In most widely discussed discrete time quantum walk model, after every unitary shift operator, the particle evolves into the superposition of position space and settles down in one of its basis states, loosing entanglement in the coin space in the new position. The Hadamard operation is applied to let the particle to evolve into the superposition in the coin space and the walk is iterated. We present a model with a additional degree of freedom for the unitary shift operator $U^{\prime}$. The unitary operator with additional degree of freedom will evolve the quantum particle into superposition of position space retaining the entanglement in coin space. This eliminates the need for quantum coin toss (Hadamard operation) after every unitary displacement operation as used in most widely studied version of the discrete time quantum walk model. This construction is easily extended to a multiple particle quantum walk and in this article we extend it for a pair of particles in pure state entangled in coin degree of freedom by simultaneously subjecting it to a pair of unitary displacement operators which were constructed for single particle. We point out that unlike for single particle quantum walk, upon measurement of its position after $N$ steps, the entangled particles are found together with 1/2 probability and at different positions with 1/2 probability. This can act as an advantage in applications of the quantum walk. A special case is also treated using a complex physical system such as, inter species two-particle entangled Bose-Einstein condensate, as an example.
We present a mathematical formalism for the description of unrestricted quantum walks with entangled coins and one walker. The numerical behaviour of such walks is examined when using a Bell state as the initial coin state, two different coin operators, two different shift operators, and one walker. We compare and contrast the performance of these quantum walks with that of a classical random walk consisting of one walker and two maximally correlated coins as well as quantum walks with coins sharing different degrees of entanglement. We illustrate that the behaviour of our walk with entangled …
Generation of entangled state is of paramount importance both from quantum theoretical foundation and technology applications. Entanglement swapping provides an efficient method to generate entanglement in quantum communication protocols. However, perfect Bell measurements for qudits, the key to entanglement swapping, have been proven impossible to achieve by using only linear elements and particle detectors. To avoid this bottleneck, we propose a novel scheme to generate entangled state including two-qubit entangled state, two-qudit entangled state, three-qubit GHZ state and three-qudit GHZ s…
We study one-dimensional quantum walk with four internal degrees of freedom resulted from two entangled qubits. We will demonstrate that the entanglement between the qubits and its corresponding coin operator enable one to steer the walker's state from a classical to standard quantum-walk behavior, and a novel one. Additionally, we report on self-trapped behavior and perfect transfer with highest velocity for the walker. We also show that symmetry of probability density distribution, the most probable place to find the walker and evolution of the entropy are subject to initial entanglement bet…
We advance the previous studies of quantum walks on the line with two coins. Such four-state quantum walks driven by a three-direction shift operator may have nonzero stationary distributions (localization), thus distinguishing themselves from the quantum walks on the line in the basic scenario (i.e., driven by a single coin). In this work, asymptotic position distributions of the quantum walks are examined. We derive a weak limit for the quantum walks and explicit formulas of stationary probability distribution, whose dependencies on the coin parameter and the initial state of quantum walks a…
Ultra-high-rate detection of entangled photon pairs
Basic Research Laboratories, NTT, Inc.（NTT公司基础研究实验室）；Advanced ICT Research Institute, National Institute of Information and Communications Technology（信息通信技术研究院高级ICT研究所）
In a local realist world view, physical properties are defined prior to and independent of measurement, and no physical influence can propagate faster than the speed of light. Proper experimental violation of a Bell inequality would show that the world cannot be described within local realism. Such experiments usually require additional assumptions that make them vulnerable to a number of "loopholes." A recent experiment [Giustina et al, Nature, 2013] violated a Bell inequality without being vulnerable to the detection (or fair-sampling) loophole, therefore not needing the fair-sampling assump…
A hypothesis testing scheme for entanglement has been formulated based on the Poisson distribution framework instead of the POVM framework. Three designs were proposed to test the entangled states in this framework. The designs were evaluated in terms of the asymptotic variance. It has been shown that the optimal time allocation between the coincidence and anti-coincidence measurement bases improves the conventional testing method. The test can be further improved by optimizing the time allocation between the anti-coincidence bases.
A method for determining the positions of hologram dislocations relative to the optical axes of entangled Laguerre Gaussian modes is proposed. In our method, the coincidence count rate distribution was obtained by scanning the position of one of the holograms in two dimensions. Then, the relative position of the hologram dislocation was determined quantitatively from the positions of the minimum and maximum coincidence count rates. The validity of the method was experimentally verified, and in addition, an experiment demonstrating the violation of the Clauser-Horne-Shimony-Holt inequality was …
Generation and characterization of entanglement are crucial tasks in quantum information processing. A hypothesis testing scheme for entanglement has been formulated. Three designs were proposed to test the entangled photon states created by the spontaneous parametric down conversion. The time allocations between the measurement vectors were designed to consider the anisotropic deviation of the generated photon states from the maximally entangled states. The designs were evaluated in terms of the p-value based on the observed data. It has been experimentally demonstrated that the optimal time …
We offer theoretical explanations for some recent observations in numerical simulations of quantum random walks (QRW). Specifically, in the case of a QRW on the line with one particle (walker) and two entangled coins, we explain the phenomenon, called "localization", whereby the probability distribution of the walker's position is seen to exhibit a persistent major "spike" (or "peak") at the initial position and two other minor spikes which drift to infinity in either direction. Another interesting finding in connection with QRW's of this sort pertains to the limiting behavior of the position …
We investigate how quantum coincidence interferometry is affected by a controllable manipulation of transverse wave-vectors in type-II parametric down conversion using adaptive optics techniques. In particular, we discuss the possibility of spatial walk-off compensation in quantum interferometry and a new effect of even-order spatial aberration cancellation.
An unconditionally secure quantum cion tossing protocol for two remote participants via entangled swapping is presented. The security of this protocol is guaranteed by the nonlocal property of quantum entanglement and the classical complexity.
We report measurements of time-frequency entangled photon pairs and heralded single photons at telecommunications wavelengths, generated using a periodically-poled, lithium niobate on insulator (LNOI) waveguide pumped optically by a diode laser. We achieve a high Coincidences-to-Accidentals Ratio (CAR) at high pair brightness, a low value of the conditional self-correlation function [$g^{(2)}$(0)], and high two-photon energy-time Franson interferometric visibility, which demonstrate the high quality of the entangled photon pairs and heralded single photons.
Entangled photon pair excitation and time-frequency-filtered multidimensional photon correlation spectroscopy as a probe for dissipative exciton kinetics
Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY（自由电子激光科学中心，德国电子同步加速器）；University of California, Irvine（加州大学尔湾分校）
Quantum spectroscopy was performed using the frequency-entangled broadband photon pairs generated by spontaneous parametric down-conversion. An absorptive sample was placed in front of the idler photon detector, and the frequency of signal photons was resolved by a diffraction grating. The absorption spectrum of the sample was measured by counting the coincidences, and the result is in agreement with the one measured by a conventional spectrophotometer with a classical light source.
Quantum-cryptography key distribution (QCKD) experiments have been recently reported using polarization-entangled photons. However, in any practical realization, quantum systems suffer from either unwanted or induced interactions with the environment and the quantum measurement system, showing up as quantum and, ultimately, statistical noise. In this paper, we investigate how ideal polarization entanglement in spontaneous parametric downconversion (SPDC) suffers quantum noise in its practical implementation as a secure quantum system, yielding errors in the transmitted bit sequence. Because al…
We present a tunable, frequency-stabilized, narrow-bandwidth source of frequency-degenerate, entangled photon pairs. The source is based on spontaneous parametric downconversion (SPDC) in periodically-poled KTiOPO4 (PPKTP). Its wavelength can be stabilized to 850 or 854 nm, thus allowing to address two D-P transitions in 40Ca+ ions. Its output bandwidth of 22 MHz coincides with the absorption bandwidth of the calcium ions. Its spectral power density is 1.0 generated pairs/(s MHz mW).
Sub-picosecond coincidence timing from nonlocal intensity interference of entangled photons allows quantum interferometry for plasmas. Using a warm plasma dispersion relation, we correlate phase measurement sensitivity with different plasma properties or physics mechanisms over 6 orders of magnitude. Due to $N^α$ ($α\leq -1/2$) scaling with the photon number $N$, quantum interferometry using entangled light can probe small signals in plasmas not previously accessible. As an example, it is predicted that plasmas will induce shifts to a Gaussian dip, a well-known quantum optics phenomenon that i…
Energy-time entangled photon holes are shown to be relatively insensitive to photon loss due to absorption by atoms whose coherence times are longer than the time delays typically employed in nonlocal interferometry (a fraction of a nanosecond). Roughly speaking, the excited atoms do not retain any significant "which-path" information regarding the time at which a photon was absorbed. High-intensity entangled photon holes can also be amplified under similar conditions. Decoherence does occur from losses at beam splitters, and these results show that photon loss cannot always be adequately mode…
The quantum characteristics of sum-frequency process in an optical cavity with an input signal optical beam, which is a half of entangled optical beams, are analyzed. The calculated results show that the quantum properties of the signal beam can be maintained after its frequency is conversed during the intracavity nonlinear optical interaction. The frequency-conversed output signal beam is still in an entangled state with the retained other half of initial entangled beams. The resultant quantum correlation spectra and the parametric dependences of the correlations on the initial squeezing fact…
We describe an entanglement purification protocol (EPP) for multipartite three-level atomic entangled pair using photonic Faraday rotation. In this EPP, the multipartite atomic entangled state can be purified with the help of some single photons. This protocol resorts to the photonic Faraday rotation to realize the function of the controlled-Not (CNOT) gate. The purified multipartite atomic entangled state can be retained and to be repeated to reach a higher fidelity.
We have developed a scheme to generate, control, transmit and measure entangled photonic qutrits (two photons each of dimension d = 3). A Bell test of this source has previously been reported elsewhere [1], therefore, here we focus on how the control of the system is realized. Motivated by these results, we outline how the scheme can be used for two specific quantum protocols, namely key distribution and coin tossing and discuss some of their advantages and disadvantages.
Quantum lithography achieves phase super-resolution using fragile, experimentally challenging entangled states of light. We propose a scalable scheme for creating features narrower than classically achievable, with reduced use of quantum resources and consequently enhanced resistance to loss. The scheme is an implementation of interferometric lithography using a mixture of an SPDC entangled state with intense classical coherent light. We measure coincidences of up to four photons mimicking multiphoton absorption. The results show a narrowing of the interference fringes of up to 30% with respec…
We present a way for the entanglement distillation of genuine mixed state. Different from the conventional mixed state in entanglement purification protocol, each components of the mixed state in our protocol is a less-entangled state, while it is always a maximally entangled state. With the help of the weak cross-Kerr nonlinearity, this entanglement distillation protocol does not require the sophisticated single-photon detectors. Moreover, the distilled high quality entangled state can be retained to perform the further distillation. These properties make it more convenient in practical appli…
High-precision time transfer is of fundamental interest in physics and metrology. Quantum time transfer technologies that use frequency-entangled pulses and their coincidence detection have been proposed, offering potential enhancements in precision and better guarantees of security. In this paper, we describe a fiber-optic two-way quantum time transfer experiment. Using quantum nonlocal dispersion cancellation, time transfer over a 20-km fiber link achieves a time deviation of 922 fs over 5 s and 45 fs over 40960 s. The time transfer accuracy as a function of fiber lengths from 15 m to 20 km …
We have generated a new type of biphoton state by cavity-enhanced down-conversion in a type-II phase-matched, periodically-poled KTiOPO_4 (PPKTP) crystal. By introducing a weak intracavity birefringence, the polarization-entangled output was modulated between the singlet and triplet states according to the arrival-time difference of the signal and idler photons. This cavity-enhanced biphoton source is spectrally bright, yielding a single-mode fiber-coupled coincidence rate of 0.7 pairs/s per mW of pump power per MHz of down-conversion bandwidth. Its novel biphoton behavior may be utilized in s…
The second-order Talbot effect is analyzed for a periodic object illuminated by entangled photon pairs in both the quantum imaging and quantum lithography configurations. The Klyshko picture is applied to describe the quantum imaging scheme, in which self-images of the object that may or may not be magnified can be observed nonlocally in the photon coincidences but not in the singles count rate. In the quantum lithography setup, we find that the second-order Talbot length is half that of the classical first-order case, thus the resolution may be improved by a factor of two.
In this letter we present the first implementation of a quantum coin tossing protocol. This protocol belongs to a class of ``two-party'' cryptographic problems, where the communication partners distrust each other. As with a number of such two-party protocols, the best implementation of the quantum coin tossing requires qutrits. In this way, we have also performed the first complete quantum communication protocol with qutrits. In our experiment the two partners succeeded to remotely toss a row of coins using photons entangled in the orbital angular momentum. We also show the experimental bound…
We demonstrate a new class of frequency-entangled states generated via spontaneous parametric down-conversion under extended phase matching conditions. Biphoton entanglement with coincident signal and idler frequencies is observed over a broad bandwidth in periodically poled KTiOPO$_4$. We demonstrate high visibility in Hong-Ou-Mandel interferometric measurements under pulsed pumping without spectral filtering, which indicates excellent frequency indistinguishability between the down-converted photons. The coincident-frequency entanglement source is useful for quantum information processing an…
We experimentally demonstrate amplitude and phase modulation of a time-energy entangled two-photon wave function. The entangled photons are produced by spontaneous parametric down-conversion, spectrally dispersed in an prism compressor, modulated in amplitude and/or phase, and detected in coincidence by sum-frequency generation. First, we present a Fourier optical analysis of the optical setup yielding an analytic expression for the resulting field distribution at the exit plane of the shaping apparatus. We then introduce amplitude and/or phase shaping and present results which can only be obt…
Entangled photons are a crucial resource for quantum communication and linear optical quantum computation. Unfortunately, the applicability of many photon-based schemes is limited due to the stochastic character of the photon sources. Therefore, a worldwide effort has focused in overcoming the limitation of probabilistic emission by generating two-photon entangled states conditioned on the detection of auxiliary photons. Here we present the first heralded generation of photon states that are maximally entangled in polarization with linear optics and standard photon detection from spontaneous p…
The pure quantum entanglement is generalized to the case of mixed compound states on an operator algebra to include the classical and quantum encodings as particular cases. The true quantum entanglements are characterized by quantum couplings which are described as transpose-CP, but not Completely Positive (CP), trace-normalized linear positive maps of the algebra. The entangled (total) information is defined in this paper as a relative entropy of the conditional (the derivative of the compound state with respect to the input) and the unconditional output states. Thus defined the total informa…
Lamata et al. use an inductive approach to classify the entangled pure states of four qubits under stochastic local operations and classical communication (SLOCC) [PRA 75(2), 022318 (2007)]. The inductive method yields a priori ten different entanglement superclasses, of which they discard three as empty. One of the remaining superclasses is split in two, resulting in eight superclasses of genuine four-qubit entanglement. Here, we show that two of the three discarded superclasses are in fact non-empty and should have been retained. We give explicit expressions for the canonical states for thos…
An interference experiment with entangled particles is theoretically analyzed, where one of the entangled pair (particle 1) goes through a multi-slit before being detected at a fixed detector. In addition, one introduces a mechanism for finding out which of the n slits did particle 1 go through. The other particle of the entangled pair (particle 2) goes in a different direction, and is detected at a variable, spatially separated location. In coincident counting, particle 2 shows n-slit interference. It is shown that the normalized quantum coherence of particle 2, $\mathcal{C}_2$, and the path-…
We experimentally realize a high-intensity three-photon Greenberger-Horne-Zeilinger (GHZ) entanglement source directly following the proposal by Rarity and Tapster [J. G. Rarity and P. R. Tapster, Phys. Rev. A 59, R35 (1999)]. The threefold coincidence rate can be more than 200 Hz with a fidelity of 0.811, and the intensity can be further improved with moderate fidelity degradation. The GHZ entanglement is characterized by testing the Bell-Mermin inequality and using an entanglement witness operator. To optimize the polarization-entangled source, we theoretically analyze the relationship betwe…
We investigate the relation between indistinguishability and quantum entanglement in Hong- Ou-Mandel-interference experiments theoretically and relate these quantum mechanical principles to the theorem of entanglement monogamy. Employing Glaubers theory of quantum coherence we compute the detection statistics in HOM-interference of frequency entangled photons, and find a new additional term in the coincidence detection probability, which is related to the spectral indistinguishability of the considered photons that arises from finite bandwidth effects, and therefore is relevant in the limit of…
We show that the entanglement of an initially frequency-entangled photon pair propagating through a disordered scattering medium can be read off in transmission from the coincidence counting rate. The very same quantity also encodes the Thouless time of the medium.
We present a scheme to realize a deterministic solid state source of time-bin entangled photon pairs using cavity-assisted stimulated Raman adiabatic passage (STIRAP) in a single quantum dot. The quantum dot is embedded inside a semiconductor cavity, and the interaction of a coherent superposition of two temporally separated input pulses and the cavity mode leads to a two-photon Raman transition, which produces a time-bin entangled photon pair through the biexciton-exciton cascade. We show that the entanglement of the generated state can be measured using triple coincidence detection, and the …
We introduce and analyze a one-dimensional quantum walk with two time-independent rotations on the coin. We study the influence on the property of quantum walk due to the second rotation on the coin. Based on the asymptotic solution in the long time limit, a ballistic behaviour of this walk is observed. This quantum walk retains the quadratic growth of the variance if the combined operator of the coin rotations is unitary. That confirms no localization exhibits in this walk. This result can be extended to the walk with multiple time-independent rotations on the coin.
Quantum entangled states of light are essential for quantum technologies and fundamental tests of physics. While quantum information science has relied on systems with entanglement in 2D degrees of freedom, e.g. quantum bits with polarization states, the field is moving towards ever-higher dimensions of entanglement. Increasing the dimensionality enhances the channel capacity and security of quantum communication protocols, gives rise to exponential speed-up of quantum computation, and is necessary for quantum imaging. Yet, characterization of even bipartite quantum states of high-dimensional …
Entanglement swapping at telecom wavelengths is at the heart of quantum networking in optical fiber infrastructures. Although entanglement swapping has been demonstrated experimentally so far using various types of entangled photon sources both in near-infrared and telecom wavelength regions, the rate of swapping operation has been too low to be applied to practical quantum protocols, due to limited efficiency of entangled photon sources and photon detectors. Here we demonstrate drastic improvement of the efficiency at telecom wavelength by using two ultra-bright entangled photon sources and f…
A novel ultrabright parametric source of polarization entangled photon pairs with striking spatial characteristics is reported. The distribution of the output electromagnetic k-modes excited by Spontaneous Parametris Down Conversion and coupled to the output detectors can be very broad. It could coincide with the full set of phase-matched excited modes, at least in principle. In this case a relevant conditional quasi-pure output state should be realized. By these (approximate) states realized over a full Entanglement-Ring output distribution, the non local properties of the generated entanglem…
Quantum measurements that use the entangled photons' polarization to encode quantum information require calibration and alignment of the measurement bases between spatially separate observers. Because of the changing birefringence in optical fibers arising from temperature fluctuations or external mechanical vibrations, the polarization state at the end of a fiber channel is unpredictable and time-varying. Polarization tracking and stabilization methods originally developed for classical optical communications cannot be applied to polarization-entangled photons, where the separately detected p…
The entangled quantum state of a photon pair propagating through atmospheric turbulence suffers decay of entanglement due to the scintillation it experiences. Here we investigate the robustness against this decay for different qutrit states. We use an infinitesimal-propagation equation to obtain the density matrix as a function of the propagation distance and we use the tangle to quantify the entanglement between a pair of qutrits. The evolution of various initial states as they propagate through turbulence is considered. Using optimization of the initial parameters, we obtain expressions for …
The use of entangled light to illuminate objects is shown to provide significant enhancements over unentangled light for detecting and imaging those objects in the presence of high levels of noise and loss. Each signal sent out is entangled with an ancilla, which is retained. Detection takes place via an entangling measurement on the returning signal together with the ancilla. Quantum illumination with e bits of entanglement increases the effective signal-to-noise ratio of detection and imaging by a factor of 2^e, an exponential improvement over unentangled illumination.
Entanglement, describing the inseparability of a quantum multiparty system, is one of the most intriguing features of quantum mechanics. Violation of Bell inequality, for ruling out the possibility of local hidden variable theories, is commonly used as a strong witness for quantum entanglement. In previous Bell test experiments with photonic entanglement based on two-photon coincidence measurement, the photon temporal wave packets are absorbed completely by the detectors. That is, the photon coherence time is much shorter than the detection time window. Here we demonstrate generation of freque…
We present two two-step practical entanglement concentration protocols (ECPs) for concentrating an arbitrary three-particle less-entangled W state into a maximally entangled W state assisted with single photons. The first protocol uses the linear optics and the second protocol adopts the cross-Kerr nonlinearity to perform the protocol. In the first protocol, based on the post-selection principle, three parties say Alice, Bob and Charlie in different distant locations can obtain the maximally entangled W state from the arbitrary less-entangled W state with a certain success probability. In the …
