We demonstrate a new class of frequency-entangled states generated via spontaneous parametric down-conversion under extended phase matching conditions. Biphoton entanglement with coincident signal and idler frequencies is observed over a broad bandwidth in periodically poled KTiOPO$_4$. We demonstrate high visibility in Hong-Ou-Mandel interferometric measurements under pulsed pumping without spectral filtering, which indicates excellent frequency indistinguishability between the down-converted photons. The coincident-frequency entanglement source is useful for quantum information processing and quantum measurement applications.
Two quantum states of two half-charge optical vortexes with relative azimuthal angle π are orthogonal, by which two half-charge spiral phase plates with intersection angle π can be used to demonstrate a parabolic coincident fringe in the Bell inequality experiment with high-dimensional two-photon orbital angular momentum entanglement and to thereby obtain a strong Bell parameter of 3.2. I theoretically demonstrate various orthogonal relations between two quantum states, each of which is a state with a rotational symmetry superposition made up of n fractional orbital angular momentum states, wh…
We show that for two initially excited qubits, interacting via dipole forces and with a common reservoir, entanglement is preceded by the emergence of quantum and classical correlations. After a time lag, entanglement finally starts building up, giving rise to a peculiar entangled state, with very small classical correlations. Different measures of quantum correlations are discussed, and their dynamics are compared and shown to lead to coincident values of these quantifiers for several ranges of time.
We use a single trapped 40Ca+ ion as a resonant, polarization-sensitive absorber to detect and characterize the entanglement of tunable narrowband photon pairs from a spontaneous parametric down-conversion source. Single-photon absorption is marked by a quantum jump in the ion and heralded by coincident detection of the partner photon. For three polarization basis settings of absorption and detection of the herald, we find maximum coincidences always for orthogonal polarizations. The polarization entanglement is further evidenced by tomographic reconstruction of the biphoton quantum state.
We describe a classical model that may serve as an analog for joint and local measurements of an entanglement witness. The analogous experimental procedure and data analysis protocol of the model follow those of a previous experiment to measure an entanglement witness with polarized photons prepared in a mixed state [Phys. Rev. Lett. \textbf{91}, 227901 (2003)]. Numerical simulations show excellent agreement with both experimental results and quantum-mechanical predictions. This agreement is made possible by the fact that the model exhibits contextuality due to the postselection of coincident …
Extended phase-matching conditions for spontaneous parametric down-conversion are examined. By augmenting the conventional phase-matching conditions, they permit the creation of a class of frequency-entangled states that generalizes the usual twin-beam biphoton state. An experimental characterization of these states is possible through interferometric coincidence counting.
Teleportation may be taken as sending and extracting quantum information through quantum channels. In this report, it is shown that to get the maximal probability of exact teleportation through partially entangled quantum channels, the sender (Alice) need only to operate a measurement which satisfy an ``entanglement matching'' to this channel. An optimal strategy is also provided for the receiver (Bob) to extract the quantum information by adopting general evolutions.
We report the simultaneous quasi-phase-matching of all three possible nonlinearities for propagation along the X axis of periodocally poled (PP) KTiOPO4 (KTP) for second-harmonic generation of 745 nm pulsed light from 1490nm subpicosecond pulses in a PPKTP crystal with a 45.65 micrometer poling period. This confirms the recent Sellmeier fits of KTP by K. Kato and E. Takaoka [Appl. Opt. 41, 5040 (2002)]. Such coincident nonlinearities are of importance for realizing compact sources of multipartite continuous-variable entanglement [Pfister et al., Phys. Rev. A 70, 020302 (2004)] and we propose a…
A simple experimental setup consisting of a spontaneous parametric down-conversion source and passive linear optics is proposed for conditional preparation of a maximally entangled polarization state of two photons. Successful preparation is unambiguously heralded by coincident detection of four auxiliary photons. The proposed scheme utilizes the down-conversion term corresponding to the generation of three pairs of photons. We analyze imperfect detection of the auxiliary photons and demonstrate that its deleterious effect on the fidelity of the prepared state can be suppressed at the cost of …
We present a security analysis against collective attacks for the recently proposed time-energy entanglement-based quantum key distribution protocol, given the practical constraints of single photon detector efficiency, channel loss, and finite-key considerations. We find a positive secure-key capacity when the key length increases beyond $10^4$ for eight-dimensional systems. The minimum key length required is reduced by the ability to post-select on coincident single-photon detection events. Including finite-key effects, we show the ability to establish a shared secret key over a 200 km fiber…
Here we present an experimentally feasible scheme to entangle flying qubit (individual photon with polarization modes) and stationary qubit (atomic ensembles with long-lived collective excitations). This entanglement integrate two different species can act as a critical element for the coherent transform of quantum information between flying and stationary qubits. The entanglement degree can be also adjusted expediently with linear optics. Furthermore, the present scheme can be modified to generate this entanglement in a way event-ready with the employment of a pair of entangled photons. Then …
Classical matching theory can be defined in terms of matrices with nonnegative entries. The notion of Positive operator, central in Quantum Theory, is a natural generalization of matrices with nonnegative entries. Based on this point of view, we introduce a definition of perfect Quantum (operator) matching . We show that the new notion inherits many "classical" properties, but not all of them . This new notion goes somewhere beyound matroids . For separable bipartite quantum states this new notion coinsides with the full rank property of the intersection of two corresponding geometric matroids…
Two time-reversal quantum key distribution (QKD) schemes are the quantum entanglement based device-independent (DI)-QKD and measurement-device-independent (MDI)-QKD. The recently proposed twin field (TF)-QKD, also known as phase-matching (PM)-QKD, has improved the key rate bound from $O\left( η\right )$ to $O\left( \sqrt η \right )$ with $η$ the channel transmittance. In fact, TF-QKD is a kind of MDI-QKD but based on single-photon detection. In this paper, we propose a different PM-QKD based on single-photon entanglement, referred to as single-photon entanglement-based phase-matching (SEPM)-QK…
We investigate theoretically quantum entanglement of light with the collective spin polarization of a cold atomic ensemble in cavity-assisted Raman schemes. Previous works concentrated mostly on the bad cavity limit where the signals are much longer than the cavity field lifetime. In view of atomic relaxation and other imperfections, there may arise a need to speed-up the light-atoms interface operation. By increasing the cavity field lifetime, one can achieve better light-matter coupling and entanglement. In our work, we consider the non-adiabatic effects that become important beyond the bad …
We show that it is possible to generate entanglement between two distant Bose-Einstein condensates by detection of Hanbury Brown-Twiss type correlations in photons Bragg-scattered by the condensates. Upon coincident detection of two photons by two detectors, the projected joint state of two condensates is shown to be non-Gaussian. We verify the existence of entanglement by showing that the partially transposed state is negative. Further we use the inequality in terms of higher order moments to confirm entanglement. Our proposed scheme can be generalized for multiple condensates and also for sp…
Wavevector quasi-phase matching was devised in the 1960s as a way to boost nonlinear interactions with efficient quantum noise squeezing as one outstanding outcome. In the era of quantum technologies, we propose a new coupling quasi-phase matching for efficient generation of multimode downconverted quantum light in nonlinear waveguide arrays. We highlight this technique achieving multimode quantum entanglement and Einstein-Podolsky-Rosen steering buildup. We discuss the feasibility of this method with current technology and demonstrate its competitiveness as a resource for continuous variables…
quantum theory of generalized $\mathrm{X}$ waves with orbital angular momentum in dispersive media, and the interaction of quantized $\mathrm{X}$ waves in quadratic nonlinear media were studied in (J. opt,20,065201(2018)). We present a kind of phase matching, which is called velocity phase matching, and this phase matching can be used for determining the length of the nonlinear crystal or the interaction time in the experiment setup, to produce $\mathrm{X}$ waves with particular velocity $v$. Moreover, we introduce more analysis for the dependence of squeezing of $\mathrm{X}$ waves on its spec…
Any practical experiment utilising the innate D-dimensional entanglement of the orbital angular momentum (OAM) state space of photons is subject to the modal capacity of the detection system. We show that given such a constraint, the number of measured, entangled OAM modes in photon pairs generated by spontaneous parametric down-conversion (SPDC) can be maximised by tuning the phase-matching conditions in the SPDC process. We demonstrate a factor of 2 increase on the half-width of the OAM-correlation spectrum, from 10 to 20, the latter implying \approx 50 -dimensional two-photon OAM entangleme…
In [Phys. Rev. Lett. 113, 210501 (2014)], to achieve the optimal fixed-point quantum search in the case of unknown fraction (denoted by $λ$) of target items, the analytical multiphase matching (AMPM) condition has been proposed. In this paper, we find out that the AMPM condition can also be used to design the exact quantum search algorithm in the case of known $λ$, and the minimum number of iterations reaches the optimal level of existing exact algorithms. Experiments are performed to demonstrate the proposed algorithm on IBM's quantum computer. In addition, we theoretically find two coinciden…
Quantum entanglement associated with transverse wave vectors of down conversion photons is investigated based on the Schmidt decomposition method. We show that transverse entanglement involves two variables: orbital angular momentum and transverse frequency. We show that in the monochromatic limit high values of entanglement are closely controlled by a single parameter resulting from the competition between (transverse) momentum conservation and longitudinal phase matching. We examine the features of the Schmidt eigenmodes, and indicate how entanglement can be enhanced by suitable mode selecti…
We have distributed entangled photons directly through the atmosphere to a receiver station 7.8 km away over the city of Vienna, Austria at night. Detection of one photon from our entangled pairs constitutes a triggered single photon source from the sender. With no direct time-stable connection, the two stations found coincidence counts in the detection events by calculating the cross-correlation of locally-recorded time stamps shared over a public internet channel. For this experiment, our quantum channel was maintained for a total of 40 minutes during which time a coincidence lock found appr…
From the partition function for two classes of classically non-local actions containing the fractional Laplacian, we show that as long as there exists a suitable (non-local) Hilbert-space transform the underlying action can be mapped onto a purely local theory. In all such cases the partition function is equivalent to that of a local theory and an area law for the entanglement entropy obtains. When such a reduction fails, the entanglement entropy deviates strongly from an area law and can in some cases scale as the volume. As these two criteria are coincident, we conjecture that they are equiv…
We demonstrate a new technique for characterizing two-photon quantum states based on joint temporal correlation measurements using time resolved single photon detection by femtosecond upconversion. We measure for the first time the joint temporal density of a two-photon entangled state, showing clearly the time anti-correlation of the coincident-frequency entangled photon pair generated by ultrafast spontaneous parametric down-conversion under extended phase-matching conditions. The new technique enables us to manipulate the frequency entanglement by varying the down-conversion pump bandwidth …
Scaling native entanglement generation in layered semiconductors with quasi-phase matching
University of Vienna（维也纳大学）；ICFO-Institut de Ciències Fotòniques, The Barcelona Institute of Science and Technology（ICFO-光子科学研究所，巴塞罗那科学技术研究院）；University of L’Aquila（拉奎拉大学）；CNR-SPIN（意大利国家研究委员会自旋物理研究所）；Columbia University（哥伦比亚大学）
In this paper, we focus on the quantum communication complexity of functions of the form $f \circ G = f(G(X_1, Y_1), \ldots, G(X_n, Y_n))$ where $f: \{0, 1\}^n \to \{0, 1\}$ is a symmetric function, $G: \{0, 1\}^j \times \{0, 1\}^k \to \{0, 1\}$ is any function and Alice (resp. Bob) is given $(X_i)_{i \leq n}$ (resp. $(Y_i)_{i \leq n}$). Recently, Chakraborty et al. [STACS 2022] showed that the quantum communication complexity of $f \circ G$ is $O(Q(f)\mathrm{QCC}_\mathrm{E}(G))$ when the parties are allowed to use shared entanglement, where $Q(f)$ is the query complexity of $f$ and $\mathrm{Q…
While the on-chip processing power in circuit QED devices is growing rapidly, an open challenge is to establish high-fidelity quantum links between qubits on different chips. Here, we show entanglement between transmon qubits on different cQED chips with $49\%$ concurrence and $73\%$ Bell-state fidelity. We engineer a half-parity measurement by successively reflecting a coherent microwave field off two nearly-identical transmon-resonator systems. By ensuring the measured output field does not distinguish $\vert 01 \rangle$ from $\vert 10 \rangle$, unentangled superposition states are probabili…
It is shown, theoretically and experimentally, that at any type-II spontaneous parametric down-conversion (SPDC) phase matching, the decoherence-free singlet Bell state is always present within the natural bandwidth and can be filtered out by a proper spectral selection. Instead of the frequency selection, one can perform time selection of the two-photon time amplitude at the output of a dispersive fibre. Applications to quantum communication are outlined.
We theoretically evaluate establishing remote entanglement between distinguishable matter qubits through interference and detection of two emitted photons. The fidelity of the entanglement operation is analyzed as a function of the temporal and frequency mode-matching between the photons emitted from each quantum memory. With a general analysis, we define limits on the absolute magnitudes of temporal and frequency mode-mismatches in order to maintain entanglement fidelities greater than 99% with two-photon detection efficiencies greater than 90%. We apply our analysis to several selected syste…
We give trade-offs between classical communication, quantum communication, and entanglement for processing information in the Shannon-theoretic setting. We first prove a unit-resource capacity theorem that applies to the scenario where only the above three noiseless resources are available for consumption or generation. The optimal strategy mixes the three fundamental protocols of teleportation, super-dense coding, and entanglement distribution. We then provide an achievable rate region and a matching multi-letter converse for the direct static capacity theorem. This theorem applies to the sce…
Crossovers between Time-Bin and Energy-Time Entanglement in Homodyned Resonance Fluorescence
Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）；Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；University of Chinese Academy of Sciences（中国科学院大学）
By making use of the spatial shape of paired photons, parametric down-conversion allows the generation of two-photon entanglement in a multidimensional Hilbert space. How much entanglement can be generated in this way? In principle, the infinite-dimensional nature of the spatial degree of freedom renders unbounded the amount of entanglement available. However, in practice, the specific configuration used, namely its geometry, the length of the nonlinear crystal and the size of the pump beam, can severely limit the value that could be achieved. Here we show that the use of quasi-phase-matching …
Quantum entanglement of two photons created by spontaneous parametric downconversion (SPDC) can be used to probe quantum optical phenomena during a single cycle of light. Harris [Phys. Rev. Lett. 98, 063602 (2007)] suggested using ultrabroad parametric fluorescence generated from a quasi-phase-matched (QPM) device whose poling period is chirped. In the Harris\' s original proposal, it is assumed that the photons are collinearly generated and then spatially separated by frequency filtering. Here, we alternatively propose using noncollinearly generated SPDC. In our numerical calculation, to achi…
Controllable multipartite entanglement is a crucial element in quantum information processing. Here we present a scheme that generates switchable bipartite and genuine tripartite entanglement between microwave and optical photons via an optoelectromechanical interface, where microwave and optical cavities are coupled to a mechanical mode with controllable coupling constants. We show that by tuning an effective gauge phase between the coupling constants to the "sweet spots", bipartite entanglement can be generated and switched between designated output photons. The bipartite entanglement is rob…
A detailed treatment of the entanglement dynamics of two distant but non-identical systems is presented. We study the entanglement evolution of two remote atoms interacting independently with a cavity field, as in the double Jaynes-Cummings (JC) model. The four-qubit pairwise concurrences are studied, allowing for asymmetric atom-cavity couplings and off-resonant ineractions. Counter to intuition, imperfect matching can prove advantageous to entanglement creation and evolution. For two types of initial entanglement, corresponding to spin correlated and anti-correlated Bell states Φand Ψ, a ful…
We consider the quantum analogue of the pattern matching problem, which consists of classifying a given unknown system according to certain predefined pattern classes. We address the problem of quantum template matching in which each pattern class ${\cal C}_i$ is represented by a known quantum state $\hat g_i$ called a template state, and our task is to find a template which optimally matches a given unknown quantum state $\hat f$. We set up a precise formulation of this problem in terms of the optimal strategy for an associated quantum Bayesian inference problem. We then investigate various e…
We study a class of nonlinear waveguide arrays where the waveguides are endowed with quadratic non- linearity and are coupled through the evanescent overlap of the guided modes. We study both the stimulated and spontaneous process in the array and show the viability of such an array as a platform for generating both bipartite and tripartite continuous variable entanglement on demand. We explicitly address the affect of realistic losses on the entanglement produced, briefly discuss the possible types of nonlinear materials that could be used, and suggest solutions to the possible phase matching…
Quantum repeaters are indispensable tools for long-distance quantum communication. However, frequency matching between entangled photon sources and remote quantum memories (QMs) is difficult, which is an obstacle to the implementation of quantum repeaters. In this paper, we demonstrate a method to achieve the coupling of a Pr:YSO as a fixed-time QM with a single telecommunication-wavelength photon through frequency stabilization using an optical frequency comb over all applied laser wavelengths. The demonstrated method can lead to the implementation of a quantum repeater scheme enabling an imp…
We present a quantum analysis of three-mode optoacoustic parametric interactions in an optical cavity, in which two orthogonal transverse optical-cavity modes are coupled to one acoustic mode through radiation pressure. Due to the optimal frequency matching -- the frequency separation of two cavity modes is equal to the acoustic-mode frequency -- the carrier and sideband fields simultaneously resonate and coherently build up. This mechanism significantly enhances the optoacoustic couplings in the quantum regime. It allows exploration of quantum behavior of optoacoustic interactions in small-sc…
Re-entrance is a novel feature where the phase boundaries of a system exhibit a succession of transitions between two phases A and B, like A-B-A-B, when just one parameter is varied monotonically. This type of re-entrance is displayed by the 1D Bose Hubbard model between its Mott insulator (MI) and superfluid phase as the hopping amplitude is increased from zero. Here we analyse this counter-intuitive phenomenon directly in the thermodynamic limit by utilizing the infinite time-evolving block decimation algorithm to variationally minimize an infinite matrix product state (MPS) parameterized by…
The method of "Isotropic Entanglement" (IE), inspired by Free Probability Theory and Random Matrix Theory, predicts the eigenvalue distribution of quantum many-body (spin) systems with generic interactions. At the heart is a "Slider", which interpolates between two extrema by matching fourth moments. The first extreme treats the non-commuting terms classically and the second treats them isotropically. Isotropic means that the eigenvectors are in generic positions. We prove Matching Three Moments and Slider Theorems and further prove that the interpolation is universal, i.e., independent of the…
The indistinguishability of quantum particles is widely used as a resource for the generation of entanglement. Linear quantum networks (LQNs), in which identical particles linearly evolve to arrive at multimode detectors, exploit the indistinguishability to generate various multipartite entangled states by the proper control of transformation operators. However, it is challenging to devise a suitable LQN that carries a specific entangled state or compute the possible entangled state in a given LQN as the particle and mode number increase. This research presents a mapping process of arbitrary L…
We propose a protocol to perform long-range distribution of near-maximally entangled multiphoton states, allowing versatile applications such as quantum key distribution (QKD) and quantum metrology which can provide alternatives to state-of-the-art protocols. Our scheme uses resources available within the current integrated quantum photonic technology: squeezed vacuum states and photon-number-resolving detectors. The distributed entanglement can be certified by Bell tests which have the potential to be loophole free, and may be directly used in well established QKD protocols. Generally, this p…
In this work the Schmidt number of the two-photon state generated by parametric-down conversion (PDC) is evaluated in the framework of a fully spatio-temporal model for PDC. A comparison with the results obtained in either purely spatial or purely temporal models shows that the degree of entanglement of the PDC state cannot be trivially reduced to the product of the Schmidt numbers obtained in models with lower dimensionality, unless the detected bandwidth is very narrow. This result is a consequence of the non-factorability of the state in the spatial and temporal degrees of freedoms of twin …
We propose a method of generating entanglement using single photons and electron spins in the regime of resonance scattering. The technique involves matching the spontaneous emission rate of the spin dipole transition in bulk dielectric to the modified rate of spontaneous emission of the dipole coupled to the fundamental mode of an optical microcavity. We call this regime resonance scattering where interference between the input photons and those scattered by the resonantly coupled dipole transition result in a reflectivity of zero. The contrast between this and the unit reflectivity when the …
Classical Cellular Automaton for Measurement-Only Entanglement Transitions
Western Washington University（西华盛顿大学）；Advanced Materials Science and Engineering Center, Western Washington University（西华盛顿大学先进材料科学与工程中心）；Kavli Institute for Theoretical Physics, University of California, Santa Barbara（加州大学圣塔芭芭拉分校卡弗里理论物理研究所）
Photonic entanglement is a crucial resource for quantum information technologies, including quantum information processing and long-distance communication. These applications call for narrow-band entanglement sources, being compatible with the photon-electron interfaces and relax the dispersion-induced entanglement-degradation in the network mediums. However, such Giga-hertz-level bandwidth is a challenge for the photonic entanglement based on conventional spontaneous parametric down-conversion. Here we introduce a state-of-art domain-engineering technology for the counterpropagating phase mat…
We inspect different quantum optical setups from the viewpoint of entanglement generation and detection. As a first step we consider a planar semiconductor microcavity and optimize the Bell-type correlations and their robustness against dephasing to create strong bipartite entanglement between polariton branches, which subsequently can be transfered to the emitted photons. In a second step, in order to create multipartite entangled light, we place the microcavity in an optical resonator driven by pump pulses with a frequency comb spectrum. For this system we show how phase matching of all comb…
