The magnetic behaviors of a spin-1/2 alternating Heisenberg antiferromagnetic chain in a staggered transverse magnetic field is studied by means of the density-matrix renormalization group method and Jordan-Wigner transformation. Quantum phase transitions of different types are observed in the S=1 Neel and XY-like gapless phases, which result from the competitions between the staggered transverse field and magnetic orders induced by anisotropy and alternating interactions. The results are compared with the mean-field and some exactly resolved results.
We study a two-leg antiferromagnetic spin-1/2 ladder in the presence of a staggered magnetic field. We consider two parameter regimes: strong (weak) coupling along the legs and weak (strong) coupling along the rungs. In both cases, the staggered field drives the Haldane spin-liquid phase of the ladder towards a Gaussian quantum criticality. In a generalized spin ladder with a non-Haldane, spontaneously dimerized phase, the staggered magnetic field induces an Ising quantum critical regime. In the vicinity of the critical lines, we derive low-energy effective field theories and use these descrip…
The EPR spectra along different crystallographic axes for single crystals of CuGeO3 containing 1% of Fe impurity have been studied in the frequency range 60-360 GHz at temperatures 0.5-30 K. The analysis based on the Oshikawa-Affleck (OA) theory suggests that the temperature dependences of the line width and g-factor are formed as a result of the competition between interchain antiferromagnetic interactions and staggered Zeeman energy. It is found that staggered magnetic moments in CuGeO3:Fe are located predominantly along b axis.
Heavy fermion compounds consisting of two or more inequivalent local moment sites per unit cell have been a promising platform of investigating the interplay between distinct Kondo screenings that is absent in the conventional systems containing only one rare-earth ion per unit cell. We report a remarkable enhancement of the antiferromagnetic (AF) ordering tendency in the staggered periodic Anderson model (PAM) with two alternating inequivalent local moments if their hybridization strengths reside in the Kondo singlet and antiferromagnetic insulator regime separately of the phase diagram of ho…
We investigate the behavior of antiferromagnetic integer-spin chains in a staggered magnetic field, by means of the density-matrix renormalization group, carefully addressing the role of finite-size effects within the Haldane phase at small fields. In the case of spin S=2, we determine the dependence of the groundstate energy and magnetization on the external field, in the thermodynamic limit, and show how the peculiar finite-size behavior can be connected with the crossover in the groundstate from a spin liquid to a polarized Néel state.
We develop a boundary field theory approach to electron spin resonance in open $S=1/2$ Heisenberg antiferromagnetic chains with an effective staggered field. In terms of the sine Gordon effective field theory with boundaries,we point out the existence of boundary bound states of elementary excitations, and modification of the selection rules at the boundary. We argue that several "unknown modes" found in electron spin resonance experiments on KCuGaF$_6$ [I. Umegaki et al., Phys. Rev. B 79, 184401 (2009)] and Cu-PM [S. A. Zvyagin et al., Phys. Rev. Lett. 93, 027201 (2004)] can be understood as …
Anticipating realization of interacting fermions in an optical lattice with a large gauge field, we consider phase transitions and loop currents in a two-dimensional S=1/2 fermionic-Hubbard model with $π$/2-staggered flux at half filling. We use a variational Monte Carlo method, which is reliable even for strong correlations. As a trial wave function, a coexistent state of antifferomagnetic and staggered-flux orders is studied. In a strongly correlated regime, the ground state becomes an insulating coexistent state with loop currents. By comparing fermions with bosons, we discuss an important …
We consider the spin-1/2 antiferromagnetic Heisenberg chain in a staggered magnetic field describing materials such as copper benzoate and copper pyrimidine dinitrate. Using the density-matrix renormalization group for transfer matrices (TMRG) we calculate the magnetization of these materials at finite temperature and arbitrary magnetic field. These results are in excellent agreement with experimental data, allowing for a determination of the inhomogeneity parameter c of copper benzoate (c = 0.043) and copper pyrimidine dinitrate (c= 0.11). The TMRG approach can be applied to rather low temper…
We study low-energy excitations in antiferromagnetic Heisenberg chains with a staggered field which splits the spectrum into a longitudinal and a transverse branch. Bound states are found to exist inside the field induced gap in both branches. They originate from the edge effects and are inherent to spin-chain materials. The sine-Gordon scaling $h_s^{2/3}|\log h_s|^{1/6}$ ($h_s$: the staggered field) provides an accurate description for the gap and midgap energies in the transverse branch for $S=1/2$ and the midgap energies in both branches for $S=3/2$ over a wide range of magnetic field; howe…
We present in this paper a nonlinear sigma-model analysis of a spin-1 antiferromagnetic Heisenberg chain in an external commensurate staggered magnetic field. After rediscussing briefly and extending previous results for the staggered magnetization curve, the core of the paper is a novel calculation, at the tree level, of the Green functions of the model. We obtain precise results for the elementary excitation spectrum and in particular for the spin gaps in the transverse and longitudinal channels. It is shown that, while the spectral weight in the transverse channel is exhausted by a single m…
We present a systematic study of coupled $S=1/2$ Heisenberg antiferromagnetic chains in an effective staggered field. We investigate several effects of the staggered field in the {\em higher} ({\em two or three}) {\em dimensional} spin system analytically. In particular, in the case where the staggered field and the inter-chain interaction compete with each other, we predict, using mean-field theory, a characteristic phase transition. The spin-wave theory predicts that the behavior of the gaps induced by the staggered field is different between the competitive case and the non-competitive case…
Considering interacting (antiferromagnetically correlated) electrons, we derive a generalized Harper's equation for the square lattice of infinite size. We obtain an analytic expression for the density of states from the newly derived Harper's equation. We present a predicted phase diagram of staggered magnetization in the plane of temperature vs doping rate and discover a possibility of reentrant behavior of the staggered magnetization even in the presence of applied magnetic field. It is shown that below a critical electron correlation strength (Coulomb repulsion) the staggered magnetization…
Inelastic neutron scattering was used to measure the magnetic field dependence of spin excitations in the antiferromagnetic S=1/2 chain CuCl_2 2(dimethylsulfoxide) (CDC) in the presence of uniform and staggered fields. Dispersive bound states emerge from a zero-field two-spinon continuum with different finite energy minima at wave numbers q=pi and q_i approx pi (1-2<S_z>). The ratios of the field dependent excitation energies are in excellent agreement with predictions for breather and soliton solutions to the quantum sine-Gordon model, the proposed low-energy theory for S=1/2 chains in a stag…
At low temperature the holes doped into the NiO(2) planes of La(2)NiO(4.133) by the excess oxygen collect in diagonal stripes that separate narrow antiferromagnetic domains. The magnetic order drops abruptly to zero at T_m = 110.5 K, but charge order remains with a period of 3a/2. We show that application of a magnetic field in the regime T > T_m induces staggered magnetic order of period 3a due to the net magnetic moment of the high-temperature bond-centered stripes, together with the odd number of Ni spins across an antiferromagnetic domain.
We investigate the thermodynamic behavior of antiferromagnetic films in external magnetic fields oriented perpendicular to the staggered magnetization. Within the systematic effective Lagrangian framework we first calculate the two-point function and the dispersion relation for the two types of magnons up to one-loop order. This allows us to split the two-loop free energy density into a piece that originates from noninteracting dressed magnons, and a second piece that corresponds to the genuine magnon-magnon interaction. We then discuss the low-temperature series for various thermodynamic quan…
We study the low-energy excitations of the spin-1/2 antiferromagnetic Heisenberg chain and $N$-leg ($N$=2, 3, 4) ladders in a staggered magnetic field $h_s$. We show that $h_s$ induces gap and midgap states in all the cases and examine their field scaling behavior. A modified boundary scheme is devised to extract accurate bulk excitation behavior. The gap values converge rapidly as $N$ increases, leading to a field scaling exponent $γ=1/2$ for both the longitudinal and transverse gaps of the square lattice ($N \to \infty$). The midgap states induced by the boundary edge effects share the bulk …
The magnitude of the staggered field is calculated from the EPR data for CuGeO3 doped with Co and Fe magnetic impurities. It is found that this parameter demonstrate an anomalous temperature and magnetic field dependence probably due to (i) the specific mechanism of the staggered field generation in doped CuGeO3 and (ii) a competition between antiferromagnetic interchain exchange and staggered Zeeman energy.
Ground state and low-energy excitations of the quasi-one-dimensional antiferromagnet CuSe$_2$O$_5$ were experimentally studied using bulk magnetization, neutron diffraction, muon spin relaxation and antiferromagnetic resonance measurements. Finite interchain interactions promote long-range antiferromagnetic order below $T_N=17$ K. The derived spin canted structure is characterized by the magnetic propagation vector $\mathbf{k}=(1, 0, 0)$ and the reduced magnetic moment $\bm{m}=[0.13(7), 0.50(1), 0.00(8)]μ_B$. The values of the magnetic anisotropies determined from the field and angular depende…
A spin-singlet ground state with a spin gap has been discovered in antiferromagnetic spin chain substances when the spin value is 1/2, 1 or 2. To find spin gap (singlet-triplet) excitations in spin-3/2 chain substances, we performed inelastic neutron scattering and magnetization measurements on {\it R}CrGeO$_5$ ({\it R} = Y or Sm) powders. As expected, we observed spin gap excitations and the dispersion relation of the lowest magnetic excitations. We proved that the spin system of Cr$^{3+}$ was an antiferromagnetic alternating spin-3/2 chain.
The Heisenberg XXZ spin-1/2 chain is considered in the massive antiferromagnetic regime in the presence of a staggered longitudinal magnetic field. The Hamiltonian of the model is characterised by the anisotropy parameter $Δ<-1$, and by the magnetic field strength h. At zero magnetic field, the model is exactly solvable. In the thermodynamic limit, it has two degenerate vacua and the kinks (which are also called spinons) interpolating between these vacua, as elementary excitations. Application of the staggered magnetic field breaks integrability of the model and induces the long-range attracti…
We present the first experimental realization of an $S=2$ ferromagnetic-antiferromagnetic (F-AF) alternating chain in a new Mn-verdazyl complex [Mn(hfac)$_2$]$\cdot$($o$-Py-V) [hfac=1,1,1,5,5,5-hexafluoroacetylacetonate; $o$-Py-V=3-(2-pyridyl)-1,5-diphenylverdazyl]. Through the $ab$ $initio$ molecular orbital calculation, magnetization, and ESR measurements, this compound is confirmed to form an $S=2$ F-AF alternating chain with Ising anisotropy below about 100 K. Furthermore, we find an anomalous change in magnetization at 1/4 of the saturation value, which is probably a manifestation of the …
We study the low-temperature behavior of antiferromagnets in two spatial dimensions that are subjected to a magnetic field oriented perpendicular to the staggered magnetization order parameter. The evaluation of the partition function is carried to two-loop order within the systematic effective Lagrangian technique. Low-temperature series that are valid in weak magnetic and staggered fields are derived for the pressure, staggered magnetization, and magnetization. Remarkably, at $T$=0, the staggered magnetization is enhanced by the magnetic field, implying that the phenomenon of magnetic cataly…
Local-susceptibility measurements via the NMR shifts of $^{31}$P and $^{51}$V nuclei in the high-pressure phase of (VO)$_{2}$P$_{2}$O$_{7}$ confirmed the existence of a unique alternating antiferromagnetic chain with a zero-field spin gap of 34 K. The $^{31}$P nuclear spin-lattice relaxation rate scales with the uniform spin susceptibility below about 15 K which shows that the temperature dependence of both the static and dynamical spin susceptibilities becomes identical at temperatures not far below the spin-gap energy.
We investigate the scaling properties of the excitation energies and transition amplitudes of the one-dimensional spin-$1\over 2$ antiferromagnetic Heisenberg model exposed to an external perturbation. Two types of perturbations are discussed in detail: a staggered field and a dimerized field.
We study quantum phase transitions in Heisenberg antiferromagnetic chains with a staggered power-law decaying long-range interactions. Employing the density-matrix renormalization group (DMRG) algorithm and the fidelity susceptibility as the criticality measure, we establish more accurate values of quantum critical points than the results obtained from the spin-wave approximation, quantum Monte Carlo and DMRG in literatures. The deviation is especially evident for strong long-range interactions. We extend isotropic long-range interactions to the anisotropic cases and find that kaleidoscope of …
We present a study of the spin-1/2 Heisenberg chain with alternating ferro- and antiferromagnetic exchange, focusing on the role of the exchange couplings to cover both, dimer and Haldane limit. Employing a complementary combination of perturbation theory and quantum Monte Carlo simulation, we report results for the magnetic susceptibility as well as the dynamic structure factor over a wide range of coupling constants and for different temperatures to extract the spin gap. For a small ferromagnetic coupling, we find good agreement between perturbation theory and quantum Monte Carlo. For arbitr…
Using the experimental data given in Phys. Rev. B70, 220507 (2004), we show that -- unlike the effective coupling discussed in this paper -- the net average antiferromagnetic interlayer coupling in doped lanthanum cuprates depends only weakly on the doping or on the temperature. We argue that the effective coupling is proportional to the square of the staggered magnetization, and does not supply new information about the origin of the suppression of the magnetic order in doped samples. Our analysis is based on a modified version of the equation describing the spin-flip transition, which takes …
In conventional quasi-one-dimensional antiferromagnets with quantum spins, magnetic excitations are carried by either magnons or spinons in different energy regimes: they do not coexist independently, nor could they interact with each other. In this Letter, by combining inelastic neutron scattering, quantum Monte Carlo simulations and Random Phase Approximation calculations, we report the discovery and discuss the physics of the coexistence of magnons and spinons and their interactions in Botallackite-Cu2(OH)3Br. This is a unique quantum antiferromagnet consisting of alternating ferromagnetic …
The present work addresses YBa$_{2}$Cu$_{3}$O$_{y}$ at doping below x=6% where the compound is a collinear antiferromagnet. In this region YBa$_{2}$Cu$_{3}$O$_{y}$ is a normal conductor with a finite resistivity at zero temperature. The value of the staggered magnetization at zero temperature is 0.6μ_B, the maximum value allowed by spin quantum fluctuations. The staggered magnetization is almost independent of doping. On the other hand, the Neel temperature decays very quickly from T_N=420K at x=0 to practically zero at x = 0.06. The present paper explains these remarkable properties and demon…
We have studied the ground state phase diagram of a spin ladder with alternating rung exchange $J^{n}_{\perp} = J_{\perp}[1 + (-1)^{n} δ]$ in a magnetic filed, in the limit where the rung coupling is dominant. In this limit the model is mapped onto an $XXZ$ Heisenberg chain in a uniform and staggered longitudinal magnetic fields, where the amplitude of the staggered field is $\sim δ$. We have shown that the magnetization curve of the system exhibits a plateau at magnetization equal to the half of the saturation value. The width of a plateau scales as $δ^ν$, where $ν=4/5$ in the case of ladder …
Using systematic effective field theory, we explore the properties of antiferromagnetic films subjected to magnetic and staggered fields that are either mutually aligned or mutually orthogonal. We provide low-temperature series for the entropy density in either case up to two-loop order. Invoking staggered, uniform and sublattice magnetizations of the bipartite antiferromagnet, we investigate the subtle order-disorder phenomena in the spin arrangement, induced by temperature, magnetic and staggered fields -- some of which are quite counterintuitive. In the figures we focus on the spin-$\frac{1…
By using mainly numerical methods, we investigate the ground-state phase diagram (GSPD) of an $S=1$ ferromagnetic-antiferromagnetic bond-alternating chain with the $XXZ$ and the on-site anisotropies. This system can be mapped onto an anisotropic spin-2 chain when the ferromagnetic interaction is much stronger than the antiferromagnetic interaction. Since there are many quantum parameters in this system, we numerically obtained the GSPD on the plane of the magnitude of the antiferromagnetic coupling versus its $XXZ$ anisotropy, by use of the exact diagonalization, the level spectroscopy as well…
Based on the linear response of the fermion propagator with respect to an external field, we first derive a model-independent expression for the staggered spin susceptibility in which the influence of the full pseudoscalar vertex function is included. This expression for the staggered spin susceptibility is quite different from that given in the previous literature. The numerical values of the staggered spin susceptibility are calculated within the framework of the Dyson-Schwinger approach. Our numerical result shows that the nonperturbative dressing effects on the fermion propagator is very i…
The ground state phase diagrams and thermodynamic properties of a spin-1 bond-alternating Heisenberg antiferromagnetic chain with a single-ion anisotropy in longitudinal and transverse magnetic fields are investigated jointly by means of the infinite time evolving block decimation, the linearized tensor renormalization group and the density matrix renormalization group methods. It is found that in the magnetic field-bond alternating ratio plane six phases such as singlet dimer, Haldane, two Tomonaga-Luttinger liquid, 1/2 magnetization plateau and spin polarized phases are identified in a longi…
We derive an effective spin Hamiltonian for the one-dimensional half-filled asymmetric ionic Hubbard model with alternating on-site interaction in the limit of strong repulsion. It is shown that the effective Hamiltonian is that of a spin $S=1/2$ anisotropic $XXZ$ Heisenberg chain with alternating next-nearest-neighbor and three-spin couplings in the presence of a uniform and a staggered magnetic field.
The continuous imaginary-time quantum Monte Carlo method with the worm update algorithm is applied to explore the ground state properties of the spin-1/2 Heisenberg model with antiferromagnetic (AF) coupling $J>0$ and ferromagnetic (F) coupling $J^{\prime}<0$ along zigzag and armchair directions, respectively, on honeycomb lattice. It is found that by enhancing the F coupling $J^{\prime}$ between zigzag AF chains, the system is smoothly crossover from one-dimensional zigzag spin chains to a two-dimensional magnetic ordered state. In absence of an external field, the system is in a stripe order…
We study the effects of quantum fluctuations and the excitation spectrum for the antiferromagnetic Heisenberg model on a two-dimensional quasicrystal, by numerically solving linear spin-wave theory on finite approximants of the octagonal tiling. Previous quantum Monte Carlo results for the distribution of local staggered magnetic moments and the static spin structure factor are reproduced well within this approximate scheme. Furthermore, the magnetic excitation spectrum consists of magnon-like low-energy modes, as well as dispersionless high-energy states of multifractal nature. The dynamical …
We study the spin-1/2 antiferromagnetic Heisenberg chain in both uniform and (perpendicular) staggered magnetic fields using the density-matrix renormalization-group method. This model has been shown earlier to describe the physics of the copper benzoate materials in magnetic field. In the present work, we extend the study to more general case for a systematic investigation of the field-induced gap and related properties of the spin-1/2 antiferromagnetic Heisenberg chain. In particular, we explore the high magnetic field regime where interesting behaviors in the field-induced gap, magnetizatio…
The fidelity and entanglement entropy in an antiferromagnetic-ferromagnetic alternating Heisenberg chain are investigated by using the method of density-matrix renormalization-group. The effect of anisotropy on fidelity and entanglement entropy are investigated. The relations between fidelity, entanglement entropy and quantum phase transition are analyzed. It is found that the quantum phase transition point can be well characterized by both the ground-state entropy and fidelity for large system.
We establish a novel mechanism of stripe formation in doped systems with alternating $t_{2g}$ orbital order --- the stripe takes the form of a ferro-orbitally ordered domain wall separating domains with staggered order and allowing for deconfined motion of holes along the stripe. At a finite level of hole concentration this gives rise to the stability of this solitonic type of stripes, while we show that the phase change of the staggered order by $π$ plays a minor role in orbitally ordered systems. These results shed new light on the physics of doped materials in which orbital degeneracy is pr…
A series of symmetry-protected topological(SPT) and trivial spin-gap phases in the spin-1/2 ferromagnetic--antiferromagnetic alternating Heisenberg chain with alternating next-nearest-neighbour interaction are investigated using two kinds of entanglement spectra defined by different divisions of the whole chain. In the case one of the next-nearest-neighbor interaction vanishes, the model reduces to the $Δ$-chain in which a series of spin-gap phases are found in J. Phys. Soc. Jpn. 77, 044707 (2008). From the degeneracy of the entanglement spectra, these phases are identified as the SPT and triv…
The response of an open spin chain with isotropic antiferromagnetic interactions to a uniform magnetic field is studied by classical Monte Carlo simulations. It is observed how the induced on-site magnetization is non uniform, due to the occurrence of edge staggered terms which decay exponentially over a distance equal to the zero field correlation length of the infinite chain. The total magnetic moment associated to each staggered term is found to be about half of the original single-spin magnitude and to decrease as the inverse of temperature (i.e. to behave as a Curie-like moment). The nume…
By performing exact quantum Monte Carlo simulations of a model of interacting Dirac Fermions with staggered potential, we reveal a novel intermediate phase where the electronic correlations drive a band insulator metallic, and at a larger interaction, drive the metal to Mott insulator. We also show that the Mott insulating phase is antiferromagnetic. A complete phase diagram is achieved by studying the phase transitions at large staggered potential and interaction strengths, which shows that the intermediate state is robust and occupies a large part of the phase diagram and that it should be m…
We present results for the dynamic structure factor of the S=1/2 bond alternating Heisenberg chain over a large range of frequencies and temperatures. Data are obtained from a numerical evaluation of thermal averages based on the calculation of all eigenvalues and eigenfunctions for chains of up to 20 spins. Interpretation is guided by the exact temperature dependence in the noninteracting dimer limit which remains qualitatively valid up to an interdimer exchange $λ\approx 0.5$. The temperature induced central peak around zero frequency is clearly identified and aspects of the crossover to spi…
By using the coupled cluster method, the numerical exact diagonalization method, and the numerical density matrix renormalization group method, we investigated the properties of the one-dimensional Heisenberg chain with alternating antiferromagnetic and ferromagnetic next nearest neighbor interactions. In the classical limit, the ground state is in the collinear Neel state if a<1/2, while for a>1/2, there is an noncollinear canted state. For the quantum case, we found that, although the classical Neel state is absent, the canted state exists if the frustration parameter a exceeds a critical po…
The topological classification of a series of frustration-induced spin-gap phases in the spin-1/2 ferromagnetic--antiferromagnetic alternating Heisenberg chain with next-nearest-neighbour interaction reported in J. Phys. Soc. Jpn. 82, 064703 (2013) is confirmed using two kinds of entanglement spectra defined by different divisions of the whole chain. For the numerical calculation, the iDMRG method is used. The results are consistent with the valence bond solid picture proposed in the previous paper.
We revisit bulk FeSe through the systematic first-principles electronic structure calculations. We find that there are a series of staggered $n$-mer antiferromagnetic (AFM) states with corresponding energies below that of the collinear AFM state which is the ground state for the parent compounds of most iron-based superconductors. Here the staggered $n$-mer ($n$ any integer $>1$) means that a set of $n$ adjacent spins parallel on a line along $b$-axis with spins in antiparallel between $n$-mers and along $a$-axis. Among them, the lowest energy states are quasi-degenerate staggered dimer and st…
The spin-1/2 ferromagnetic-antiferromagnetic alternating Heisenberg chain with ferromagnetic next-nearest-neighbour (NNN) interaction is investigated. The ground state is the Haldane phase for weak NNN interaction, and is the ferromagnetic phase for weak antiferromagnetic interaction. We find a series of topologically distinct spin-gap phases with various magnitudes of edge spins for strong NNN interaction. The phase boundaries between these phases are determined on the basis of the DMRG calculation with additional spins that compensate the edge spins. It is found that each of the exact soluti…
We obtain the phase diagram in the parameter space $(J'/J, γ)$ and an accurate estimate of the critical line separating the different phases. We show several measuments of the magnetization, dimerization, nearest neighbours correlation, and density of energy in the different zones of the phase diagram, as well as a measurement of the string order parameter proposed as the non vanishing phase order parameter characterizing Haldane phases. All these results will be compared in the limit $J'/J\gg 1$ with the behaviour of the $\textbf{S}=1$ Bond Alternated Heisenberg Chain (BAHC). The analysis of …
We present a static, model-independent, experimental determination of the spin-spin correlation length ξin a quantum spin system. This is achieved in doped Haldane (i.e., S=1 Heisenberg antiferromagnetic) chain Y(2)BaNi(1-x)Mg(x)O(5) by Y NMR imaging of the staggered magnetization induced around the Mg-impurities (i.e., chain boundaries) by magnetic field. The magnitude of this magnetization is found to decay exponentially with ξequal to the theoretical prediction for an infinite S=1 chain, and the staggered magnetic moment at the edge site showing the Curie behavior of an effective S=1/2 spin…
We investigate a possibility of odd-parity multipole orderings in a locally noncentrosymmetric tetragonal compound CeCoSi. By performing symmetrical and microscopic mean-field analyses on a two-orbital tight-binding model, we propose potential odd-parity multipoles hidden in staggered antiferromagnetic and antiferroquadrupole orderings in CeCoSi. We show that $3z^2-r^2$ type of the magnetic quadrupole is induced by the staggered magnetic dipole ordering for a large crystal-field splitting between two orbitals, while $xy$ type of the electric toroidal quadrupole is emergent by the staggered ele…
Nuclear magnetic resonance (NMR) of 31P and 51V nuclei has been measured in a spin-1/2 alternating-chain compound (VO)_2P_2O_7. By analyzing the temperature variation of the 31P NMR spectra, we have found that (VO)_2P_2O_7 has two independent spin components with different spin-gap energies. The spin gaps are determined from the temperature dependence of the shifts at 31P and 51V sites to be 35 K and 68 K, which are in excellent agreement with those observed in the recent inelastic neutron scattering experiments [A.W. Garrett et al., Phys. Rev. Lett. 79, 745 (1997)]. This suggests that (VO)_2P…
In the weak-coupling regime of the continuous theories, two sets of one-loop renormalization group equations are derived and solved to disclose the phase diagrams of the antiferromagnetic generalized two-leg spin-1/2 ladder under the effect of (I) a staggered external magnetic field and (II) an explicit dimerization. In model (I), the splitting of the SU(2)$_2$ critical line into U(1) and Z$_2$ critical surfaces is observed; while in model (II), two critical surfaces arising from their underlying critical lines with SU(2)$_2$ and Z$_2$ characteristics merge into an SU(2)$_1$ critical surface o…
The low temperature magnetization process of the ferromagnetic-antiferromagnetic Heisenberg chain is studied using the interacting boson approximation. In the low field regime and near the saturation field, the spin wave excitations are approximated by the $δ$ function boson gas for which the Bethe ansatz solution is available. The finite temperature properties are calculated by solving the integral equation numerically. The comparison is made with Monte Carlo calculation and the limit of the applicability of the present approximation is discussed.
The ground state phase diagram of the alternating spin-1/2 chains with anisotropic ferromagnetic coupling under the influence of a symmetry breaking transverse magnetic field is studied. We have used the exact diagonalization technique. In the limit where the antiferromagnetic coupling is dominant, we have identified two Ising-type quantum phase transitions. We have calculated two critical fields $h_{c_{1}}$ and $h_{c_{2}}$, corresponding to the transition between different magnetic phases of the system. It is found that the intermediate state ($h_{c_{1}}<h<h_{c_{2}}$) is gapful, describing th…
We successfully synthesized the zinc-verdazyl complex [Zn(hfac)$_2$]$\cdot$($o$-Py-V) [hfac = 1,1,1,5,5,5-hexafluoroacetylacetonate; $o$-Py-V = 3-(2-pyridyl)-1,5-diphenylverdazyl], which is an ideal model compound with an $S$ = 1/2 ferromagnetic-antiferromagnetic alternating Heisenberg chain (F-AF AHC). $Ab$ $initio$ molecular orbital (MO) calculations indicate that two dominant interactions $J_{\rm{F}}$ and $J_{\rm{AF}}$ form the $S=1/2$ F-AF AHC in this compound. The magnetic susceptibility and magnetic specific heat of the compound exhibit thermally activated behavior below approximately 1 …
Doping the high-Tc superconductor YBa2Cu3O6.7 with 1.5 % of non-magnetic Zn impurities in CuO2 planes is shown to produce a considerable broadening of 63Cu NMR spectra, as well as an increase of low-energy magnetic fluctuations detected in 63Cu spin-lattice relaxation measurements. A model-independent analysis demonstrates that these effects are due to the development of staggered magnetic moments on many Cu sites around each Zn and that the Zn-induced moment in the bulk susceptibility might be explained by this staggered magnetization. Several implications of these enhanced antiferromagnetic …
