A single layer ferromagnetic film magnetized in the plane of an ac current flow, exhibits a characteristic Hall voltage with harmonic and second harmonic components, which is attributed to the presence of spin currents with polarization non-collinear with the magnetization. A set of 30 nm thick permalloy (Py) films used in this study are deposited at an oblique angle with respect to the substrate plane which induces an in-plane easy axis in the magnetization of the initial nucleating layers of the films which is distinct from the overall bulk magnetic properties of the film. This unusual magnetic texture provides a platform for the direct detection of inverse spin Hall effect in Hall bar shaped macroscopic devices at room temperatures which we denote as Anomalous Inverse Spin Hall Effect (AISHE). Control samples fabricated by normal deposition of permalloy with slow rotation of substrate shows significant reduction of the harmonic Hall signal that further substantiates the model. The analysis of the second harmonic Hall signal corroborates the presence of spin-orbit torque arising from the unconventional spin-currents in the single-layer ferromagnets.
In a topological insulator (TI)/magnetic insulator (MI) hetero-structure, large spin-orbit coupling of the TI and inversion symmetry breaking at the interface could foster non-planar spin textures such as skyrmions at the interface. This is observed as topological Hall effect in a conventional Hall set-up. While this effect has been observed at the interface of TI/MI, where MI beholds perpendicular magnetic anisotropy, non-trivial spin-textures that develop in interfacial MI with in-plane magnetic anisotropy is under-reported. In this work, we study Bi$_2$Te$_3$/EuS hetero-structure using plan…
Observation of Unconventional Ferroelectricity in Non-Moir'\e Graphene on Hexagonal Boron Nitride Boundaries and Interfaces
The University of Hong Kong（香港大学）；HK Institute of Quantum Science & Technology, The University of Hong Kong（香港大学量子科学与技术研究所）；National Institute for Materials Science（物质材料研究机构）
We investigate an interfacial spin-transfer torque and $β$-term torque with alternating current (AC) parallel to a magnetic interface. We find that both torques are resonantly enhanced as the AC frequency approaches to the exchange splitting energy. We show that this resonance allows us to estimate directly the interfacial exchange interaction strength from the domain wall motion. We also find that the $β$-term includes an unconventional contribution which is proportional to the time derivative of the current and exists even in absence of any spin relaxation processes.
Interfacial Noncollinear Filtering of Spin Hall Currents
Key Laboratory of Materials Physics, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences（中国科学院合肥物质科学研究院固体物理研究所材料物理重点实验室）；University of Science and Technology of China（中国科学技术大学）；School of Physics, Nankai University（南开大学物理学院）；Tsung-Dao Lee Institute, Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), School of Physics and Astronomy, Shanghai Jiao Tong University（上海交通大学物理与天文学院、人工结构量子控制教育部重点实验室、李政道研究所）；MOE Key Laboratory for Nonequilibrium Synthesis and Modulation of Condensed Matter, Shaanxi Province Key Laboratory of Quantum Information and Quantum Optoelectronic Devices, School of Physics, Xi’an Jiaotong University（西安交通大学物理学院、陕西省量子信息与光电子器件重点实验室、非平衡合成与调控凝聚态物质教育部重点实验室）；Anhui Province Key Laboratory of Low-Energy Quantum Materials and Devices, High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences（中国科学院合肥物质科学研究院强磁场科学中心安徽省低能量子材料与器件重点实验室）；Collaborative Innovation Center of Microstructures, Nanjing University（南京大学微观结构协同创新中心）
The anomalous Hall effect (AHE) is a quantum coherent transport phenomenon that conventionally vanishes at elevated temperatures because of thermal dephasing. Therefore, it is puzzling that the AHE can survive in heavy metal (HM)/antiferromagnetic (AFM) insulator (AFMI) heterostructures at high temperatures yet disappears at low temperatures. In this paper, we report that an unconventional high-temperature AHE in HM/AFMI is observed only around the Néel temperature of AFM, with large anomalous Hall resistivity up to 40 n$Ω$ cm. This mechanism is attributed to the emergence of a noncollinear AF…
Orbital Hybridization-Induced Ising-Type Superconductivity in a Confined Gallium Layer
The Pennsylvania State University（宾夕法尼亚州立大学）；Shanghai Jiao Tong University（上海交通大学）；University of Oxford（牛津大学）；Zhejiang University（浙江大学）；Diamond Light Source（钻石光源研究所）；University of North Texas（北德克萨斯大学）
We study inserting Co layer thickness-dependent spin transport and spin-orbit torques (SOTs) in the Pt/Co/Py trilayers by spin-torque ferromagnetic resonance. The interfacial perpendicular magnetic anisotropy energy density ($K_s = 2.7~erg/cm^2$), which is dominated by interfacial spin-orbit coupling (ISOC) in the Pt/Co interface, total effective spin-mixing conductance ($G_{eff,tot} = 0.42 {\times} 10^{15}~Ω^{-1} m^{-2}$) and two-magnon scattering ($β_{TMS} = 0.46~nm^2$) are first characterized, and the damping-like torque ($ξ_{DL}$ = 0.103) and field-like torque ($ξ_{FL}$ = -0.017) efficienc…
Heavy metal/ferromagnet interfaces feature emergent spin-orbit effects absent in the bulk materials. Because of their inherent strong coupling between spin, charge and orbital degrees of freedom, such systems provide a platform for technologically sought-after spin-orbit torques (SOTs). However, the microscopic origin of purely interfacial antidamping SOT, especially in the ultimate atomically thin limit, has proven elusive. Here, using two-dimensional (2D) van der Waals materials as a testbed for interfacial phenomena, we address this problem by means of a microscopic framework accounting for…
Superconductivity and magnetism are generally incompatible because of the opposing requirement on electron spin alignment. When combined, they produce a multitude of fascinating phenomena, including unconventional superconductivity and topological superconductivity. The emergence of two-dimensional (2D)layered superconducting and magnetic materials that can form nanoscale junctions with atomically sharp interfaces presents an ideal laboratory to explore new phenomena from coexisting superconductivity and magnetic ordering. Here we report tunneling spectroscopy under an in-plane magnetic field …
The static and dynamic properties of skyrmions have recently received increased attention due to the potential application of skyrmions as information carriers and for unconventional computing. While the current-driven dynamics has been explored deeply, both theoretically and experimentally, the theory of temperature gradient-induced dynamics - Skyrmion-Caloritronics - is still at its early stages of development. Here, we move the topic forward by identifying the role of entropic torques due to the temperature dependence of magnetic parameters. Our results show that, skyrmions move towards hig…
Topological spin textures in an itinerant ferromagnet, SrRuO$_3$ is studied combining Hall transport measurements and numerical simulations. We observe characteristic signatures of the Topological Hall Effect associated with skyrmions. A relatively large thickness of our films and absence of heavy metal layers make the interfacial Dzyaloshinskii-Moriya interaction an unlikely source of these topological spin textures. Additionally, the transport anomalies exhibit an unprecedented robustness to magnetic field tilting and temperature. Our numerical simulations suggest that this unconventional be…
In a bilayer consisting of an insulator (I) and a ferromagnetic metal (FM), interfacial spin orbit scattering leads to spin mixing of the two conducting channels of the FM, which results in an unconventional anisotropic magnetoresistance (AMR). We theoretically investigate the magnetotransport in such bilayer structures by solving the spinor Boltzmann transport equation with generalized Fuchs-Sondheimer boundary condition that takes into account the effect of spin orbit scattering at the interface. We find that the new AMR exhibits a peculiar angular dependence which can serve as a genuine exp…
In spintronics applications, ultrafast spin dynamics have to be controlled at femtosecond (fs) timescales via fs-laser radiation. At such ultrafast timescales, the effect of the Gilbert damping factor α on ultrafast demagnetization time should be considered. In previous explorations for the relationship between these two parameters, it was found that the theoretical calculations based on the local spin-flip scattering model do not agree with the experimental results. Here, we find that in Fe81Ga19(FeGa)/Ir20Mn80(IrMn) bilayers, the unconventional IrMn thickness dependence of α results from the…
Large Field-Free Superconducting Diode Effect with Nonmonotonic Polarity Reversals in NbSe$_2$/CrBr$_3$ Heterostructures
Southern University of Science and Technology（南方科技大学）；International Quantum Academy, and Shenzhen Branch, Hefei National Laboratory（国际量子科学院，合肥国家实验室深圳分院）；Eastern Institute for Advanced Study, Eastern Institute of Technology（宁波东方理工大学（暂名）先进研究院）；State Key Laboratory of Optoelectronic Materials and Technologies, Sun Yat‑sen University（中山大学光电信息材料与技术国家重点实验室）
