We explore the behavior of the order parameter and the magnetization of antiferromagnetic solids subjected to mutually parallel staggered and magnetic fields. The effective field theory analysis of the partition function is taken up to the two-loop level, where the magnon-magnon interaction comes into play. These interaction effects, however, are small. A phenomenon that comes rather unexpectedly is that the finite-temperature magnetization increases with temperature when the strengths of the staggered and magnetic field are held constant.
We investigate the thermodynamic behavior of antiferromagnetic films in external magnetic fields oriented perpendicular to the staggered magnetization. Within the systematic effective Lagrangian framework we first calculate the two-point function and the dispersion relation for the two types of magnons up to one-loop order. This allows us to split the two-loop free energy density into a piece that originates from noninteracting dressed magnons, and a second piece that corresponds to the genuine magnon-magnon interaction. We then discuss the low-temperature series for various thermodynamic quan…
We study the low-temperature behavior of antiferromagnets in two spatial dimensions that are subjected to a magnetic field oriented perpendicular to the staggered magnetization order parameter. The evaluation of the partition function is carried to two-loop order within the systematic effective Lagrangian technique. Low-temperature series that are valid in weak magnetic and staggered fields are derived for the pressure, staggered magnetization, and magnetization. Remarkably, at $T$=0, the staggered magnetization is enhanced by the magnetic field, implying that the phenomenon of magnetic cataly…
The thermal properties of antiferromagnetic films -- in particular, the square-lattice antiferromagnet -- subjected to an external magnetic field pointing into the direction of the staggered magnetization are explored. The effective field theory analysis of the free energy density is carried out to two-loop order. While the emphasis is on finite temperature, we also discuss the behavior of the magnetization and staggered magnetization at zero temperature. Our results imply that the staggered magnetization increases in presence of the magnetic field -- reminiscent of magnetic catalysis. Most re…
Using systematic effective field theory, we explore the properties of antiferromagnetic films subjected to magnetic and staggered fields that are either mutually aligned or mutually orthogonal. We provide low-temperature series for the entropy density in either case up to two-loop order. Invoking staggered, uniform and sublattice magnetizations of the bipartite antiferromagnet, we investigate the subtle order-disorder phenomena in the spin arrangement, induced by temperature, magnetic and staggered fields -- some of which are quite counterintuitive. In the figures we focus on the spin-$\frac{1…
Using a model-independent low-energy effective field theory, we calculate the free energy of three-dimensional antiferromagnets in a combination of mutually perpendicular external magnetic and staggered fields at the next-to-next-to-leading, two-loop order. Renormalization is carried out analytically, and the renormalization group invariance of the result is checked explicitly. The free energy is thus expressed solely in terms of temperature, the external fields, and a set of low-energy coupling constants, to be determined by experiment or by matching to the microscopic model of a given concre…
Inspired by the recently theoretical development relevant to the experimental data of TlCuCl$_3$, particularly those associated with the universal scaling between the Néel temperature $T_N$ and the staggered magnetization density $M_s$, we carry a detailed investigation of 3-dimensional (3D) dimerized quantum antiferromagnets using the first principles quantum Monte Carlo calculations. The motivation behind our study is to better understand the microscopic effects on these scaling relations of $T_N$ and $M_s$, hence to shed some light on some of the observed inconsistency between the theoretic…
S=1/2 antiferromagnetic Heisenberg chain with staggered fields: Copper pyrimidine and copper benzoate using the density matrix renormalization group for transfer matrices
We study quantum phase transitions in Heisenberg antiferromagnetic chains with a staggered power-law decaying long-range interactions. Employing the density-matrix renormalization group (DMRG) algorithm and the fidelity susceptibility as the criticality measure, we establish more accurate values of quantum critical points than the results obtained from the spin-wave approximation, quantum Monte Carlo and DMRG in literatures. The deviation is especially evident for strong long-range interactions. We extend isotropic long-range interactions to the anisotropic cases and find that kaleidoscope of …
The Heisenberg XXZ spin-1/2 chain is considered in the massive antiferromagnetic regime in the presence of a staggered longitudinal magnetic field. The Hamiltonian of the model is characterised by the anisotropy parameter $Δ<-1$, and by the magnetic field strength h. At zero magnetic field, the model is exactly solvable. In the thermodynamic limit, it has two degenerate vacua and the kinks (which are also called spinons) interpolating between these vacua, as elementary excitations. Application of the staggered magnetic field breaks integrability of the model and induces the long-range attracti…
We investigate the spin-1/2 Heisenberg model on a rectangular lattice, using the Gutzwiller projected variational wave function known as the staggered flux state. Using Monte Carlo techniques, the variational parameters and static spin-structure factor for different coupling anisotropies $γ=J_y/J_x$ are calculated. We observe a gradual evolution of the ground state energy towards a value which is very close to the 1D estimate provided by the Bethe ansatz and a good agreement between the finite size scaling of the energies. The spin-spin correlation functions exhibit a power-law decay with vary…
We investigated magnetic and thermodynamic properties of $S$ = 1/2 quasi-one-dimensional antiferromagnet KCuMoO$_4$(OH) through single crystalline magnetization and heat capacity measurements. At zero field, it behaves as a uniform $S$ = 1/2 Heisenberg antiferromagnet with $J$ = 238 K, and exhibits a canted antiferromagnetism below $T_\mathrm{N}$ = 1.52 K. In addition, a magnetic field $H$ induces the anisotropy in magnetization and opens a gap in the spin excitation spectrum. These properties are understood in terms of an effective staggered field induced by staggered g-tensors and Dzyaloshin…
We analyze the thermodynamic properties of antiferromagnetic solids subjected to a combination of mutually orthogonal uniform magnetic and staggered fields. Low-temperature series for the pressure, order parameter and magnetization up to two-loop order in the effective expansion are established. We evaluate the self-energy and the dispersion relation of the dressed magnons in order to discuss the impact of spin-wave interactions on thermodynamic observables.
We report studies of the magnetic properties of a staggered stacked triangular lattice Ba$_2$MnTeO$_6$ using magnetic susceptibility, specific heat, neutron powder diffraction and inelastic neutron scattering measurements, as well as first principles density functional theory calculations. Neutron diffraction measurements reveal an antiferromagnetic order with a propagated vector $\textbf{\emph{k}}=(0.5, 0.5, 0)$ and N{é}el transition temperature of $T_\text{N}\approx20$ K. The dominant interaction derived from the Curie-Weiss fitting to the inverse DC susceptibility is antiferromagnetic. Thro…
Counterintuitive order-disorder phenomena emerging in antiferromagnetically coupled spin systems have been reported in various studies. Here we perform a systematic effective field theory analysis of two-dimensional bipartite quantum Heisenberg antiferromagnets subjected to either mutually aligned -- or mutually orthogonal -- magnetic and staggered fields. Remarkably, in the aligned configuration, the finite-temperature uniform magnetization $M_T$ grows as temperature rises. Even more intriguing, in the orthogonal configuration, $M_T$ first drops, goes through a minimum, and then increases as …
The Néel temperature, staggered magnetization density, as well as the spinwave velocity of a three-dimensional (3D) quantum Heisenberg model with antiferromagnetic disorder (randomness) are calculated using first principles non-perturbative quantum Monte Carlo simulations. In particular, we examine the validity of universal scaling relations that are related to these three studied physical quantities. These relations are relevant to experimental data and are firmly established for clean (regular) 3D dimerized spin-1/2 Heisenberg models. Remarkably, our numerical results show that the considere…
The continuous imaginary-time quantum Monte Carlo method with the worm update algorithm is applied to explore the ground state properties of the spin-1/2 Heisenberg model with antiferromagnetic (AF) coupling $J>0$ and ferromagnetic (F) coupling $J^{\prime}<0$ along zigzag and armchair directions, respectively, on honeycomb lattice. It is found that by enhancing the F coupling $J^{\prime}$ between zigzag AF chains, the system is smoothly crossover from one-dimensional zigzag spin chains to a two-dimensional magnetic ordered state. In absence of an external field, the system is in a stripe order…
The Heisenberg model for S=1/2 describes the interacting spins of electrons localized on lattice sites due to strong repulsion. It is the simplest strong-coupling model in condensed matter physics with wide-spread applications. Its relevance has been boosted further by the discovery of curate high-temperature superconductors. In leading order, their undoped parent compounds realize the Heisenberg model on square-lattices. Much is known about the model, but mostly at small wave vectors, i.e., for long-range processes, where the physics is governed by spin waves (magnons), the Goldstone bosons o…
Magnetic properties of lightly doped antiferromagnetic YBa$_{2}$Cu$_{3}$O$_{y}$
本工作解决YBa $_{2}$ Cu $_{3}$ O $_{y}$在掺杂低于x=6%，其中该化合物是共线反铁磁体。在该区域中，YBa $_{2}$ Cu $_{3}$ O $_{y}$是在零温度下具有有限电阻率的正常导体。零温时的交错磁化强度为0.6μ B，这是自旋量子涨落所允许的最大值。交错磁化几乎与掺杂无关。另一方面，Neel温度从x=0时的T_N=420K迅速衰减到x = 0.06时的几乎为零。本文解释了这些显着的性能，并表明，从物理的轻掺杂莫特绝缘体与小孔口袋的属性结果。核四极共振数据进行了讨论。这些数据揭示了x <6%时反铁磁有序稳定性的机制。
Probing Anomalous Longitudinal Fluctuations of the Interacting Bose Gas via Bose-Einstein Condensation of Magnons
在均匀磁场中量子海森堡反铁磁体中有限交错磁化的出现可以看作是磁振子的玻色-爱因斯坦凝聚。利用相互作用玻色气体红外行为的非微扰结果，给出了零温下磁场中量子反铁磁体的交错自旋关联函数的精确结果.特别是，我们表明，在1 < D <= 3的纵向动态结构因子S_parallel（q，ω）描述的交错自旋起伏的方向上的交错磁化表现出一个临界连续的重量可以通过改变磁场实验控制。
We study a frustrated spin-$S$ staggered-dimer Heisenberg model on square lattice by using the bond-operator representation for quantum spins, and investigate the emergence of classical magnetic order from the quantum mechanical (staggered-dimer singlet) ground state for increasing $S$. Using triplon analysis, we find the critical couplings for this quantum phase transition to scale as $1/S(S+1)$. We extend the triplon analysis to include the effect of quintet dimer-states, which proves to be essential for establishing the classical order (Néel or collinear in the present study) for large $S$,…
Manipulating spin currents in magnetic insulators is a key technology in spintronics. We theoretically study a simple inversion-asymmetric model of quantum antiferromagnets, where both the exchange interaction and the magnetic field are staggered. We calculate spin currents generated by external electric and magnetic fields by using a quantum master equation. We show that an ac electric field with amplitude $E_0$ leads, through exchange-interaction modulation, to the dc and second-harmonic spin currents proportional to $E_0^2$. We also show that dc and ac staggered magnetic fields $B_0$ genera…
