We employ an improved estimator to calculate the constraint effective potential of the staggered magnetization in the spin $\tfrac{1}{2}$ quantum Heisenberg model using a loop-cluster algorithm. The first and second moment of the probability distribution of the staggered magnetization are in excellent agreement with the predictions of the systematic low-energy magnon effective field theory. We also compare the Monte Carlo data with the universal shape of the constraint effective potential of the staggered magnetization and study its approach to the convex effective potential in the infinite volume limit. In this way the higher-order low-energy parameter $k_0$ is determined from a fit to the numerical data.
We explore the behavior of the order parameter and the magnetization of antiferromagnetic solids subjected to mutually parallel staggered and magnetic fields. The effective field theory analysis of the partition function is taken up to the two-loop level, where the magnon-magnon interaction comes into play. These interaction effects, however, are small. A phenomenon that comes rather unexpectedly is that the finite-temperature magnetization increases with temperature when the strengths of the staggered and magnetic field are held constant.
We study the low-temperature behavior of antiferromagnets in two spatial dimensions that are subjected to a magnetic field oriented perpendicular to the staggered magnetization order parameter. The evaluation of the partition function is carried to two-loop order within the systematic effective Lagrangian technique. Low-temperature series that are valid in weak magnetic and staggered fields are derived for the pressure, staggered magnetization, and magnetization. Remarkably, at $T$=0, the staggered magnetization is enhanced by the magnetic field, implying that the phenomenon of magnetic cataly…
Using a model-independent low-energy effective field theory, we calculate the free energy of three-dimensional antiferromagnets in a combination of mutually perpendicular external magnetic and staggered fields at the next-to-next-to-leading, two-loop order. Renormalization is carried out analytically, and the renormalization group invariance of the result is checked explicitly. The free energy is thus expressed solely in terms of temperature, the external fields, and a set of low-energy coupling constants, to be determined by experiment or by matching to the microscopic model of a given concre…
The thermal properties of antiferromagnetic films -- in particular, the square-lattice antiferromagnet -- subjected to an external magnetic field pointing into the direction of the staggered magnetization are explored. The effective field theory analysis of the free energy density is carried out to two-loop order. While the emphasis is on finite temperature, we also discuss the behavior of the magnetization and staggered magnetization at zero temperature. Our results imply that the staggered magnetization increases in presence of the magnetic field -- reminiscent of magnetic catalysis. Most re…
Inspired by the recently theoretical development relevant to the experimental data of TlCuCl$_3$, particularly those associated with the universal scaling between the Néel temperature $T_N$ and the staggered magnetization density $M_s$, we carry a detailed investigation of 3-dimensional (3D) dimerized quantum antiferromagnets using the first principles quantum Monte Carlo calculations. The motivation behind our study is to better understand the microscopic effects on these scaling relations of $T_N$ and $M_s$, hence to shed some light on some of the observed inconsistency between the theoretic…
We simulate the three-dimensional quantum Heisenberg model with a spatially anisotropic ladder pattern using the first principles Monte Carlo method. Our motivation is to investigate quantitatively the newly established universal relation $T_N/\sqrt{c^3}$ $\propto$ ${\cal M}_s$ near the quantum critical point (QCP) associated with dimerization. Here $T_N$, $c$, and ${\cal M}_s$ are the Néel temperature, the spinwave velocity, and the staggered magnetization density, respectively. For all the physical quantities considered here, such as $T_N$ and ${\cal M}_s$, our Monte Carlo results agree nice…
We propose an efficient numerical method to obtain local order parameter in two-dimensional systems using spiral boundary conditions. As a benchmark, we first estimate the magnitude of staggered magnetization for the $S=1/2$ XXZ Heisenberg model on a square lattice in the whole range of the XXZ anisotropy by density-matrix renormalization group technique. The validity of our method is confirmed by comparing our results with the previous analytical and numerical studies. Then, as further demonstration, we apply our method to obtain the staggered magnetization for the higher-spin cases from $S=1…
Ground state and low-energy excitations of the quasi-one-dimensional antiferromagnet CuSe$_2$O$_5$ were experimentally studied using bulk magnetization, neutron diffraction, muon spin relaxation and antiferromagnetic resonance measurements. Finite interchain interactions promote long-range antiferromagnetic order below $T_N=17$ K. The derived spin canted structure is characterized by the magnetic propagation vector $\mathbf{k}=(1, 0, 0)$ and the reduced magnetic moment $\bm{m}=[0.13(7), 0.50(1), 0.00(8)]μ_B$. The values of the magnetic anisotropies determined from the field and angular depende…
Counterintuitive order-disorder phenomena emerging in antiferromagnetically coupled spin systems have been reported in various studies. Here we perform a systematic effective field theory analysis of two-dimensional bipartite quantum Heisenberg antiferromagnets subjected to either mutually aligned -- or mutually orthogonal -- magnetic and staggered fields. Remarkably, in the aligned configuration, the finite-temperature uniform magnetization $M_T$ grows as temperature rises. Even more intriguing, in the orthogonal configuration, $M_T$ first drops, goes through a minimum, and then increases as …
We calculate exactly cumulant generating functions (full counting statistics) for the transverse, staggered magnetization and the domain walls at zero temperature for a finite interval of the XY spin chain. In particular, we also derive a universal interpolation formula in the scaling limit for the full counting statistics of the transverse magnetization and the domain walls which is based on the solution of a Painlevé V equation. By further determining subleading corrections in a large interval asymptotics, we are able to test the applicability of conformal field theory predictions at critica…
We propose an efficient method to identify the degree of frustration in quasi-2D antiferromagnets described by the J_1-J_2 Heisenberg model. The frustration ratio J_2/J_1 is usually obtained from analysis of susceptibility, specific heat and saturation field. We show that the non-monotonic field dependence of the staggered moment caused by the suppression of quantum fluctuations in a field depends strongly on the frustration ratio. This gives a powerful criterion to determine J_2/J_1 using a combination of exact diagonalization (ED) method for finite clusters and spin wave analysis. We apply t…
We investigate the spin-1/2 Heisenberg model on a rectangular lattice, using the Gutzwiller projected variational wave function known as the staggered flux state. Using Monte Carlo techniques, the variational parameters and static spin-structure factor for different coupling anisotropies $γ=J_y/J_x$ are calculated. We observe a gradual evolution of the ground state energy towards a value which is very close to the 1D estimate provided by the Bethe ansatz and a good agreement between the finite size scaling of the energies. The spin-spin correlation functions exhibit a power-law decay with vary…
We investigated magnetic and thermodynamic properties of $S$ = 1/2 quasi-one-dimensional antiferromagnet KCuMoO$_4$(OH) through single crystalline magnetization and heat capacity measurements. At zero field, it behaves as a uniform $S$ = 1/2 Heisenberg antiferromagnet with $J$ = 238 K, and exhibits a canted antiferromagnetism below $T_\mathrm{N}$ = 1.52 K. In addition, a magnetic field $H$ induces the anisotropy in magnetization and opens a gap in the spin excitation spectrum. These properties are understood in terms of an effective staggered field induced by staggered g-tensors and Dzyaloshin…
We report studies of the magnetic properties of a staggered stacked triangular lattice Ba$_2$MnTeO$_6$ using magnetic susceptibility, specific heat, neutron powder diffraction and inelastic neutron scattering measurements, as well as first principles density functional theory calculations. Neutron diffraction measurements reveal an antiferromagnetic order with a propagated vector $\textbf{\emph{k}}=(0.5, 0.5, 0)$ and N{é}el transition temperature of $T_\text{N}\approx20$ K. The dominant interaction derived from the Curie-Weiss fitting to the inverse DC susceptibility is antiferromagnetic. Thro…
The Néel temperature, staggered magnetization density, as well as the spinwave velocity of a three-dimensional (3D) quantum Heisenberg model with antiferromagnetic disorder (randomness) are calculated using first principles non-perturbative quantum Monte Carlo simulations. In particular, we examine the validity of universal scaling relations that are related to these three studied physical quantities. These relations are relevant to experimental data and are firmly established for clean (regular) 3D dimerized spin-1/2 Heisenberg models. Remarkably, our numerical results show that the considere…
The 2-d spin 1/2 Heisenberg antiferromagnet with exchange coupling $J$ is investigated on a periodic square lattice of spacing $a$ at very small temperatures using the loop-cluster algorithm. Monte Carlo data for the staggered and uniform susceptibilities are compared with analytic results obtained in the systematic low-energy effective field theory for the staggered magnetization order parameter. The low-energy parameters of the effective theory, i.e.\ the staggered magnetization density ${\cal M}_s = 0.30743(1)/a^2$, the spin stiffness $ρ_s = 0.18081(11) J$, and the spin wave velocity $c = 1…
Using quantum Monte Carlo, we study the non-equilibrium transport of magnetization in large open strongly correlated quantum spin $\frac{1}{2}$ systems driven by purely dissipative processes that conserve the uniform or staggered magnetization. We prepare both a low-temperature Heisenberg ferromagnet and an antiferromagnet in two parts of the system that are initially isolated from each other. We then bring the two subsystems in contact and study their real-time dissipative dynamics for different geometries. The flow of the uniform or staggered magnetization from one part of the system to the …
The magnetization process of the isotropic Heisenberg antiferromagnet on the kagome lattice is studied. Data obtained from the numerical-diagonalization method are reexamined from the viewpoint of the derivative of the magnetization with respect to the magnetic field. We find that the behavior of the derivative at approximately one-third of the height of the magnetization saturation is markedly different from that for the cases of typical magnetization plateaux. The magnetization process of the kagome-lattice antiferromagnet reveals a new phenomenon, which we call the "magnetization ramp".
Heisenberg Spin-One Chain in Staggered Magnetic Field : A Density Matrix Renormalization Group Study
利用密度矩阵重整化群方法，数值计算了自旋为1的反铁磁链在交错磁场中的低能激发谱和磁化强度曲线，以期描述磁性稀土（$R$）亚晶格Néel温度以下的$R_2 Ba Ni O_5 (R \neq Y) $族物理.这些结果在交错场的整个范围内都是有效的，并且对于小场与非线性$σ$模型研究的结果一致，但是对于大场与后者不同。它们与现有的实验数据是一致的。计算了该模型的关联函数。横向相关显示预期的指数衰减与较短的相关长度，而纵向相关显示明确的诱导交错磁化。
We apply the coupled cluster method and exact diagonalzation to study the uniform susceptibility and the ground-state magnetization curve of the triangular-lattice spin-1 Heisenberg antiferromagnet. Comparing our theoretical data for the magnetization curve with recent measurements on the s=1 triangular lattice antiferromagnet Ba3NiSb2O9 we find a very good agreement.
Motivated by recent experiments on TmB4 (arXiv:0712.1537), we examine the phase diagram of the Shastry-Sutherland antiferromagnet in an applied magnetic field in the limit of strong Ising anisotropy. In classical Ising limit, we demonstrate that the only fractional magnetization plateau is at 1/3 of the saturated magnetization. We study the perturbative influence of transverse quantum spin fluctuations, and present evidence that they can stabilize a narrow 1/2 magnetization plateau.
We consider the magnetic-field dependent spatial magnetization pattern around a general impurity embedded in a Heisenberg antiferromagnet using both an analytical and a numerical spin wave approach. The results are compared to quantum Monte Carlo simulations. The decay of the magnetization pattern away from the impurity follows a universal form which reflects the properties of the pure antiferromagnetic Heisenberg model. Only the overall magnitude of the induced magnetization depends also on the size of the impurity spin and the impurity coupling.
The magnetization of two spin-1/2 kagome antiferromagnets, volborthite and vesignieite, has been measured in pulsed magnetic fields up to 68 T. A magnetization plateau is observed for each compound near the highest magnetic field. Magnetizations at saturation are approximately equal to 0.40Ms for both compounds, where Ms is the fully saturated magnetization, irrespective of a difference in the distortion of the kagome lattice between the two compounds. It should be noted that these values of magnetizations are significantly larger than Ms/3 predicted theoretically for the one-third magnetizati…
We report the results of magnetization and specific heat measurements on Ba$_3$NiSb$_2$O$_9$, which is a quasi-two-dimensional spin-1 triangular-lattice antiferromagnet. We observed a nonclassical magnetization plateau at one-third of the saturation magnetization that is driven by spin frustration and quantum fluctuation. Exact diagonalization for a 21-site rhombic cluster was performed to analyze the magnetization process. Experimental and calculated results agree well.
We clarify the existence of several magnetization plateaux for the kagome $S=1/2$ antiferromagnetic Heisenberg model in a magnetic field. Using approximate or exact localized magnon eigenstates, we are able to describe in a similar manner the plateau states that occur for magnetization per site $m=1/3$, $5/9$, and $7/9$ of the saturation value. These results are confirmed using large-scale Exact Diagonalization on lattices up to 63 sites.
We investigate the $S=1/2$ quantum spin antiferromagnets on the triangular and Kagome lattices in magnetic field, using the numerical exact diagonalization. Particularly we focus on an anomalous magnetization behavior of each system at 1/3 of the saturation magnetization. The critical exponent analyses suggest that it is a conventional magnetization plateau on the triangular lattice, while an unconventional phenomenon, called the magnetization ramp, on the Kagome lattice.
We study the magnetization process of the spin-1/2 antiferromagnetic Heisenberg model on a layered triangular lattice by means of a numerical cluster mean-field method with a scaling scheme (CMF+S). It has been known that antiferromagnetic spins on a two-dimensional (2D) triangular lattice with quantum fluctuations exhibit a one-third magnetization plateau in the magnetization curve under magnetic field. We demonstrate that the CMF+S quantitatively reproduces the magnetization curve including the stabilization of the plateau. {We also discuss the effects of a finite interlayer coupling, which …
The present work addresses YBa$_{2}$Cu$_{3}$O$_{y}$ at doping below x=6% where the compound is a collinear antiferromagnet. In this region YBa$_{2}$Cu$_{3}$O$_{y}$ is a normal conductor with a finite resistivity at zero temperature. The value of the staggered magnetization at zero temperature is 0.6μ_B, the maximum value allowed by spin quantum fluctuations. The staggered magnetization is almost independent of doping. On the other hand, the Neel temperature decays very quickly from T_N=420K at x=0 to practically zero at x = 0.06. The present paper explains these remarkable properties and demon…
Probing Anomalous Longitudinal Fluctuations of the Interacting Bose Gas via Bose-Einstein Condensation of Magnons
在均匀磁场中量子海森堡反铁磁体中有限交错磁化的出现可以看作是磁振子的玻色-爱因斯坦凝聚。利用相互作用玻色气体红外行为的非微扰结果，给出了零温下磁场中量子反铁磁体的交错自旋关联函数的精确结果.特别是，我们表明，在1 < D <= 3的纵向动态结构因子S_parallel（q，ω）描述的交错自旋起伏的方向上的交错磁化表现出一个临界连续的重量可以通过改变磁场实验控制。
To capture the high-field magnetization process of herbertsmithite (ZnCu3(OH)6Cl2), Faraday rotation (FR) measurements were carried out on a single crystal in magnetic fields of up to 190 T. The magnetization data evaluated from the FR angle exhibited a saturation behavior above 150 T at low temperatures, which was attributed to the 1/3 magnetization plateau. The overall behavior of the magnetization process was reproduced by theoretical models based on the nearest-neighbor Heisenberg model. This suggests that herbertsmithite is a proximate kagome antiferromagnet hosting an ideal quantum spin …
The phenomenon of magnetization plateaus in antiferromagnets under magnetic field has always been an important topic in magnetism. We propose to probe the elusive physics of plateaus in 2-d by considering hole-doped antiferromagnet and studying the signatures of magnetization plateaus in terms of the properties of holes, coupled to an effective gauge field generated by the spin sector. The latter mediates interaction between the holes, found to be algebraically decaying long-ranged with both Coulombic and dipolar forms outside plateau and short-ranged (local) inside plateau. The resulting hole…
We use general hydrodynamic equations to determine the long-wavelength spin excitations in isotropic antiferromagnets in the presence of a homogeneous magnetization. The latter may be induced, such as in antiferromagnets in an external magnetic field, or spontaneous, such as in ferrimagnetic or canted phases that are characterized by the coexistence of antiferromagnetic and ferromagnetic order. Depending on the physical situation, we find propagating spin waves that are gapped in some cases and gapless in others, diffusive modes, or relaxational modes. The excitation spectra turn out to be qua…
We study the S=1/2 Heisenberg antiferromagnet on the Cairo pentagon lattice by the numerical-diagonalization method. We tune the ratio of two antiferromagnetic interactions coming from two kinds of inequivalent sites in this lattice, examining the magnetization process of the antiferromagnet; particular attention is given to one-third of the height of the saturation. We find that quantum phase transition occurs at a specific ratio and that a magnetization plateau appears in the vicinity of the transition. The plateau is accompanied by a magnetization jump on one side among the edges due to the…
