We measured the spin rectify effect and the inverse spin Hall effect in Nb-doped SrTiO$_3$ by injecting the spins from ferromagnetic thin films to SrTiO$_3$ using spin pumping. It was shown that the spin injection is increased when the doping level is increased. However, the spin Hall angle decreases when Nb occupies more than $\sim$2\% of the Ti sites, which is due to that beyond this concentration, the electron contributed the spin Hall effect is from the $d-$orbitals of Nb instead those from the Ti. Our work points to the importance of orbital occupations in the (inverse) spin Hall effect. We may explore controllable spin and charge interconversion in oxide spintronics.
The spin Hall angle (SHA) is a measure of the efficiency with which a transverse spin current is generated from a charge current by the spin-orbit coupling and disorder in the spin Hall effect (SHE). In a study of the SHE for a Pt$|$Py (Py=Ni$_{80}$Fe$_{20}$) bilayer using a first-principles scattering approach, we find a SHA that increases monotonically with temperature and is proportional to the resistivity for bulk Pt. By decomposing the room temperature SHE and inverse SHE currents into bulk and interface terms, we discover a giant interface SHA that dominates the total inverse SHE current…
The measured Hall angle in a ferromagnetic nanomagnet shows a substantial non-linear dependence on an external magnetic field, which cannot be explained by adopted mechanisms of the Ordinary and Anomalous (AHE) Hall effects implying a linear plus constant dependence on the external magnetic field. We suggest that there is an additional non-linear contribution from the Inverse Spin Hall effect (ISHE). The significant contribution of ISHE in a ferromagnet is supported by perfect agreement of experiment with a phenomenological theory of ISHE. We observed different dependencies of AHE and ISHE on …
Here, we investigate spin Hall angle of Pt in Ni80Fe20/Pt bilayer system by using a broadband spin pumping and inverse spin Hall effect measurement. An out-of-plane excitation geometry with application of external magnetic field perpendicular to the charge current direction is utilized in order to suppress unwanted galvanomagnetic effects. Magnetization precession angle on ferromagnetic resonance for wide excitation frequency range (4-14 GHz) is estimated from the rectification voltage of anisotropic magnetoresistance (AMR) and a conventional method of using microwave power in a coplanar waveg…
We investigated the self-induced inverse spin Hall effect in ferromagnets. Temperature (T), thickness (t) and angular-dependent measurements of transverse voltage in spin pumping experiments were performed with permalloy films. Results revealed non-monotonous T-dependence of the self-induced transverse voltage. Qualitative agreement was found with first-principle calculations unravelling the skew scattering, side-jump, and intrinsic contributions to the T-dependent spin Hall conductivity. Experimental data were similar whatever the material in contact with permalloy (oxides or metals), and rev…
Pure spin current based research is mostly focused on ferromagnet (FM)/heavy metal (HM) system. Because of the high spin orbit coupling (SOC) these HMs exhibit short spin diffusion length and therefore possess challenges for device application. Low SOC (elements of light weight) and large spin diffusion length make the organic semiconductors (OSCs) suitable for future spintronic applications. From theoretical model it is explained that, due to $π$ - $σ$ hybridization the curvature of the C$_{60}$ molecules may increase the SOC strength. Here, we have investigated spin pumping and inverse spin …
We measure magnetic field dependence of the Hall angle in a metallic ferromagnetic nanomagnet with stable local magnetic moments where the adopted mechanisms of Hall effect predict linear plus a constant dependence on the external field originating from the ordinary and anomalous Hall effects, respectively. We suggest that the experimentally observed deviations from this dependence is caused by the inverse spin Hall effect (ISHE) and develop a phenomenological theory, which predicts a unique nonlinear dependence of the ISHE contribution on the external magnetic field. Perfect agreement between…
In an easy-plane antiferromagnet with the Dzyaloshinskii-Moriya interaction (DMI), magnons are subject to an effective spin-momentum locking. An in-plane temperature gradient can generate interfacial accumulation of magnons with a specified polarization, realizing the magnon thermal Edelstein effect. We theoretically investigate the injection and detection of this thermally-driven spin polarization in an adjacent heavy metal with strong spin Hall effect. We find that the inverse spin Hall voltage depends monotonically on both temperature and the DMI but non-monotonically on the hard-axis aniso…
Spin transport in thin-film materials can be studied by ferromagnetic resonantly (FMR) driven spin pumping of a charge-free spin current which induces an electromotive force through the inverse spin Hall effect (ISHE). For quantitative ISHE experiments, precise control of the FMR driving field amplitude $B_1$ is crucial. This study exploits in situ monitoring of $B_1$ by utilization of electron paramagnetic resonantly (EPR) induced transient nutation of paramagnetic molecules (a 1:1 complex of α,γ-bisdiphenylene-β-phenylallyl and benzene, BDPA) placed as $B_1$ probe in proximity of a NiFe/Pt-b…
Electric gating can strongly modulate a wide variety of physical properties in semiconductors and insulators, such as significant changes of conductivity in silicon, appearance of superconductivity in SrTiO3, the paramagnet-ferromagnet transition in (In,Mn)As and so on. The key to such modulation is charge accumulation in solids. Thus, it has been believed that such modulation is out of reach for conventional metals where the number of carriers is too large. However, success in tuning the Curie temperature of ultrathin cobalt gave hope of finally achieving such degree of control even in metall…
Using circularly polarized light is an alternative to electronic ways for spin injection into materials. Spins are injected at a point of the light illumination, and then diffuse and spread radially due to the in-plane gradient of the spin density. This diffusion is converted into a circular charge current by the inverse spin Hall effect (ISHE). With shining the circularly polarized light at asymmetric parts of the sample, such as near edges, we detected this current as a helicity-dependent component in the photocurrent. We present a model for this ISHE based on the experimental results and th…
We study theoretically and experimentally the spin pumping signals induced by the resonance of canted antiferromagnets with Dzyaloshinskii-Moriya interaction and demonstrate that they can generate easily observable inverse spin-Hall voltages. Using a bilayer of hematite/heavy metal as a model system, we measure at room temperature the antiferromagnetic resonance and an associated inverse spin-Hall voltage, as large as in collinear antiferromagnets. As expected for coherent spin-pumping, we observe that the sign of the inverse spin-Hall voltage provides direct information about the mode handedn…
Unambiguous separation of the inverse spin Hall and anomalous Nernst Effects within a ferromagnetic metal using the spin Seebeck effect
用铁磁金属Co $_{0.2}$ Fe $_{0.6}$ B $_{0.2}$（CoFeB）作为自旋探测器，测量了铁磁绝缘体Fe $_3$ O $_4$上的纵向自旋塞贝克效应.通过在两种材料（Ti）之间使用非磁性间隔物材料，可以使两种铁磁材料去耦，并直接观察从Fe $_3$ O $_4$到CoFeB的纯自旋流。结果表明，在单一铁磁金属中，逆自旋霍尔效应（ISHE）和反常能斯特效应（ANE）可以同时发生，但极性相反。利用这一点以及两个磁体之间矫顽场的巨大差异，可以明确地将自旋塞贝克效应的贡献与ANE分开，并观察每种效应对总响应的贡献程度。这些实验最终表明，ISHE和ANE在CoFeB是不同的起源独立的现象，可以共存于同一种材料中，对热梯度有相反的反应。
By studying the Hall effect in a series of low resistivity Ga1-xMnxAs samples, accurate values for the hole density p, Mn concentration x, and Curie temperature Tc are obtained over the range 0.015=<x=<0.08. The hole density corresponds to 90% of the Mn concentration at low x, and has a maximum value of 1.0x10-27 m-3 when Tc=125K for x=0.06. This data allows the first meaningful comparison of mean field predicted Curie temperatures with experiment over a wide range of x. The theory is in qualitative agreement with experiment, but overestimates Tc at large x and underestimates TC at low x.
We quantify the relative weight of inverse spin Hall and spin rectification effects occurring in RF-sputtered polycrystalline permalloy, molecular beam epitaxy-grown epitaxial iron and liquid phase epitaxy-grown yttrium-iron-garnet bilayer systems with different capping materials. To distinguish the spin rectification signal from the inverse spin Hall voltage the external magnetic field is rotated in-plane to take advantage of the different angular dependencies of the prevailing effects. We prove that in permalloy anisotropic magnetoresistance is the dominant source for spin rectification whil…
It is shown that magnetic forces as the Lorentz force, exerted on electric currents, and the force μDiv(B), exerted on electron spins at rest, account for both the transverse spin imbalance typical of spin Hall effect and the transverse charge imbalance associated with pure spin currents (inverse spin Hall effect). Considering that for stationary currents the laboratory reference frame and those for which the spin up and spin down carriers are at rest are inertial systems, one can easily find the forces exerted by the lattice on both spin sub-bands, as well as the force between sub-bands.
We report the observation of the crossover between the extrinsic and intrinsic spin Hall effect induced by alloying. We found that the spin Hall angle, the ratio of the spin Hall conductivity to the electric conductivity, changes drastically by tuning the composition of Au-Cu alloy. The spin Hall angle changes the sign only in a limited range of the Cu concentration due to the extrinsic skew scattering, while the intrinsic contribution becomes dominant with increasing the Cu concentration. This observation provides essential information for fundamental understanding of spin-orbit physics.
Understanding the evolution of spin-orbit torque (SOT) with increasing heavy-metal thickness in ferromagnet/normal metal (FM/NM) bilayers is critical for the development of magnetic memory based on SOT. However, several experiments have revealed an apparent discrepancy between damping enhancement and damping-like SOT regarding their dependence on NM thickness. Here, using linewidth and phase-resolved amplitude analysis of vector network analyzer ferromagnetic resonance (VNA-FMR) measurements, we simultaneously extract damping enhancement and both field-like and damping-like inverse SOT in Ni$_…
Dynamical antiferromagnets pump spins efficiently into adjacent conductors as ferromagnets. The high antiferromagnetic resonance frequencies represent a challenge for experimental detection, but magnetic fields can reduce these resonance frequencies. We compute the inverse spin Hall voltages resulting from dynamical spin excitations as a function of a magnetic field along the easy axis and the polarization of the driving AC magnetic field perpendicular to the easy axis. We consider the insulating antiferromagnets MnF$_2$, FeF$_2$, and NiO. Near the spin-flop transition, there is a significant …
The anomalous Hall effect (AHE) is studied on the surface of a 3D magnetic topological insulator. By applying a modified semi-classical framework, all three contributions to the AHE, the intrinsic Berry phase curvature effect, the side-jump effect and the skew scattering effects are systematically treated, and analytical expressions for the conductivities are obtained in terms of the Fermi level, the spatial orientation of the surface magnetization and the concentration of magnetic and non-magnetic impurities. We demonstrate that the AHE can change sign by altering the orientation of the surfa…
Among antiferromagnetic materials, Mn$_2$Au is one of the most intensively studied, and it serves as a very popular platform for testing various ideas related to antiferromagnetic magnetotransport and dynamics. Since recently, this material has also attracted considerable interest in the context of optical properties and optically-driven antiferromagnetic switching. In this work, we use first principles methods to explore the physics of charge photocurrents, spin photocurrents and inverse Faraday effect in antiferromagnetic Mn$_2$Au. We predict the symmetry and magnitude of these effects, and …
There exists considerable confusion in estimating the spin diffusion length of materials with high spin-orbit coupling from spin pumping experiments. For designing functional devices, it is important to determine the spin diffusion length with sufficient accuracy from experimental results. An inaccurate estimation of spin diffusion length also affects the estimation of other parameters (e.g., spin mixing conductance, spin Hall angle) concomitantly. The spin diffusion length for platinum (Pt) has been reported in literature in a wide range of 0.5 - 14 nm, and particularly it is a constant value…
