We report a continuous phase transition between quantum-anomalous-Hall and trivial-insulator phases in a magnetic topological insulator upon magnetization rotation. The Hall conductivity transits from one plateau of quantized Hall conductivity $e^2/h$ to the other plateau of zero Hall conductivity. The transition curves taken at various temperatures cross almost at a single point, exemplifying the critical behavior of the transition. The slope of the transition curves follows a power-law temperature dependence with a critical exponent of $-0.61$. This suggests a common underlying origin in the plateau transitions between the QAH and quantum Hall systems, which is a percolation of one-dimensional chiral edge channels.
Using the Green functions method we study transport properties of surface electrons in topological insulators in the presence of a correlated random exchange field. Such an exchange field may be due to random magnetization with correlated fluctuations. We determine the relaxation time due to scattering from the magnetization fluctuations and from other structural defects. Then we calculate the longitudinal charge conductivity taking into account the contribution due to vertex correction.
The magnetoelectric effect predicted in topological insulators makes heterostructures that combine magnetic materials and such insulators promising candidates for spintronics applications. Here, we theoretically consider a setup that exhibits two well-separated interfaces between a topological insulator and a ferromagnetic insulator. We show that there is a topological magnetic dipole-dipole interaction stemming from long-range Coulomb interactions. We analytically derive the magnetization dynamics at the two interfaces and discuss how the long-range coupling can be applied to non-locally indu…
Spin-orbit torque (SOT) magnetization switching of ferromagnets with large perpendicular magnetic anisotropy has a great potential for the next-generation non-volatile magnetoresistive random-access memory (MRAM). It requires a high-performance pure spin current source with a large spin Hall angle and high electrical conductivity, which can be fabricated by a mass production technique. In this work, we demonstrate ultrahigh efficient and robust SOT magnetization switching in all-sputtered BiSb topological insulator - perpendicularly magnetized Co/Pt multilayers. Despite fabricated by the indus…
Topological insulators (TIs) with spin momentum locked topological surface states (TSS) are expected to exhibit a giant spin-orbit torque (SOT) in the TI/ferromagnet systems. To date, the TI SOT driven magnetization switching is solely reported in a Cr doped TI at 1.9 K. Here, we directly show giant SOT driven magnetization switching in a Bi2Se3/NiFe heterostructure at room temperature captured using a magneto-optic Kerr effect microscope. We identify a large charge to spin conversion efficiency of ~1-1.75 in the thin TI films, where the TSS is dominant. In addition, we find the current densit…
Graphene multilayers with flat moiré minibands can exhibit the quantized anomalous Hall effect due to the combined influence of spontaneous valley polarization and topologically non-trival valley-projected bands. The sign of the Hall effect in these Chern insulators can be reversed either by applying an external magnetic field, or by driving a transport current through the system. We propose a current-driven mechanism whereby reversal occurs along lines in the (current $I$, magnetic-field $B$) control parameter space with slope $dI/dB = (e/h)\, M A_{M} \, (1-γ^2)/γ$, where $M$ is the magnetiza…
The origins of the spin-orbit torque (SOT) at ferromagnet/topological insulator (FM/TI) interfaces are incompletely understood. Theory has overwhelmingly focussed on the Edelstein effect due to the surface states in the presence of a scalar scattering potential. We investigate here the contribution to the SOT due to extrinsic spin-orbit scattering of the surface states, focusing on the case of an out-of-plane magnetization. We show that spin-orbit scattering brings about a sizable renormalization of the field-like SOT, which exceeds 20$\%$ at larger strengths of the extrinsic spin-orbit parame…
Recently, the intrinsic magnetic topological insulator MnBi2Te4 has attracted enormous research interest due to the great success in realizing exotic topological quantum states, such as the quantum anomalous Hall effect (QAHE), axion insulator state, high-Chern-number and high-temperature Chern insulator states. One key issue in this field is to effectively manipulate these states and control topological phase transitions. Here, by systematic angle-dependent transport measurements, we reveal a magnetization-tuned topological quantum phase transition from Chern insulator to magnetic insulator w…
Established forms of electromagnetic coupling are usually conservative (in insulators) or dissipative (in metals and semiconductors). Here we point out the possibility of nondissipative electric driving of magnetization dynamics, if the valence electronic states have nontrivial topology in the combined space of crystal momentum and magnetization configuration. We provide a hybrid insulator system to demonstrate that the topology-based nonconservative electrical generalized force is capable of supporting sustained magnetization motion in the presence of Gilbert damping, with quantized and stead…
Precise estimation of spin Hall angle as well as successful maximization of spin-orbit torque (SOT) form a basis of electronic control of magnetic properties with spintronic functionality. Until now, current-nonlinear Hall effect, or second harmonic Hall voltage has been utilized as one of the methods for estimating spin Hall angle, which is attributed to the magnetization oscillation by SOT. Here, we argue the second harmonic Hall voltage in magnetic/nonmagnetic topological insulator (TI) heterostructures, Cr$_x$(Bi$_{1-y}$Sb$_y$)$_{2-x}$Te$_3$/(Bi$_{1-y}$Sb$_y$)$_2$Te$_3$. From the angular, …
We study the dynamics of spin valves consisting of two layers of magnetic insulators separated by a normal metal in the macrospin model. A current through the spacer generates a spin Hall current that can actuate the magnetization via the spin-transfer torque. We derive expressions for the effective Gilbert damping and the critical currents for the onset of magnetization dynamics including the effects of spin pumping that can be tested by ferromagnetic resonance experiments. The current generates an amplitude asymmetry between the in-phase and out-of-phase modes. We briefly discuss superlattic…
Electric-field control of magnetization dynamics is fundamentally and technologically important for future spintronic devices. Here, based on electric-field control of both magnetic anisotropy and spin--orbit torque, two distinct methods are presented for switching the magnetization in topological insulator (TI)/magnetic-TI hybrid systems. The magnetic anisotropy energy in magnetic TIs is formulated analytically as a function of the Fermi energy, and it is confirmed that the out-of-plane magnetization is always favored for the partially occupied surface band. Also proposed is a transistor-like…
We study the interaction between a ferromagnetically ordered medium and the surface states of a topological insulator with a general surface termination. This interaction is strongly crystal face dependent and can generate chiral states along edges between crystal facets even for a uniform magnetization. While magnetization parallel to quintuple layers shifts the momentum of Dirac point, perpendicular magnetization lifts the Kramers degeneracy at any Dirac points except on the side face where the spectrum remains gapless and the Hall conductivity switches sign. Chiral states can be found at an…
We theoretically study the spin and charge generation along with the electron transport on a disordered surface of a doped three-dimensional topological insulator/magnetic insulator junction by using Green's function techniques. We find that the spin and charge current are induced by not only local but also nonlocal magnetization dynamics through nonmagnetic impurity scattering on the disordered surface of the doped topological insulator. We also clarify that the spin current as well as charge density are induced by spatially inhomogeneous magnetization dynamics, and the spin current diffusive…
We study dynamics of the magnetization coupled to the surface Dirac fermions of a three di- mensional topological insulator. By solving the Landau-Lifshitz-Gilbert equation in the presence of charge current, we find current induced magnetization dynamics and discuss the possibility of mag- netization reversal. The torque from the current injection depends on the transmission probability through the ferromagnet and shows nontrivial dependence on the exchange coupling. The mag- netization dynamics is a direct manifestation of the inverse spin-galvanic effect and hence another ferromagnet is unne…
We study supercurrent and proximity vortices in a Josephson junction made of disordered surface states of a three-dimensional topological insulator with a proximity induced in-plane helical magnetization. In a regime where the rotation period of helical magnetization is larger than the junction width, we find supercurrent 0-π crossovers as a function of junction thickness, magnetization strength, and parameters inherent to the helical modulation and surface states. The supercurrent reversals are associated with proximity induced vortices, nucleated along the junction width, where the number of…
The spin-torque ferromagnetic resonance (ST-FMR) in a bilayer system consisting of a magnetic insulator such as Y3Fe5O12 and a normal metal with spin-orbit interaction such as Pt is addressed theoretically. We model the ST-FMR for all magnetization directions and in the presence of field-like spin-orbit torques based on the drift-diffusion spin model and quantum mechanical boundary conditions. ST-FMR experiments may expose crucial information about the spin-orbit coupling between currents and magnetization in the bilayers.
We report the observation of efficient charge-to-spin conversion in the three-dimensional topological insulator (TI) Bi2Se3 and Ag bilayer by the spin-torque ferromagnetic resonance technique. The spin orbit torque ratio in the Bi2Se3/Ag/CoFeB heterostructure shows a significant enhancement as the Ag thickness increases to ~2 nm and reaches a value of 0.5 for 5 nm Ag, which is ~3 times higher than that of Bi2Se3/CoFeB at room temperature. The observation reveals the interfacial effect of Bi2Se3/Ag exceeds that of the topological surface states (TSS) in the Bi2Se3 layer and plays a dominant rol…
We uncover a new family of few-body topological phases in periodically driven fermionic systems in two dimensions. These phases, which we term correlation-induced anomalous Floquet insulators (CIAFIs), are characterized by quantized contributions to the bulk magnetization from multi-particle correlations, and are classified by a family of integer-valued topological invariants. The CIAFI phases do not require many-body localization, but arise in the generic situation of k-particle localization, where the system is localized (due to disorder) for any finite number of particles up to a maximum nu…
We theoretically study the magnetization dynamics of a thin ferromagnetic film exchange-coupled with a surface of a strong three-dimensional topological insulator. We focus on the role of electronic zero modes imprinted by domain walls (DW's) or other topological textures in the magnetic film. Thermodynamically reciprocal hydrodynamic equations of motion are derived for the DW responding to electronic spin torques, on the one hand, and fictitious electromotive forces in the electronic chiral mode fomented by the DW, on the other. An experimental realization illustrating this physics is propose…
We theoretically study the magnetoresistance (MR) of two-dimensional massless Dirac electrons as found on the surface of three-dimensional topological insulators (3D TIs) that is capped by a ferromagnetic insulator (FI). We calculate charge and spin transport by Kubo and Boltzmann theories, taking into account the ladder-vertex correction and the in-scattering due to normal and magnetic disorder. The induced exchange splitting is found to generate an electric conductivity that depends on the magnetization orientation, but its form is very different from both the anisotropic and spin Hall MR. T…
We study the magnetoelectric coupling at the surface of a topological insulator. We are in particular interested in the surface current induced by a static Zeeman/exchange field. This surface current can be related to the orbital magnetization of the system. For an insulator with zero Chern number, the orbital magnetization is independent of the details at the boundary. With the appearance of surface states in the topological insulator, it is not immediately obvious if the response is not affected by the conditions at the surface. We investigate this question using exact diagonalization to a l…
The orbital magnetic moment of a finite piece of matter is expressed in terms of the one-body density matrix as a simple trace. We address a macroscopic system, insulating in the bulk, and we show that its orbital moment is the sum of a bulk term and a surface term, both extensive. The latter only occurs when the transverse conductivity is nonzero and owes to conducting surface states. Simulations on a model Hamiltonian validate our theory.
An approach to the electrostatic control of $90^{\circ}$ magnetization rotation in the hybrid structures composed of topological insulators (TIs) and adjacent ferromagnetic insulators (FMI) is proposed and studied. The concept is based on TI electron energy variation with in-plane to put-of plane FMI magnetization turn. The calculations explicitly expose the effect of free energy variability in the form of the electrically controlled uniaxial magnetic anisotropy, which depends on proximate exchange interaction and TI surface electron density. Combining with inherent anisotropy, the magnetizati…
The anomalous Hall effect (AHE) is studied on the surface of a 3D magnetic topological insulator. By applying a modified semi-classical framework, all three contributions to the AHE, the intrinsic Berry phase curvature effect, the side-jump effect and the skew scattering effects are systematically treated, and analytical expressions for the conductivities are obtained in terms of the Fermi level, the spatial orientation of the surface magnetization and the concentration of magnetic and non-magnetic impurities. We demonstrate that the AHE can change sign by altering the orientation of the surfa…
We present the second-order phase transition from a band insulator to metal that is induced by a strong magnetic field. The magnetic-field dependences of the magnetization and energy band gap of a crystalline silicon immersed in a magnetic field are investigated by means of the nonperturbative magnetic-field-containing relativistic tight-binding approximation method [Phys. Rev. B 97, 195135 (2018)]. It is shown that the energy band gap disappears at the critical magnetic field of 2.22x$10^4$ (T). At the critical magnetic field, the magnetic-field dependence of the magnetization exhibits a kink…
Strong dependence of the Josephson energy on the magnetization orientation in Josephson junctions with ferromagnetic interlayers and spin-orbit coupling opens a way to control magnetization by Josephson current or Josephson phase. Here we investigate the perspectives of magnetization control in superconductor/ferromagnet/superconductor (S/F/S) Josephson junctions on the surface of a 3D topological insulator hosting Dirac quasiparticles. Due to the spin-momentum locking of these Dirac quasiparticles a strong dependence of the Josephson current-phase relation on the magnetization orientation is …
Both spin and orbital degrees of freedom contribute to the magnetic moment of isolated atoms. However, when inserted in crystals, atomic orbital moments are quenched because of the lack of rotational symmetry that protects them when isolated. Thus, the dominant contribution to the magnetization of magnetic materials comes from electronic spin. Here we show that nanoislands of quantum spin Hall insulators can host robust orbital edge magnetism whenever their highest occupied Kramers doublet is singly occupied, upgrading the spin edge current into a charge current. The resulting orbital magnetiz…
Many proposed experiments involving topological insulators (TIs) require spatial control over time-reversal symmetry and chemical potential. We demonstrate reconfigurable micron-scale optical control of both magnetization (which breaks time-reversal symmetry) and chemical potential in ferromagnetic thin films of Cr-(Bi,Sb)$_2$Te$_3$ grown on SrTiO$_3$. By optically modulating the coercivity of the films, we write and erase arbitrary patterns in their remanent magnetization, which we then image with Kerr microscopy. Additionally, by optically manipulating a space charge layer in the underlying …
We show that a spontaneous strain and spontaneous magnetization can arise in the doped topological insulators with a two-component superconducting vector order parameter. The details of the effects crucially depend on the symmetry of the superconducting order parameter, whether it is nematic or chiral. The transition from the nematic state to the chiral one can be performed by application of a magnetic field while the transition from the chiral state to the nematic one is tuned by the external strain. These transitions associated with a jump of the magnetic susceptibility and mechanical stiffn…
We study current carrying helical edge states in a two-dimensional topological insulator coupled to an environment of localized spins, i.e. a spin bath. The localized spins mediate elastic spin-flip scattering between the helical edge states, and we show how this induces a spin-bath magnetization for a finite current through the edge states. The magnetization appears near the boundaries of the topological insulator, while the bulk remains unmagnetized, and it reaches its maximal value in the high bias regime. Furthermore, the helical edge states remain ballistic in steady state, if no addition…
We calculate the magnetization of the helical metallic surface states of a topological insulator. We account for the presence of a small sub-dominant Schr{ö}dinger piece in the Hamiltonian in addition to the dominant Dirac contribution. This breaks particle-hole symmetry. The cross-section of the upper Dirac cone narrows while that of the lower cone broadens. The sawtooth pattern seen in the magnetization of the pure Dirac limit as a function of chemical potential ($μ$) is shifted; but, the quantization of the Hall plateaus remains half integral. This is verified by taking the derivative of th…
Among the potential applications of topological insulators, we investigate theoretically the effect of coexistence of proximity-induced ferromagnetism and superconductivity on the surface states of 3-dimensional topological insulator, where the superconducting electron-hole excitations can be significantly affected by the magnetization of ferromagnetic order. We find that, Majorana mode energy, as a verified feature of TI F/S structure, along the interface sensitively depends on the magnitude of magnetization $m_{zfs}$ in FS region, while its slope in perpendicular incidence presents steep and…
We address the nature of spin-orbit torques at the magnetic surfaces of topological insulators, using both Kubo formula and Keldysh formalism. Through the analysis of the derived spin-charge equations, we find that the so-called Dirac torques possess a different symmetry compared to their Rashba counterpart, as well as a high anisotropy as a function of the magnetization direction. In particular, the damping torque vanishes when the magnetization lies in the plane of the topological insulator surface. This peculiarity has important consequences in terms of magnetization dynamics and switching,…
Strong nonmagnetic impurities on the surface of three-dimensional topological insulators (TIs) generate localized resonance peaks close to the Dirac point. We show that this results in a strongly reduced critical Coulomb interaction strength to reach a magnetic surface state, following a Stoner-like criterion. Thus even weakly interacting TIs host a finite (local) magnetization around strong nonmagnetic impurities. The local magnetization gives rise to a global energy gap, linearly dependent on the maximum value of the magnetization but decreasing with reduced impurity concentration.
Pure spin currents transport angular momentum without an associated charge flow. This unique property makes them attractive for spintronics applications, such as torque induced magnetization control in nanodevices that can be used for sensing, data storage, interconnects and logics. Up to now, however, most spin transfer torque studies focused on metallic ferromagnets, while magnetic insulators were largely ignored, in spite of superior magnetic quality factors. Here, we report the observation of spin torque-induced magnetization dynamics in a magnetic insulator. Our experiments show that in u…
We derive the Onsager response matrix of fluctuation-mediated spin-collinear transport through a ferromagnetic insulator and normal metal interface driven by a temperature difference, spin accumulation, or magnetic field. We predict magnon-squeezing spin currents, magnetic field-induced cooling (magnon Peltier effect), temperature induced magnetization (thermal magnetic field) as well as universal spin Seebeck/Peltier coefficients.
In magnetic topological insulators, quantized electronic transport is interwined with spontaneous magnetic ordering, as magnetization controls band gaps, hence band topology, through the exchange interaction. We show that considering the exchange gaps at the mean-field level is inadequate to predict phase transitions between electronic states of distinct topology. Thermal spin fluctuations disturbing the magnetization can act as frozen disorders that strongly scatter electrons, reducing the onset temperature of quantized transport appreciably even in the absence of structural impurities. This …
Transition metal dichalcogenides XTe$_{2}$ (X=Mo,W) have been shown to be second-order topological insulators based on first-principles calculations, while topological hinge states have been shown to emerge based on the associated tight-binding model. The model is equivalent to the one constructed from a loop-nodal semimetal by adding mass terms and spin-orbit interactions. We propose to study a chiral-symmetric model obtained from the original Hamiltonian by simplifying it but keeping almost identical band structures and topological hinge states. A merit is that we are able to derive various …
We propose magnetic second-order topological insulators (SOTIs). First, we study a three-dimensional model. It is pointed out that the previously proposed topological hinge insulator has actually surface states along the [001] direction in addition to hinge states. We gap out these surface states by introducing magnetization, obtaining a SOTI only with hinge states. The bulk topological number is the $Z_2$ index protected by the combined symmetry of the four-fold rotation and the inversion symmetry. We next study two dimensional magnetic SOTIs, where the corner states are robust also in the pr…
The magneto-transport and magnetization measurements of Sb1.90Cu0.10Te3 were performed at different temperatures and different fields. Magneto-transport measurement at high field indicates the coexistence of both bulk and surface states. The magnetization shows the induced antiferromagnetic ordering with Cu doping and the observed quantum oscillation in it indicates that magnetization in Sb1.90Cu0.10Te3 is the bulk property. The non linearity in Hall data suggests the existence of anomalous and topological Hall effect. The anomalous and topological Hall effect (THE) from measured hall data of …
We study the magnon-mediated pairing between fermions on the surface of a topological insulator (TI) coupled to a ferromagnetic insulator with a tilted mean field magnetization. Tilting the magnetization towards the interfacial plane reduces the magnetic band gap and leads to a shift in the effective TI dispersions. We derive and solve the self-consistency equation for the superconducting gap in two different situations, where we neglect or include the frequency dependence of the magnon propagator. Neglecting the frequency dependence results in p-wave Amperean solutions. We also find that tilt…
The interplay between band topology and magnetic order could generate a variety of time-reversal-breaking gapped topological phases with exotic topological quantization phenomena, such as quantum anomalous Hall (QAH) insulators and axion insulators (AxI). Here by combining analytic models and first-principles calculations, we predict QAH and AxI phases can be realized in thin film of an intrinsic antiferromagnetic van der Waal material Mn$_2$Bi$_2$Te$_5$. The phase transition between QAH and AxI is tuned by the layer magnetization, which would provide a promising platform for chiral supercondu…
We propose and demonstrate spin manipulation by magnetically controlled modulation of pure spin currents in cobalt/copper lateral spin valves, fabricated on top of the magnetic insulator Y$_3$Fe$_5$O$_{12}$ (YIG). The direction of the YIG magnetization can be controlled by a small magnetic field. We observe a clear modulation of the non-local resistance as a function of the orientation of the YIG magnetization with respect to the polarization of the spin current. Such a modulation can only be explained by assuming a finite spin-mixing conductance at the Cu/YIG interface, as it follows from the…
We investigate the magnetization dynamics that arise when a thin-film ferromagnet is deposited on a topological insulator (TI), focusing in particular on domain-wall motion via current and the possibility of a spin-wave torque acting on the magnetization. We show analytically that the coupling between the magnetic domain wall and the TI removes the degeneracy of the wall profile with respect to its chirality and topological charge. Moreover, we find that the threshold for Walker breakdown of domain wall motion is substantially increased and determined by the interaction with the TI, allowing f…
It is commonly believed that organic molecules are physisorbed on the ideal non-polar surfaces of wide band gap insulators with limited variation of the electronic properties of the adsorbate molecule. On the basis of first principles calculations within density functional theory (DFT) and $GW$ approximation, we show that this is not generally true. We find that the molecular frontier orbitals undergo significant changes when a hydroxy acid (here we chose gluconic acid) is adsorbed on MgSO$_4$$\cdot$H$_2$O(100) surface due to the complex interaction between the molecule and the insulating surf…
We investigate theoretically the spin torque and magnetization dynamic in a thin ferromagnetic (FM) layer with spatially varying magnetization. The FM layer is deposited on the surface of a topological insulator (TI). In the limit of the adiabatic relaxation of electron spin along the magnetization, the interaction between the exchange interaction and the Rashba-like surface texture of a TI yields a topological gauge field. Under the gauge field and an applied current, spin torque is induced according to the direction of the current. We derived the corresponding effective anisotropy field and …
We show that the magneto-electric coupling in 3D (strong) topological insulators is related to a second derivative of the bulk magnetization. The formula we derive is the non-linear response analog of the Streda formula for Hall conductivity (P. Streda, J. Phys. C: Solid State Physics, 15, 22 (1982)), which relates the Hall conductivity to the derivative of the magnetization with respect to chemical potential. Our finding allows one to extract the magneto-electric coefficient by measuring the magnetization, while varying the chemical potential and one more perturbing field. Such an experimenta…
