In a proposed book chapter surface plasmon polariton assisted optical switching in noble metal nanoparticle systems is discussed in the sub-band gap formalism.
The use of magneto-optical techniques to tune the plasmonic response of nanostructures is a hot topic in active plasmonics, with fascinating implications for several plasmon-based applications and devices. For this emerging field, called magnetoplasmonics, plasmonic nanomaterials with strong optical response to magnetic field are desired, which is generally challenging to achieve with pure noble metals. To overcome this issue, several efforts have been carried out to design and tailor the magneto-optical response of metal nanostructures, mainly by combining plasmonic and magnetic materials in …
Optical field interacting with a topologically protected one-dimensional helical state is shown to support a one-dimensional plasmon-polariton that is characterized by a non-linear dispersion. In a two-dimensional Dirac magnet these electro-optical excitations are confined to domain walls, thus, offering a possibility to manipulate quantum optical states by altering magnetic domain configurations. An exact spectral equation for such a topological plasmon-polariton is derived.
Phonon polaritons in natural anisotropic crystals hold great promise for infrared nano-optics. However, the direct electrical control of these polaritons is difficult, preventing the development of active polaritonic devices. Here we propose the heterostructures of graphene on a biaxial crystal (α-phase molybdenum trioxide) slab and theoretically study the hybridized plasmon-phonon polaritons with dependence on the Fermi level of graphene from three aspects: dispersion relationships, iso-frequency contours, and the quantum spin Hall effects. We demonstrate the distinct wavelength tunability of…
The collective oscillations of surface charges (surface plasmons) induced by light-matter interactions were predicted in the 1950s to influence electrical conduction in 2D noble metals. Primarily two mechanisms were predicted and later by Frohlich which could affect the electron transport in metals; (1) Umklapp electron-electron scattering and (2) attractive interaction between free electrons in transition metals because of screening of the d-band electrons by the s-band electrons. [1] However, there is no experimental evidence to date on how such oscillations might influence the electrical co…
Plasmonic structures are known to support the modes with subwavelength volumes in which the field matter interactions are greatly enhanced. Coupling between the molecular excitations and plasmons leading to formation of plexcitons has been investigated for a number of organic molecules. However, plasmon-exciton coupling in metal semiconductor structures have not experienced the same degree of attention. In this work we show that the very strong coupling regime in which the Rabi energy exceeds the exciton binding energy is attainable in semiconductor cladded plasmonic nanoparticles and leads to…
We theoretically investigate plasmon polaritons in cubic lattices of spherical metallic nanoparticles. The nanoparticles, each supporting triply-degenerate localized surface plasmons, couple through the Coulomb dipole-dipole interaction, giving rise to collective plasmons that extend over the whole metamaterial. The latter hybridize with photons forming plasmon polaritons, which are the hybrid light-matter eigenmodes of the system. We derive general analytical expressions to evaluate both plasmon and plasmon-polariton dispersions, and the corresponding eigenstates. These are obtained within a …
Surface plasmon polaritons on soft-boundary graphene nanoribbons and their application as voltage controlled plasmonic switches and frequency demultiplexers
Polaritons are compositional light-matter quasiparticles that have recently enabled remarkable breakthroughs in quantum and nonlinear optics, as well as in material science. Despite the enormous progress, however, a direct nanometer-scale visualization of polaritons has remained an open challenge. Here, we demonstrate that plasmon-exciton polaritons, or plexcitons, generated by a hybrid system composed of an individual silver nanoparticle and a few-layer transition metal dichalcogenide can be spectroscopically mapped with nanometer spatial resolution using electron energy loss spectroscopy in …
In the present work we theoretically investigated the excitation of surface plasmon-polaritons (SPPs) in deformed graphene by attenuated total reflection method. We considered the Otto geometry for SPPs excitation in graphene. Efficiency of SPPs excitation strongly depends on the SPPs propagation direction. The frequency and the incident angle of the most effective excitation of SPPs strongly depend on the polarization of the incident light. Our results may open up the new possibilities for strain-induced molding flow of light at nanoscales.
We propose a mechanism of angular momentum conversion from optical transverse spin in surface plasmon polaritons (SPPs) to conduction electron spin. Free electrons in the metal follow the transversally spinning electric field of SPP, and the resulting orbital motions create inhomogeneous static magnetisation in the metal. By solving the spin diffusion equation in the SPP, we find that the magnetisation field generates an electron spin current. We show that there exists a resonant condition where the spin current is resonantly enhanced, and the polarisation of the spin current is flipped. Our t…
Laser-launched evanescent surface plasmon polariton field utilized as a direct coherent pumping source to generate emitted nonlinear four-wave mixing radiation
We investigated, both experimentally and theoretically, the reflection phase shift (RPS) of one-dimensional plasmon polaritons. We launched 1D plasmon polaritons in carbon nanotube and probed the plasmon interference pattern using scanning near-field optical microscopy (SNOM) technique, through which a non-zero phase shift was observed. We further developed a theory to understand the nonzero phase shift of 1D polaritons, and found that the RPS can be understood by considering the evanescent field beyond the nanotube end. Interesting, our theory shows a strong dependence of RPS on polaritons wa…
We study a surface plasmon polariton mode that is strongly confined in the transverse direction and propagates along a periodically nanostructured metal-dielectric interface. We show that the wavelength of this mode is determined by the period of the structure, and may therefore, be orders of magnitude smaller than the wavelength of a plasmon-polariton propagating along a flat surface. This plasmon polariton exists in the frequency region in which the sum of the real parts of the permittivities of the metal and dielectric is positive, a frequency region in which surface plasmon polaritons do n…
We have investigated the spectrum of two-dimensional (2D) plasmon polaritons over the full range of magnetic fields. In our study, we investigate a disk-shaped two-dimensional electron system (2DES) with a metallic gate on the backside of the substrate. Importantly, we show that 2D plasmon polaritons hybridize with the TM$_0$ photonic mode of a dielectric waveguide formed by a sample substrate. We have developed a theory for plasmon-polaritons in an infinite 2DES. We find the experimental data to be in good agreement with the developed theory.
Surface plasmon polariton (SPP) is an electromagnetic wave which is tightly localised beyond the diffraction limit at metallic surfaces. Recently, it is theoretically proposed that the angular momentum conversion between the SPP and electrons. In this work, we have successfully measured SPP induced spin currents, which proves the fact that the angular momenta are interconverted. Such conversion from light to a spin current can be used as a coupler in a next generation spintronic computing with optical data transfer or storage.
Weyl semimetals have recently attracted extensive attention due to their anomalous band structure manifested by topological properties that lead to some unusual and unique physical properties. We investigate novel features of surface plasmon polaritons in a slot waveguide comprised from two semi-infinite Weyl semimetals. We consider symmetric Voigt-Voigt and Faraday-Faraday configurations for plasmon polaritons in two interfaces of waveguide and show that the resulting dispersion is symmetric and the propagation of surface plasmon polaritons is bidirectional. We introduce exotic and novel asym…
We consider a hybrid structure formed by graphene and an insulating antiferromagnet, separated by a dielectric of thickness up to $d\simeq 500 \,nm$. When uncoupled, both graphene and the antiferromagnetic surface host their own polariton modes coupling the electromagnetic field with plasmons in the case of graphene, and with magnons in the case of the antiferromagnet. We show that the hybrid structure can host two new types of hybrid polariton modes. First, a surface magnon-plasmon polariton whose dispersion is radically changed by the carrier density of the graphene layer, including a change…
We theoretically investigate surface plasmon polaritons propagating in the thin-film Weyl semimetals. We show how the properties of surface plasmon polaritons are affected by hybridization between plasmons localized at the two metal-dielectric interfaces. Generally, this hybridization results in new mixed plasmon modes, which are called short-range surface plasmons and long-range surface plasmons, respectively. We calculate dispersion curves of these mixed modes for three principle configurations of the axion vector describing axial anomaly in Weyl semimetals. We show that the partial lack of …
Surface plasmon polaritons in planar graphene superlattices with one-dimensional periodic mo-dulation of the band gap were studied. The interminiband contribution to the optical conductivity of this system was found by the equation of motion method for two cases: the Fermi level falls within one of the minigaps and the Fermi level is located within one of the minibands. It was shown that the optical conductivity of the system varies significantly in these cases. The spectra of surface plasmon polaritons in the system differs for them.
Surface plasmon polaritons in a strained slab of a Weyl semimetal with broken time-reversal symmetry are investigated. It is found that the strain-induced axial gauge field reduces frequencies of these collective modes for intermediate values of the wave vector. Depending on the relative orientation of the separation of Weyl nodes in momentum space, the surface normal, and the direction of propagation, the dispersion relation of surface plasmon polaritons could be nonreciprocal even in a thin slab. In addition, strain-induced axial gauge fields can significantly affect the localization propert…
Conventional and Acoustic Surface Plasmons on Noble Metal Surfaces: A Time-dependent Density Functional Theory Study
采用第一性原理计算方法研究了Cu、Ag和Au(111)表面的常规表面等离子体和声学表面等离子体。通过比较局域密度近似和轨道相关交换相关(xc)势的结果(该势改善了$d$带的位置和宽度),研究了$s-d$带间跃迁对两种类型等离子体激元的影响。用后者xc势计算的等离子体色散与电子能量损失谱(EELS)实验吻合得很好。对于CSP和ASP,对于等离子体激元能量,发现Cu $<$ Au $<$ Ag的相同趋势,并且归因于从Cu到Au和Ag的带间跃迁的减少的屏蔽。然而,ASP的这种趋势与先前的模型预测相矛盾。虽然ASP在EELS中被视为弱特征,但它可以在静态和动态介电能带结构中被清楚地识别。
It is well known that collective electronic excitations in fullerene C$_{60}$ are manifested as Mie plasmons, and in graphene (the limiting case of an infinitely large fullerene) collective excitations are of plasmon-polariton type. How the properties of plasmons change in fullerenes with intermediate sizes is poorly understood. This problem is considered in current paper in the framework of the GW approximation on the example of fullerenes C$_{60}$, C$_{240}$ and C$_{540}$. The calculations show that a high-frequency plasmon-polariton resonance begins to form in C$_{240}$, and in C$_{540}$ th…
Transverse-electric (TE) surface plasmon polaritons are unique eigenmodes of a homogeneous graphene layer that are tunable with the chemical potential and temperature. However, as their dispersion curve spectrally lies just below the light line, they cannot be resonantly excited by an externally incident wave. Here, we propose a way of exciting the TE modes and tuning their peaks in the transmission by introducing a one-dimensional graphene grating. Using the scattering-matrix formalism, we show that periodic modulations of graphene make the transmission more pronounced, potentially allowing f…
The dispersion relation of surface plasmon polaritons in graphene that includes optical losses is often obtained for complex wave vectors while the frequencies are assumed to be real. This approach, however, is not suitable for describing the temporal dynamics of optical excitations and the spectral properties of graphene. Here, we propose an alternative approach that calculates the dispersion relation in the complex frequency and real wave vector space. This approach provides a clearer insight into the optical properties of a graphene layer and allows us to find the surface plasmon modes of a…
The plasmon and phonon polaritons of two-dimensional (2d) and van-der-Waals materials have recently gained substantial interest. Unfortunately, they are notoriously hard to observe in linear response because of their strong confinement, low frequency and longitudinal mode symmetry. Here, we propose a fundamentally new approach of harnessing nonlinear resonant scattering that we call stimulated plasmon polariton scattering (SPPS) in analogy to the opto-acoustic stimulated Brillouin scattering (SBS). We show that SPS allows to excite, amplify and detect 2d plasmon and phonon polaritons all acros…