We propose a quantum computation architecture of double-dot molecules, where the qubit is encoded in the molecule two-electron spin states. By arranging the two dots inside each molecule perpendicular to the qubit scaling line, the interactions between neighboring qubits are largely simplified and the scaling to multi-qubit system becomes straightforward. As an Ising-model effective interaction can be expediently switched on and off between any two neighboring molecules by adjusting the potential offset between the two dots, universal two-qubit gates can be implemented without requiring time-dependent control of the tunnel coupling between the dots. A Bell-state measurement scheme for qubit encoded in double-dot singlet and triplet states is also proposed for quantum molecules arranged in this way.
We show how to improve the efficiency for preparing Bell states in coupled two quantum dots system. A measurement to the state of driven quantum laser field leads to wave function collapse. This results in highly efficiency preparation of Bell states. The effect of decoherence on the efficiency of generating Bell states is also discussed in this paper. The results show that the decoherence does not affect the relative weight of $|00>$ and $|11>$ in the output state, but the efficiency of finding Bell states.
We propose a Bell measurement free scheme to implement a quantum repeater in GaAs/AlGa double qunatum dot systems.we prove the four pairs of double quantum dots compose an entanglement unit, given the the initial state is singlet states. Our shceme differs from the famous Duan-Lukin-Cirac-zoller(DLCZ) protocol in that Bell measurements are unneccessary for the entanglement swapping,which provides great advantages and conveniences in experimental implementaion. Our scheme significantly improve the success probability of quantum repeaters based on solid state quantum devices.
We introduce Bell-type inequalities allowing for non-locality and entanglement tests with two cold heteronuclear molecules. The proposed inequalities are based on correlations between each molecule spatial orientation, an observable which can be experimentally measured with present day technology. Orientation measurements are performed on each subsystem at diferent times. These times play the role of the polarizer angles in Bell tests realized with photons. We discuss the experimental implementations of the proposed tests, which could also be adapted to other high dimensional quantum angular m…
By exploiting the fermionic qubit parity measurement, we present a scheme to realize quantum non-demolition (QND) measurement of Bell-states and generate n-party GHZ state in quantum dot. Compared with the original protocol, the required electron transfer before and after parity measurement can be nonadiabatic, which may speed up the operation speed and make the omitting of spin-orbit interaction more reasonable. This may help us to construct CNOT gate without highly precise control of coupling as the way of D. Gottesman and I. L. Chuang.
Entanglement generated from polar molecules of two-dimensional rotation is investigated in a static electric field. The electric field modulates the rotational properties of molecules, leading to distinctive entanglement. The concurrence is used to estimate the degree of entanglement. When the electric field is applied parallel or perpendicular to the intermolecular direction, the concurrences reveal two overlapping features. Such a pronounced signature corresponds to the coexistence of all Bell-like states. The characteristics of Bell-like states and overlapping concurrences are kept independ…
Bell-state analysis (BSA) is essential in quantum communication, but it is impossible to distinguish unambiguously the four Bell states in the polarization degree of freedom (DOF) of two-photon systems with only linear optical elements, except for the case in which the BSA is assisted with hyperentangled states, the simultaneous entanglement in more than one DOF. Here, we propose a scheme to distinguish completely the 16 hyperentangled Bell states in both the polarization and the spatial-mode DOFs of two-photon systems, by using the giant nonlinear optics in quantum dot-cavity systems. This sc…
Recently, experiments showed that the spatial-mode states of entangled photons are more robust than their polarization-mode states in quantum communications. Here we construct a complete and deterministic protocol for analyzing the spatial Bell states using the interaction between a photon and an electron spin in a charged quantum dot inside a one-side micropillar microcavity. A quantum nondemolition detector (QND) for checking the parity of a two-photon system can be constructed with the giant optical Faraday rotation in this solid state system. With this parity-check QND, we present a comple…
Hyperentangled Bell-state analysis (HBSA) is critical for high-capacity quantum communication. Here we design two effective schemes for error-heralded deterministic generation and self-assisted complete analysis of hyperentangled Bell states for two-photon systems in both the polarization and spatial-mode degrees of freedom, assisted by single-sided quantum-dot-cavity systems. We construct an error-heralded block with a singly charged quantum dot inside a single-sided optical microcavity, two circular polarization beam splitters, one half-wave plate, and one single-photon detector, in which th…
We construct an error-detected block, assisted by the quantum-dot spins in double-sided optical microcavities. With this block, we propose three error-detected schemes for the deterministic generation, the complete analysis, and the complete nondestructive analysis of hyperentangled Bell states in both the polarization and spatial-mode degrees of freedom of two-photon systems. In these schemes, the errors can be detected, which can improve their fidelities largely, far different from other previous schemes assisted by the interaction between the photon and the quantum-dot-cavity system. Our sc…
We investigate the possibility of realizing a loophole-free violation of Bell's inequality using deterministic single-photon sources. We provide a detailed analysis of a scheme to achieve such violations over long distances with immediate extensions to device-independent quantum key distribution. We investigate the effect of key experimental imperfections that are unavoidable in real-world single-photon sources including the finite degree of photon indistinguishability, single-photon purity, and the overall source efficiency. We benchmark the performance requirements to state-of-the-art determ…
Cluster states, a special type of highly entangled states, are a universal resource for measurement-based quantum computation. Here, we propose an efficient one-step generation scheme for cluster states in semiconductor quantum dot molecules, where qubits are encoded on singlet and triplet state of two coupled quantum dots. By applying a collective electrical field or simultaneously adjusting interdot bias voltages of all double-dot molecule, we get a switchable Ising-like interaction between any two adjacent quantum molecule qubits. The initialization, the single qubit measurement, and the ex…
We develop a scalable architecture for quantum computation using controllable electrons of double-dot molecules coupled to a microwave stripline resonator on a chip, which satisfies all Divincenzo criteria. We analyze the performance and stability of all required operations and emphasize that all techniques are feasible with current experimental technologies.
We propose a scheme for full Bell state measurement of spin qubits in a double quantum dot. Our scheme consists of Pauli spin-blockade measurements and biaxial electron-spin resonance. In order to eliminate the average of the Zeeman fields, the double quantum dot is designed so that the Landé g-factors of first and second dots satisfy g1=g2 with the use of g-factor engineering. Thus, we can swap one of the three spin-triplet states for the spin-singlet state without disturbing the other states. Our study shows that the sequential spin-to-charge conversions enable us to implement the full Bell …
We theoretically investigate the joint photodetection probabilities of the biexciton-exciton cascade in single semiconductor quantum dots and analytically derive the density matrix and the Bell's inequalities of the entangled state. Our model includes different mechanisms that may spoil or even destroy entanglement such as dephasing, energy splitting of the relay excitonic states and incoherent population exchange between these relay levels. We explicitly relate the fidelity of entanglement to the dynamics of these processes and derive a threshold for violation of Bell's inequalities. Applied …
We show that excitons in coupled quantum dots are ideal candidates for reliable preparation of entangled states in solid-state systems. An optically controlled exciton transfer process is shown to lead to the generation of Bell and GHZ states in systems comprising two and three coupled dots, respectively. The strength and duration of selective light-pulses for producing maximally entangled states are identified by both analytic, and full numerical, solution of the quantum dynamical equations. Experimental requirements to build such entangled states are discussed.
Here we demonstrate, for the first time, violation of Bell's inequality using a triggered quantum dot photon-pair source without post-selection. Furthermore, the fidelity to the expected Bell state can be increased above 90% using temporal gating to reject photons emitted at times when collection of uncorrelated light is more probable. A direct measurement of a CHSH Bell inequality is made showing a clear violation, highlighting that a quantum dot entangled photon source is suitable for communication exploiting non-local quantum correlations.
Geometric manipulation of a quantum system offers a method for fast, universal, and robust quantum information processing. Here, we propose a scheme for universal all-geometric quantum computation using non-adiabatic quantum holonomies. We propose three different realizations of the scheme based on an unconventional use of quantum dot and single-molecule magnet devices, which offer promising scalability and robust efficiency.
In this Letter, we present a physical scheme for implementing the discrete quantum Fourier transform in a coupled semiconductor double quantum dot system. The main controlled-R gate operation can be decomposed into many simple and feasible unitary transformations. The current scheme would be a useful step towards the realization of complex quantum algorithms in the quantum dot system.
Bell's inequality in three coupled quantum dots (QDs) within cavity QED, including Forster and exciton-phonon interactions, is investigated theoretically. For an initially entangled state, Bell's inequality is valid for certain times and violated for some other times. It is shown that the system moves from a product state to a entangled state and back again during it's time evolution.
We theoretically investigate the phenomenon of voltage-controlled intracavity electromagnetically induced transparency with asymmetric double quantum dot system. The impact of voltage on frequency pulling and cavity linewidth narrowing are discussed. The linewidth and position of the cavity transmission can be engineered by the bias voltage. The scheme may be useful in integrated electro-optical device in quantum information process.
We propose a method for implementation of a quantum computer using artificial molecules. The artificial molecule consists of two coupled quantum dots stacked along z direction and one single electron. One-qubit and two-qubit gates are constructed by one molecule and two coupled molecules, respectively.The ground state and the first excited state of the molecule are used to encode the |0> and |1> states of a qubit. The qubit is manipulated by a resonant electromagnetic wave that is applied directly to the qubit through a microstrip line. The coupling between two qubits in a quantum controlled N…
In this paper we make a detailed study of the role of coherent tunneling, on the photocurrent and power delivered by a quantum dot molecule (QDM) in the presence of solar light. We focus our analysis on the coherence driven by tunneling and its impact on the photovoltaic properties of the QDM. The coherence developed by the system raises as a resource from the interplay between the strength of the tunneling coupling, the QDM band alignment, and the coupling rates with the reservoirs of thermal phonons. Our results show that a QDM can deliver up to 30% more power than a single quantum dot, and …
This work provides a complete description of entanglement properties between electrons inside coupled quantum molecules, nanoestructures which consist of two quantum dots. Each electron can tunnel between the two quantum dots inside the molecule, being also coupled by Coulomb interaction. First, it is shown that Bell states act as a natural basis for the description of this physical system, defining the characteristics of the energy spectrum and the eigenstates. Then, the entanglement properties of the eigenstates are discussed, shedding light on the roles of each physical parameters on experi…
Successful generation of photonic cluster states is the key step in the realization of measurement-based quantum computation and quantum network protocols. Several proposals for the generation of such entangled states from different solid-state emitters have been put forward. Each of these protocols come with their own challenges in terms of both conception and implementation. In this work we propose deterministic generation of these photonic cluster states from a spin-photon interface based on a hole spin qubit hosted in a quantum dot molecule. Our protocol resolves many of the difficulties o…
We propose a two-qubit optically controlled phase gate in quantum dot molecules via adiabatic passage and hole tunneling. Our proposal combines the merits of the current generation of vertically stacked self-assembled InAs quantum dots and adiabatic passage. The simulation shows an implementation of the gate with a fidelity exceeding 0.98.
We demonstrate the effects of cavity quantum electrodynamics for a quantum dot coupled to a photonic molecule, consisting of a pair of coupled photonic crystal cavities. We show anti-crossing between the quantum dot and the two super-modes of the photonic molecule, signifying achievement of the strong coupling regime. From the anti-crossing data, we estimate the contributions of both mode-coupling and intrinsic detuning to the total detuning between the super-modes. Finally, we also show signatures of off-resonant cavity-cavity interaction in the photonic molecule.
The puzzling behavior of the transition phase through a quantum dot can be understood in a natural way via a formation of the electron molecule in the quantum dot. In this case the resonance tunneling takes place through the quasi-stationary (doorway) state, which emerges when the number of electrons occupying the dot reaches a certain ``critical'' value, $N_{cr}$. Our estimation of this quantity agrees with the experimental data. The dependence of $N_{cr}$ on the dot's size is predicted as well.
We use photoluminescence spectroscopy to investigate the ground state of single self-assembled InGaAs lateral quantum dot molecules. We apply a voltage along the growth direction that allows us to control the total charge occupancy of the quantum dot molecule. Using a combination of computational modeling and experimental analysis, we assign the observed discrete spectral lines to specific charge distributions. We explain the dynamic processes that lead to these charge configurations through electrical injection and optical generation. Our systemic analysis provides evidence of inter-dot tunne…
We investigate the dynamical purification of maximally entangled electron states by transport through coupled quantum dots. Under resonant ac driving and coherent tunneling, even-parity Bell states perform Rabi oscillations that decouple from the environment, leading to a dark state. The two electrons remain spatially separated, one in each quantum dot. We propose configurations where this effect will prove as antiresonances in transport spectroscopy experiments.
Using single-particle pseudopotential and many-particle configuration interaction methods, we compare various physical quantities of (In,Ga)As/GaAs quantum dot molecules (QDMs) made of dissimilar dots (heteropolar QDMs) with QDMs made of identical dots (homopolar QDMs). The calculations show that the electronic structures of hetero-QDMs and homo-QDMs differ significantly at large inter-dot distance. In particular (i) Unlike those of homo-QDMs, the single-particle molecular orbitals of hetero-QDMs convert to dot localized orbitals at large inter-dot distance. (ii) Consequently, in a hetero-QMD …
We discuss the optical response of a quantum molecule under the action of two lasers fields. Using a realistic model and parameters, we map the physical conditions to find three different phenomena reported in the literature: the tunneling induced transparency, the formation of Autler-Townes doublets, and the creation of a Mollow-like triplet. We found that the electron tunneling between quantum dots is the responsible for the different optical regime. Our results not only explain the experimental results in the literature but also give insights for future experiments and applications in optic…
In this work, it is investigated the behavior of the efficiency at maximum power of a quantum dot molecule, acting as a device for photovoltaic conversion. A theoretical approach using a master equation, considering the effect of the energy offsets, and the width of the quantum barrier, identifies realistic physical conditions that enhance the photovoltaic response of the photocell. The results show the potentiality of increasing the gain in 30\% of maximum power delivered per molecule if compared with a single quantum dot. Also, the system exhibits gain when compared to the Chambadal-Novikov …
Pauli spin blockade in quantum dot systems occurs when the charge transport is allowed only for some spin states, and it has been an efficient tool in spin-based qubit devices in semiconductors. We theoretically investigate a Pauli spin blockade in a triple quantum dot molecule consisting of three identical quantum dots in a semiconductor in the presence of an external magnetic field through the molecule. When the three-electron state is on resonance with two- or four-electron states, the Aharonov-Bohm oscillation and the Zeeman splitting lead to a periodic spin blockade effect. We focus on th…
Two main mechanisms dictate the tunneling process in a double quantum dot: overlap of excited wave functions, effectively described as a tunneling rate, and phonon-assisted tunneling. In this paper, we study different regimes of tunneling that arise from the competition between these two mechanisms in a double quantum dot molecule immersed in a unimodal optical cavity. We show how such regimes affect the mean number of excitations in each quantum dot and in the cavity, the spectroscopic resolution and emission peaks of the photoluminescence spectrum, and the second-order coherence function whi…
The spin of an electron in a self-assembled InAs/GaAs quantum dot molecule is optically prepared and measured through the trion triplet states. A longitudinal magnetic field is used to tune two of the trion states into resonance, forming a superposition state through asymmetric spin exchange. As a result, spin-flip Raman transitions can be used for optical spin initialization, while separate trion states enable cycling transitions for non-destructive measurement. With two-laser transmission spectroscopy we demonstrate both operations simultaneously, something not previously accomplished in a s…
We report on a single photon and spin storage device based on a semiconductor quantum dot molecule. Optically excited single electron-hole pairs are trapped within the molecule and their recombination rate is electrically controlled over three orders of magnitude. Single photons are stored up to 1 microsecond and read out on a sub-nanosecond timescale. Using resonant excitation, the circular polarisation of individual photons is transferred into the spin state of electron-hole pairs with a fidelity above 80%, which does not degrade for storage times up to the 12.5ns repetition period of the ex…
We give three methods for entangling quantum states in quantum dots. We do this by showing how to tailor the resonant energy (Foerster-Dexter) transfer mechanisms and the biexciton binding energy in a quantum dot molecule. We calculate the magnitude of these two electrostatic interactions as a function of dot size, interdot separation, material composition, confinement potential and applied electric field by using an envelope function approximation in a two-cuboid dot molecule. In the first implementation, we show that it is desirable to suppress the Foerster coupling and to create entanglemen…
We study phonon-assisted electron tunneling in semiconductor quantum dot molecules. In particular, singlet-singlet relaxation in a two-electron doped structure is considered. The influence of Coulomb interaction is discussed via comparison with a single electron system. We find that the relaxation rate reaches similar values in the two cases but the Coulomb interaction shifts the maximum rates towards larger separations between the dots. The difference in electron-phonon interaction between deformation potential and piezoelectric coupling is investigated. We show that the phonon-induced tunnel…
We investigate the generation of entanglement through a quantum dot molecule under the influence of vibrational phonon modes in a bias voltage junction. The molecular quantum dot system is realized by coupled quantum dots inside a suspended carbon nanotube. We consider the dynamical entanglement as a function of bias voltage and temperature by taking into account the electron-phonon interaction. In order to generate the robust entanglement between quantum dots and preserve it to reach the maximal achievable amount steadily, we introduce an asymmetric coupling protocol and apply the easy tunabl…
We propose an all-optical scheme to perform a non-demolition measurement of a single hole spin localized in a quantum-dot molecule. The latter is embedded in a microcavity and driven by two lasers. This allows to induce Raman transitions which entangle the spin state with the polarization of the emitted photons. We find that the measurement can be completed with high fidelity on a timescale of 100 ps, shorter than the typical T2. Furthermore, we show that the scheme can be used to induce and observe spin oscillations without the need of time-dependent magnetic fields.
Multi-electron semiconductor quantum dots have found wide application in qubits, where they enable readout and enhance polarizability. However, coherent control in such dots has typically been restricted to only the lowest two levels, and such control in the strongly interacting regime has not been realized. Here we report quantum control of eight different resonances in a silicon-based quantum dot. We use qubit readout to perform spectroscopy, revealing a dense set of energy levels with characteristic spacing far smaller than the single-particle energy. By comparing with full configuration in…
The wide set of control parameters and reduced size scale make semiconductor quantum dots attractive candidates to implement solid-state quantum computation. Considering an asymmetric double quantum dot coupled by tunneling, we combine the action of a laser field and the spontaneous emission of the excitonic state to protect an arbitrary superposition state of the indirect exciton and ground state. As a by-product we show how to use the protected state to solve the Deutsch problem.
We demonstrate the extension of coherence between all four two-electron spin ground states of an InAs quantum dot molecule (QDM) via non-local suppression of nuclear spin fluctuations in both constituent quantum dots (QDs), while optically addressing only the upper QD transitions. Long coherence times are revealed through dark-state spectroscopy as resulting from nuclear spin locking mediated by the exchange interaction between the QDs. Lineshape analysis provides the first measurement of the quieting of the Overhauser field distribution correlating with reduced nuclear spin fluctuations.
In this theoretical work, we study a double quantum dot interacting strongly with a microcavity, while undergoing resonant tunneling. Effects of interdot tunneling on the light-matter hybridized states are determined, and tunability of their brightness degrees and associated dipole moments is demonstrated. These results predict dipolariton generation in artificial molecules coupled to optical resonators, and provide a promising scenario for control of emission efficiency and coherence times of exciton polaritons.
The spin states of electrons and holes confined in InAs quantum dot molecules have recently come to fore as a promising system for the storage or manipulation of quantum information. We describe here a feasible scheme for complete quantum optical control of two electron spin qubits in two vertically-stacked singly-charged InAs quantum dots coupled by coherent electron tunneling. With an applied magnetic field transverse to the growth direction, we construct a universal set of gates that corresponds to the possible Raman transitions between the spin states. We detail the procedure to decompose …
Atomistic electronic structure calculations are performed to study the coherent inter-dot couplings of the electronic states in a single InGaAs quantum dot molecule. The experimentally observed excitonic spectrum [12] is quantitatively reproduced, and the correct energy states are identified based on a previously validated atomistic tight binding model. The extended devices are represented explicitly in space with 15 million atom structures. An excited state spectroscopy technique is presented in which the externally applied electric field is swept to probe the ladder of the electronic energy …
An ideal source of entangled photon pairs combines the perfect symmetry of an atom with the convenient electrical trigger of light sources based on semiconductor quantum dots. We create a naturally symmetric quantum dot cascade that emits highly entangled photon pairs on demand. Our source consists of strain-free GaAs dots self-assembled on a triangular symmetric (111)A surface. The emitted photons strongly violate Bell's inequality and reveal a fidelity to the Bell state as high as 86 (+-2) % without postselection. This result is an important step towards scalable quantum-communication applic…
The effects caused by phonon-assisted tunnelling (PhAT) in a double quantum dot (QD) molecule immersed in a cavity were studied under the quantum Markovian master equation formalism in order to account for dissipation phenomena. We explain how for higher PhAT rates, a stronger interaction between a QD and the cavity at off-resonance takes place through the resonant interaction of another QD and the cavity, where the QDs interact through tunnelling. A closer look at the system's allowed optical transitions as a function of PhAT rates showed coalescence of the transition energies, leading to a l…
Starting with an accurate pseudopotential description of the single-particle states, and following by configuration-interaction treatment of correlated electrons in vertically coupled, self-assembled InAs/GaAs quantum dot-molecules, we show how simpler, popularly-practiced approximations, depict the basic physical characteristics including the singlet-triplet splitting, degree of entanglement (DOE) and correlation. The mean-field-like single-configuration approaches such as Hartree-Fock and local spin density, lacking correlation, incorrectly identify the ground state symmetry and give inaccur…
A semiconductor based scheme has been proposed for generating entangled photon pairs from the radiative decay of an electrically-pumped biexciton in a quantum dot. Symmetric dots produce polarisation entanglement, but experimentally-realised asymmetric dots produce photons entangled in both polarisation and frequency. In this work, we investigate the possibility of erasing the `which-path' information contained in the frequencies of the photons produced by asymmetric quantum dots to recover polarisation-entangled photons. We consider a biexciton with non-degenerate intermediate excitonic state…
Two-electron charged self-assembled quantum dot molecules exhibit a decoherence-avoiding singlet-triplet qubit subspace and an efficient spin-photon interface. We demonstrate quantum entanglement between emitted photons and the spin-qubit after the emission event. We measure the overlap with a fully entangled state to be $69.5\pm2.7\,\%$, exceeding the threshold of $50\,\%$ required to prove the non-separability of the density matrix of the system. The photonic qubit is encoded in two photon states with an energy difference larger than the timing resolution of existing detectors. We devise a n…
Self-assembled optically active quantum dot molecules (QDMs) allow the creation of protected qubits via singlet-triplet spin states. The qubit energy splitting of these states is defined by the tunnel coupling strength and is, therefore, determined by the potential landscape and thus fixed during growth. Applying an in-plane magnetic field increases the confinement of the hybridized wave functions within the quantum dots, leading to a decrease of the tunnel coupling strength. We achieve a tuning of the coupling strength by $(53.4\pm1.7)$ %. The ability to fine-tune this coupling is essential f…
Semiconductor quantum dots coherently driven by pulsed laser are fundamental physical systems which allow studying the dynamical properties of confined quantum states. These systems are attractive candidates for a solid-state qubit, which open the possibility for several investigations in quantum information processing. In this work we study the effects of a specific decoherence process, the spontaneous emission of excitonic states, in a quantum dot molecule. We model our system considering a three-level Hamiltonian and solve the corresponding master equation in the Lindblad form. Our results …
