A high repetition rate, picosecond THz parametric amplifier (TPA) with a LiNbO3 (LN) crystal has been demonstrated in this work. At 10 kHz repetition rate, a peak power of 200 W and an average power of 12 μW have been obtained over a wide range around 2 THz; at 100 kHz repetition rate, a maximum peak power of 18 W and average power of 10.8 μW have been obtained. The parametric gain of the LN crystal was also investigated and a modified Schwarz-Maier model was introduced to interpret the experimental results.
We theoretically and experimentally demonstrate a new electro-optic linear approach to generate high repetition-rate picosecond pulse trains. This simple cavity-free method is based on a temporal sinusoidal phase modulation combined with a triangular spectral phase processing. Experimental results validate the concept at repetition rates ranging from 10 GHz up to 40 GHz with the generation of background-free pulse trains made of nearly Gaussian Fourier-transform limited pulses.
We demonstrate the operation of an ultra low repetition rate, high peak power, picosecond diode pumped Nd:YVO4 passively mode locked laser oscillator. Repetition rates even below 1 MHz were achieved with the use of a new design multiple-pass cavity and a semiconductor saturable absorber. Long term stable operation at 1.2 MHz, pulse duration of 16.3 ps and average output power of 470 mW corresponding to 24 KW peak power pulses is reported. This is, to our knowledge, the lowest repetition rate high peak power pulses ever generated directly from a picosecond laser resonator without cavity dumping…
Here, we demonstrate all-fiber direct amplification of 11 picosecond pulses from a gain-switched laser diode at 1063nm. The diode was driven at a repetition rate of 40MHz and delivered 13$μ$W of fiber-coupled average output power. For the low output pulse energy of 0.33pJ we have designed a multi-stage core pumped preamplifier based on single clad Yb-doped fibers in order to keep the contribution of undesired amplified spontaneous emission as low as possible and to minimize temporal and spectral broadening. After the preamplifier we reduced the 40MHz repetition rate to 1MHz using a fiber coupl…
We experimentally demonstrate intensity amplification of repetitive picosecond optical pulses with an input-to-output gain up to 5.5 dB using a passive Talbot amplifier. Through the dispersion-induced temporal Talbot effect, the amplifier uses electro-optic phase modulation and a low-loss dispersive medium to exploit and coherently redistribute the energy of the original pulse train into fewer, replica, amplified pulses. In addition, we show how our passive amplifier mitigates the pulse train timing-jitter and pulse-to-pulse intensity fluctuations above a specific cutoff frequency.
We present a Ho:YLF Chirped-Pulse Amplification (CPA) laser for pumping a longwave infrared Optical Parametric Chirped Pulse Amplifier (OPCPA) at a 1 kHz repetition rate. By utilizing a Ti:Sapphire laser as a frontend, 5-μJ seed pulses at 2051 nm laser pulse are generated in a Dual-Chirp Optical Parametric Amplifier (DC-OPA), which are amplified to 28 mJ pulses with a pulse duration of 6.8 ps. The scheme offers a potential driver for two-color (800 nm and 8 μm) high harmonic generation with an increased keV X-ray photon flux.
We demonstrated all-fiber amplification of 11 ps pulses from a gain-switched laser diode at 1064 nm. The diode was driven at a repetition rate of 40 MHz and delivered 13 $μ$W of fiber-coupled average output power. For the low output pulse energy of 325 fJ we have designed a multi-stage core pumped pre-amplifier in order to keep the contribution of undesired amplified spontaneous emission as low as possible. By using a novel time-domain approach for determining the power spectral density ratio (PSD) of signal to noise, we identified the optimal working point for our pre-amplifier. After the pre…
We report on the generation of a train of ~ 2 ps, 10 um laser pulses via multiple four-wave mixing and compression of an infrared laser beat-wave propagating in the negative group velocity dispersion region of bulk GaAs and a combination of GaAs and NaCl. The use of a 200 ps, 106 GHz beat-wave, produced by combining laser pulses amplified on the 10P(20) and 10P(16) transition of a CO2 laser, provides a novel method for generating high-power, picosecond, mid-IR laser pulses at a high repetition rate. By using 165 and 882 GHz beat-waves we show that cascaded phase-mismatched difference frequency…
We demonstrate a compact source of energetic and phase-locked multi-terahertz pulses at a repetition rate of 190 kHz. Difference frequency mixing of the fundamental output of an Yb:KGW amplifier with the idler of an optical parametric amplifier in GaSe and LiGaS2 crystals yields a passively phase-locked train of waveforms tunable between 12 and 42 THz. The shortest multi-terahertz pulses contain 1.8 oscillation cycles within the intensity FWHM. Pulse energies of up to 0.16 μJ and peak electric fields of 13 MV/cm are achieved. Electro-optic sampling reveals a phase stability better than 0.1 $π$…
This paper reports the study and demonstration of a new variable temporal shaping method capable of generating linearly polarized picosecond laser pulses with arbitrary predefined shapes, which are highly desired by various applications including low emittance high brightness electron bunch generation in photocathode guns. It is found that both high transmittance and high stability of the shaped pulses can be achieved simultaneously when birefringent stages (BSs) are set at specific phase delay. Such variable temporal shaping technique may lead to new opportunities for many potential applicati…
We report the study and demonstration of a new laser pulse shaping system capable of generating linearly polarized picosecond laser pulses with variable temporal profiles including symmetric intensity distributions such as parabolic, flattop, elliptical, triangular, as well as non-symmetric distributions, which are highly desired by various applications. It is found that both high transmittance and high stability of the shaped pulse can be achieved simultaneously when crystals are set at a specific phase delay through fine control of the crystal temperature. Although multi-crystal pulse stacki…
Optical pump-probe spectroscopy is a powerful tool to directly probe the carrier dynamics in materials down to sub-femtosecond resolution. To perform such measurement, while keeping the pump induced perturbation to the sample as small as possible, it is essential to have a detection scheme with high signal to noise ratio. Achieving such high signal to noise ratio is easy with phase sensitive detection based on lock-in-amplifier when a high repetition rate laser is used as the optical pulse source. However such a lock-in-amplifier based method does not work well when a low repetition rate laser…
The output of a 200 kHz, 34 W, 300 fs Yb amplifier is compressed to 31 fs with > 88 % efficiency to reach a peak power of 2.5 GW, which to date is a record for a single-stage bulk multi-pass cell. Despite operation 80 times above the critical power for self-focusing in bulk material, the setup demonstrates excellent preservation of the input beam quality. Extensive beam and pulse characterizations are performed to show that the compressed pulses are promising drivers for high harmonic generation and nonlinear optics in gases or solids.
We demonstrate THz generation using the tilted pulse front method in Lithium Niobate, driven at unprecedented high average power of more than 100 W and at 13.3 MHz repetition rate, provided by a compact amplifier-free modelocked thin-disk oscillator. The conversion efficiency was optimized with respect to pump spot size and pump pulse duration, enabling us to generate a maximum THz average power of 66 mW, which is the highest reported to date from a laser-driven, few-cycle THz source. Furthermore, we identify beam walk-off as the main obstacle that currently limits the conversion efficiency in…
We present a comprehensive study of laser pulse amplification with respect to operation regimes, gain dynamics, and highly stable operation points of Ho:YLF regenerative amplifiers (RAs). The findings are expected to be more generic than for this specific case. Operation regimes are distinguished with respect to pulse energy and the appearance of pulse instability, and are studied as a function of the repetition rate, seed energy, and pump intensity. The corresponding gain dynamics are presented, identifying highly stable operation points related to high gain build -up during pumping and high …
We report on the design and whole characterization of low-noise and affordable-cost Yb-doped double-clad fiber amplifiers operating at room temperature in the near-infrared spectral region at pulse repetition rate of 160 MHz. Two different experimental configurations are discussed. In the first one, a broadband seed radiation with a transform limited pulse duration of 71 fs, an optical spectrum of 20 nm wide at around 1040 nm, and 20 mW average power is adopted. In the second configuration, the seed radiation is constituted by stretched pulses with a time duration as long as 170 ps, with a 5-n…
Sub 100-fs, 5.2-$μ$m ZGP Parametric Amplifier Driven by a ps Ho:YAG Chirped Pulse Amplifier and its application to high harmonic generation
Vienna University of Technology（维也纳工业大学）；The University of Tokyo（东京大学）；Menlo Systems GmbH（Menlo Systems有限公司）；University of Erlangen-Nuremberg（埃尔朗根-纽伦堡大学）；Center for Physical Sciences & Technology（物理科学和技术中心）
We demonstrate an all-fiber mode-locked laser at all-normal dispersion with a saturable absorber, which is based on a section of grade-index multimode fiber with inner microcavity embedded in the splice points. The absorption modulation depth of this nonlinear saturable absorber is 2.2% in the suitable bent state. The fiber laser operates at central wavelength of 1035nm with average power of ~1.26mW, pulse-duration of 17.05 ps, repetition rate of 37.098MHz. This kind of saturable absorber has superiorities of low cost, high stability and high damage threshold, which may facilitate applications…
The Free-Electron Laser (FEL) FLASH offers the worldwide still unique capability to study ultrafast processes with high-flux, high-repetition rate XUV and soft X-ray pulses. The vast majority of experiments at FLASH are of pump-probe type. Many of them rely on optical ultrafast lasers. Here, a novel FEL facility laser is reported which combines high average power output from Yb:YAG amplifiers with spectral broadening in a Herriott-type multi-pass cell and subsequent pulse compression to sub-100 fs durations. Compared to other facility lasers employing optical parametric amplification, the new …
We demonstrate a single-stage, multipass Ti:sapphire amplifier capable of delivering sub-13 fs, 3.2 mJ pulses at 1 kHz repetition rate. Gaussian filters are used to suppress the gain-narrowing effect, thereby enabling the achievement of an ultrabroadband flat-top spectrum with a FWHM > 130 nm. The carrier-envelope phase (CEP) of the output pulses is actively stabilized via the feed-forward scheme (for the oscillator) and a fast 1 kHz f-to-2f interferometer, which corrects the amplifier-induced CEP drift. The single-shot 75 h CEP measurement yielded rms noise of <150 mrad.
A tapered semiconductor amplifier is injection seeded by a femtosecond optical frequency comb at 780 nm from a mode-locked Ti:sapphire laser. Energy gains over 17 dB (12 dB) are obtained for 1 mW (20 mW) of average input power when the input pulses are stretched into the picosecond range. A spectral window of supercontinuum light generated in a photonic fiber has also been amplified. Interferometric measurements show sub-hertz linewidths for a heterodyne beat between the input and amplified comb components, yielding no detectable phase-noise degradation under amplification. These amplifiers ca…
Lasers capable of generating attosecond X-ray pulses in the water window (282 to 533 eV) through high-order harmonic generation are normally based on inefficient, multi-stage optical parametric amplifiers or optical parametric chirped pulse amplifiers pumped by femtosecond or picosecond lasers. Here we report a very efficient single amplification stage laser based on traditional chirped pulse amplification capable of producing 3 mJ, near-transform limited 44 fs (<6 cycles), 1 kHz pulses centered at 2.5 micrometer. The 68 GW peak power is the highest value ever reached at this wavelength. In or…
Ultrafast optical Kerr Gate at 1 GHz repetition rate by focusing on BBS glass
University of Siegen（锡根大学）；Alfred University（阿尔弗雷德大学）；European Laboratory for Non-Linear Spectroscopy（欧洲非线性光谱学实验室）；Università di Parma（帕尔马大学）；Istituto Nazionale di Ottica (INO), Consiglio Nazionale delle Ricerche (CNR)（意大利国家光学研究所，意大利国家研究委员会）
We present a comprehensive model for predicting the full performance of a second harmonic generationoptical parametric amplification system that aims at enhancing the temporal contrast of laser pulses. The model simultaneously takes into account all the main parameters at play in the system such as the group velocity mismatch, the beam divergence, the spectral content, the pump depletion, and the length of the nonlinear crystals. We monitor the influence of the initial parameters of the input pulse and the interdependence of the two related non-linear processes on the performance of the system…
Manipulating the atomic and electronic structure of matter with strong terahertz (THz) fields while probing the response with ultrafast pulses at x-ray free electron lasers (FELs) has offered unique insights into a multitude of physical phenomena in solid state and atomic physics. Recent upgrades of x-ray FEL facilities are pushing to much higher repetition rates, enabling unprecedented signal to noise for pump probe experiments. This requires the development of suitable THz pump sources that are able to deliver intense pulses at compatible repetition rates. Here we present a high power laser-…
We present the first direct observation of the bound state of multiple dissipative optical solitons in which bond length and bond strength can be individually controlled in a broad range in a regular manner. We have observed experimentally a new type of stable and extremely elastic soliton crystals that can be stretched and compressed many times conserving their structure by adjusting the bond properties in real time in a specially designed passively mode-locked fiber laser incorporating highly asymmetric tunable Mach-Zehnder interferometer. The temporal structure and dynamics of the generated…
The thermal lensing effects in the lasing crystal appear to be dominant when the pump laser focused on the lasing crystal which causes the local heating effect. The spatial refractive index variations observed if the crystal has non-uniform temperature distribution. In the present study, the demonstration of thermal lensing effect of Brewster-cut Ti: Sapphire crystal carried out when pumped by 25 ps pulses at 80 MHz repetition rate with 532 nm central wavelength, while the average pump power controlled by the attenuator. The thermal lensing effects measured first at the ~293 K temperature and …
We report on a multi-mJ 2.1-$μ$m OPCPA system operating at a 1-kHz repetition rate, pumped by a picosecond cryogenic Yb:YAG pump laser, and the phase-matched high-flux high-harmonic soft X-ray generation.
An optical parametric chirped pulse amplifier fully based on Yb lasers at 500 kHz is described. Passive optical-synchronization is achieved between a fiber laser-pumped white-light and a 515 nm pump produced with a 200 W picosecond Yb:YAG InnoSlab amplifier. An output power up to 19.7 W with long-term stability of 0.3% is demonstrated for wavelength tunable pulses between 680 nm and 900 nm and spectral stability of 0.2%; 16.5 W can be achieved with a bandwidth supporting 5.4 fs pulses. We demonstrate compression of 30 microjoule pulses to sub-20 fs duration with a prism compressor, suitable fo…
A power enhancement optical cavity is a compelling means of realizing a pulsed laser with a high peak power and high repetition frequency, which is not feasible using a simple amplifier scheme. However, a precise feedback system is necessary for maintaining the narrow resonance condition of the optical cavity; this has become a major technical issue in developing such cavities. We have developed a new approach that does not require any active feedback system, by placing the cavity in the outer loop of a laser amplifier. We report on the first demonstration of a mode-locked pulse oscillation us…
Coherent soft x-ray (SXR) sources enable fundamental studies in the important water window spectral region. Until now, such sources have been limited to repetition rates of 1 kHz or less, which limits count rates and signal-to-noise ratio for a variety of experiments. SXR generation at high repetition rate has remained challenging because of the missing high-power mid-infrared (mid-IR) laser sources to drive the high-harmonic generation (HHG) process. Here we present a mid-IR optical parametric chirped pulse amplifier (OPCPA) centered at a wavelength of 2.2 μm and generating 16.5-fs pulses (2.…
Time-resolved femtosecond stimulated Raman spectroscopy (FSRS) is a powerful tool for investigating ultrafast structural and vibrational dynamics in light absorbing systems. However, the technique generally requires exposing a sample to high laser pulse fluences and long acquisition times to achieve adequate signal-to-noise ratios. Here, we describe a timeresolved FSRS instrument built around a Yb ultrafast amplifier operating at 200 kHz, and address some of the unique challenges that arise at high repetition-rates. The setup includes detection with a 9 kHz CMOS camera and an improved dual-cho…
Characterizing and controlling electronic properties of quantum materials require direct measurements of non-equilibrium electronic band structures over large regions of momentum space. Here, we demonstrate an experimental apparatus for time- and angle-resolved photoemission spectroscopy using high-order harmonic probe pulses generated by a robust, moderately high power (20 W) Yb:KGW amplifier with tunable repetition rate between 50 and 150 kHz. By driving high-order harmonic generation (HHG) with the second harmonic of the fundamental 1025 nm laser pulses, we show that single-harmonic probe p…
We present a 2-\mum frequency comb based on a reliable mode-locked Er:fiber laser with 100 MHz repetition rate. After shifting the spectrum of the amplified Er:fiber comb to longer wavelengths, a single-clad Tm/Ho:fiber is used as a self-pumped pre-amplifier to generate a coherent and broadband spectrum centered at 1.93 \mum. Subsequently, a cladding-pumped Tm:fiber amplifier boosts the system to a maximum output power of 4.8 W at 1.96 \mum. After compression in a compact grating compressor, our amplified Er:fiber/Tm:fiber hybrid system delivers as much as 2.9 W with a pulse duration of 141 fs…
Picosecond Schrödinger cat states for ultrafast optical quantum processing
The University of Tokyo（东京大学）；RIKEN Center for Quantum Computing（理化学研究所量子计算研究中心）；OptQC Inc.（OptQC公司）；National Institute of Advanced Industrial Science and Technology（国立研究开发法人产业技术综合研究所）；NTT Inc.（日本电信电话株式会社）；Johannes Gutenberg-Universität Mainz（美因茨约翰内斯·古腾堡大学）
A femtosecond frequency-doubled Erbium-doped fiber laser with adjustable pulse repetition rate is developed and applied in two-photon excited fluorescence microscopy. The all-fiber laser system provides the fundamental pulse at 1560 nm wavelength with 22 fs duration for the second harmonic generation, resulting in 1.35 nJ, 60 fs pulses at 780 nm. The repetition rate is adjusted by a pulse picker unit built-in within the amplifier chain, directly providing transform-limited pulses for any chosen repetition rate between 1 and 12 MHz. We employed the laser source to drive a scanning two-photon ex…
A Portable Optical Frequency Comb with Low Repetition-Rate Drift Based on "Optical Cubes"
Institute of Quantum Electronics, School of Electronics, Peking University（北京大学电子工程学院量子电子学研究所）；Tianjin Key Laboratory of Quantum Precision Measurement Technology（天津量子精密测量技术重点实验室）；China Quantum Measurement Tek Co., Ltd.（中国量子测量科技有限公司）；Hefei National Laboratory（合肥国家实验室）
Supercontinuum generation in optical fibers is one of the most dramatic nonlinear effects discovered, allowing short pulses to be converted into multi-octave spanning coherent spectra. However, generating supercontinua that are both coherent and broadband requires pulses that are simultaneously ultrashort with high peak power. This results in a reducing efficiency with increasing pulse repetition rate, that has hindered supercontinua at microwave line spacing, i.e. 10s of GHz. Soliton microcombs by contrast, can generate octave-spanning spectra, but with good conversion efficiency only at vast…
