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arXiv 1608.03565cond-mat.str-el
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电子掺杂Sr $_{3}$ Ir $_{2}$ O $_{7}$中的无序二聚体态

Disordered dimer state in electron-doped Sr$_{3}$Ir$_{2}$O$_{7}$

Tom Hogan, Rebecca Dally, Mary Upton, J. P. Clancy, Kenneth Finkelstein, Young-June Kim, M. J. Graf, Stephen D. Wilson

摘要:

研究了电子掺杂自旋轨道Mott绝缘体(Sr $_{1-x}$ La $_{x}$)$_3$ Ir $_2$ O $_7$中的自旋激发.当这个双层正方形晶格系统被掺杂到金属制度中时,长程反铁磁性消失,但带隙自旋激发的光谱仍然存在。随着载流子浓度的增加,激发寿命被强烈阻尼,并且能量积分谱权重变得几乎与动量无关,因为静态自旋序被抑制。本地磁矩,在母体系统中不存在,在金属样品中生长,并接近与每个电子掺杂一个$J=\frac{1}{2}$杂质相一致的值。我们的综合数据表明,金属(Sr $_{1-x}$ La $_{x}$)$_3$ Ir $_2$ O $_7$的磁谱最好描述的激发出的无序二聚体状态。

英文摘要:

Spin excitations are explored in the electron-doped spin-orbit Mott insulator (Sr$_{1-x}$La$_{x}$)$_3$Ir$_2$O$_7$. As this bilayer square lattice system is doped into the metallic regime, long-range antiferromagnetism vanishes, yet a spectrum of gapped spin excitation remains. Excitation lifetimes are strongly damped with increasing carrier concentration, and the energy integrated spectral weight becomes nearly momentum independent as static spin order is suppressed. Local magnetic moments, absent in the parent system, grow in metallic samples and approach values consistent with one $J=\frac{1}{2}$ impurity per electron doped. Our combined data suggest that the magnetic spectra of metallic (Sr$_{1-x}$La$_{x}$)$_3$Ir$_2$O$_7$ are best described by excitations out of a disordered dimer state.

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