Noise is a result of stochastic processes that originate from quantum or classical sources. Higher-order cumulants of the probability distribution underlying the stochastic events are believed to contain details that characterize the correlations within a given noise source and its interaction with the environment, but they are often difficult to measure. Here we report measurements of the transient cumulants <<n^m>> of the number n of passed charges to very high orders (up to m=15) for electron transport through a quantum dot. For large m, the cumulants display striking oscillations as functions of measurement time with magnitudes that grow factorially with m. Using mathematical properties of high-order derivatives in the complex plane we show that the oscillations of the cumulants in fact constitute a universal phenomenon, appearing as functions of almost any parameter, including time in the transient regime. These ubiquitous oscillations and the factorial growth are system-independent and our theory provides a unified interpretation of previous theoretical studies of high-order cumulants as well as our new experimental data.
We investigate the quantum transport in a generalized N-particle Hanbury Brown--Twiss setup enclosing magnetic flux, and demonstrate that the Nth-order cumulant of current cross correlations exhibits Aharonov-Bohm oscillations, while there is no such oscillation in all the lower-order cumulants. The multiparticle interference results from the orbital Greenberger-Horne-Zeilinger entanglement of N indistinguishable particles. For sufficiently strong Aharonov-Bohm oscillations the generalized Bell inequalities may be violated, proving the N-particle quantum nonlocality.
We discuss the counting statistics and current noise associated with the double Josephson quasiparticle resonance point in a superconducting single electron transistor. The counting statistics are in general phase-dependent, despite the fact that the average current has no dependence on phase. Focusing on parameter regimes where the counting statistics have no phase-dependence, we use a general relation first derived by MacDonald in 1948 to obtain the full frequency-dependent shot noise directly from the counting statistics, without any further approximations. We comment on problems posed by t…
We review the relations between the full counting statistics and the field theory of electric circuits. We demonstrate that for large conductances the counting statistics is determined by non-trivial saddle-point of the field. Coulomb effects in this limit are presented as quantum corrections that can stongly renormalize the action at low energies.
We study analytically the full counting statistics of charge transport through single molecules, strongly coupled to a weakly damped vibrational mode. The specifics of transport in this regime - a hierarchical sequence of avalanches of transferred charges, interrupted by "quiet" periods - make the counting statistics strongly non-Gaussian. We support our findings for the counting statistics as well as for the frequency-dependent noise power by numerical simulations, finding excellent agreement.
We derive the full counting statistics of charge transfer through a voltage biased superconducting junction. We find that for measurement times much longer than the inverse Josephson frequency, the counting statistics describes a correlated transfer of quanta of multiple electron charges, each quantum associated with the transfer of a single quasiparticle. An expression for the the counting statistics in terms of the quasiparticle scattering amplitudes is derived.
Full counting statistics is a fundamentally new concept in quantum transport. After a review of basic statistics theory, we introduce the powerful Green's function approach to full counting statistics. To illustrate the concept we consider a number of examples. For generic two-terminal contacts we show how counting statistics elucidates the common (and different) features of transport between normal and superconducting contacts. Finally, we demonstrate how correlations in multi-terminal structures are naturally included in the formalism.
In the hot electron regime, electron-electron scattering strongly modifies not only the shot noise but also the full counting statistics. We employ a method based on a stochastic path integral to calculate the counting statistics of two systems in which noise in the hot electron regime has been experimentally measured. We give an analytical expression for the counting statistics of a chaotic cavity and find that heating due to electron-electron scattering renders the distribution of transmitted charge symmetric in the shot noise limit. We also discuss the frequency dispersion of the third orde…
We present measurements of the time-dependent fluctuations in electrical current in a voltage-biased tunnel junction. We were able to simultaneously extract the first three moments of the tunnel current counting statistics. Detailed comparison of the second and the third moment reveals that counting statistics is accurately described by the Poissonian distribution expected for spontaneous current fluctuations due to electron charge discreteness, realized in tunneling transport at negligible coupling to environment.
Full counting statistics is a powerful tool to characterize the noise and correlations in transport through mesoscopic systems. In this work, we propose the theory of conditional spin counting statistics, i.e., the statistical fluctuations of spin-up (down) current given the observation of the spin-down (up) current. In the context of transport through a single quantum dot, it is demonstrated that a strong Coulomb interaction leads to a conditional spin counting statistics that exhibits a substantial change in comparison to that without Coulomb repulsion. It thus can be served as an effective …
We present a stochastic path integral method to calculate the full counting statistics of conductors with energy conserving dephasing probes and dissipative voltage probes. The approach is explained for the experimentally important case of a Mach-Zehnder interferometer, but is easily generalized to more complicated setups. For all geometries where dephasing may be modeled by a single one-channel dephasing probe we prove that our method yields the same full counting statistics as phase averaging of the cumulant generating function.
We study the full counting statistics of current of large open systems through the application of random matrix theory to transition-rate matrices. We develop a method for calculating the ensemble-averaged current-cumulant generating functions based on an expansion in terms of the inverse system size. We investigate how different symmetry properties and different counting schemes affect the results.
We discuss how threshold detectors can be used for a direct measurement of the full counting statistics (FCS) of current fluctuations and how to implement Jose phson junctions in this respect. We propose a scheme to characterize the full co unting statistics from the current dependence of the escape rate measured. We il lustrate the scheme with explicit results for tunnel, diffusive and quasi-ballis tic mesoscopic conductors.
We study the full counting statistics of heterostructures consisting of normal metal parts connected to a superconducting terminal. Assuming that coherent superconducting correlations are suppressed in the normal metals we show, using Keldysh-Nambu Green's functions, that the system can be mapped onto a purely normal system with twice the number of elements. For a superconducting beam splitter with several normal terminals we obtain general results for the counting statistics.
We present a theory for the full distribution of current fluctuations in incoherent diffusive superconducting junctions, subjected to a voltage bias. This theory of full counting statistics of incoherent multiple Andreev reflections is valid for arbitrary applied voltage. We present a detailed discussion of the properties of the first four cumulants as well as the low and high voltage regimes of the full counting statistics. The work is an extension of the results of Pilgram and the author, Phys. Rev. Lett. 94, 086806 (2005).
We consider current shot noise and the full counting statistics in a chain of quantum dots which exhibits a continuous non-equilibrium phase transition as a function of the tunnel couplings of the chain with the electrodes. Using a combination of analytical and numerical methods, we establish that the full counting statistics is conventional away from the phase transition, but becomes, in a well-defined sense, essentially non-Gaussian on the critical line, where the current fluctuations are controlled by the dynamic critical exponent $z$. We find that signatures of the critical full counting s…
Using a microscopic model for stochastic transport through a single quantum dot that is modified by the Coulomb interaction of environmental (weakly coupled) quantum dots, we derive generic properties of the full counting statistics for multi-stable Markovian transport systems. We study the temporal crossover from multi-modal to broad uni-modal distributions depending on the initial mixture, the long-term asymptotics and the divergence of the cumulants in the limit of a large number of transport branches. Our findings demonstrate that the counting statistics of a single resonant level may be u…
We explore the full counting statistics of single electron tunneling through a quantum dot using a quantum point contact as non-invasive high bandwidth charge detector. The distribution of counted tunneling events is measured as a function of gate and source-drain-voltage for several consecutive electron numbers on the quantum dot. For certain configurations we observe super-Poissonian statistics for bias voltages at which excited states become accessible. The associated counting distributions interestingly show a bimodal characteristic. Analyzing the time dependence of the number of electron …
Measurements of single electron tunneling through a quantum dot using a quantum point contact as charge detector have been performed for very long time traces with very large event counts. This large statistical basis is used for a detailed examination of the counting statistics for varying symmetry of the quantum dot system. From the measured statistics we extract high order cumulants describing the distribution. Oscillations of the high order cumulants are observed when varying the symmetry. We compare this behavior to the observed oscillation in time dependence and show that the variation o…
We study the full counting statistics of electric current to several drain terminals with spin-dependent entrance conductances. We show that the statistics of charge transfers can be interpreted in terms of single electrons and spin-singlet pairs coming from the source. If the source contains transport channels of high transparency, a significant fraction of electrons comes in spin-singlet pairs.
Full counting statistics of electron transport is a powerful diagnostic tool for probing the nature of quantum transport beyond what is obtainable from the average current or conductance measurement alone. In particular, the non-Markovian dynamics of quantum dot molecule plays an important role in the nonequilibrium electron tunneling processes. It is thus necessary to understand the non-Markovian full counting statistics in a quantum dot molecule. Here we study the non-Markovian full counting statistics in two typical quantum dot molecules, namely, serially coupled and side-coupled double qua…
We describe a method for calculating the counting statistics of electronic transport through nanoscale devices with both sequential and cotunneling contributions. The method is based upon a perturbative expansion of the von Neumann equation in Liouvillian space, with current cumulants calculated from the resulting nonMarkovian master equation without further approximation. As application, we consider transport through a single quantum dot and discuss the effects of cotunneling on noise and skewness, as well as the properties of various approximation schemes.
We derive a stochastic path integral representation of counting statistics in semi-classical systems. The formalism is introduced on the simple case of a single chaotic cavity with two quantum point contacts, and then further generalized to find the propagator for charge distributions with an arbitrary number of counting fields and generalized charges. The counting statistics is given by the saddle point approximation to the path integral, and fluctuations around the saddle point are suppressed in the semi-classical approximation. We use this approach to derive the current cumulants of a chaot…
We investigate the effect of weak interactions on the full counting statistics of charge transfer through an arbitrary mesoscopic conductor. We show that the main effect can be incorporated into an energy dependence of the transmission eigenvalues and study this dependence in a non-perturbative approach. An unexpected result is that all mesoscopic conductors behave at low energies like either a single or a double tunnel junction, which divides them into two broad classes.
We develop a self-consistent version of perturbation theory in Liouville space which seeks to combine the advantages of master equation approaches in quantum transport with the nonperturbative features that a self-consistent treatment brings. We describe how counting fields may be included in a self-consistent manner in this formalism such that the full counting statistics can be calculated. NonMarkovian effects are also incorporated. Several different self-consistent approximations are introduced and we discuss their relative strengths with a simple example.
Destructive interference of single-electron tunneling between three quantum dots can trap an electron in a coherent superposition of charge on two of the dots. Coupling to external charges causes decoherence of this superposition, and in the presence of a large bias voltage each decoherence event transfers a certain number of electrons through the device. We calculate the counting statistics of the transferred charges, finding a crossover from sub-Poissonian to super-Poissonian statistics with increasing ratio of tunnel and decoherence rates.
We present here a quantum mechanical framework for defining the statistics of measurements of time integrals of A(t), A(t) being a quantum mechanical variable. This is a generalization of the so-called full counting statistics proposed earlier for DC electric currents. We develop an influence functional formalism that allows us to study the quantum system along with the measuring device thus fully accounting for the action of the detector on the system to be measured. We define the full counting statistics of an arbitrary variable by means of an evolution operator that relates initial and fina…
The article develops a powerful theoretical tool to obtain the full counting statistics. By a slight extension of the standard Keldysh method we can access immediately all correlation functions of the current operator. Embedded in a quantum generalization of the circuit theory of electronic transport, we are able to study the full counting statistics of a large class of two-terminal contacts and multi-terminal structures, containing superconductors and normal metals as elements. The practical use of the method is demonstrated in many examples.
We revisit the problem of full counting statistics of particles on a segment of a one-dimensional gas of free fermions. Using a combination of analytical and numerical methods, we study the crossover between the counting of discrete particles and of the continuous particle density as a function of smoothing in the counting procedure. In the discrete-particle limit, the result is given by the Fisher--Hartwig expansion for Toeplitz determinants, while in the continuous limit we recover the bosonization results. This example of full counting statistics with smoothing is also related to orthogonal…
We use the inchworm Quantum Monte Carlo method to investigate the full counting statistics of particle and energy currents in a strongly correlated quantum dot. Our method is used to extract the heat fluctuations and entropy production of a quantum thermoelectric device, as well as cumulants of the particle and energy currents. The energy--particle current cross correlations reveal information on the preparation of the system and the interplay of thermal and electric currents. We furthermore demonstrate the signature of a crossover from Coulomb blockade to Kondo physics in the energy current f…
We consider full counting statistics of spin in matrix product states. In particular, we study the approach to gaussian distribution for magnetization. We derive the asymptotic corrections to the central limit theorem for magnetization distribution for finite but large blocks in analogy to the Edgeworth series. We also show how central limit theorem like behavior is modified for certain states with topological characteristics such as the AKLT state.
We study Markovian stochastic motion on a graph with finite number of nodes and adiabatically periodically driven transition rates. We show that, under general conditions, the quantized currents that appear at low temperatures are a manifestation of topological invariants in the counting statistics of currents. This observation provides an approach for classification of topological properties of the counting statistics, as well as for extensions of the phenomenon of the robust quantization of currents at low temperatures to the properties of the counting statistics which persist to finite temp…
We present a theory of full counting statistics for electron transport through interacting electron systems with non-Markovian dynamics. We illustrate our approach for transport through a single-level quantum dot and a metallic single-electron transistor to second order in the tunnel-coupling strength, and discuss under which circumstances non-Markovian effects appear in the transport properties.
The joint probability distribution in the full counting statistics (FCS) for noninteracting electrons is discussed for an arbitrary number of initially separate subsystems which are connected at t=0 and separated at a later time. A simple method to obtain the leading order long time contribution to the logarithm of the characteristic function is presented which simplifies earlier approaches. New explicit results for the determinant involving the scattering matrices are found. The joint probability distribution for two leads is discussed for Y-junctions and dots connected to four leads.
We study the trace of the exponentials of general fermion bi-linears, including pairing terms, and including non Hermitian forms. In particular, we give elementary derivations for determinant and pfaffian formulae for such traces, and use these to obtain general expressions for the full counting statistics in states associated with quadratic Hamiltonians including BCS-like pairing terms and fermion parity in a prescribed region or set of modes. We also derive pfaffian expressions for state overlaps and counting statistics in states built out of the vacuum by creation of pairs of particles.
We calculate the charge transport in a flux biased dissipative Cooper pair pump using the method of full counting statistics (FCS). This is instead of a more traditional technique of integrating a very small expectation value of the instantaneous current over the pumping period. We show that the rotating wave approximation (RWA), which fails in the traditional technique, produces accurate results within the FCS method.
Stochastic systems feature, in general, both coherent dynamics and incoherent transitions between different states. We propose a method to identify the coherent part in the full counting statistics for the transitions. The proposal is illustrated for electron transfer through a quantum-dot spin valve, which combines quantum-coherent spin precession with electron tunneling. We show that by counting the number of transferred electrons as a function of time, it is possible to distill out the coherent dynamics from the counting statistics even in transport regimes, in which other tools such as the…
We study full counting statistics of coherent electron transport through multi-terminal interacting quantum-dots under a finite magnetic field. Microscopic reversibility leads to the symmetry of the cumulant generating function, which generalizes the fluctuation theorem in the context of quantum transport. Using this symmetry, we derive the Onsager-Casimir relation in the linear transport regime and universal relations among nonlinear transport coefficients.
We investigate the dynamics of electron spin qubits in quantum dots. Measurement of the qubit state is realized by a charge current through the dot. The dynamics is described in the framework of the quantum trajectory approach, widely used in quantum optics, and we show that it can be applied successfully to problems in condensed matter physics. The relevant master equation dynamics is unravelled to simulate stochastic tunneling events of the current through the dot.Quantum trajectories are then used to extract the counting statistics of the current. We show how, in combination with an electro…
Explicit formulas are obtained for all moments and for all cumulants of the electric current through a quantum chaotic cavity attached to two ideal leads, thus providing the full counting statistics for this type of system. The approach is based on random matrix theory, and is valid in the limit when both leads have many open channels. For an arbitrary number of open channels we present the third cumulant and an example of non-linear statistics.
We review several ways of defining the statistics of charge that is transmitted through an electric circuit, the so-called "counting statistics". We first pursue two approaches that explain the origin of "negative probabilities" that have been found earlier in this context. The first analysis involves degrees of freedom of the electric circuit only. In the second approach an idealized charge detector is introduced. We study then general linear detectors and how their back action on the electric conductor affects the statistics of transferred charge. Phase-coherent conductors in the presence of…
Using a simple quantum master equation approach, we calculate the Full Counting Statistics of a single electron transistor strongly coupled to vibrations. The Full Counting Statistics contains both the statistics of integrated particle and energy currents associated to the transferred electrons and phonons. A universal as well as an effective fluctuation theorem are derived for the general case where the various reservoir temperatures and chemical potentials are different. The first relates to the entropy production generated in the junction while the second reveals internal information of the…
A complete characterization of quantum fluctuations in many-body systems is accessible through the full counting statistics. We present an exact computation of statistical properties of light in a basic model of light-matter interaction: a multimode photonic field coupled to a single two-level emitter. We mostly consider an initial coherent state in a given mode and demonstrate how the original Poissonian statistics gets modified because of quantum many-body scattering effects leading to non-Poissonian distributions. We argue that measuring this statistics in a simple quantum optical setup pro…
We demonstrate time-resolved counting of single atoms extracted from a weakly interacting Bose-Einstein condensate of $^{87}$Rb atoms. The atoms are detected with a high-finesse optical cavity and single atom transits are identified. An atom laser beam is formed by continuously output coupling atoms from the Bose-Einstein condensate. We investigate the full counting statistics of this beam and measure its second order correlation function $g^{(2)}(τ)$ in a Hanbury Brown and Twiss type experiment. For the monoenergetic atom laser we observe a constant correlation function $g^{(2)}(τ)=1.00\pm0.0…
Exact numerical results for the full counting statistics (FCS) of a one-dimensional tight-binding model of noninteracting electrons are presented at finite temperatures using an identity recently presented by Abanov and Ivanov. A similar idea is used to derive a new expression for the cumulant generating function for a system consisting of two quasi-one-dimensional leads connected by a quantum dot in the long time limit. This provides a generalization of the Levitov-Lesovik formula for such systems.
We present a general technique to obtain the zero temperature full counting statistics of charge transfer in interacting impurity models out of equilibrium from time-dependent simulations on a lattice. We demonstrate the technique with application to the self-dual interacting resonant level model, where very good agreement between numerical simulations using the density matrix renormalization group and those obtained analytically from the thermodynamic Bethe ansatz is found. We show from the exact form of counting statistics that the quasiparticles involved in transport carry charge $2e$ in th…
We propose a procedure to reconstruct characteristic features of an unknown stochastic system from the long-time full counting statistics of some of the system's transitions that are monitored by a detector. The full counting statistics is conveniently parametrized by so-called generalized factorial cumulants. Taking only a few of them as input information is sufficient to reconstruct important features such as the lower bound of the system dimension and the full spectrum of relaxation rates. The use of generalized factorial cumulants reveals system dimensions and rates that are hidden for ord…
The full counting statistics of a non adiabatic pure spin pump are calculated with particular emphasis on the second and third moments. We show that incoherence can change the sign of spin shot noise cross-correlations from negative to positive, implying entanglement for spin-singlet electronic sources, a truly counterintuitive result. The third moment on the other hand is shown to be much more resilient to incoherence.
We study the effect of Coulomb interaction on the full counting statistics of an Aharonov-Bohm (AB) interferometer with a single-level quantum dot in one arm in the regime of weak dot-lead and lead-lead tunnel couplings. In the absence of Coulomb interaction, the interference processes are of nonresonant nature with an even AB flux dependence and obey bidirectional Poissonian statistics. For large charging energy, the statistic of these processes changes. In addition, processes of resonant nature with an odd flux dependence appear. In the limit of strongly asymmetric tunnel couplings from the …
In order to fully characterize the noise associated with electron transport, with its severe consequences for solid-state quantum information systems, the theory of full counting statistics has been developed. It accounts for correlation effects associated with the statistics and effects of entanglement, but it remains a non-trivial task to account for interaction effects. In this article we present two examples: we describe electron transport through quantum dots with strong charging effects beyond perturbation theory in the tunneling, and we analyze current fluctuations in a diffusive intera…
The full counting statistics of a molecular level weakly interacting with a local phonon mode is derived. We find an analytic formula that gives the behavior of arbitrary irreducible moments of the distribution upon phonon excitation. The underlying competition between quasi-elastic and inelastic processes results in the formation of domains in parameter space characterized by a given sign in the jump of the irreducible moments. In the limit of perfect transmission, the corresponding distribution is distorted from Gaussian statistics for electrons to Poissonian transfer of holes above the inel…
We propose a theory that treats the current, noise, and, generally, the full current statistics of electron transfer in a mesoscopic system in a unified, simple and efficient way. The theory appears to be a circuit theory of $2\times 2$ matrices associated with Keldysh Green functions. We illustrate the theory by considering the big fluctuations of currents in various three-terminal circuits.
We examine the full counting statistics of electron transport through double quantum dots coupled in series, with particular attention being paid to the unique features originating from level renormalization. It is clearly illustrated that the energy renormalization gives rise to a dynamic charge blockade mechanism, which eventually results in super-Poissonian noise. Coupling of the double dots to an external heat bath leads to dephasing and relaxation mechanisms, which are demonstrated to suppress the noise in a unique way.
We study the charge transfer in a small grain oscillating between two leads. Coulomb blockade restricts the charge fluctuations in such a way that only zero or one additional electrons can sit on the grain. The system thus acts as a charge shuttle. We obtain the full counting statistics of charge transfer and discuss its behavior. For large oscillation amplitude the probability of transferring $\tilde n$ electrons per cycle is strongly peaked around one. The peak is asymmetric since its form is controlled by different parameters for $\tilde n>1$ and $\tilde n < 1$. Under certain conditions the…
We propose a dynamical scheme for measuring the full counting statistics in a mesoscopic conductor using an electronic Mach-Zehnder interferometer. The conductor couples capacitively to one arm of the interferometer and causes a phase shift which is proportional to the number of transferred charges. Importantly, the full counting statistics can be obtained from average current measurements at the outputs of the interferometer. The counting field can be controlled by varying the time delay between two separate voltage signals applied to the conductor and the interferometer, respectively. As a s…
We present a general theory for the full counting statistics of multiple Andreev reflections in incoherent superconducting-normal-superconducting contacts. The theory, based on a stochastic path integral approach, is applied to a superconductor-double barrier system. It is found that all cumulants of the current show a pronounced subharmonic gap structure at voltages $V=2Δ/en$. For low voltages $V\llΔ/e$, the counting statistics results from diffusion of multiple charges in energy space, giving the $p$th cumulant $<Q^p> \propto V^{2-p}$, diverging for $p\geq 3$. We show that this low-voltage r…
We consider the transport of electrons passing through a mesoscopic device possessing internal dynamical quantum degrees of freedom. The mutual interaction between the system and the conduction electrons contributes to the current fluctuations, which we describe in terms of full counting statistics. We identify conditions where this discriminates coherent from incoherent internal dynamics, and also identify and illustrate conditions under which the device acts to dynamically bunch transmitted or reflected electrons, thereby generating super-Poissonian noise.
Non-adiabatic charge pumping through a single-level quantum dot with periodically modulated parameters is studied theoretically. By means of a quantum-master-equation approach the full counting statistics of the system is obtained. We find a trinomial-probability distribution of the charge transfer, which adequately describes the reversal of the pumping current by sweeping the driving frequency. Further, we derive equations of motion for current and noise, and solve those numerically for two different driving schemes. Both show interesting features which can be fully analyzed due to the simple…
The Cooper pair shuttle is a simple model system that combines features of coherent and incoherent transport. We evaluate the full counting statistics (FCS) of charge transfer via the shuttle in the incoherent regime. We describe two limiting cases when the FCS allows for classical interpretation. Generally, the classical interpretation fails yielding negative and imaginary "probabilities". This signals that superconducting coherence survives even in incoherent regime. We evaluate the current noise in some detail.
