtering applications in mini- and micro-lasers. The technique allows the fabrication of efficient photonic crystal spatial filters in glass, with a narrow angle (~1 degree) nearly 100%-transmission pass-band between broad angle (up…
Electron-beam Writing of Spectrally Uniform Green Single-photon Emitters in Hexagonal Boron Nitride
Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences（中国科学院大学杭州高等研究院）；Zhejiang University（浙江大学）；University of Science and Technology of China（中国科学技术大学）；Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences（中国科学院上海光学精密机械研究所）
Non-Hermitian Interaction between Light and Photonic Time Crystal Beyond the Floquet Quasinormal Mode Approximation
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；School of Physical Sciences, University of Chinese Academy of Sciences（中国科学院大学物理科学学院）；State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University（北京大学物理学院介观物理国家重点实验室及纳米光电子前沿科学中心）
Optically active point defects in crystals have gained widespread attention as photonic systems that can find use in quantum information technologies. However challenges remain in the placing of individual defects at desired locations, an essential element of device fabrication. Here we report the controlled generation of single nitrogen-vacancy (NV) centres in diamond using laser writing. The use of aberration correction in the writing optics allows precise positioning of vacancies within the diamond crystal, and subsequent annealing produces single NV centres with up to 45% success probabili…
Photonic crystals with a sufficiently high refractive index contrast display partial or full band gaps. However, imperfections in the metamaterial cause light scattering and extinction of the interfering propagating waves. Positive as well as negative defect volumes may contribute to this kind of optical perturbation. In this study, we fabricate and characterize three-dimensional woodpile photonic crystals, with a pseudo-bandgap for near-infrared optical wavelengths. By direct laser writing, we intentionally introduce random defects in the periodic structure. We show that we can model random d…
We report on the mesoscale fabrication and characterization of polymeric templates for isotropic photonic materials derived from hyper- uniform point patterns using direct laser writing in a polymer photoresist. We study experimentally the microscopic structure by electron microscopy and small angle light scattering. Reducing the refractive index mismatch by liquid infiltration we find good agreement between the scattering data and numerical calculations based on a discrete dipole approximation. Our work demonstrates the feasibility of fabricating such random designer materials on technologica…
