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arXiv 1703.00780cond-mat.str-el
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用$^{75}$ As NMR谱研究$A$ Fe PDMATHAAB As PDMATHAAB($A$ = K,Rb,Cs)超导体中的增感条纹型涨落

Increasing stripe-type fluctuations in $A$Fe$_{2}$As$_{2}$ ($A$ = K, Rb, Cs) superconductors probed by $^{75}$As NMR spectroscopy

Z. T. Zhang, D. Dmytriieva, S. Molatta, J. Wosnitza, S. Khim, S. Gass, A. U. B. Wolter, S. Wurmehl, H. -J. Grafe, H. Kühne

摘要:

本文报道了$^{75}$ As对RbFe $_{2}$ As $_{2}$和CsFe $_{2}$ As $_{2}$单晶的核磁共振测量。考虑到以前报道的KFe $_{2}$ As $_{2}$的结果,我们发现,各向异性的电子相关的$A$ Fe $_{2}$ As $_{2}$系列(与$A$ = K,Rb,Cs)的磁不稳定性发展。在与较大的碱金属离子的等价取代,各向异性的核自旋晶格弛豫速率的急剧增强和减少奈特位移揭示了形成明显的自旋波动与条纹型调制。此外,下降的幂律指数的核自旋晶格弛豫速率$(1/T_{1})_{H\parallel{ab}}$,探测面内自旋波动,证据从费米液体行为的紧急偏离。所有这些发现清楚地表明,在$A$ Fe $_{2}$ As $_{2}$系列中的晶格膨胀将电子相关性向量子临界点调谐,在该量子临界点处过渡到尚未观察到的有序相。

英文摘要:

We report $^{75}$As nuclear magnetic resonance measurements on single crystals of RbFe$_{2}$As$_{2}$ and CsFe$_{2}$As$_{2}$. Taking previously reported results for KFe$_{2}$As$_{2}$ into account, we find that the anisotropic electronic correlations evolve towards a magnetic instability in the $A$Fe$_{2}$As$_{2}$ series (with $A$ = K, Rb, Cs). Upon isovalent substitution with larger alkali ions, a drastic enhancement of the anisotropic nuclear spin-lattice relaxation rate and decreasing Knight shift reveal the formation of pronounced spin fluctuations with stripe-type modulation. Furthermore, a decreasing power-law exponent of the nuclear spin-lattice relaxation rate $(1/T_{1})_{H\parallel{ab}}$, probing the in-plane spin fluctuations, evidences an emergent deviation from Fermi-liquid behavior. All these findings clearly indicate that the expansion of the lattice in the $A$Fe$_{2}$As$_{2}$ series tunes the electronic correlations towards a quantum critical point at the transition to a yet unobserved, ordered phase.

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