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arXiv 1704.01481cond-mat.mes-hallcond-mat.other
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石墨烯的液门霍尔效应测量用于分子检测

Molecular detection by liquid gated Hall effect measurement of graphene

Hualin Zhan, Jiri Cervenka, Steven Prawer, David J. Garrett

摘要:

在石墨烯的液体门控霍尔效应测量中获得的霍尔电阻对于pM范围内的不同浓度的L-组氨酸表现出比薄层电阻和栅极-源极电流更高的灵敏度。这表明石墨烯的液体门控霍尔测量提供的额外信息可以提高基于晶体管的电位生物传感器的灵敏度,并且它也可以是电化学惰性分子的安培技术的补充方法。对该系统的进一步分析表明,由液体中的离子引起的电子-空穴迁移率的不对称性作为传感机制。对电容值的计算表明,量子电容只在“狄拉克”点附近占主导地位。这一结论对于涉及石墨烯-电解质系统的许多应用都很有用,例如生物传感、能量存储、神经刺激等。

英文摘要:

The Hall resistance obtained in liquid gated Hall effect measurement of graphene demonstrates a higher sensitivity than the sheet resistance and the gate-source current for L-histidine of different concentrations in the pM range. This indicates that the extra information offered by the liquid gated Hall measurement of graphene can improve the sensitivity of the transistor-based potentiometric biosensors, and it could also be a supplementary method to the amperometric techniques for electrochemically inactive molecules. Further analysis of the system suggests that the asymmetry of the electron-hole mobility induced by the ions in the liquid serves as the sensing mechanism. The calculation on the capacitance values shows that the quantum capacitance is only dominant near the "Dirac" point in our system. This conclusion is useful for many applications involving graphene-electrolyte systems, such as bio-sensing, energy storage, neural stimulation, and so on.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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