In this paper, we theoretically and numerically demonstrate a two-dimensional Metal-Dielectric-Metal (MDM) waveguide based on finite-difference time-domain simulation of the propagation characteristics of surface plasmon polaritons (SPPs). For practical applications, we propose a plasmonic Y-branch waveguide based on MDM structure for high integration. The simulation results show that the Y-branch waveguide proposed here makes optical splitter with large branching angle (~180 degree) come true. We also introduce a finite array of periodic tooth structure on one surface of the MDM waveguide which is in a similar way as FBGs or Bragg reflectors, potentially as filters for WDM applications. Our results show that the novel structure not only can realize filtering function of wavelength with a high transmittance over 92%, but also with an ultra-compact size in the length of a few hundred nanometers, in comparison with other grating-like SPPs filters. The MDM waveguide splitters and filters could be utilized to achieve ultra-compact photonic filtering devices for high integration in SPPs-based flat metallic surfaces.
We propose and design an ultra-compact and broadband tunable multimode interference (MMI) splitter in mid-infrared based on graphene plasmonic waveguides. The size of the device is only 0.56μm*1.2μm, which corresponds to device area of only about 0.014λ^2, where λ is the vacuum wavelength. And the center wavelength of the device can be tuned in a broad band from 7μm to 9μm with the Fermi level of graphene varied from 0.5eV to 1eV. Furthermore, the device is easy to be fabricated on chip.
Transformational optics are shown to markedly enhance the control of the electromagnetic wave trajectories within metamaterials with unconventional functionalities such as a beam splitter, a toroidal carpet, a Luneburg lens and a black hole, all of which are specially designed for surface plasmon polaritons propagating on a metal plate
We present a quantitative experimental analysis of a surface plasmon polariton (SPP) interferometer relying on elliptical Bragg mirrors. By using a leakage radiation microscope we observe oscillation fringes with unit visibility at the two interferometer exits. We study the properties of the SPP beam splitter and determine experimentally both the norm and phase of the SPP reflection and transmission coefficients.
We propose using the effective spin-orbit interaction of light in Bragg-modulated cylindrical waveguides for the effcient separation of spin-up and spin-down photons emitted by a single photon emitter. Due to the spin and directional dependence of photonic stopbands in the waveguides, spin-up (down) photon propagation in the negative (positive) direction along the waveguide axis is blocked while the same photon freely propagates in the opposite direction.
We investigate the performance of bends and splitters in graphene nanoribbon waveguides. Although the graphene waveguides are lossy themselves, we show that bends and splitters do not induce any additional loss provided that the nanoribbon width is sub-wavelength. We use transmission line theory to qualitatively interpret the behavior observed in our simulation. Our results pave a promising way to realize ultra-compact devices operating in the terahertz region.
In this paper, tooth-shaped and multiple-teeth-shaped plasmonic filters in the metal-insulator-metal (MIM) waveguides are demonstrated numerically. By introducing a three-port waveguide splitter, a modified model based on the multiple-beam-interference and the scattering matrix is given. The ransmittance spectrum as a function of teeth width, depth, period and period number are respectively addressed. The result shows the new structure not only performs the filtering function as well as MIM grating-like structures, but also is of submicrometer size for ultra-high integration and relatively eas…
Surface plasmon resonance in super-period metal nanoslits can be observed in the first order diffraction as well in the zeroth order transmission. In this paper, surface plasmon resonance modes in various super-period gold nanoslit arrays are investigated. It is found that the surface plasmon resonance frequencies are determined by the small period of the nanoslits in super-period nanoslits. The number of nanoslits in the unit cell super-period and the nanoslit width do not control the surface plasmon resonance frequencies. It is also found that the resonance wavelength observed in the first o…
We introduce the concept of polychromatic plasmonics and suggest an broadband plasmonic lens for nanofocusing of surface plasmon polaritons. The lens employs a parabolically modulated metal-dielectric-metal structure. This plasmonic lens has a bandwidth of more than an optical octave thus opening new opportunities for broadband plasmonic applications.
In this manuscript we report on a near-feld study of two-dimensional plasmonic gold nano-wedges using electron energy loss spectroscopy in combination with scanning transmission electron microscopy, as well as discontinuous Galerkin time-domain computations. With increasing nano-wedge size, we observe a transition from localized surface plasmons on small nano-wedges to non-resonant propagating surface plasmon polaritons on large nano-wedges. Furthermore we demonstrate that nano-wedges with a groove cut can support localized as well as propagating plasmons in the same energy range.
Nanostructured metal surfaces comprised of periodically arranged spherical voids are grown by electrochemical deposition through a self-assembled template. Detailed measurements of the angle- and orientation-dependent reflectivity reveal the spectral dispersion, from which we identify the presence of both delocalized Bragg- and localized Mie-plasmons. These couple strongly producing bonding and anti-bonding mixed plasmons with anomalous dispersion properties. Appropriate plasmon engineering of the void morphology selects the plasmon spatial and spectral positions, allowing these plasmonic crys…
Tightly confined plasmon waveguide modes supported by semicircular cross section top silver nanoridges are investigated in this paper. Mode field profiles, dispersion curves, propagation distances, confinement factors, and figure-of-merits of semicircular top silver nanoridge plasmon waveguide mode are calculated for different radii of curvature at different wavelengths. It is found that semicircular top silver nanoridges support tightly confined quasi-TEM plasmon waveguide modes. Semicircular top silver nanoridge mode has longer propagation distance and higher figure-of-merit than that of the…
It is now well established that, due to excitation of localized surface plasmon resonances in plasmonic nanosystems, the electric field from an external irradiation source is greatly amplified in their vicinity. Surface plasmon mediated electric field amplification near plasmonic nanosystems is of vital importance for; light absorption enhancement of solar cells, molecular detection using surface enhanced Raman spectroscopy, proximity measurement of biological macromolecules such as proteins, lipids and nucleic acids using plasmon enhanced FRET, cancer therapy using photothermal effects, just …
Spasers have been theoretically predicted and experimentally observed and promise to deliver new exciting nanophotonic and biomedical applications. Here we theoretically investigate ultrafast dynamical properties of spasers with external plasmonic feedback. We consider a spaser both as a nanoscale source and detector of plasmons which could be used to design novel nano-imaging and sensing techniques. We show that, as with conventional lasers, spasers are sensitive to external feedback. However, unlike the lasers, spasers have faster relaxation dynamics which could be used to develop new ultras…
Sharp metal corners and tips support plasmons localized on the scale of the curvature radius -- superlocalized plasmons. We analyze plasmonic properties of nanoparticles with small and sharp corner- and tip-shaped surface perturbations in terms of hybridization of the superlocalized plasmons, which frequencies are determined by the perturbations shape, and the ordinary plasmons localized on the whole particle. When the frequency of a superlocalized plasmon gets close to that of the ordinary plasmon, their strong hybridization occurs and facilitates excitation of an optical hot-spot near the co…
We derive and present systematic relationships between the analytical formulas for calculation of the localized surface plasmon resonances (LSPR) of some plasmonic nano-structures which we have categorized as simple. These relationships, including some new formulas, are summarized in a tree diagram which highlights the core-shell plasmons as the generators of solid and cavity plasmons. In addition, we show that the LSPR of complex structures can be reduced to that of simpler ones, using the LSPR of a nanorice as a case study, in the dipole limit. All the formulas were derived using a combinati…
We develop a theory to model the interaction of graphene substrate with localized plasmon resonances in metallic nanoparticles. The influence of a graphene substrate on the surface plasmon resonances is described using an effective background permittivity that is derived from a pseudoparticle concept using the electrostatic method. For this purpose, the interaction of metal nanoparticle with graphene sheet is studied to obtain the optical spectrum of gold nanoparticles deposited on a graphene substrate. Then, we introduce a factor based on dipole approximation to predict the influence of the s…
We use focused-ion-beam milling of a single-crystal Au surface to fabricate a 590-nm-long linear ridge that acts as a surface plasmon nanoresonator. Cathodoluminescence imaging spectroscopy is then used to excite and image surface plasmons on the ridge. Principal component analysis reveals distinct plasmonic modes, which proves confinement of surface-plasmon oscillations to the ridge. Boundary-element-method calculations confirm that a linear ridge is able to support highly-localized surface-plasmon modes (mode diameter < 100 nm). The results demonstrate that focused-ion-beam milling can be us…
Artificially built periodic optical structures in dielectric and metallic media have generated considerable interest due to their potential for optical device miniaturization. In this context plasmonics, i.e., optics based on surface plasmon polaritons (SPPs) offers new exciting prospects. SPPs are hybrid light/electron surface waves at the interface between a dielectric and a metal and as such hold the potential for 2D optical functionality. Indeed, SPP elements as mirrors, splitters and interferometers have been recently demonstrated. However, for plasmonics to qualify at the information tec…
While long-range propagating plasmons have been extensively investigated for implementing on-chip optical sensing platforms, waveguide-excited localized surface plasmon resonance (LSPR) based sensing systems have not yet received much attention. Waveguide excitation and readout as an alternative to free-space light based single-particle spectroscopy are particularly attractive for high-throughput sensing and on-chip drug discovery platforms. Here we present a numerical investigation of the optical response of a waveguide-excited plasmonic dolmen-shaped compound nanoantenna that exhibits a Fano…
High-performance optical beam splitters are of fundamental importance for the development of advanced silicon photonics integrated circuits. However, due to the high refractive index contrast of the silicon-on-insulator platform, state of the art Si splitters are hampered by trade-offs in bandwidth, polarization dependence and sensitivity to fabrication errors. Here, we present a new strategy that exploits modal engineering in slotted waveguides to overcome these limitations, enabling ultra-wideband polarization-insensitive optical power splitters, with relaxed fabrication tolerances. The prop…
We propose a novel Conditional Variational Autoencoder (CVAE) model, enhanced with adversarial censoring and active learning, for the generation of 550 nm broad bandwidth (1250 nm to 1800 nm) power splitters with arbitrary splitting ratio. The device footprint is 2.25 x 2.25 μ m2 with a 20 x 20 etched hole combination. It is the first demonstration to apply the CVAE model and the adversarial censoring for the photonics problems. We confirm that the optimized device has an overall performance close to 90% across all bandwidths from 1250 nm to 1800 nm. To the best of our knowledge, this is the s…
Assuming that the resonant surface plasmons on a spherical nanoparticle is formed by standing waves of two counter-propagating surface plasmon waves along the surface, by using Mie theory simulation, we find that the dispersions of surface plasmon resonant modes supported by silver nanospheres match that of the surface plasmons on a semi-infinite medium-silver interface very well. This suggests that the resonant surface plasmons of a metal nanosphere can be treated as a propagating surface plasmon wave.
By using the real-space method, switching of a single plasmon interacting with a hybrid nanosystem composed of a semiconductor quantum dot (SQD) and a metallic nanoparticle (MNP) coupled to one-dimensional surface plasmonic waveguide is investigated theoretically. We discussed that the dipole coupling between an exciton and a localized surface plasmon results in the formation of a hybrid exciton and the transmission and reflection of the propagating single plasmon could be controlled by changing the interparticle distance between the SQD and the MNP and the size of the nanoparticles. The contr…
The effect of confinement on surface plasmon polariton in a planar nanocavity was studied. The generalized modes were obtained and studied in detail. It was demonstrated that these modes result from the strong coupling of plasmon-like and photon-like modes.
Transport properties of a single plasmon interacting with a hybrid system composed of a semiconductor quantum dot (SQD) and a metal nanoparticle (MNP) coupled to one-dimensional surface plasmonic waveguide are investigated theoretically via the real-space approach. We considered that the MNP-SQD interaction leads to the formation of a hybrid exciton and the transmission and reflection of a single incident plasmon could be controlled by adjusting the frequency of the classical control field applied to the MNP-SQD hybrid nanosystem, the kinds of metallic nanoparticles and the background media, r…
Silicon vacancy (SiV) centers in diamonds have emerged as a very promising candidate for quantum emitter due to their narrow emission line resulting in their indistinguishability. While many different quantum emitters have already been used for excitation of various propagating plasmonic modes, the corresponding exploitation of SiV centers remained so far uncharted territory. Here, we report on excitation of surface plasmon modes supported by silver nanowires using SiV centers in nanodiamonds. The coupling of SiV center fluorescence to surface plasmons is observed, when a nanodiamond situated …
Plasmonic waveguides are an essential element of nanoscale coherent sources, including nanolasers and four-wave mixing (FWM) devices. Here we report how the design of the plasmonic waveguide needs to be guided by the ultimate application. This contrasts with traditional approaches in which the waveguide is considered in isolation. We find that hybrid plasmonic waveguides, with a nonlinear material sandwiched between the metal substrate and a high-index layer, are best suited for FWM applications, whereas metallic wedges are preferred in nanolasers. We also find that in plasmonic nanolasers hig…
Plasmonic nanolithography is a nanofabrication technique which exploits surface plasmons to generate subdiffraction patterns. In this review, we highlight the key concepts in plasmonic nanolithography, review the pioneering papers and provide a classification that can be useful in determining the proper method and tool for subdiffraction patterning. Considering the ongoing developments in the field of plasmonics, lithography using surface plasmons is an extremely promising approach for development of high-throughput nanofabrication techniques.
A rigorous theory of photon emission accompanied inelastic tunnelling inside the gap of plasmonic nanoantennas has been developed. The disappointingly low efficiency of the electrical excitation of surface plasmon polaritons in these structures can be increased by orders of magnitude when a resonant tunnelling structure is incorporated inside the gap. Resonant tunnelling assisted surface plasmon emitter may become a key element in future electrically-driven nanoplasmonic circuits.
Quantum dots optically excited in close proximity to a silver nanowire can launch nanowire surface plasmons. The challenge related to this promising hybrid system is to control the position of nanoemitters on the nanowire. We report on the use of two-photon photopolymerization process to strategically position quantum dots on nanowires at controlled sites. A parametric study of the distance between the quantum dots and the nanowire extremity shows that precise control of the position of the launching sites enables control of light intensity at the wire end, through surface plasmon propagation.
Plasmonic circuitry is considered as a promising solution-effective technology for miniaturizing and integrating the next generation of optical nano-devices. A key element is the shared metal network between electrical and optical information enabling an efficient hetero-integration of an electronic control layer and a plasmonic data link. Here, we investigate to what extend surface plasmons and current-carrying electrons interfere in such a shared circuitry. By synchronously recording surface plasmon propagation and electrical output characteristics of single chemically-synthesized silver nan…
Metal-dielectric interfaces of various geometries are fundamental photonic material platforms for surface plasmons. Surface plasmon polaritons and localized surface plasmons are two surface plasmon modes that are excited on planar and curved metal-dielectric interfaces, respectively. Herein, we demonstrate in-situ formation of silver nanoparticles by diffusion at a planar interface between sputter-deposited silver and nitride dielectrics. In one step, we synthesize a nanostructure that exhibits both localized surface plasmon resonances at silver nanoparticles and surface plasmon resonances at …
We launch surface plasmons from one end of a silver nanowire by asymmetric illumination with white light and use plasmon-to-light scattering at the nanowire ends to probe spectroscopically the plasmonic Fabry-Perot wire modes. The spectral positions of the maxima and minima in the scattered intensity from both nanowire ends are found to be either in phase or out-of phase, depending on the nanowire length and the spectral range. This behavior can be explained by a generalized Fabry-Perot model. The turnover-point between the two regimes is sensitive to the surface plasmon round trip losses and …
We demonstrate plasmon-enhanced photoconduction in Au bowtie nanojunctions containing nanogaps overlaid with an amorphous Ge film. The role of plasmons in the production of nanogap photocurrent is verified by studying the unusual polarization dependence of the photoresponse. With increasing Ge thickness, the nanogap polarization of the photoresponse rotates 90 degrees, indicating a change in the dominant relevant plasmon mode, from the resonant transverse plasmon at low thicknesses to the nonresonant "lightning rod" mode at higher thicknesses. To understand the plasmon response in the presence…
Carbon nanotubes provide a rare access point into the plasmon physics of one-dimensional electronic systems. By assembling purified nanotubes into uniformly sized arrays, we show that they support coherent plasmon resonances, that these plasmons enhance and hybridize with phonons, and that the phonon-plasmon resonances have quality factors as high as 10. Because coherent nanotube plasmonics can strengthen light-matter interactions, it provides a compelling platform for surface-enhanced infrared spectroscopy and tunable, high-performance optical devices at the nanometer scale.
We investigate theoretically the optical properties associated to plasmon resonances of metal nanowires with cross section given by low-order Chebyshev nanoparticles (like rounded-tip nanostars or nanoflowers). The impact of the nanoflower shape is analyzed for varying symmetry and deformation parameter through the spectral dependence of resonances, and their corresponding near field distributions. Large field intensity enhancements are obtained at the gaps between petals, apart from the tips themselves, which make these nanostars/nanoflowers specially suitable to host molecules for SERS sensi…
In a proposed book chapter surface plasmon polariton assisted optical switching in noble metal nanoparticle systems is discussed in the sub-band gap formalism.
We develop a quantum-mechanical theory for Landau damping of surface plasmons in metal nanostructures larger that the characteristic length for nonlocal effects. We show that the electron surface scattering, which facilitates plasmon decay in small nanostructures, can be incorporated into the metal dielectric function on par with phonon and impurity scattering. The derived surface scattering rate is determined by the plasmon local field polarization relative to the metal-dielectric interface and is highly sensitive to the system geometry. We illustrate our model by providing analytical results…
Ultrabroad resonance of localized plasmon on a nanoparticle coupled with surface plasmon on a nanowire enabling two-photon excited emission via continuous-wave laser
We develop a theory for spontaneous decay of a quantum emitter (QE) situated near metal-dielectric structure supporting localized surface plasmons. If plasmon resonance is tuned close to the QE emission frequency, the emission is enhanced due to energy transfer from the QE to a localized plasmon mode followed by photon emission by plasmonic antenna. The emission rate is determined by intimate interplay between the plasmon coupling to radiation field and the Ohmic losses in metal. Here we develop plasmon Green's function approach that includes plasmon's interaction with radiation to obtain expl…
We present theoretical and experimental studies of the optical response of L-shaped silver nanoparticles. The scattering spectrum exhibits several plasmon resonances that depend sensitively on the polarization of the incident electromagnetic field. The physical origin of the resonances is traced to different plasmon phenomena. In particular, a high energy band with unusual properties is interpreted in terms of volume plasmon oscillations arising from the asymmetry of a nanoparticle.
We report sensing of single nanoparticles using disordered metallic nanoisland substrates supporting surface plasmon polaritons (SPPs). Speckle patterns arising from leakage radiation of elastically scattered SPPs provides a unique fingerprint of the scattering microstructure at the sensor surface. Experimental measurements of the speckle decorrelation are presented and shown to enable detection of sorption of individual gold nanoparticles and polystyrene beads. Our approach is verified through bright-field and fluorescence imaging of particles adhering to the nanoisland substrate.
Plasmon-assisted hot carrier processes in metal nanoparticles can be described either classically or using the full strength of quantum mechanics. We reconfirm that from the practical applications point of view, when it comes to description of the decay of plasmons in nanoparticles, classical description is sufficiently adequate for all but the smallest of the nanoparticles. At the same time, the electron temperature rise in nanoparticles is discrete (quantized) and neglecting this fact can lead to significant underestimating of hot carrier assisted effects, such as photo-catalysis.
A canonical quantization scheme for localized surface plasmons (LSPs) in a metal nanosphere is presented based on a microscopic model composed of electromagnetic fields, oscillators that describe plasmons, and a reservoir that describes excitations other than plasmons. The eigenmodes of this fully quantum electrodynamic theory show a spectrum that includes radiative depolarization and broadening, including redshifting from the quasi-static LSP modes, with increasing particle size. These spectral profiles correctly match those obtained with exact classical electrodynamics (Mie theory). The pres…
We predict the simultaneous occurrence of two fundamental phenomena for metal nanoparticles possessing sharp corners: First, the main plasmonic dipolar mode experiences strong red shift with decreasing corner curvature radius; its resonant frequency is controlled by the apex angle of the corner and the normalized (to the particle size) corner curvature. Second, the split-off plasmonic mode experiences strong localization at the corners. Altogether, this paves the way for tailoring of metal nano-structures providing wavelength-selective excitation of localized plasmons and a strong near-field e…
Single-molecule surface enhanced Raman scattering (SM-SERS) is one of the vital applications of plasmonic nanoparticles. The SM-SERS sensitivity critically depends on plasmonic hot-spots created at the vicinity of such nanoparticles. In conventional fluid-phase SM-SERS experiments, plasmonic hot-spots are facilitated by chemical aggregation of nanoparticles. Such aggregation is usually irreversible, and hence, nanoparticles cannot be re-dispersed in the fluid for further use. Here, we show how to combine SM-SERS with plasmon-polariton assisted, reversible assembly of plasmonic nanoparticles at…
