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arXiv 1012.0611cond-mat.str-el
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四面体受抑自旋量子系统Cu2Te2O5Br2顺磁相的NMR和NQR研究

NMR and NQR study of the tetrahedral frustrated quantum spin system Cu2Te2O5Br2 in its paramagnetic phase

Arnaud Comment, Hadrien Mayaffre, Vesna Mitrovic, Mladen Horvatic, Claude Berthier, Beatrice Grenier, Patrice Millet

摘要:

用NMR和NQR研究了量子反铁磁体Cu_2Te_2O_5Br_2。~(125)Te核磁共振研究表明,在9 T下,在10.5K附近有一个磁转变,这与前人的研究结果一致。从自旋-晶格弛豫速率的发散,我们排除了这种转变可能是由自旋-自旋关联函数的一维发散所控制的可能性。所观察到的125 Te位移的各向异性被证明是由于[TeO 3E]四面体的5s 2“E”双峰的自旋极化,突出了碲在交换路径中的重要性。在顺磁状态下,Br NQR和NMR测量导致的Br超精细耦合和电场梯度张量的确定,和Br p轨道的自旋极化。结果表明,溴在铜自旋之间的相互作用路径中发挥着至关重要的作用。

英文摘要:

The quantum antiferromagnet Cu2Te2O5Br2 was investigated by NMR and NQR. The 125Te NMR investigation showed that there is a magnetic transition around 10.5K at 9T, in agreement with previous studies. From the divergence of the spin-lattice relaxation rate, we ruled out the possibility that the transition could be governed by a one-dimensional divergence of the spin-spin correlation function. The observed anisotropy of the 125Te shift was shown to be due to a spin polarization of the 5s2 "E" doublet of the [TeO3E] tetrahedra, highlighting the importance of tellurium in the exchange paths. In the paramagnetic state, Br NQR and NMR measurements led to the determination of the Br hyperfine coupling and the electric field gradient tensor, and to the the spin polarization of Br p orbitals. The results demonstrate the crucial role of bromine in the interaction paths between Cu spins.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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