We describe a new regime of magnetotransport in two dimensional electron systems in the presence of a narrow potential barrier imposed by external gates. In such systems, the Landau level states, confined to the barrier region in strong magnetic fields, undergo a deconfinement transition as the field is lowered. We present transport measurements showing Shubnikov-de Haas (SdH) oscillations which, in the unipolar regime, abruptly disappear when the strength of the magnetic field is reduced below a certain critical value. This behavior is explained by a semiclassical analysis of the transformation of closed cyclotron orbits into open, deconfined trajectories. Comparison to SdH-type resonances in the local density of states is presented.
We demonstrate that single layer graphene exhibits the electronic structure of a bilayer when it is connected to two gated bilayers. The energy gap characteristic for gated bilayer is induced in the single layer and it persists for distances separating the bilayers up to 20 nm. Most importantly, we report on the appearance of topologically protected gapless state localized in a single graphene layer when the distant bilayers differ in the stacking order. The one-dimensional current in the topological state flows in a single layer graphene, and this finding suggests a new exploitation of graphe…
We investigate gated trilayer graphene partially devoid of outer layers and forming a system of two trilayers connected by a single layer of graphene. A difference in the stacking order of trilayers leads to the appearance of gapless states, one of which is mainly localized in the single graphene layer. We demonstrate that by changing the value of the gate voltage applied to the outer layers one can change the slope of E(k) of this state. As a consequence the direction of current flowing in the single layer graphene can also be changed, the effect that could be useful in practical applications…
We develop a microscopic theory of a strong electromagnetic field interaction with gated bilayer graphene. Quantum kinetic equations for density matrix are obtained using a tight binding approach within second quantized Hamiltonian in an intense laser field. We show that adiabatically changing the gate potentials with time may produce (at resonant photon energy) a full inversion of the electron population with high density between valence and conduction bands. In the linear regime, excitonic absorption of an electromagnetic radiation in a graphene monolayer with opened energy gap is also studi…
We report on asymmetric electron-hole decoherence in epitaxial graphene gated by an ionic liquid. The observed negative magnetoresistance near zero magnetic field for different gate voltages, analyzed in the framework of weak localization, gives rise to distinct electron-hole decoherence. The hole decoherence rate increases prominently with decreasing negative gate voltage while the electron decoherence rate does not exhibit any substantial gate dependence. Quantitatively, the hole decoherence rate is as large as the electron decoherence rate by a factor of two. We discuss possible microscopic…
Gated bilayer graphene exhibits spin-degenerate gapless states with a topological character localized at stacking domain walls. These states allow for one-dimensional currents along the domain walls. We herein demonstrate that these topologically protected currents are spin -polarized and locked in a single layer when bilayer graphene contains stacking domain walls decorated with magnetic defects. The magnetic defects, which we model as π-vacancies, perturb the topological states but also lift their spin degeneracy. One gapless state survives the perturbation of these defects, and its spin pol…
We report on transport properties in dual-gated hexagonal boron nitride (hBN)/bilayer-graphene (BLG) superlattices. Here, BLG is nontwisted, i.e., plain. This paper focuses on the charge neutrality point (CNP) for a plain BLG. Under a perpendicular magnetic field, transitions between two insulating phases at the CNP are detected by varying a displacement field with the study on the resistance-temperature characteristics and the magnetoresistance. This work opens avenues for exploring the global phase diagram of the hBN/BLG superlattices beyond the CNP.
We report simultaneous transport and scanning microwave impedance microscopy to examine the correlation between transport quantization and filling of the bulk Landau levels in the quantum Hall regime in gated graphene devices. Surprisingly, a comparison of these measurements reveals that quantized transport typically occurs below the complete filling of bulk Landau levels, when the bulk is still conductive. This result points to a revised understanding of transport quantization when carriers are accumulated by gating. We discuss the implications on transport study of the quantum Hall effect in…
Gated trilayer graphene exhibits energy gap in its most stable ABC stacking. Here we show that when the stacking order changes from ABC to CBA, three gapless states appear in each valley. The states are topologically protected and their number is related to the change of the valley Chern number across the stacking boundary. The stacking change is achieved by corrugation or delamination in the top and bottom layers, which simultaneously yields two AB/BA stacking domain walls in the pairs of adjacent layers (in bilayers). This in turn causes that for some gate voltages two pairs of topological r…
An efficient method with no numerical diagonalization of a huge Hamiltonian matrix and calculation of a tedious Green's function is proposed to acquire the exact energy spectrum and dynamical conductivity in a gated AA-stacking $N$-layer Graphene (AANLG) with the intrinsic spin-orbital coupling (SOC). $2N \times 2N$ tight-binding Hamiltonian matrix, velocity operator and Green's function representation of an AANLG are simultaneously reduced to $N$ $2\times 2$ diagonal block matrices through a proper transformation matrix. A gated AANLG with intrinsic SOC is reduced to $N$ graphene-like layers.…
Excitonic effects in the optical conductivity of gated graphene
我们研究了电子-电子相互作用的影响下施加偏压的石墨烯的光学电导率,并推导出一个概括的艾略特公式,通常用于半导体,光强度。我们表明,{ \it激子共振}是负责的实验测量的中红外响应的石墨烯,如增加的电导率超过“通用”值以上的费米阻断制度,在阈值处的吸收加宽,并在较高的频率下的光学电导率的降低的几个功能。我们的结果也符合{ \it ab initio}计算的中性制度。
Graphene field-effect transistors are widely used for development of biosensors. However, certain fundamental questions about details of their functioning are not fully understood yet. One of these questions is the presence of gate (leakage) currents in the electrolyte-gated configuration. Here, we report our observations considering causes of this phenomena on chemical vapor deposition (CVD) grown graphene. We observed that gate currents reflect currents that occur on the transistor surface similarly to a working electrode - counter electrode pair currents in an electrochemical cell. Gate cur…
Quantum dynamics and kinetics of electrically gated graphene ribbons with lateral n-p and e-n-p junctions under magnetic field are investigated. It is shown that the snake-like states of quasiparticles skipping along the n-p interface do not manifest themselve in the main semiclassical part of the ribbon conductance. Giant oscillations of the conductance of a ribbon with an n-p-n junction are predicted and analytically calculated. Depending on the number of junctions inside the ribbon its magnetoresistance may be controllably changed by 50% - 90% by an extremely small change of the magnetic fi…
Transient stimulated emission from multi-split-gated graphene structure
在中红外光谱区,提出了具有多分裂(叉指)顶栅和接地背栅的石墨烯中瞬态布居反转的机制,并对其进行了研究。有效的受激发射后,由于漂移扩散过程中的载流子的快速横向扩展被发现的情况下,缓慢的电子空穴复合在无源区。我们表明,与大的栅极到石墨烯的距离的漂移过程总是先于扩散过程,由于无效的屏蔽面内电场的栅极。对于放置在由顶栅和背栅形成的波导中的单层和多层石墨烯的情况,发现具有高于100 cm $^{-1}$的增益的激光发射的条件。分析了波导损耗和温度效应。
We present a novel measurement approach which combines the electrical characterization of solution-gated field effect transistors based on epitaxial bilayer graphene on 4H-SiC (0001) with simultaneous Raman spectroscopy. By changing the gate voltage, we observed Raman signatures related to the resonant electron-phonon coupling. An analysis of these Raman bands enabled the extraction of the geometrical capacitance of the system and an accurate calculation of the Fermi levels for bilayer graphene. An intentional application of higher gate voltages allowed us to trigger electrochemical reactions,…
Tuning of quantum interference in top-gated graphene on SiC
我们报告的量子干涉测量在顶部栅霍尔条的单层石墨烯外延生长在Si面的SiC,其中实现了从负到正的磁阻的转变,不同的温度和电荷密度。系统地研究了准粒子量子干涉和电子-电子相互作用对磁电阻效应的量子修正。我们分析了影响磁输运的不同散射机制在$-2.0 \times 10^{10}$ cm $^{-2}$到$3.75 \times 10^{11}$ cm $^{-2}$密度区域的贡献,并发现电荷密度对谷内散射时间的显著影响。此外,我们观察到调制的电子-电子相互作用的电荷密度不占目前的理论。我们的研究结果阐明了量子输运在基于SiC的器件中的作用,这将与基于石墨烯的相干电子技术的发展相关。
Metal-semiconductor interfaces, known as Schottky junctions, have long been hindered by defects and impurities. Such imperfections dominate the electrical characteristics of the junction by pinning the metal Fermi energy. We report measurements on a boron nitride encapsulated graphene-tungsten diselenide (WSe$_2$) Schottky junction which exhibits ideal diode characteristics and a complete lack of Fermi-level pinning. The Schottky barrier height of the device is rigidly tuned by electrostatic gating of the WSe$_2$, enabling experimental verification of the Schottky-Mott limit in a single device…
Graphene/silicon (G/Si) heterojunction based devices have been demonstrated as high responsivity photodetectors that are potentially compatible with semiconductor technology. Such G/Si Schottky junction diodes are typically in parallel with gated G/silicon dioxide (SiO$_2$)/Si areas, where the graphene is contacted. Here, we utilize scanning photocurrent measurements to investigate the spatial distribution and explain the physical origin of photocurrent generation in these devices. We observe distinctly higher photocurrents underneath the isolating region of graphene on SiO$_2$ adjacent to the…
We investigate the effects of homogeneous and inhomogeneous deformations and edge disorder on the conductance of gated graphene nanoribbons. Under increasing homogeneous strain the conductance of such devices initially decreases before it acquires a resonance structure, and finally becomes completely suppressed at larger strain. Edge disorder induces mode mixing in the contact regions, which can restore the conductance to its ballistic value. The valley-antisymmetric pseudo-magnetic field induced by inhomogeneous deformations leads to the formation of additional resonance states, which either …
Graphene-based heterostructures display a variety of phenomena that are strongly tunable by electrostatic local gates. Monolayer graphene (MLG) exhibits tunable surface plasmon polaritons, as revealed by scanning nano-infrared experiments. In bilayer graphene (BLG), an electronic gap is induced by a perpendicular displacement field. Gapped BLG is predicted to display unusual effects such as plasmon amplification and domain wall plasmons with significantly larger lifetime than MLG. Furthermore, a variety of correlated electronic phases highly sensitive to displacement fields have been observed …
Electronic current densities can reach extreme values in highly conducting nanostructures where constrictions limit current. For bias voltages on the 1 volt scale, the highly non-equilibrium situation can influence the electronic density between atoms, leading to significant inter-atomic forces. An easy interpretation of the non-equilibrium forces is currently not available. In this work, we present an ab-initio study based on density functional theory of bias-induced atomic forces in gated graphene nanoconstrictions consisting of junctions between graphene electrodes and graphene nano-ribbons…