Tunable Luttinger liquid physics in biased bilayer graphene
Matthew Killi, Tzu-Chieh Wei, Ian Affleck, Arun Paramekanti
备注：
Modified to address referee comments - added references, added discussion of disorder and modified setup which allows tuning of carrier density and electric field (version to appear in PRL).
Electronically gated bilayer graphene behaves as a tunable gap semiconductor under a uniform interlayer bias $V_{g}$. Imposing a spatially varying bias, which changes polarity from $-V_g$ to $+V_g$, leads to one dimensional (1D) chiral modes localized along the domain wall of the bias. Due to the broad transverse spread of their low-energy wavefunctions, we find that the dominant interaction between these 1D electrons is the forward scattering part of the Coulomb repulsion. Incorporating these interactions and the gate voltage dependence of the dispersion and wavefunctions, we find that these 1D modes behave as a strongly interacting Tomonaga-Luttinger liquid with three distinct mode velocities and a bias dependent Luttinger parameter, and discuss its experimental signatures.
The conductivity properties between Luttinger liquids are analyzed by exact Renormalization Group methods. We prove that in a two chain system or in a model of bilayer graphene, described by two coupled fermionic honeycomb lattices interacting with a gauge field, the transverse optical conductivity at finite temperature is anomalous and decreasing together with the frequency as a power law with Luttinger liquid exponent.
We calculate the tunneling density of states for a Tomonaga-Luttinger liquid placed under a strong bias voltage. For the tunneling through a side-coupled point contact, one can observe the power law singularities in the tunneling density of states separately for the right- and left-movers despite the point-like tunnel contact. Deviations of the nonequilibrium tunneling exponents from the equilibrium case are discussed.
We investigate the many-body instabilities of electrons interacting near Van Hove singularities arising in monolayer and twisted bilayer graphene. We show that a pairing instability must be dominant over the tendency to magnetic order as the Fermi level is tuned to the Van Hove singularity in the conduction band of graphene. As a result of the extended character of the saddle points in the dispersion, we find that the pairing of the electrons takes place preferentially in a channel of f-wave symmetry, with an order parameter vanishing at the position of the saddle points along the Fermi line. …
Mean-field theory predicts that bilayer quantum Hall systems at odd integer total filling factors can have stripe ground states in which the top Landau level is occupied alternately by electrons in one of the two layers. We report on an analysis of the properties of these states based on a coupled Luttinger liquid description that is able to account for quantum fluctuations of charge-density and position along each stripe edge. The soft modes associated with the broken symmetries of the stripe state lead to an unusual coupled Luttinger liquid system with strongly enhanced low-temperature heat …
We study the localized magnetic states of impurity in biased bilayer and trilayer graphene. It is found that the magnetic boundary for bilayer and trilayer graphene presents the mixing features of Dirac and conventional fermion. For zero gate bias, as the impurity energy approaches the Dirac point, the impurity magnetization region diminishes for bilayer and trilayer graphene. When a gate bias is applied, the dependence of impurity magnetic states on the impurity energy exhibits a different behavior for bilayer and trilayer graphene due to the opening of a gap between the valence and the condu…
We explore in detail the electronic phases of a system consisting of three non-colinear arrays of coupled quantum wires, each rotated 120 degrees with respect to the next. A perturbative renormalization-group analysis reveals that multiple correlated states can be stabilized: a $s$-wave or $d \pm id$ superconductor, a charge density wave insulator, a two-dimensional Fermi liquid, and a 2D Luttinger liquid (also known as smectic metal or sliding Luttinger liquid). The model provides an effective description of electronic interactions in small-angle twisted bilayer graphene and we discuss its im…
We compute the phase diagram of a biased graphene bilayer. The existence of a ferromagnetic phase is discussed with respect both to carrier density and temperature. We find that the ferromagnetic transition is first order, lowering the value of $U$ relatively to the usual Stoner criterion. We show that in the ferromagnetic phase the two planes have unequal magnetization and that the electronic density is hole like in one plane and electron like in the other.
The phase diagram of a biased graphene bilayer is computed and the existence of a ferromagnetic phase is discussed both in the critical on-site interaction $U_{c}$ versus doping density and versus temperature. We show that in the ferromagnetic phase the two planes have unequal magnetization and that the electronic density is hole like in one plane and electron like in the other. We give evidence for a \emph{first-order} phase transition between paramagnetic and ferromagnetic phases induced by doping at zero temperature.
We study magnetism of an adatom adsorbed on AA-stacked bilayer graphene (BLG) in both unbiased and biased cases, using the Anderson impurity model. We find different magnetic phase diagrams for the adatom, depending on the energy level of the adatom, which varies from the magnetic phase diagram of adatom in normal metals to that in graphene. This is due to the individual energy dependence of the density of states (DOS) of AA-stacked BLG and anomalous broadening of the adatom energy level. Furthermore we investigate the effect of a bias voltage on DOS of AA-stacked and show that the magnetizati…
We address the optical conductivity of undoped bilayer graphene in the presence of a finite bias voltage at finite temperature. The effects of gap parameter and stacking type on optical conductivity are discussed in the context of tight binding model Hamiltonian. Green's function approach has been implemented to find the behavior of optical conductivity of bilayer graphene within linear response theory. We have found the frequency dependence of optical conductivity for different values of gap parameter and bias voltage. Also the dependence of optical conductivity on the temperature has been in…
Monte Carlo simulation of a 2+1 dimensional model of voltage-biased bilayer graphene, consisting of relativistic fermions with chemical potential mu coupled to charged excitations with opposite sign on each layer, has exposed non-canonical scaling of bulk observables near a quantum critical point found at strong coupling. We present a calculation of the quasiparticle dispersion relation E(k) as a function of exciton source j in the same system, employing partially twisted boundary conditions to boost the number of available momentum modes. The Fermi momentum k_F and superfluid gap Delta are ex…
We demonstrate that the electronic gap of a graphene bilayer can be controlled externally by applying a gate bias. From the magneto-transport data (Shubnikov-de Haas measurements of the cyclotron mass), and using a tight binding model, we extract the value of the gap as a function of the electronic density. We show that the gap can be changed from zero to mid-infrared energies to a value as large as 0.3 eV by using fields of < 1 V/nm, below the electric breakdown of SiO2. The opening of a gap is clearly seen in the quantum Hall regime.
Excitonic bound states are characterised by a binding energy $ε_b$ and a single-particle band gap $Δ_b$. This work provides a theoretical description for both strong ($ε_b\simΔ_b$) and weak ($ε_b\llΔ_b$) excitonic bound states, with particular application to biased bilayer graphene. Standard description of excitons is based on a wave function that is determined by a Schrödinger-like equation with screened attractive potential. The wave function approach is valid only in the weak binding regime $ε_b\llΔ_b$. The screening depends on frequency (dynamical screening) and this implies retardation. I…
We study, within the tight-binding approximation, the electronic properties of a graphene bilayer in the presence of an external electric field applied perpendicular to the system -- \emph{biased bilayer}. The effect of the perpendicular electric field is included through a parallel plate capacitor model, with screening correction at the Hartree level. The full tight-binding description is compared with its 4-band and 2-band continuum approximations, and the 4-band model is shown to be always a suitable approximation for the conditions realized in experiments. The model is applied to real bias…
Motivated by experiments on twisted bilayer graphene, we study the emergence of superconductivity from $\textit{weak}$ repulsive interactions in the Hubbard model on a honeycomb lattice, with both spin and orbital degeneracies, and with the filling treated as a tunable control parameter. The attraction is generated through the Kohn-Luttinger mechanism. We find, similar to old studies of single layer graphene, that the leading superconducting instability is in a $d$-wave pairing channel close to Van Hove filling, and is in an $f$-wave pairing channel away from Van Hove filling. The $d$-wave pai…
We suggest an experiment to study Luttinger liquid behavior in a one-dimensional nanostructure, avoiding the usual complications associated with transport measurements. The proposed setup consists of a quantum box, biased by a gate voltage, and side-coupled to a quantum wire by a point contact. Close to the degeneracy points of the Coulomb blockaded box, and in the presence of a magnetic field sufficiently strong to spin polarize the electrons, the setup can be described as a Luttinger liquid interacting with an effective Kondo impurity. Using exact nonperturbative techniques we predict that t…
The Fermi liquid paradigm for metals has contributed enormously to our understanding of condensed matter systems. However a growing number of quantum critical systems have been shown to exhibit non Fermi liquid behavior. A full understanding of such systems is still lacking and in particular analytical results away from equilibrium are rare. In this work, we provide a distinct example of such kind in a two channel Kondo Luttinger model where a Kondo impurity couples to two voltage biased interacting electron leads, experimentally realizable in a dissipative quantum dot. An exotic quantum phase…
We evaluate tunneling rates into/from a voltage biased quantum wire containing weak backscattering defect. Interacting electrons in such a wire form a true nonequilibrium state of the Luttinger liquid (LL). This state is created due to inelastic electron backscattering leading to the emission of nonequilibrium plasmons with typical frequency $\hbar ω\leq U$. The tunneling rates are split into two edges. The tunneling exponent at the Fermi edge is positive and equals that of the equilibrium LL, while the exponent at the side edge $E_F-U$ is negative if Coulomb interaction is not too strong.
We consider suspened bilayer graphene under applied perpendicular electric bias field that is known to generate a single particle gap $2Δ$ and a related electric polarization ${\cal P}$. We argue that the bias also drives a quantum phase transition from band insulator to superfluid exciton condensate. The transition occurs when the exciton binding energy exceeds the band gap $2Δ$. We predict the critical bias (converted to band gap), $Δ_c\approx 60$ meV, below which the excitons condense. The critical temperature, $T_c(Δ)$, is maximum at $Δ\approx 25$ meV, $T_c^\text{max}\approx 115$ K, decrea…
Magnetic state of exchanged biased CoO(20nm)/Co($d_F$) bilayer ($d_F$=5-20nm) was studied by means of polarized neutron reflectometry. By spacing of CoO/Co bilayer and Al$_2$O$_3$ substrate with Nb(20nm) layer we created waveguide structure which allowed us to significantly enhance intensity of spin-flip (SF) scattering in the position of optical resonances. For the trained sample with thinnest Co(5nm) we detected strong SF scattering at the resonance position (up to 30\% of incoming intensity) speaking about high non-collinearity of the system. As $d_F$ increases, the intensity of SF scatteri…
We demonstrate that the plasmon in one-dimensional Coulomb interacting electron fluids can develop a finite-momentum maxon-roton-like nonmonotonic energy-momentum dispersion. Such an unusual nonmonotonicity arises from the strongly interacting $1/r$ Coulomb potential going beyond the conventional band linearization approximation used in the standard bosonization theories of Luttinger liquids. We provide details for the nonmonotonic plasmon dispersion using both bosonization and RPA theories. We also calculate the specific heat including the nonmonotonicity and discuss possibilities for observi…
The current noise of a voltage biased interacting quantum wire adiabatically connected to metallic leads is computed in presence of an impurity in the wire. We find that in the weak backscattering limit the Fano factor characterizing the ratio between noise and backscattered current crucially depends on the noise frequency $ω$ relative to the ballistic frequency $v_F/gL$, where $v_F$ is the Fermi velocity, $g$ the Luttinger liquid interaction parameter, and $L$ the length of the wire. In contrast to chiral Luttinger liquids the noise is not only due to the Poissonian backscattering of fraction…
We have investigated exchange bias effects in bilayers composed by the antiferromagnetic o-YMnO$_3$ and ferromagnetic Co thin film by means of SQUID magnetometry, magnetoresistance, anisotropic magnetoresistance and planar Hall effect. The magnetization and magnetotransport properties show pronounced asymmetries in the field and magnetization axes of the field hysteresis loops. Both exchange bias parameters, the exchange bias field $H_{E}(T)$ as well as the magnetization shift $M_E(T)$, vanish around the Néel temperature $T_N \simeq 45$ K. We show that the magnetization shift $M_E(T)$ is also …
Since the discovery of superconductivity and correlated insulator at fractional electron fillings in the twisted bilayer graphene, most theoretical efforts have been focused on describing this system in terms of an effective extended Hubbard model. However, it was recognized that an exact tight binding model on the Moiré superlattice which captures all the subtleties of the bands can be exceedingly complicated. Here we pursue an alternative coupled wire description of the system based on the observation that the lattice relaxation effect is strong at small twist angle, which substantially enla…
We investigate the time evolution towards the asymptotic steady state of a one dimensional interacting system after a quantum quench. We show that at finite time the latter induces entanglement between right- and left- moving density excitations, encoded in their cross-correlators, which vanishes in the long-time limit. This behavior results in a universal time-decay in system spectral properties $ \propto t^{-2} $, in addition to non-universal power-law contributions typical of Luttinger liquids. Importantly, we argue that the presence of quench-induced entanglement clearly emerges in transpo…
We study the emergence of superconductivity in rhombohedral trilayer graphene due purely to the long-range Coulomb repulsion. This repulsive-interaction-driven phase in rhombohedral trilayer graphene is significantly different from those found in twisted bilayer and trilayer graphenes. In the latter case, the nontrivial momentum-space geometry of the Bloch wavefunctions leads to an effective attractive electron-electron interaction; this allows for less modulated order parameters and for spin-singlet pairing. In rhombohedral trilayer graphene, we instead find spin-triplet superconductivity wit…
We formulate a model of N_f=4 flavors of relativistic fermion in 2+1d in the presence of a chemical potential mu coupled to two flavor doublets with opposite sign, akin to isopsin chemical potential in QCD. This is argued to be an effective theory for low energy electronic excitations in bilayer graphene, in which an applied voltage between the layers ensures equal populations of particles on one layer and holes on the other. The model is then reformulated on a spacetime lattice using staggered fermions, and in the absence of a sign problem, simulated using an orthodox hybrid Monte Carlo algor…
The current noise of a voltage biased interacting quantum wire adiabatically connected to metallic leads is computed in presence of an impurity in the wire. We find that in the weak backscattering limit the Fano factor characterizing the ratio between shot noise and backscattering current crucially depends on the noise frequency relative to the ballistic frequency v_F/gL, where v_F is the Fermi velocity, g the Luttinger liquid interaction parameter, and L the length of the wire. In contrast to chiral Luttinger liquids, the noise is not only due to the Poissonian backscattering of fractionally …
Imaging flat band electron hydrodynamics in biased bilayer graphene
University of California, Santa Barbara（加州大学圣塔芭芭拉分校）；University of Colorado, Boulder（科罗拉多大学博尔德分校）；National Institute for Materials Science（国立材料研究所）；University of Colorado, Denver（科罗拉多大学丹佛分校）
Albeit difficult to access experimentally, the density of states (DOS) is a key parameter in solid state systems which governs several important phenomena including transport, magnetism, thermal, and thermoelectric properties. We study DOS in an ensemble of potassium intercalated single-wall carbon nanotubes (SWCNT) and show using electron spin resonance spectroscopy that a sizeable number of electron states are present, which gives rise to a Fermi-liquid behavior in this material. A comparison between theoretical and the experimental DOS indicates that it does not display significant correlat…
Physical properties reflecting valley asymmetry of Landau levels in a biased bilayer graphene under magnetic field are discussed. Within the $4-$band continuum model with Hartree-corrected self-consistent gap and finite damping factor we predict the appearance of anomalous steps in quantized Hall conductivity due to the degeneracy lifting of Landau levels. Moreover, the valley symmetry breaking effect appears as a non-semiclassical de Haas-van Alphen effect where the reduction of the oscillation period to half cannot be accounted for through quasi-classical quantization of the orbits in recipr…
A real-space formulation is given for the recently discussed exciton condensate in a symmetrically biased graphene bilayer. We show that in the continuum limit an oddly-quantized vortex in this condensate binds exactly one zero mode per valley index of the bilayer. In the full lattice model the zero modes are split slightly due to intervalley mixing. We support these results by an exact numerical diagonalization of the lattice Hamiltonian. We also discuss the effect of the zero modes on the charge content of these vortices and deduce some of their interesting properties.
Luttinger Liquid Behavior in a Single-Layer Nickelate La1.4Sr0.6NiO4
Tsinghua University（清华大学）；Yale University（耶鲁大学）；University of Oxford（牛津大学）；Diamond Light Source（钻石光源）；SLAC National Accelerator Laboratory（斯坦福直线加速器中心）；Shanghai Advanced Research Institute, Chinese Academy of Sciences（中国科学院上海高等研究院）；University of Science and Technology of China（中国科学技术大学）；ShanghaiTech University（上海科技大学）
We study charge transport through $N$-lead junctions ($N\geq 3$) of spinless Luttinger liquid wires with bias voltages applied to Fermi-liquid reservoirs. In particular, we consider a Y junction, which is a setup characteristic of the tunneling experiment. In this setup, the strength of electron-electron interactions in one of the arms ("tunneling tip") is different from that in the other two arms (which form together the "main wire"). For a generic single-particle $S$ matrix of the junction, we find that the bias voltage $V$ applied---even symmetrically---to the main wire generates a current …
The Luttinger liquid (LL) model of one-dimensional (1D) electronic systems provides a powerful tool for understanding strongly correlated physics including phenomena such as spin-charge separation. Substantial theoretical efforts have attempted to extend the LL phenomenology to two dimensions (2D), especially in models of closely packed arrays of 1D quantum wires, each being described as a LL. Such coupled-wire models have been successfully used to construct 2D anisotropic non-Fermi liquids, quantum Hall states, topological phases, and quantum spin liquids. However, an experimental demonstrati…
Bilayer graphene -- two coupled single graphene layers stacked as in graphite -- provides the only known semiconductor with a gap that can be tuned externally through electric field effect. Here we use a tight binding approach to study how the gap changes with the applied electric field. Within a parallel plate capacitor model and taking into account screening of the external field, we describe real back gated and/or chemically doped bilayer devices. We show that a gap between zero and midinfrared energies can be induced and externally tuned in these devices, making bilayer graphene very appea…
This thesis studies how the rudimentary attributes of graphene's charge carriers, and local moments on its surface, can be directly manipulated and controlled with electrostatic potentials. We first consider bilayer graphene subject to a spatially varying electrostatic potential that forms two neighbouring regions with opposite interlayer bias. Along the boundary, 1D chiral "kink" states emerge. We find that these 1D modes behave as a strongly interacting Luttinger liquid whose properties can be tuned via an external gate. Next, we consider superlattices in bilayer graphene. Superlattices are …
The allegedly unconventional superconducting phase of magic-angle twisted bilayer graphene (MATBG)1 has been predicted to possess extraordinary thermal properties, as it is formed from a highly diluted electron ensemble with both a record-low carrier density n ~ 10^11 cm-2 and electronic heat capacity Ce < 100 kB. While these attributes position MATBG as a ground-breaking material platform for revolutionary calorimetric applications2, these properties have so far not been experimentally shown. Here we reveal the ultra-sensitive calorimetric properties of a superconducting MATBG device, by moni…
