By using Nuclear Magnetic Resonance and ac-susceptibility, the characteristic correlation times for the vortex dynamics, in an iron-based superconductor, have been derived. Upon cooling, the vortex dynamics displays a crossover consistent with a vortex glass transition. The correlation times, in the fast motions regime, merge onto a universal curve which is fit by the Vogel-Fulcher law, rather than by an Arrhenius law. Moreover, the pinning barrier shows a weak dependence on the magnetic field which can be heuristically justified within a fragile glass scenario. In addition, the glass freezing temperatures obtained by the two techniques merge onto the de Almeida-Thouless line. Finally the phase diagram for the mixed phase has been derived.
Doping dependence of Normal-state Property in the Iron-based Oxypnictide Superconductors LaFeAsO1-y probed by 57Fe-NMR and 75As-NMR/NQR
本文报道了贫氧铁基氧氮族化合物超导体LaFeAsO_{1-y} $. A microscopic phase separation between superconducting domains and magnetic domains is shown to take place in the underdoped sample, indicating a local inhomogeneity in association with the density distribution of oxygen deficiencies. As a result, 1/T_1T in the normal state of the superconducting domain decreases significantly upon cooling at both the Fe and As sites regardless of the electron-doping level in LaFeAsO_{1-y}. On the basis of this result, we claim that $ 1/T_1 T $ is not always enhanced by antiferromagnetic fluctuations close to an antiferromagn…
High-$T_c$ Iron-phosphide Superconductivity Enhanced by Reemergent Antiferromagnetic Spin Fluctuations in (Sr$_4$Sc$_2$O$_6$)Fe$_2$(As$_{1-x}$P$_{x}$)$_2$ probed by NMR
本文报道了[SrPDMATHABMM ScPDMATHABMN O $_6$ ] FePDMATHABMN的系统NMR研究(As $_{1-x}$ P $_x$)$_2$,其中铁氮族元素的局部晶格参数(Fe $Pn$)层与LaFe系列的层相似(As $_{1-x'}$ P $_{x'}$)O,其表现出两个分离的反铁磁(AFM)有序相,$x'$ =0-0.2时的AFM 1和$x'$ =0.4-0.7时的AFM 2。结果表明,当$x$ =0时,母体AFM 1相在$x$ =0.3-0.4时消失,对应的磷族元素高度($h_{pn}$)为1.3-1.32 μ m,这与LaFe(As $_{1-x'}$ P $_{x'}$)O和各种母体铁磷族元素化合物相似。相比之下,AFM 2秩序报道的LaFe(作为$_{0.4}$ P $_{0.6}$)O不出现在$x\sim$ 0.8,虽然局部晶格参数的Fe $Pn$层和微观电子状态是非常相似的。尽管没有{ \it静态} AFM 2阶,但在大约$x\sim$ 0.8处观察到重新出现的{ \it动态} AFM自旋波动,这可以归因于AFM 2相的不稳定性。我们建议这种重新增强的AFM自旋波动发挥了重要作用,提高$T_c$到17 K的$x$ =0.8-1。最后,我们从微观角度讨论了复杂磁基态的普遍性和多样性,包括AFM 1和AFM 2相起源的差异,以及它们与铁磷…
Unconventional superconductivity and antiferromagnetic quantum critical behavior in the isovalent-doped BaFe2(As1-xPx)2
用$^{31}$ P NMR研究了BaFe $_2$(As $_{1-x}$ P $_x$)$_2$的自旋动力学随P浓度的变化.我们的核磁共振研究表明,二维反铁磁(AF)的波动显着增强与静态磁化率的变化不大接近AF阶段从超导圆顶。此外,磁有序温度$θ$推导出的弛豫速率在最佳掺杂消失。这些结果为量子临界点(QCP)提供了明确的证据,表明与QCP相关的AF涨落在高- $T_c$超导性中发挥着核心作用。
Quasiparticle spin susceptibility in heavy-fermion superconductors : An NMR study compared with specific heat results
在Kramers双重态晶体电场(CEF)费米液体模型的基础上,根据电子比热($γ_{el}$)、核磁共振奈特位移($K$)和核磁共振弛豫速率($1/T_1$)的实验结果,讨论了各种重费米子(HF)超导体的准粒子自旋磁化率($χ^{qp}$). $χ^{qp}_γ$由增强索末菲系数$γ_{el}$和$χ^{qp}_{T_1}$通过$χ^{qp}_{T_1}=(N_Aμ_B/A_{hf})K^{qp}_{T_1}$关系式由准粒子柯林加关系式$T_1T(K^{qp}_{T_1})^2=const.$计算得到,其中$A_{hf}$是超精细耦合常数,$N_A$是玻尔磁子数,$μ_B$是玻尔磁子。对于偶宇称(自旋单重态)超导体CeCu $_2$ Si $_2$,CeCoIn $_5$和UPd $_2$ Al $_3$,在低于超导转变温度($T_c$)时,奈特位移$δK^{obs}$的分数减小是由于由$χ^{qp}_γ$和$χ^{qp}_{T_1}$一致估计的重准粒子自旋磁化率的减小。这一结果使我们得出结论,重准粒子形成自旋单态库珀对CeCu $_2$ Si $_2$,CeCoIn $_5$和UPd $_2$ Al $_3$。另一方面,在UPt $_3$和UNi $_2$ Al $_3$中没有观察到奈特位移的减少,然而,$χ^{qp}_γ$和$χ^{qp}_{T_1}$的估计值足够大,可以通过实…
No anomalous spin fluctuation in optimally doped and overdoped iron-based oxypnictide superconductors LaFeAsO$_{1-x}$F$_x$ probed by muon spin relaxation
在最佳掺杂和过掺杂超导体LaFeAsO $_{1-x}$ F $_x$中进行了零场和纵向场μ子自旋弛豫测量,以研究在较宽的温度和纵向场范围内的磁涨落.在μ子的时间窗(10 $^{-5}\sim$ 10 $^{-9}$ s)内,我们没有观察到磁涨落随温度变化的迹象.考虑到目前的结果和其他结果,即,通过中子散射观察到的自旋涨落、核磁共振和光电子能谱观察到的类赝能隙行为,表明不仅自旋涨落,而且费米表面具有几种不同轨道贡献的多带特征可能在LaFeAsO $_{1-x}$ F $_x$的超导配对机制中发挥重要作用。
Dynamics of the Local Moment Induced by Nonmagnetic Defects in Cuprates
本文研究了$_2$ O $_3$正常态中Li取代平面Cu所引起的磁缺陷的自旋动力学。用近邻的$^{89}$ Y { \it}和$^7$ Li NMR自旋晶格弛豫探测了Li附近的耦合Cu磁矩的涨落。数据表明,磁扰动波动作为一个单一的实体与相关时间$τ$的规模与当地的静态磁化率。这种行为让人联想到传统金属中磁性杂质的低$T$近藤态。令人惊讶的是,它延伸到远高于“近藤”温度的掺杂不足的赝隙的情况下。
Competing effects of Mn and Y doping on the low-energy excitations and phase diagram of La$_{1-y}$Y$_{y}$Fe$_{1-x}$Mn$_x$AsO$_{0.89}$F$_{0.11}$ iron-based superconductors
用μ子自旋旋转($μ$ SR)和$^{19}$ F核磁共振(NMR)研究了Mn对La $_{1-y}$ Y $_{y}$ Fe $_{1-x}$ Mn $_x$ AsO $_{0.89}$ F $_{0.11}$超导体中Fe替代的影响.虽然对于$y = 0$,需要非常低的临界浓度的Mn($x = 0.2$ %)来淬灭超导电性,但是随着$y$增加,由Y引入的用于La取代的负化学压力稳定了超导电性,并且对于$y= 20$ %,其在Mn含量大一个数量级时被抑制。一旦超导性被抑制,对于$y$ =0和$y= 20$ %,磁相就会出现。低能量的自旋波动引起$^{19}$ F NMR $1/T_1$中的峰值,其起始温度远高于超导转变温度,并且其幅度随着$x$而增加。此外,静态磁相关探测$^{19}$ F NMR线宽测量显示显着增加与Mn含量。根据LaFeAsO $_{0.89}$ F $_{0.11}$接近量子临界点的观点,讨论了超导电性的破坏和磁基态的起始.