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arXiv 1107.6034cond-mat.supr-con
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压力和Ru取代对BaFe2As2的联合影响

Combined effects of pressure and Ru substitution on BaFe2As2

S. K. Kim, M. S. Torikachvili, E. Colombier, A. Thaler, S. L. Bud'ko, P. C. Canfield

摘要:

为了研究Ba(Fe_(1-x)Rux)_2As_2(x = 0.00,0.09,0.16,0.21,0.28)的T-P相图,比较等电子Ru取代和压力的联合效应,在近静水压力下(最高压力为7.4GPa)研究了Ba(Fe_(1-x)Rux)_2As_2(x = 0.00,0.09,0.16,0.21,0.28)的ab面电阻率.母体化合物BaFe 2 As 2在134 K附近发生结构/磁性相变。在环境压力下,逐步增加钌浓度抑制这种相变到较低的温度在约5 K/%钌的速率,并与超导性的出现。通过对该系统施加压力,对于每个浓度都可以看到类似的行为:结构/磁性相变被进一步抑制,超导性被诱导,并且最终,对于较大的x Ru和P,被抑制。所有Ru浓度的T-P相图的详细比较表明,3 GPa的压力大致相当于10%的Ru替代。此外,由于Ba(Fe 1-xRux)2As 2对压力条件的敏感性,在本研究中使用的液体介质(4:6轻质矿物油:正戊烷和1:1异戊烷:正戊烷)的熔化可以在电阻率测量中容易地看到。这一功能被用来确定这些介质的冻结曲线,并推断其室温,流体静力学极限:3.5和6.5 GPa,分别。

英文摘要:

The ab-plane resistivity of Ba(Fe1-xRux)2As2 (x = 0.00, 0.09, 0.16, 0.21, and 0.28) was studied under nearly hydrostatic pressures, up to 7.4 GPa, in order to explore the T-P phase diagram and to compare the combined effects of iso-electronic Ru substitution and pressure. The parent compound BaFe2As2 exhibits a structural/magnetic phase transition near 134 K. At ambient pressure, progressively increasing Ru concentration suppresses this phase transition to lower temperatures at the approximate rate of ~5 K/% Ru and is correlated with the emergence of superconductivity. By applying pressure to this system, a similar behavior is seen for each concentration: the structural/magnetic phase transition is further suppressed and superconductivity induced and ultimately, for larger x Ru and P, suppressed. A detailed comparison of the T-P phase diagrams for all Ru concentrations shows that 3 GPa of pressure is roughly equivalent to 10% Ru substitution. Furthermore, due to the sensitivity of Ba(Fe1-xRux)2As2 to pressure conditions, the melting of the liquid media, 4 : 6 light mineral oil : n-pentane and 1 : 1 iso-pentane : n-pentane, used in this study could be readily seen in the resistivity measurements. This feature was used to determine the freezing curves for these media and infer their room temperature, hydrostatic limits: 3.5 and 6.5 GPa, respectively.

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